arXiv subjects

O. Gileva

Publications and source records attributed to O. Gileva.

14 recordsLinked to original sources

arXiv2026

Preventing quart-NaI adhesion in Bridgman growth using ammonium iodide

Adhesion between NaI(Tl) single crystals and the walls of quartz ampoules remains a major limitation for Bridgman growth under sealed conditions, particularly for applications requiring ultra-radiopure scintillators for dark matter searches, where sealed handling is essential. In this study, ammonium iodide (NH4I) was used as an additive to generate HI in situ, thereby suppressing the NaOH-SiO2 reaction that forms adhesive sodium silicate phases. Small-diameter crystals (8 mm) were first grown to determine the NH4I concentration required to eliminate adhesion. The optimized condition was then applied to the growth of a large NaI(Tl) crystal. A crack-free and bubble-free NaI(Tl) crystal with dimensions of 3 inches in diameter by 3 inches in length was successfully grown. The crystal exhibited a light output of 59,000 photons/MeV, which is higher than that of the commercial NaI(Tl) crystals used as references in this study.

physics.ins-det↗

arXiv2026

A study of neutrinoless double electron capture in $^{40}$Ca from the AMoRE experiment

The search for neutrinoless double electron capture ($0\nu\mathrm{2EC}$) provides a sensitive probe of lepton-number violation and the Majorana nature of neutrinos. We investigate the $0\nu\mathrm{2EC}$ decay of $^{40}$Ca using cryogenic detectors equipped with metallic magnetic calorimeters in the AMoRE-I experiment. The analysis is based on a physics dataset corresponding to a total exposure of 7.32 kg$\cdot$yr from thirteen $^{40}$Ca$^{100}$MoO$_4$ crystals. No significant excess is observed, and a lower limit on the half-life is obtained as $T^{0\nu}_{1/2} > 1.7 \times 10^{22}$ yr at 90$\%$ confidence level. An improved sensitivity is expected for the upcoming AMoRE-II experiment. These results demonstrate the potential of CaMoO$_4$ detectors to explore rare decay processes beyond the primary $^{100}$Mo $0\nu\beta\beta$ search program.

nucl-ex↗

arXiv2026

The nEXO Radioassay Program

Material radioactivity compilations, such as the one presented here, are important enablers of science. They are useful for the selection of radiopure materials used in the design and construction of low-energy rare-event search experiments. They allow researchers developing such experiments to save time on material studies and avoid costly duplication of effort. The data presented here were generated in support of the planned nEXO double-beta decay search. This work contains among the most restrictive constraints on the natural radioactivity content of materials of general interest to the low-radioactivity community, found in any tabulation of this kind. In this study, various techniques were employed; they are described here.

physics.ins-det↗

arXiv2026

Probing unexplored spin-dependent dark matter-proton coupling with few-photoelectron threshold in COSINE-100

We report new constraints on the spin-dependent scattering cross section between low-mass dark matter and protons using data collected by the COSINE-100 experiment. By implementing a specialized event selection process using a multi-layer perceptron and robust noise mitigation, this analysis pioneers a detection threshold of 3 and 4 isolated peaks, corresponding to the reconstructed photoelectrons, which are significantly lower than the 8 photoelectron threshold used in previous analyses. In this unstudied few-photoelectron regime, where instrumental noise and phosphorescence are prevalent, we utilize a phenomenological background model to search for the annual modulation signal expected from the Standard Halo Model. No statistically significant annual modulation is observed in our data. We derive new 90% confidence level (C.L.) upper limits for the spin-dependent DM-proton cross section, establishing the world's most stringent constraints in the 1.75-2.25 GeV/c$^2$ mass range. Furthermore, by incorporating the Migdal effect, we extend the experimental sensitivity to the sub-GeV/c$^2$ regime, setting world-leading limits in the 15-58 MeV/c$^2$ range. These results demonstrate the capability of NaI(Tl) target materials to probe previously unexplored regions of the dark matter parameter space.

hep-ex↗

arXiv2025

Constraints on sub-GeV dark matter scattering on electrons with COSINE-100

We present results of the search for sub-GeV dark matter interaction with electrons in the NaI(Tl) crystals of the COSINE-100 experiment. The two benchmark scenarios of a heavy and a light vector boson as mediator of the interaction were studied. We found no excess events over the expected background in a data-set of 2.82 years, with a total exposure of 172.9 kg-year. The derived 90% confidence level upper limits exclude a DM-electron scattering cross section above 6.4 $\times$ 10$^{-33}$ cm$^2$ for a DM mass of 0.25 GeV, assuming a light mediator; and above 3.4 $\times$ 10$^{-37}$ cm$^2$ for a 0.4 GeV DM, assuming a heavy mediator, and represent the most stringent constraints for a NaI(Tl) target to date. We also briefly discuss a planned analysis using an annual modulation method below the current 0.7 keV threshold of COSINE-100, down to few photoelectrons yield.

hep-ex↗

arXiv2025

Improved limit on neutrinoless double beta decay of $^{100}$Mo from AMoRE-I

AMoRE searches for the signature of neutrinoless double beta decay of $^{100}$Mo with a 100 kg sample of enriched $^{100}$Mo. Scintillating molybdate crystals coupled with a metallic magnetic calorimeter operate at milli-Kelvin temperatures to measure the energy of electrons emitted in the decay. As a demonstration of the full-scale AMoRE, we conducted AMoRE-I, a pre-experiment with 18 molybdate crystals, at the Yangyang Underground Laboratory for over two years. The exposure was 8.02 kg$\cdot$year (or 3.89 kg$_{\mathrm{^{100}Mo}}\cdot$year) and the total background rate near the Q-value was 0.025 $\pm$ 0.002 counts/keV/kg/year. We observed no indication of $0νββ$ decay and report a new lower limit of the half-life of $^{100}$Mo $0νββ$ decay as $ T^{0ν}_{1/2}>2.9\times10^{24}~\mathrm{yr}$ at 90\% confidence level. The effective Majorana mass limit range is $m_{ββ}<$(210--610) meV using nuclear matrix elements estimated in the framework of different models, including the recent shell model calculations.

nucl-ex↗

arXiv2025

Development of MMC-based lithium molybdate cryogenic calorimeters for AMoRE-II

The AMoRE collaboration searches for neutrinoless double beta decay of $^{100}$Mo using molybdate scintillating crystals via low temperature thermal calorimetric detection. The early phases of the experiment, AMoRE-pilot and AMoRE-I, have demonstrated competitive discovery potential. Presently, the AMoRE-II experiment, featuring a large detector array with about 90 kg of $^{100}$Mo isotope, is under construction. This paper discusses the baseline design and characterization of the lithium molybdate cryogenic calorimeters to be used in the AMoRE-II detector modules. The results from prototype setups that incorporate new housing structures and two different crystal masses (316 g and 517 - 521 g), operated at 10 mK temperature, show energy resolutions (FWHM) of 7.55 - 8.82 keV at the 2.615 MeV $^{208}$Tl $γ$ line, and effective light detection of 0.79 - 0.96 keV/MeV. The simultaneous heat and light detection enables clear separation of alpha particles with a discrimination power of 12.37 - 19.50 at the energy region around $^6$Li(n, $α$)$^3$H with Q-value = 4.785 MeV. Promising detector performances were demonstrated at temperatures as high as 30 mK, which relaxes the temperature constraints for operating the large AMoRE-II array.

physics.ins-det↗

arXiv2024

Development of decay energy spectroscopy for radio impurity analysis

We present the development of a decay energy spectroscopy (DES) method for the analysis of radioactive impurities using magnetic microcalorimeters (MMCs). The DES system was designed to analyze radionuclides, such as Ra-226, Th-228, and their daughter nuclides, in materials like copper, commonly used in rare-event search experiments. We tested the DES system with a gold foil absorber measuring 20x20x0.05 mm^3, large enough to accommodate a significant drop of source solution. Using this large absorber and an MMC sensor, we conducted a long-term measurement over ten days of live time, requiring 11 ADR cooling cycles. The combined spectrum achieved an energy resolution of 45 keV FWHM, sufficient to identify most alpha and DES peaks of interest. Specific decay events from radionuclide contaminants in the absorber were identified. This experiment confirms the capability of the DES system to measure alpha decay chains of Ra-226 and Th-228, offering a promising method for radio-impurity evaluation in ultra-low background experiments.

physics.ins-det↗

arXiv2024

Projected background and sensitivity of AMoRE-II

AMoRE-II aims to search for neutrinoless double beta decay with an array of 423 Li$_2$$^{100}$MoO$_4$ crystals operating in the cryogenic system as the main phase of the Advanced Molybdenum-based Rare process Experiment (AMoRE). AMoRE has been planned to operate in three phases: AMoRE-pilot, AMoRE-I, and AMoRE-II. AMoRE-II is currently being installed at the Yemi Underground Laboratory, located approximately 1000 meters deep in Jeongseon, Korea. The goal of AMoRE-II is to reach up to $T^{0νββ}_{1/2}$ $\sim$ 6 $\times$ 10$^{26}$ years, corresponding to an effective Majorana mass of 15 - 29 meV, covering all the inverted mass hierarchy regions. To achieve this, the background level of the experimental configurations and possible background sources of gamma and beta events should be well understood. We have intensively performed Monte Carlo simulations using the GEANT4 toolkit in all the experimental configurations with potential sources. We report the estimated background level that meets the 10$^{-4}$counts/(keV$\cdot$kg$\cdot$yr) requirement for AMoRE-II in the region of interest (ROI) and show the projected half-life sensitivity based on the simulation study.

physics.ins-det↗

arXiv2024

Background study of the AMoRE-pilot experiment

We report a study on the background of the Advanced Molybdenum-Based Rare process Experiment (AMoRE), a search for neutrinoless double beta decay (\znbb) of $^{100}$Mo. The pilot stage of the experiment was conducted using $\sim$1.9 kg of \CAMOO~ crystals at the Yangyang Underground Laboratory, South Korea, from 2015 to 2018. We compared the measured $β/γ$ energy spectra in three experimental configurations with the results of Monte Carlo simulations and identified the background sources in each configuration. We replaced several detector components and enhanced the neutron shielding to lower the background level between configurations. A limit on the half-life of $0νββ$ decay of $^{100}$Mo was found at $T_{1/2}^{0ν} \ge 3.0\times 10^{23}$ years at 90\% confidence level, based on the measured background and its modeling. Further reduction of the background rate in the AMoRE-I and AMoRE-II are discussed.

nucl-ex↗

arXiv2022

Alpha backgrounds in the AMoRE-Pilot experiment

The Advanced Mo-based Rare process Experiment (AMoRE)-Pilot experiment is an initial phase of the AMoRE search for neutrinoless double beta decay of $^{100}$Mo, with the purpose of investigating the level and sources of backgrounds. Searches for neutrinoless double beta decay generally require ultimately low backgrounds. Surface $α$ decays on the crystals themselves or nearby materials can deposit a continuum of energies that can be as high as the $Q$-value of the decay itself and may fall in the region of interest (ROI). To understand these background events, we studied backgrounds from radioactive contaminations internal to and on the surface of the crystals or nearby materials with Geant4-based Monte Carlo simulations. In this study, we report on the measured $α$ energy spectra fitted with the corresponding simulated spectra for six crystal detectors, where sources of background contributions could be identified through high energy $α$ peaks and continuum parts in the energy spectrum for both internal and surface contaminations. We determine the low-energy contributions from internal and surface $α$ contaminations by extrapolating from the $α$ background fitting model.

physics.ins-det↗

arXiv2020

Development of ultra-pure NaI(Tl) detectors for the COSINE-200 experiment

The annual modulation signal observed by the DAMA experiment is a long-standing question in the community of dark matter direct detection. This necessitates an independent verification of its existence using the same detection technique. The COSINE-100 experiment has been operating with 106~kg of low-background NaI(Tl) detectors providing interesting checks on the DAMA signal. However, due to higher backgrounds in the NaI(Tl) crystals used in COSINE-100 relative to those used for DAMA, it was difficult to reach final conclusions. Since the start of COSINE-100 data taking in 2016, we also have initiated a program to develop ultra-pure NaI(Tl) crystals for COSINE-200, the next phase of the experiment. The program includes efforts of raw powder purification, ultra-pure NaI(Tl) crystal growth, and detector assembly techniques. After extensive research and development of NaI(Tl) crystal growth, we have successfully grown a few small-size (0.61$-$0.78 kg) thallium-doped crystals with high radio-purity. A high light yield has been achieved by improvements of our detector assembly technique. Here we report the ultra-pure NaI(Tl) detector developments at the Institute for Basic Science, Korea. The technique developed here will be applied to the production of NaI(Tl) detectors for the COSINE-200 experiment.

physics.ins-det↗

arXiv2020

Growth and development of pure Li2MoO4 crystals for rare event experiment at CUP

The Center for Underground Physics (CUP) of the Institute for Basic Science (IBS) is searching for the neutrinoless double-beta decay (0ν\b{eta}\b{eta}) of 100Mo in the molybdate crystals of the AMoRE experiment. The experiment requires pure scintillation crystals to minimize internal backgrounds that can affect the 0ν\b{eta}\b{eta} signal. For the last few years, we have been growing and studying Li2MoO4 crystals in a clean-environment facility to minimize external contamination during the crystal growth. Before growing Li2100MoO4 crystal, we have studied Li2natMoO4 crystal growth by a conventional Czochralski (CZ) grower. We grew a few different kinds of Li2natMO4 crystals using different raw materials in a campaign to minimize impurities. We prepared the fused Al2O3 refractories for the growth of ingots. Purities of the grown crystals were measured with high purity germanium detectors and by inductively coupled plasma mass spectrometry. The results show that the Li2MoO4 crystal has purity levels suitable for rare-event experiments. In this study, we present the growth of Li2MoO4 crystals at CUP and their purities.

physics.ins-det↗

arXiv2020

Purification and recovery of 100MoO3 in crystal production for AMoRE experiment

The AMoRE collaboration searches for the neutrinoless double-beta decay of 100Mo with ultra-radiopure molybdate crystals operated as low-temperature scintillating bolometers. For such a rare event search experiment, the techniques for investigating and reducing radioactive background contaminants in detector materials are extremely crucial. This paper discusses techniques for deep purification of enriched molybdenum for growing the crystals and the recovery of 100MoO3 from the residual melt left after growing lithium molybdate crystals. The purities of enriched molybdenum trioxide powders before and after the purification and that of the recovered powder were tested with ICP-MS; results of these tests are presented.

physics.ins-det↗