SearcharxivSearch

arXiv subjects

O. Gingras

Publications and source records attributed to O. Gingras.

6 recordsLinked to original sources

Accelerating dynamical mean-field theory convergence by preconditioning with computationally cheaper quantum embedding methods

Dynamical mean-field theory (DMFT) is a cornerstone technique for studying strongly correlated electronic systems. However, each DMFT step is computationally demanding, and many iterations can be required to achieve convergence. Here, we accelerate the convergence of DMFT by initializing its self-consistent cycle with solutions from computationally cheaper and more approximate methods. We compare the initialization with the non-interacting solution to a range of quantum embedding compatible approaches: Hartree-Fock, the Hubbard-I approximation, rotationally invariant slave bosons (RISB), and its ghost extension (g-RISB). We find that these initializations can reduce the number of DMFT iterations by up to an order of magnitude, with g-RISB providing the most effective and reliable benefits. In most regimes, initializing with g-RISB and performing a single DMFT iteration suffices to recover the full dynamical structure. The improvement in convergence is controlled by the initial solution's accuracy in the low-energy part of the self-energy, on the scale of the non-interacting bandwidth. This strategy is especially effective at the Mott insulator-metal transition, where an initialization from the non-interacting limit can lead to a breakdown of DMFT due to the sign problem. Our results establish the usage of accurate yet cheaper quantum embedding methods as a powerful means to substantially reduce the computational cost of DMFT, particularly in regimes where convergence is slow or prone to failure.

cond-mat.str-el

Light-induced Asymmetric Pseudogap below T$_\text{c}$ in cuprates

To this day, high-temperature cuprate superconductors remain an unparalleled platform for studying the competition and coexistence of emergent, static and dynamic, quantum phases of matter exhibiting high transition temperature non-s-wave superconductivity, non-Fermi liquid transport and a still enigmatic pseudogap regime. However, how superconductivity emerges alongside and competes with the pseudogap regime remains an open question. Here, we present a high-resolution, time- and angle-resolved photoemission study of the near-antinodal region of optimally-doped Bi$_2$Sr$_2$CaCu$_2$O$_{8+\delta}$. For a sufficiently high excitation fluence, we disrupt superconductivity and drive a transient change from a symmetric superconducting-like to an asymmetric pseudogap-like density of states, for electronic temperatures well below the equilibrium superconducting critical temperature. Conversely, when the superconductivity is fully restored, the pseudogap is suppressed, as signaled by a fully particle-hole symmetric density of states. A unique aspect of our experiments is that the pseudogap coexists with superconducting features at intermediate times or at intermediate fluence. Our findings challenge the paradigm that superconductivity emerges by establishing phase coherence in the pseudogap. Instead, our experimental results, supported by phenomenological theory, demonstrate that the two states compete, and that the low-temperature ground state of the cuprates originates from a competition between superconducting and pseudogap states.

cond-mat.supr-con

The Frenkel line and the pseudogap: an analogy between classical and electronic fluids

Asymptotically close to critical end-points of first-order transitions, maxima in thermodynamic quantities occur along a line called the Widom line, a concept first introduced in classical fluids. This concept has been extended to strongly correlated electronic fluids in the context of the Mott transition. Namely, upon increasing interaction strength in the Hubbard model at half-filling, one finds a first-order Mott metal-insulator transition with a critical endpoint at high temperature, above which several crossover lines are observable. Using the dynamical cluster approximation for the triangular-lattice Hubbard model, we compute a new crossover line, the Frenkel line, a concept borrowed from classical fluids that is useful for defining a sharp crossover between the pseudogap and the correlated Fermi liquid. The Frenkel line in the electron fluid is defined by the appearance of back-scattering upon entering the pseudogap. The signature of back-scattering is the existence of a negative value in the time-domain optical conductivity. The Frenkel line extends to high temperatures.

cond-mat.str-el

Doping the Mott insulating state of the triangular-lattice Hubbard model reveals the Sordi transition

It has been reported that upon doping a Mott insulator, there can be a crossover to a pseudogaped metallic phase followed by a first-order transition to another thermodynamically stable metallic phase. We call this first-order metal-metal transition the Sordi transition. It was argued that the initial reports of Sordi transitions at finite temperature could be explained by finite size effects and biases related to the model and method used. In this work, we report the Sordi transition on larger clusters at finite temperature on a triangular lattice, where long-range antiferromagnetic fluctuations are frustrated, using a different method, the dynamical cluster approximation instead of the cellular dynamical mean-field theory. This demonstrates that this first-order transition is a directly observable transition in doped Mott insulators and that it is relevant for experiments on candidate spin-liquid organic materials.

cond-mat.str-el

Mott transition, Widom line and pseudogap in the half-filled triangular lattice Hubbard model

The Mott transition is observed experimentally in materials that are magnetically frustrated so that long-range order does not hide the Mott transition at finite temperature. The Hubbard model on the triangular lattice at half-filling is a paradigmatic model to study the interplay of interactions and frustration on the normal-state phase diagram. We use the dynamical cluster approximation with continuous time auxiliary field quantum Monte Carlo to solve this model for 1, 4, 6, 12, and 16 site clusters with detailed analysis performed for the 6 site cluster. We show that a) for every cluster there is an inflection point in the double occupancy as a function of interaction, defining a Widom line that extends above the critical point of the first-order Mott transition; b) the presence of this line and the cluster size dependence argue for the observability of the Mott transition at finite temperature in the thermodynamic limit; c) the loss of spectral weight in the metal to Mott insulator transition as a function of temperature and for strong interactions is momentum dependent, the hallmark of a pseudogap. That pseudogap spans a large region of the phase diagram near the Mott transition.

cond-mat.str-el

Superintegrable systems with spin induced by coalgebra symmetry

A method for deriving superintegrable Hamiltonians with a spin orbital interaction is presented. The method is applied to obtain a new superintegrable system in Euclidean space $\mathbb{E}_3$ with the following properties. It describes a rotationally invariant interaction between a particle of spin $\frac{1}{2}$ and one of spin 0. Its Hamiltonian commutes with total angular momentum $\vec{\mathcal{J}}$ and with additional vector integrals of motion $\vec{X}$, $\vec{Y}$ with components that are third order differential operators. The integrals of motion form a polynomial algebra under commutation. The system is exactly solvable (in terms of Laguerre polynomials) and the bound state energy levels are degenerate and described by a Balmer type formula. When the spin orbital potential is switched off the system reduces to a hydrogen atom.

math-ph