arXiv subjects

O. Serot

Publications and source records attributed to O. Serot.

6 recordsLinked to original sources

arXiv2026

Hindered Prompt-Neutron Evaporation in Surrogate Reactions for $^{239}$Pu(n,f)

Isotopic fission-fragment distributions of $^{240}$Pu have been measured, for the first time, as a function of the initial excitation energy, and the prompt neutron multiplicity has been derived from these data. The $^{240}$Pu fissioning system was produced through the two-proton transfer reaction between $^{238}$U and $^{12}$C, a surrogate reaction for the neutron-capture-induced fission $^{239}$Pu(n,f). The reaction was measured in inverse kinematics, allowing the fission fragments to be fully identified with the VAMOS Spectrometer. When compared to neutron-capture-induced reactions, the observed prompt neutron multiplicity shows a clear reduction in the surrogate two-proton transfer, revealing an unexpected influence of the entrance channel in the fission output. At the same time, fission-fragment yield distributions obtained in neutron-capture-induced reactions show a relative fission-fragment production in the symmetry region similar to that measured in this work. The discrepancy in neutron multiplicity is attributed to the additional angular momentum induced in the multi-nucleon transfer reactions, which excites the fissioning system to higher-spin states, increasing the probability of gamma emission that competes with neutron evaporation, in particular from the fission barrier to the scission point. This observation underlines the limitations in the utilisation of properties derived from surrogate reactions in nuclear technology and other applications of nuclear fission.

nucl-ex↗

arXiv2023

Observation of a nuclear recoil peak at the 100 eV scale induced by neutron capture

Coherent elastic neutrino-nucleus scattering and low-mass Dark Matter detectors rely crucially on the understanding of their response to nuclear recoils. We report the first observation of a nuclear recoil peak at around 112 eV induced by neutron capture. The measurement was performed with a CaWO$_4$ cryogenic detector from the NUCLEUS experiment exposed to a $^{252}$Cf source placed in a compact moderator. The measured spectrum is found in agreement with simulations and the expected peak structure from the single-$γ$ de-excitation of $^{183}$W is identified with 3 $σ$ significance. This result demonstrates a new method for precise, in-situ, and non-intrusive calibration of low-threshold experiments.

nucl-ex↗

arXiv2023

Study of collision and $γ$-cascade times following neutron-capture processes in cryogenic detectors

The emission of $γ$-rays after a neutron capture in a cryogenic detector can generate mono-energetic nuclear recoils in the sub-keV regime, of direct interest for the calibration of Dark Matter and Coherent Elastic Neutrino Nucleus Scattering experiments. Here we show that accurate predictions of the nuclear recoil spectra induced by neutron captures require taking into account the interplay between the development in time of the de-excitation $γ$-cascade of the target nucleus and that of the associated atomic collisions in matter. We present detailed simulations coupling the FIFRELIN code for the description of the $γ$-cascades and the IRADINA code for the modelling of the fast atomic movements in matter. Nuclear recoil spectra are predicted, and made available to the community, for concrete cases of Al$_2$O$_3$, Si, Ge and CaWO$_4$ crystals exposed to a low intensity beam of thermal neutrons. We find that timing effects cause new calibration peaks to emerge in the recoil spectra and also impact the shape of the continuous recoil distribution. We discuss how they could give access to a rich physics program, spanning the accurate study of the response of cryogenic detectors in the sub-keV range, tests of solid state physics simulations and tests of nuclear models.

physics.ins-det↗

arXiv2021

Calibration of nuclear recoils at the 100 eV scale using neutron capture

The development of low-threshold detectors for the study of coherent elastic neutrino-nucleus scattering and for the search for light dark matter necessitates methods of low-energy calibration. We suggest this can be provided by the nuclear recoils resulting from the $γ$ emission following thermal neutron capture. In particular, several MeV-scale single-$γ$ transitions induce well-defined nuclear recoil peaks in the 100 eV range. Using the FIFRELIN code, complete schemes of $γ$-cascades for various isotopes can be predicted with high accuracy to determine the continuous background of nuclear recoils below the calibration peaks. We present a comprehensive experimental concept for the calibration of CaWO$_4$ and Ge cryogenic detectors at a research reactor. For CaWO$_4$ the simulations show that two nuclear recoil peaks at 112.5 eV and 160.3 eV should be visible above background simply in the spectrum of the cryogenic detector. Then we discuss how the additional tagging for the associated $γ$ increases the sensitivity of the method and extends its application to a wider energy range and to Ge cryogenic detectors.

physics.ins-det↗

arXiv2009

beta-decay study of Cu-77

A beta-decay study of Cu-77 has been performed at the ISOLDE mass separator with the aim to deduce its beta-decay properties and to obtain spectroscopic information on Zn-77. Neutron-rich copper isotopes were produced by means of proton- or neutron-induced fission reactions on U-238. After the production, Cu-77 was selectively laser ionized, mass separated and sent to different detection systems where beta-gamma and beta-n coincidence data were collected. We report on the deduced half-live, decay scheme, and possible spin assignment of 77Cu.

nucl-ex↗

arXiv2007

Emission of Scission Neutrons in the Sudden Approximation

At a certain finite neck radius during the descent of a fissioning nucleus from the saddle to the scission point, the attractive nuclear forces can no more withstand the repulsive Coulomb forces producing the neck rupture and the sudden absorption of the neck stubs by the fragments. At that moment, the neutrons, although still characterized by their pre-scission wave functions, find themselves in the newly created potential of their interaction with the separated fragments. Their wave functions become wave packets with components in the continuum. The probability to populate such states gives evidently the emission probability of neutrons at scission. In this way, we have studied scission neutrons for the fissioning nucleus $^{236}$U, using two-dimensional realistic nuclear shapes. Both the emission probability and the distribution of the emission points relative to the fission fragments strongly depend on the quantum numbers of the pre-scission state from which the neutron is emitted. In particular it was found that states with $Ωπ$ = 1/2+ dominate the emission. Depending on the assumed pre- and post-scission configurations and on the emission-barrier height, 30 to 50% of the total scission neutrons are emitted from 1/2+ states. Their emission points are concentrated in the region between the newly separated fragments. The upper limit for the total number of neutrons per scission event is predicted to lie between 0.16 and 1.73 (depending on the computational assumptions).

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