arXiv subjects

O. Smirnova

Publications and source records attributed to O. Smirnova.

16 recordsLinked to original sources

arXiv2022

Sub-cycle multidimensional spectroscopy of strongly correlated materials

Strongly correlated solids are extremely complex and fascinating quantum systems, where new states continue to emerge, especially when interaction with light triggers interplay between them. In this interplay, sub-laser-cycle electron response is particularly attractive as a tool for ultrafast manipulation of matter at PHz scale. Here we introduce a new type of non-linear multidimensional spectroscopy, which allows us to unravel the sub-cycle dynamics of strongly correlated systems interacting with few-cycle infrared pulses and the complex interplay between different correlated states evolving on the sub-femtosecond time-scale. We demonstrate that single particle sub-cycle electronic response is extremely sensitive to correlated many-body dynamics and provides direct access to many body response functions. For the two-dimensional Hubbard model under the influence of ultra-short, intense electric field transients, we demonstrate that our approach can resolve pathways of charge and energy flow between localized and delocalized many-body states on the sub-cycle time scale and follow the creation of a highly correlated state surviving after the end of the laser pulse. Our findings open a way towards a regime of imaging and manipulating strongly correlated materials at optical rates, beyond the multi-cycle approach employed in Floquet engineering, with the sub-cycle response being a key tool for accessing many body phenomena.

cond-mat.str-el↗

arXiv2020

Lightwave topology for strong-field valleytronics

Modern light generation technology offers extraordinary capabilities for sculpting light pulses, with full control over individual electric field oscillations within each laser cycle. These capabilities are at the core of lightwave electronics - the dream of ultrafast lightwave control over electron dynamics in solids, on a few-cycle to sub-cycle timescale, aiming at information processing at tera-Hertz to peta-Hertz rates. Here we show a robust and general approach to valley-selective electron excitations in two-dimensional solids, by controlling the sub-cycle structure of non-resonant driving fields at a few-femtosecond timescale. Bringing the frequency-domain concept of topological Floquet systems to the few-fsec time domain, we develop a transparent control mechanism in real space and an all-optical, non-element-specific method to coherently write, manipulate and read selective valley excitations using fields carried in a wide range of frequencies, on timescales that can be much shorter than the valley lifetime, crucial for implementation of valleytronic devices.

physics.optics↗

arXiv2018

Topological strong field physics on sub-laser cycle time scale

Sub-laser cycle time scale of electronic response to strong laser fields enables attosecond dynamical imaging in atoms, molecules and solids. Optical tunneling and high harmonic generation are the hallmarks of attosecond imaging in optical domain, including imaging of phase transitions in solids. Topological phase transition yields a state of matter intimately linked with electron dynamics, as manifested via the chiral edge currents in topological insulators. Does topological state of matter leave its mark on optical tunneling and sub-cycle electronic response? We identify distinct topological effects on the directionality and the attosecond timing of currents arising during electron injection into conduction bands. We show that electrons tunnel across the band gap differently in trivial and topological phases, for the same band structure, and identify the key role of the Berry curvature in this process. These effects map onto topologically-dependent attosecond delays in high harmonic emission and the helicities of the emitted harmonics, which can record the phase diagram of the system and its topological invariants. Thus, the topological state of the system controls its attosecond, highly non-equilibrium electronic response to strong low-frequency laser fields, in bulk. Our findings create new roadmaps in studies of topological systems, building on ubiquitous properties of sub-laser cycle strong field response - a unique mark of attosecond science.

physics.optics↗

arXiv2017

High harmonic imaging of ultrafast many-body dynamics in strongly correlated systems

This Letter brings together two topics that, until now, have been the focus of intense but non-overlapping research efforts. The first concerns high harmonic generation in solids, which occurs when intense light field excites highly non-equilibrium electronic response in a semiconductor or a dielectric. The second concerns many-body dynamics in strongly correlated systems such as the Mott insulator. Here we show that high harmonic generation can be used to time-resolve ultrafast many-body dynamics associated with optically driven phase transition, with accuracy far exceeding one cycle of the driving light field. Our work paves the way for time-resolving highly non-equilibrium many body dynamics in strongly correlated systems, with few femtosecond accuracy.

cond-mat.str-el↗

arXiv2016

Photoexcitation Circular Dichroism in Chiral Molecules

Chirality is ubiquitous in nature and fundamental in science, from particle physics to metamaterials.The most established technique of chiral discrimination - photoabsorption circular dichroism - relies on the magnetic properties of a chiral medium and yields an extremely weak chiral response. We propose and demonstrate a new, orders of magnitude more sensitive type of circular dichroism in neutral molecules: photoexitation circular dichroism. It does not rely on weak magnetic effects, but takes advantage of the coherent helical motion of bound electrons excited by ultrashort circularly polarized light. It results in an ultrafast chiral response and the efficient excitation of a macroscopic chiral density in an initially isotropic ensemble of randomly oriented chiral molecules. We probe this excitation without the aid of further chiral interactions using linearly polarized laser pulses. Our time-resolved study of vibronic chiral dynamics opens a way to the efficient initiation, control and monitoring of chiral chemical change in neutral molecules at the level of electrons.

physics.atm-clus↗

arXiv2016

Even harmonic generation in isotropic media of dissociating homonuclear molecules

Isotropic gases irradiated by long pulses of intense IR light can generate very high harmonics of the incident field. It is generally accepted that, due to the symmetry of the generating medium, be it an atomic or an isotropic molecular gas, only odd harmonics of the driving field can be produced. Here we show how the interplay of electronic and nuclear dynamics can lead to a marked breakdown of this standard picture: a substantial part of the harmonic spectrum can consist of even rather than odd harmonics. We demonstrate the effect using ab-initio solutions of the time-dependent Schrödinger equation for $H$$_2$$^+$ and its isotopes in full dimensionality. By means of a simple analytical model, we identify its physical origin, which is the appearance of a permanent dipole moment in dissociating homonuclear molecules, caused by light-induced localization of the electric charge during dissociation. The effect arises for sufficiently long laser pulses and the region of the spectrum where even harmonics are produced is controlled by pulse duration. Our results (i) show how the interplay of femtosecond nuclear and attosecond electronic dynamics, which affects the charge flow inside the dissociating molecule, is reflected in the nonlinear response, and (ii) force one to augment standard selection rules found in nonlinear optics textbooks by considering light-induced modifications of the medium during the generation process.

physics.atom-ph↗

arXiv2015

CEP-stable Tunable THz-Emission Originating from Laser-Waveform-Controlled Sub-Cycle Plasma-Electron Bursts

We study THz-emission from a plasma driven by an incommensurate-frequency two-colour laser field. A semi-classical transient electron current model is derived from a fully quantum-mechanical description of the emission process in terms of sub-cycle field-ionization followed by continuum-continuum electron transitions. For the experiment, a CEP-locked laser and a near-degenerate optical parametric amplifier are used to produce two-colour pulses that consist of the fundamental and its near-half frequency. By choosing two incommensurate frequencies, the frequency of the CEP-stable THz-emission can be continuously tuned into the mid-IR range. This measured frequency dependence of the THz-emission is found to be consistent with the semi-classical transient electron current model, similar to the Brunel mechanism of harmonic generation.

physics.atom-ph↗

arXiv2015

The High A(V) Quasar Survey: Reddened quasi-stellar objects selected from optical/near-infrared photometry - II

Quasi-stellar objects (QSOs) whose spectral energy distributions (SEDs) are reddened by dust either in their host galaxies or in intervening absorber galaxies are to a large degree missed by optical color selection criteria like the one used by the Sloan Digital Sky Survey (SDSS). To overcome this bias against red QSOs, we employ a combined optical and near-infrared color selection. In this paper, we present a spectroscopic follow-up campaign of a sample of red candidate QSOs which were selected from the SDSS and the UKIRT Infrared Deep Sky Survey (UKIDSS). The spectroscopic data and SDSS/UKIDSS photometry are supplemented by mid-infrared photometry from the Wide-field Infrared Survey Explorer. In our sample of 159 candidates, 154 (97%) are confirmed to be QSOs. We use a statistical algorithm to identify sightlines with plausible intervening absorption systems and identify nine such cases assuming dust in the absorber similar to Large Magellanic Cloud sightlines. We find absorption systems toward 30 QSOs, 2 of which are consistent with the best-fit absorber redshift from the statistical modeling. Furthermore, we observe a broad range in SED properties of the QSOs as probed by the rest-frame 2 μm flux. We find QSOs with a strong excess as well as QSOs with a large deficit at rest-frame 2 μm relative to a QSO template. Potential solutions to these discrepancies are discussed. Overall, our study demonstrates the high efficiency of the optical/near-infrared selection of red QSOs.

astro-ph.GA↗

arXiv2009

Optical and X-ray Observations of M31N 2007-12b: An Extragalactic Recurrent Nova with a Detected Progenitor?

We report combined optical and X-ray observations of nova M31N 2007-12b. Optical spectroscopy obtained 5 days after the 2007 December outburst shows evidence of very high ejection velocities (FWHM H$α\simeq 4500$ km s$^{-1}$). In addition, Swift X-ray data show that M31N 2007-12b is associated with a Super-Soft Source (SSS) which appeared between 21 and 35 days post-outburst and turned off between then and day 169. Our analysis implies that $M_{\rm WD} \ga 1.3 $M$_{\odot}$ in this system. The optical light curve, spectrum and X-ray behaviour are consistent with those of a recurrent nova. Hubble Space Telescope observations of the pre-outburst location of M31N 2007-12b reveal the presence of a coincident stellar source with magnitude and color very similar to the Galactic recurrent nova RS Ophiuchi at quiescence, where the red giant secondary dominates the emission. We believe that this is the first occasion on which a nova progenitor system has been identified in M31. However, the greatest similarities of outburst optical spectrum and SSS behaviour are with the supposed Galactic recurrent nova V2491 Cygni. A previously implied association of M31N 2007-12b with nova M31N 1969-08a is shown to be erroneous and this has important lessons for future searches for recurrent novae in extragalactic systems. Overall, we show that suitable complementary X-ray and optical observations can be used not only to identify recurrent nova candidates in M31, but also to determine subtypes and important physical parameters of these systems. Prospects are therefore good for extending studies of recurrent novae into the Local Group with the potential to explore in more detail such important topics as their proposed link to Type Ia Supernovae.

astro-ph.SR↗

arXiv2003

HEP Applications Evaluation of the EDG Testbed and Middleware

Workpackage 8 of the European Datagrid project was formed in January 2001 with representatives from the four LHC experiments, and with experiment independent people from five of the six main EDG partners. In September 2002 WP8 was strengthened by the addition of effort from BaBar and D0. The original mandate of WP8 was, following the definition of short- and long-term requirements, to port experiment software to the EDG middleware and testbed environment. A major additional activity has been testing the basic functionality and performance of this environment. This paper reviews experiences and evaluations in the areas of job submission, data management, mass storage handling, information systems and monitoring. It also comments on the problems of remote debugging, the portability of code, and scaling problems with increasing numbers of jobs, sites and nodes. Reference is made to the pioneeering work of Atlas and CMS in integrating the use of the EDG Testbed into their data challenges. A forward look is made to essential software developments within EDG and to the necessary cooperation between EDG and LCG for the LCG prototype due in mid 2003.

cs.DC↗

arXiv2003

Atlas Data-Challenge 1 on NorduGrid

The first LHC application ever to be executed in a computational Grid environment is the so-called ATLAS Data-Challenge 1, more specifically, the part assigned to the Scandinavian members of the ATLAS Collaboration. Taking advantage of the NorduGrid testbed and tools, physicists from Denmark, Norway and Sweden were able to participate in the overall exercise starting in July 2002 and continuing through the rest of 2002 and the first part of 2003 using solely the NorduGrid environment. This allowed to distribute input data over a wide area, and rely on the NorduGrid resource discovery mechanism to find an optimal cluster for job submission. During the whole Data-Challenge 1, more than 2 TB of input data was processed and more than 2.5 TB of output data was produced by more than 4750 Grid jobs.

physics.comp-ph↗

arXiv2003

The NorduGrid architecture and tools

The NorduGrid project designed a Grid architecture with the primary goal to meet the requirements of production tasks of the LHC experiments. While it is meant to be a rather generic Grid system, it puts emphasis on batch processing suitable for problems encountered in High Energy Physics. The NorduGrid architecture implementation uses the \globus{} as the foundation for various components, developed by the project. While introducing new services, the NorduGrid does not modify the Globus tools, such that the two can eventually co-exist. The NorduGrid topology is decentralized, avoiding a single point of failure. The NorduGrid architecture is thus a light-weight, non-invasive and dynamic one, while robust and scalable, capable of meeting most challenging tasks of High Energy Physics.

physics.comp-ph↗

arXiv2002

An Overview of a Grid Architecture for Scientific Computing

This document gives an overview of a Grid testbed architecture proposal for the NorduGrid project. The aim of the project is to establish an inter-Nordic testbed facility for implementation of wide area computing and data handling. The architecture is supposed to define a Grid system suitable for solving data intensive problems at the Large Hadron Collider at CERN. We present the various architecture components needed for such a system. After that we go on to give a description of the dynamics by showing the task flow.

cs.DC↗

arXiv2002

Performance evaluation of the GridFTP within the NorduGrid project

This report presents results of the tests measuring the performance of multi-threaded file transfers, using the GridFTP implementation of the Globus project over the NorduGrid network resources. Point to point WAN tests, carried out between the sites of Copenhagen, Lund, Oslo and Uppsala, are described. It was found that multiple threaded download via the high performance GridFTP protocol can significantly improve file transfer performance, and can serve as a reliable data

cs.DC↗

arXiv2001

Hadronization corrections to helicity components of the fragmentation function

In the hadronic decays of Z, gluon emission leads to the appearance of the longitudinal component of the fragmentation function, F_L. Measurement of F_L and the transverse component, F_T, could thus provide an insight into the gluon fragmentation function. However, hadronization corrections at low x can be significant. Here we present a method of accounting for such corrections, using the JETSET event generator as illustration.

hep-ph↗

arXiv1998

Tests of the JETSET Bose-Einstein correlation model in the e+e- annihilation process

Studies of implementation of the simulation of the Bose-Einstein correlation effects in the JETSET particle generator are performed. Analysis of dependance of the one-dimensional correlation function parameters on the presumed boson source size reveals appearance of the effective new length scale, which limits applicability of the simple momentum-shifting mechanism, employed by JETSET to simulate the Bose-Einstein correlation. Two- and three-dimensional correlation functions are analysed as well and compared to the DELPHI data.

hep-ex↗