arXiv subjects

O. Thomas

Publications and source records attributed to O. Thomas.

7 recordsLinked to original sources

arXiv2018

Photoassociation of rovibrational Rydberg molecules

In this work we discuss the rotational structure of Rydberg molecules. We calculate the complete wave function in a laboratory fixed frame and derive the transition matrix elements for the pho- toassociation of free ground state atoms. We discuss the implications for the excitation of different rotational states as well as the shape of the angular nuclear wave function. We find a rather com- plex shape and unintuitive coupling strengths, depending on the angular momenta coupling that are relevant for the states. This work explains the different steps to calculate the wave functions and the transition matrix elements in a way, that they can be directly transferred to different molecular states, atomic species or molecular coupling cases.

physics.atom-ph↗

arXiv2016

Mesoscopic Rydberg-blockaded ensembles in the superatom regime and beyond

Controlling strongly interacting many-body systems enables the creation of tailored quantum matter, with properties transcending those based solely on single particle physics. Atomic ensembles which are optically driven to a Rydberg state provide many examples of this, such as atom-atom entanglement, many-body Rabi oscillations, strong photon-photon interaction and spatial pair correlations. In its most basic form, Rydberg quantum matter consists of an isolated ensemble of strongly interacting atoms spatially confined to the blockade volume - a so-called superatom. Here we demonstrate the controlled creation and characterization of an isolated mesoscopic superatom by means of accurate density engineering and excitation to Rydberg $p$-states. Its variable size allows to investigate the transition from effective two-level physics for strong confinement to many-body phenomena in extended systems. By monitoring continuous laser-induced ionization we observe a strongly anti-bunched ion emission under blockade conditions and extremely bunched ion emission under off-resonant excitation. Our experimental setup enables in vivo measurements of the superatom, yielding insight into both excitation statistics and dynamics. We anticipate straightforward applications in quantum optics and quantum information as well as future experiments on many-body physics.

physics.atom-ph↗

arXiv2014

Retrieval of the atomic displacements in the crystal from the coherent x-ray diffraction pattern

We investigate the retrieval of spatially resolved atomic displacements via the phases of the direct(real)-space image reconstructed from the strained crystal's coherent x-ray diffraction pattern. We demonstrate that limiting the spatial variation of the first and second order spatial displacement derivatives improves convergence of the iterative phase retrieval algorithm for displacements reconstructions to the true solution. Our approach is exploited to retrieve the displacement in a periodic array of silicon lines isolated by silicon dioxide filled trenches.

cond-mat.mtrl-sci↗

arXiv2013

Combined coherent x-ray micro-diffraction and local mechanical loading on copper nanocrystals

Coherent x-ray micro-diffraction and local mechanical loading can be combined to investigate the mechanical deformation in crystalline nanostructures. Here we present measurements of plastic deformation in a copper crystal of sub-micron size obtained by loading the sample with an Atomic Force Microscopy tip. The appearance of sharp features in the diffraction pattern, while conserving its global shape, is attributed to crystal defects induced by the tip.

cond-mat.mtrl-sci↗

arXiv2011

Probing higher order correlations of the photon field with photon number resolving avalanche photodiodes

We demonstrate the use of two high speed avalanche photodiodes in exploring higher order photon correlations. By employing the photon number resolving capability of the photodiodes the response to higher order photon coincidences can be measured. As an example we show experimentally the sensitivity to higher order correlations for three types of photon sources with distinct photon statistics. This higher order correlation technique could be used as a low cost and compact tool for quantifying the degree of correlation of photon sources employed in quantum information science.

quant-ph↗

arXiv2010

Efficient photon number detection with silicon avalanche photodiodes

We demonstrate an efficient photon number detector for visible wavelengths using a silicon avalanche photodiode. Under subnanosecond gating, the device is able to resolve up to four photons in an incident optical pulse. The detection efficiency at 600 nm is measured to be 73.8%, corresponding to an avalanche probability of 91.1% of the absorbed photons, with a dark count probability below 1.1x10^{-6} per gate. With this performance and operation close to room temperature, fast-gated silicon avalanche photodiodes are ideal for optical quantum information processing that requires single-shot photon number detection.

quant-ph↗

arXiv2007

Inversion of the Diffraction Pattern from an Inhomogeneously Strained Crystal using an Iterative Algorithm

The displacement field in highly non uniformly strained crystals is obtained by addition of constraints to an iterative phase retrieval algorithm. These constraints include direct space density uniformity and also constraints to the sign and derivatives of the different components of the displacement field. This algorithm is applied to an experimental reciprocal space map measured using high resolution X-ray diffraction from an array of silicon lines and the obtained component of the displacement field is in very good agreement with the one calculated using a finite element model.

cond-mat.mtrl-sci↗