arXiv subjects

Ofer Kfir

Publications and source records attributed to Ofer Kfir.

At least 19 recordsLinked to original sources

arXiv2025

Cathodoluminescence Enhancement Mechanisms in Silica Microspheres

Cathodoluminescence (CL) enables optical-frequency analysis of samples with nanometer resolutions, originating from the interaction of a focused electron beam with radiative electronic states, or directly with the optical modes of the sample. Here we decompose the various mechanisms underlying CL generation and emission from an archetype spherical resonator using its spectral, angular and spatially resolved features. We investigate radiation of optical whispering-gallery modes in regimes of coherent and incoherent luminescence. The use of different experimental regimes allows us to disentangle the different contributions to the CL in spheres, namely, photon absorption, generation and radiative leakage, and conclude that the photon generation occurs precisely on the sphere's surface. In addition, the spheres serve as high-NA collimating lenses for CL, resulting in mode quality unprecedented for CL in free space. We believe that such collimated and directed CL in free space will enhance existing quantum measurements of CL and facilitate new ones, such as high-rate electron-photon entangled pairs, CL from quantum emitters, and homodyne analysis of CL.

physics.optics↗

arXiv2025

Elastic Quantum Coupling Between Free Electrons and Photons

The quantum coupling between free-electrons and photons enables applying quantum optics techniques in electron microscopy. Here, we formulate the elastic electron-photon quantum coupling and its possible implications. Our analysis shows that when an electron traverses the field of an optical cavity, it induces a phase shift onto its confined photonic mode, which can be quantified as a refractive index of a free electron. This principle can be applied to counting electrons in a beam without changing its quantum states. The elastic scattering operator forms an electron-counting dispersive Hamiltonian for electron-photon systems within electron microscope, and it could enable quantum- and sub-shot-noise sensing and imaging at the {\AA}-scale.

quant-ph↗

arXiv2025

Revealing domain wall stability during ultrafast demagnetization

The ultrafast control of nanoscale spin textures such as magnetic domain walls or skyrmions is essential for advancing high-speed, high-density spintronics. However, imaging their dynamics will require a technique that combines nanometer spatial and femtosecond temporal resolution. Introducing ultrafast sub-wavelength imaging in the extreme ultraviolet, we track domain wall properties during ultrafast demagnetization in ferro- and ferrimagnetic thin films. We reveal that domain walls remain invariant in position, shape, and width, down to a demonstrated sub-nanometer precision, for up to 50% demagnetization. Stronger excitation causes stochastic nanoscale domain switching. This previously unobservable robustness of laser-excited domain walls highlights the localized nature of photoinduced demagnetization and presents both challenges and opportunities for all-optical magnetic control. The presented technique can be generalized to directly probe nanoscale dynamics in spintronic materials and devices.

cond-mat.mtrl-sci↗

arXiv2025

Light's symmetry, asymmetry, and their role in nonlinear optics and ultrafast phenomena

The analysis of symmetries is extremely useful across science. In Physics, symmetries are used to derive conservation laws and selection rules for transitions in interacting systems. In the early days of nonlinear optics (NLO), symmetries were used to formulate a set of rules for photonic processes according to the medium's symmetries that are reflected in the NLO coefficient tensor. While this approach was believed to be complete and closed, the field has recently reignited as multi-color ultrashort laser pulses with tailored polarization and spatiotemporal structures become standard in NLO. A more complete theory has been recently emerging, which aims to incorporate all possible dynamical degrees of freedom of light: spin and orbital angular momentum, spatial structure, time-dependent polarizations, temporal envelopes, etc., in addition to the symmetries of the medium. This theoretical development is also accompanied by experimental advances that rely on tailored light beams that can now be generated with ever-increasing complexity, including topologies in real and a variety of synthetic dimensions, carrying poly-chromatic carrier waves, time-dependent varying angular momenta, local-chirality, and more. The nonlinear interactions between light fields with unique symmetries (or asymmetries) and matter is especially appealing, since that holds the key for developing new ultrafast spectroscopies with sub-femtosecond resolution, for exerting exact control over matter, and improving our fundamental understanding of how light and matter interact. We review these recent advances in this expanding field, focusing on the theory, its implications, and seminal experiments. We aim to establish a comprehensive database of symmetries and selection rules governing NLO light-matter interactions within the emerging new formalism, and invite the scientific community to contribute to this effort.

physics.optics↗

arXiv2025

Roadmap for Quantum Nanophotonics with Free Electrons

Over the past century, continuous advancements in electron microscopy have enabled the synthesis, control, and characterization of high-quality free-electron beams. These probes carry an evanescent electromagnetic field that can drive localized excitations and provide high-resolution information on material structures and their optical responses, currently reaching the sub-{\aa}ngstr\"om and few-meV regime. Moreover, combining free electrons with pulsed light sources in ultrafast electron microscopy adds temporal resolution in the sub-femtosecond range while offering enhanced control of the electron wave function. Beyond their exceptional capabilities for time-resolved spectromicroscopy, free electrons are emerging as powerful tools in quantum nanophotonics, on par with photons in their ability to carry and transfer quantum information, create entanglement within and with a specimen, and reveal previously inaccessible details on nanoscale quantum phenomena. This Roadmap outlines the current state of this rapidly evolving field, highlights key challenges and opportunities, and discusses future directions through a collection of topical sections prepared by leading experts.

cond-mat.mes-hall↗

arXiv2024

On spatial electron-photon entanglement

Free electron beams and their quantum coupling with photons is attracting a rising interest due to the basic questions it addresses and the cutting-edge technology these particles are involved in, such as microscopy, spectroscopy, and quantum computation. This work investigates theoretically the concept of electron-photon coupling in the spatial domain. Their interaction is discussed as a thought experiment of spontaneous photon emission from a dual-path free-electron (free-e) beam. We discuss a retro-causal paradox that may emerge from naively extending perceptions of single-path e-photon coupling to transversely separated paths, and its resolution through the physics of two-particle interference. The precise spatial control of electrons and photons within e-microscopes enables manipulation of their respective states, thus, such instruments can harness position-encoded free-e qubits for novel quantum sensing and the transfer of quantum information.

physics.gen-ph↗

arXiv2023

Sub-Terahertz Nearfields for Electron-Pulse Compression

The advent of ultrafast science with pulsed electron beams raised the need in controlling the temporal features of the electron pulses. One promising suggestion is the nano-selective quantum optics with multi-electrons, which scales quadratically with the number of electrons within the coherence time of the quantum system. Terahertz (THz) radiation from optical nonlinear crystals is an attractive methodology to generate the rapidly varying electric fields necessary for electron compression, with an advantage of an inherent temporal locking to laser-triggered electrons, such as in untrafast electron microscopes. Longer (picosecond-) pulses require sub-THz field for their compression, however, the generation of such low frequencies require pumping with energetic optical pulses and their focusability is fundamentally limited by their mm-wavelength. This work proposes electron-pulse compression with sub-THz fields directly in the vicinity of their dipolar origin, thereby avoiding mediation through radiation. We analyze the merits of nearfields for compression of slow electrons particularly in challenging regimes for THz radiation, such as small numerical apertures, micro-joule-level optical pump pulses, and low frequencies. This sheme can be implemented within the tight constraints of electron microscopes and reach fiels of a few kV/cm below 0.1 THz at high repetition rates. Our paradigm offers a realistic approach for controlling electron pulses spatially and temporally in many experiments, opening the path of flexible multi-electron manipulation for analytic and quantum sciences.

physics.optics↗

arXiv2022

Quantum state heralding using photonic integrated circuits with free electrons

Recently, integrated photonic circuits have brought new capabilities to electron microscopy and been used to demonstrate efficient electron phase modulation and electron-photon correlations. Here, we quantitatively analyze the feasibility of high fidelity and high purity quantum state heralding using a free electron and a photonic integrated circuit with parametric coupling, and propose schemes to shape useful electron and photonic states in different application scenarios. Adopting a dissipative quantum electrodynamics treatment, we formulate a framework for the coupling of free electrons to waveguide spatial-temporal modes. To avoid multimode-coupling induced state decoherence, we show that with proper waveguide design, the interaction can be reduced to a single-mode coupling to a quasi-TM00 mode. In the single-mode coupling limit, we go beyond the conventional state ladder treatment, and show that the electron-photon energy correlations within the ladder subspace can still lead to a fundamental purity and fidelity limit on complex optical and electron state preparations through heralding schemes. We propose applications that use this underlying correlation to their advantage, but also show that the imposed limitations for general applications can be overcome by using photonic integrated circuits with an experimentally feasible interaction length, showing its promise as a platform for free-electron quantum optics.

quant-ph↗

arXiv2021

Chiral high-harmonic generation and spectroscopy on solid surfaces using polarization-tailored strong fields

Strong-field methods in solids enable new strategies for ultrafast nonlinear spectroscopy and provide all-optical insights into the electronic properties of condensed matter in reciprocal and real space. Additionally, solid-state media offers unprecedented possibilities to control high-harmonic generation using modified targets or tailored excitation fields. Here we merge these important points and demonstrate circularly-polarized high-harmonic generation with polarization-matched excitation fields for spectroscopy of chiral electronic properties at surfaces. The sensitivity of our approach is demonstrated for structural helicity and termination-mediated ferromagnetic order at the surface of silicon-dioxide and magnesium oxide, respectively. Circularly polarized radiation emanating from a solid sample now allows to add basic symmetry properties as chirality to the arsenal of strong-field spectroscopy in solids. Together with its inherent temporal (femtosecond) resolution and non-resonant broadband spectrum, the polarization control of high harmonics from condensed matter can illuminate ultrafast and strong field dynamics of surfaces, buried layers or thin films.

physics.optics↗

arXiv2021

Modulation of Cathodoluminescence Emission by Interference with External Light

Spontaneous processes triggered in a sample by free electrons are commonly regarded as incoherent, and therefore unable to interfere with external light sources. Here, we challenge this concept by showing through first-principles theory that light and free-electron pulses can interfere when interacting with a nanostructure, giving rise to a modulation in the spectral distribution of the cathodoluminescence light emission that is strongly dependent on the electron wave function. Specifically, for a temporally focused electron, cathodoluminescence can be cancelled upon illumination with a spectrally modulated dimmed laser that is phase-locked relative to the electron density profile. We illustrate this idea with realistic simulations under attainable conditions in currently available ultrafast electron microscopes. We further argue that the interference between excitations produced by light and free electrons opens a new window to manipulate the ultrafast materials response by combining the spectral and temporal selectivity of the light with the atomic resolution of electron beams.

physics.optics↗

arXiv2020

Implementing strong interference in ultrathin film top absorbers for tandem solar cells

Strong interference in ultrathin film semiconductor absorbers on metallic back reflectors has been shown to enhance the light harvesting efficiency of solar cell materials. However, metallic back reflectors are not suitable for tandem cell configurations because photons cannot be transmitted through the device. Here, we introduce a method to implement strong interference in ultrathin film top absorbers in a tandem cell configuration through use of distributed Bragg reflectors (DBRs). We showcase this by designing and fabricating a photoelectrochemical-photovoltaic (PEC-PV) stacked tandem cell in a V-shaped configuration where short wavelength photons are reflected back to the photoanode material (hematite, Fe2O3), whereas long wavelength photons are transmitted to the bottom silicon PV cell. We employ optical simulations to determine the optimal thicknesses of the DBR layers and the V-shape angle to maximize light absorption in the ultrathin (10 nm thick) hematite film. The DBR spectral response can be tailored to allow for a more than threefold enhancement in absorbed photons compared to a layer of the same thickness on transparent current collectors. Using a DBR to couple a bottom silicon PV cell with an ultrathin hematite top PEC cell, we demonstrate unassisted solar water splitting and show that DBRs can be designed to enhance strong interference in ultrathin films while enabling stacked tandem cell configuration.

physics.optics↗

arXiv2020

Optical coherence transfer mediated by free electrons

We investigate theoretically the quantum-coherence properties of the cathodoluminescence (CL) emission produced by a temporally modulated electron beam. Specifically, we consider the quantum-optical correlations of CL from electrons that are previously shaped by a laser field. The main prediction here is the presence of phase correlations between the emitted CL field and the electron-modulating laser, even though the emission intensity and spectral profile are independent of the electron state. In addition, the coherence of the CL field extends to harmonics of the laser frequency. Since electron beams can be focused to below one Angstrom, their ability to transfer optical coherence could enable ultra precise excitation, manipulation, and spectroscopy of nanoscale quantum systems.

quant-ph↗

arXiv2020

Ultrafast high-harmonic nanoscopy of magnetization dynamics

Light-induced magnetization changes, such as all-optical switching, skyrmion nucleation, and intersite spin transfer, unfold on temporal and spatial scales down to femtoseconds and nanometers, respectively. Pump-probe spectroscopy and diffraction studies indicate that spatio-temporal dynamics may drastically affect the non-equilibrium magnetic evolution. Yet, direct real-space magnetic imaging on the relevant timescale has remained challenging. Here, we demonstrate ultrafast high-harmonic nanoscopy employing circularly polarized high-harmonic radiation for real-space imaging of femtosecond magnetization dynamics. We observe the reversible and irreversible evolution of nanoscale spin textures following femtosecond laser excitation. Specifically, we map quenched magnetic domains and localized spin structures in Co/Pd multilayers with a sub-wavelength spatial resolution down to 16 nm, and strobosocopically trace the local magnetization dynamics with 40 fs temporal resolution. Our approach enables the highest spatio-temporal resolution of magneto-optical imaging to date. Facilitating ultrafast imaging with an extreme sensitivity to various microscopic degrees of freedom expressed in chiral and linear dichroism, we envisage a wide range of applications spanning magnetism, phase transitions, and carrier dynamics.

physics.optics↗

arXiv2020

Probing chirality with inelastic electron-light scattering

Circular dichroism spectroscopy is an essential technique for understanding molecular structure and magnetic materials, but spatial resolution is limited by the wavelength of light, and sensitivity sufficient for single-molecule spectroscopy is challenging. We demonstrate that electrons can efficiently measure the interaction between circularly polarized light and chiral materials with deeply sub-wavelength resolution. By scanning a nanometer-sized focused electron beam across an optically-excited chiral nanostructure and measuring the electron energy spectrum at each probe position, we produce a high-spatial-resolution map of near-field dichroism. This technique offers a nanoscale view of a fundamental symmetry and could be employed as "photon staining" to increase biomolecular material contrast in electron microscopy.

physics.optics↗

arXiv2019

Controlling free electrons with optical whispering-gallery modes

Free-electron beams serve as uniquely versatile probes of microscopic structure and composition, and have repeatedly revolutionized atomic-scale imaging, from solid-state physics to structural biology. Over the past decade, the manipulation and interaction of electrons with optical fields has seen significant progress, enabling novel imaging methods, schemes of near-field electron acceleration, and culminating in 4D microscopy techniques with both high temporal and spatial resolution. However, weak coupling strengths of electron beams to optical excitations are a standing issue for existing and emerging applications of optical free-electron control. Here, we demonstrate phase matched near-field coupling of a free-electron beam to optical whispering gallery modes of dielectric microresonators. The cavity-enhanced interaction with these optically excited modes imprints a strong phase modulation on co-propagating electrons, which leads to electron-energy sidebands up to hundreds of photon orders and a spectral broadening of 700 eV. Mapping the near-field interaction with ultrashort electron pulses in space and time, we trace the temporal ring-down of the microresonator following a femtosecond excitation and observe the cavity's resonant spectral response. Resonantly enhancing the coupling of electrons and light via optical cavities, with efficient injection and extraction, can open up novel applications such as continuous-wave acceleration, attosecond structuring, and real-time all-optical electron detection.

physics.optics↗

arXiv2019

Entanglements of electrons and cavity-photons in the strong coupling regime

This work sets a road-map towards an experimental realization of strong coupling between free-electrons and photons, and analytically explores entanglement phenomena that emerge in this regime. The proposed model unifies the strong-coupling predictions with known electron-photon interactions. Additionally, this work predicts a non-Columbic entanglement between freely propagating electrons. Since strong-coupling can map entanglements between photon pairs onto photon-electron pairs, it may harness electron beams for quantum communication, thus far exclusive to photons.

quant-ph↗

arXiv2017

Nanoscale Magnetic Imaging using Circularly Polarized High-Harmonic Radiation

This work demonstrates nanoscale magnetic imaging using bright circularly polarized high-harmonic radiation. We utilize the magneto-optical contrast of worm-like magnetic domains in a Co/Pd multilayer structure, obtaining quantitative amplitude and phase maps by lensless imaging. A diffraction-limited spatial resolution of 49 nm is achieved with iterative phase reconstruction enhanced by a holographic mask. Harnessing the unique coherence of high harmonics, this approach will facilitate quantitative, element-specific and spatially-resolved studies of ultrafast magnetization dynamics, advancing both fundamental and applied aspects of nanoscale magnetism.

physics.optics↗

arXiv2014

High-order harmonics with frequency-varying polarization within each harmonic

We predict high-order harmonics in which the polarization within the spectral bandwidth of each harmonic varies continuously and significantly. For example, the interaction of counter-rotating circularly-polarized bichromatic drivers having close central frequencies with isotropic gas leads to the emission of polarization-fan harmonics which are nearly circularly-polarized in one tail of the harmonic peak, linear in the center of the peak and nearly circular with the opposite helicity in the opposite tail. Polarization fan harmonics are obtained as a result of multiple (at least two) head-on recollisions of electrons with their parent ions occurring from different angles. The process can be phase-matched using standard methods (e.g. pressure tuning phase matching) and maintains the single-atom polarization property through propagation. These polarization-fan harmonics may be used for exploring non-repetitive ultrafast chiral phenomena, e.g. dynamics of magnetic domains, in a single shot

physics.optics↗