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Olajumoke Oluwatobiloba Emmanuel

Publications and source records attributed to Olajumoke Oluwatobiloba Emmanuel.

5 recordsLinked to original sources

Dual Charge-Density-Waves in Two-dimensional DyTe3 and Their Distinct Impacts on Magneto-Transport Properties

Charge-density-waves (CDWs) are macroscopic quantum states defined by periodic modulations in electronic charge density coupled with lattice distortions. Despite significant research efforts, the evolution of electromagnetic transport properties in the presence of CDWs remains largely unexplored. Here, we report the effects of two orthogonal CDWs (CDW1 and CDW2) coexisting at low-temperature in DyTe3 on its electronic transport properties. Importantly, we find that while no clear magnetotransport anomaly is resolved across CDW1 transition under the present experimental conditions, the emergence of CDW2 drives a drastic enhancement in magnetoresistance and a multiband-governed nonlinear Hall response. These results demonstrate that CDW1 and CDW2 in DyTe3 are fundamentally different and impact its electronic transport in qualitatively distinct ways, establishing DyTe3 as a model system for understanding the transport consequences of multiple CDWs in quasi-two-dimensional materials.

cond-mat.str-el↗

Angular-Dependent Thermal Hall Effect in a Honeycomb Magnet: Disentangling Kitaev and Dzyaloshinskii-Moriya Interactions

Layered honeycomb magnets have garnered significant attention recently for their exotic quantum phenomena due to the potential anisotropic, bond-dependent Kitaev interactions. However, distinguishing the roles of Kitaev interactions and the symmetry-allowed Dzyaloshinskii-Moriya interaction (DMI) remains challenging, since both mechanisms may lead to similar magnetic excitations and thermal transport properties. To tackle this challenge, using a ferromagnetic honeycomb insulator VI3 as a model system, we systematically study the angular-dependent thermal Hall conductivity Kxy(θ, Φ) with both out-of-plane (θ) and in-plane (Φ) magnetic field rotations. Our results reveal a persistent thermal Hall response for both out-of-plane and in-plane rotating magnetic fields, devoid of the sign-reversal patterns characteristic of Kitaev physics. Instead, quantitative analysis shows that the angular dependent Kxy(θ, Φ) is governed by the projection between the magnetic moment and a tilted DM vector containing both out-of-plane and in-plane components. These results not only establish the DMI-driven topological magnetic excitations as the origin of the thermal Hall response in VI3 but also highlight the angular-dependent thermal Hall effect measurements as an effective approach for distinguishing competing interactions in quantum magnets.

cond-mat.str-el↗

Large Anomalous and Topological Hall Effect and Nernst Effect in a Dirac Kagome Magnet Fe3Ge

The search for kagome magnets with unconventional magnetic and electronic properties has gained significant attention in recent years. We report the magnetic, electronic, and thermoelectric properties of Fe3Ge single crystals, where the Fe atoms form a slightly distorted kagome lattice. Fe3Ge exhibits a large anomalous Hall effect and anomalous Nernst effect. The anomalous transverse thermoelectric conductivity reaches about 4.6 A m^-1 K^-1, exceeding values reported for conventional ferromagnets and most topological ferromagnets. First-principles calculations indicate that these transport responses are primarily governed by intrinsic mechanisms, highlighting the dominant role of Berry curvature arising from massive Dirac gaps in momentum space. In addition, we observe a topological Hall resistivity of about 0.9 microOhm cm and a topological Nernst coefficient of 1.2 microvolt K^-1, which are attributed to the Berry phase associated with field-induced scalar spin chirality. These findings demonstrate the combined influence of Berry phases in both momentum and real space, establishing Fe3Ge as a promising candidate for room-temperature transverse thermoelectric applications.

cond-mat.mtrl-sci↗

ErMn$_6$Sn$_6$: A Promising Kagome Antiferromagnetic Candidate for Room-Temperature Nernst Effect-based thermoelectrics

The Nernst effect, the generation of a transverse electric voltage in the presence of longitudinal thermal gradient, has garnered significant attention in the realm of magnetic topological materials due to its superior potential for thermoelectric applications. In this work, we investigate electronic and thermoelectric transport properties of a Kagome magnet ErMn$_6$Sn$_6$, a compound showing an incommensurate antiferromagnetic phase followed by a ferrimagnetic phase transition upon cooling. We show that in the antiferromagnetic phase ErMn$_6$Sn$_6$ exhibits both topological Nernst effect and anomalous Nernst effect, analogous to the electric Hall effects, with the Nernst coefficient reaching 1.71 uV/K at 300 K and 3 T. This value surpasses that of most of previously reported state-of-the-art canted antiferromagnetic materials and is comparable to recently reported other members of RMn$_6$Sn$_6$ (R = rare-earth, Y, Lu, Sc) compounds, which makes ErMn$_6$Sn$_6$ a promising candidate for advancing the development of Nernst effect-based thermoelectric devices.

cond-mat.mtrl-sci↗

Giant Nernst Angle in Self-Intercalated van der Waals Magnet Cr$_{1.25}$Te$_2$

The discovery of two-dimensional van der Waals (vdW) magnetic materials has propelled advancements in technological devices. The Nernst effect, which generates a transverse electric voltage in the presence of a longitudinal thermal gradient, shows great promise for thermoelectric applications. In this work, we report the electronic and thermoelectric transport properties of Cr$_{1.25}$Te$_2$, a layered self-intercalated vdW material which exhibits an antiferromagnetic ordering at TN ~ 191 K followed by a ferromagnetic-like phase transition at TC ~171 K. We observe a prominent topological Hall effect and topological Nernst effect between TC and TN, which is ascribable to non-coplanar spin textures inducing a real-space Berry phase due to competing ferromagnetic and antiferromagnetic interactions. Furthermore, we show that Cr$_{1.25}$Te$_2$ exhibits a substantial anomalous Nernst effect, featuring a giant Nernst angle of ~37% near TC and a maximum Nernst thermoelectric coefficient of 0.52 uV/K. These results surpass those of conventional ferromagnets and other two-dimensional vdW materials, highlighting Cr$_{1.25}$Te$_2$ as a promising candidate for advanced thermoelectric devices based on the Nernst effect.

cond-mat.mtrl-sci↗