arXiv subjects

Oleksandr V. Pylypovskyi

Publications and source records attributed to Oleksandr V. Pylypovskyi.

At least 19 recordsLinked to original sources

arXiv2026

Local multiferroic ordering at room temperature in collinear magnetoelectric antiferromagnets induced by flexo-Zeeman coupling

Spin-driven multiferroicity attracts significant interest due to its tunability and inherently strong magnetoelectric coupling. While this mechanism induces sizeable electric polarization, it typically occurs at low temperatures and in complex materials. In the simple oxide, the magnetoelectric antiferromagnet Cr$_2$O$_3$, we experimentally demonstrate the existence of specific domain walls that act as room-temperature multiferroic regions. This behavior stems from an anisotropic crystal-symmetry-dependent mechanism of exchange origin, which is applicable to a broad class of bipartite antiferromagnets. The key signature is the magnetization occurring at antiferromagnetic textures, driven by the flexo-Zeeman interaction. These findings establish a foundation for exploring high-temperature spin-driven multiferroicity for magnetoelectric spin-orbit memory and logic applications.

cond-mat.mtrl-sci↗

arXiv2026

Piezomagnetic Switching of Nonvolatile Antiferromagnetic States

Prospective spintronic memory and logic devices will benefit from the negligible stray field and ultrafast magnetic dynamics inherent to antiferromagnets [1]. However, realizing isothermal, nonvolatile, and deterministic switching of antiferromagnetic states remains a key challenge [2, 3]. Here, we propose a piezomagnetic writing scheme in triangular Mn3Ir-based memory cells, with readout achieved via the exchange bias effect. Our approach enables deterministic and nonvolatile switching of the antiferromagnetic states, which exhibit exceptional robustness against external perturbations. The switching mechanism is ascribed to piezomagnetic effect of Mn3Ir combined with the interfacial Dzyaloshinskii-Moriya interaction at the antiferromagnet-ferromagnet interface. This scheme overcomes the speed limitations imposed by conventional isothermal methods based on isothermal crystallization mechanism [4]. Our findings highlight the potential of piezomagnetic effects in designing advanced spintronic devices, providing an efficient pathway for manipulating antiferromagnetic states and developing energy-efficient memory technology.

cond-mat.mtrl-sci↗

arXiv2025

Curvilinear magnonic crystal based on 3D hierarchical nanotemplates

Curvilinear magnetic nanostructures enable control of magnetization dynamics through geometry-induced anisotropy and chiral interactions as well as magnetic field modulation. In this work, we report a curvilinear magnonic crystal based on large-area square arrays of truncated nanospikes fabricated by conformal coating of 3D hierarchical templates with permalloy thin films. Brillouin light scattering spectroscopy reveals anisotropic band structure with multiple dispersive and folded Bloch-type dispersive spin-wave modes as well as non-dispersive modes exhibiting direction-dependent frequency shifts and intensity asymmetries along lattice principal axes. Finite element micromagnetic simulations indicate that curvature-induced variations of the demagnetizing field govern the magnonic response, enabling the identification of modes propagating in nanochannels and other localized on nanospike apexes or along the ridges connecting adjacent nanospikes. The combination of geometric curvature and optical probing asymmetry produces directional dependence of magnonic bands, establishing 3D hierarchical templates as a versatile platform for curvature-engineered magnonics.

cond-mat.str-el↗

arXiv2025

Field-programmable dynamics in a soft magnetic actuator enabling true random number generation and reservoir computing

Complex and even chaotic dynamics, though prevalent in many natural and engineered systems, has been largely avoided in the design of electromechanical systems due to concerns about wear and controlability. Here, we demonstrate that complex dynamics might be particularly advantageous in soft robotics, offering new functionalities beyond motion not easily achievable with traditional actuation methods. We designed and realized resilient magnetic soft actuators capable of operating in a tunable dynamic regime for tens of thousands cycles without fatigue. We experimentally demonstrated the application of these actuators for true random number generation and stochastic computing. {W}e validate soft robots as physical reservoirs capable of performing Mackey--Glass time series prediction. These findings show that exploring the complex dynamics in soft robotics would extend the application scenarios in soft computing, human-robot interaction and collaborative robots as we demonstrate with biomimetic blinking and randomized voice modulation.

cs.RO↗

arXiv2024

Magnetic Vortex Dynamics on a Spherical Cap

By tailoring geometrical properties of magnetic nanocap structures, new possibilities appear to control its magnetic properties, such as the dynamics of magnetic vortices. Here, we develop an approach to describe dynamics of magnetic vortices on a spherical cap. Analytic results for the gyrofrequency of the vortex state are in a good agreement with micromagnetic simulations.

cond-mat.mes-hall↗

arXiv2024

Manipulation by magnetic frustration in ferrotoroidal spin chains via curvature and torsion

Geometric effects in curvilinear nanomagnets can enable chiral, anisotropic and even magnetoelectric responses. Here, we study the effects of magnetic frustration in curvilinear (quasi-)1D magnets represented by spin chains arranged along closed space curves of constant torsion. Considering the cases of easy- and hard-axis anisotropy in ferro- and antiferromagnetic samples, we determine their ground states and analyze the related magnetoelectric multipoles. A constant torsion along the chain results in alternating regions of high and low curvature, facilitating the spin spiral state perturbed by the (anti)periodic boundary conditions on the magnetic order parameter. While easy-axis ferromagnetic chains develop a purely toroidal configuration with the magnetic toroidal moment oriented along the geometry symmetry axis, hard-axis antiferromagnetic chains support multiple magnetic toroidal domains. Our findings suggest that tailoring curvature and torsion of a spin chain enables a new physical mechanism for magnetic frustration, which can be observed in the inhomogeneity of the magnetic order parameter and in the local ferrotoroidic responses.

cond-mat.mes-hall↗

arXiv2024

Antiferromagnetic nanoscale bit arrays of magnetoelectric Cr$_2$O$_3$ thin films

Magnetism of oxide antiferromagnets (AFMs) has been studied in single crystals and extended thin films. The properties of AFM nanostructures still remain underexplored. Here, we report on the fabrication and magnetic imaging of granular 100-nm-thick magnetoelectric Cr$_2$O$_3$ films patterned in circular bits with diameters ranging from 500 down to 100 nm. With the change of the lateral size, the domain structure evolves from a multidomain state for larger bits to a single domain state for the smallest bits. Based on spin-lattice simulations, we show that the physics of the domain pattern formation in granular AFM bits is primarily determined by the energy dissipation upon cooling, which results in motion and expelling of AFM domain walls of the bit. Our results provide a way towards the fabrication of single domain AFM-bit-patterned memory devices and the exploration of the interplay between AFM nanostructures and their geometric shape.

cond-mat.mtrl-sci↗

arXiv2023

Surface-symmetry-driven Dzyaloshinskii--Moriya interaction and canted ferrimagnetism in collinear magnetoelectric antiferromagnet Cr$_2$O$_3$

Antiferromagnets are normally thought of as materials with compensated magnetic sublattices. This adds to their technological advantages but complicates readout of the antiferromagnetic state. We demonstrate theoretically the existence of a Dzyaloshinskii-Moriya interaction (DMI) which is determined by the magnetic symmetry classes of Cr$_2$O$_3$ surfaces with an in-plane magnetic easy axis. The DMI explains a previously predicted out-of-plane magnetization at the nominally compensated surfaces of chromia, leading to a surface-localized canted ferrimagnetism. This is in agreement with magnetotransport measurements and with density functional theory predictions which further allow us to quantify the strength of DMI. The temperature dependence of the transversal resistance for these planes shows distinct behavior in comparison with that of the Cr$_2$O$_3$ $c$ plane, which we attribute to the influence of DMI. Our work provides a framework to analyze surface-driven phenomena in antiferromagnets, and motivates the use of nominally compensated chromia surfaces for antiferomagnetic spintronics and magnonics.

cond-mat.str-el↗

arXiv2022

Field-induced spin reorientation transitions in antiferromagnetic ring-shaped spin chains

Easy axis antiferromagnets are robust against external magnetic fields of moderate strength. Spin reorientations in strong fields can provide an insight into more subtle properties of antiferromagnetic materials, which are often hidden by their high ground state symmetry. Here, we investigate theoretically effects of curvature in ring-shaped antiferromagnetic achiral anisotropic spin chains in strong magnetic fields. We identify the geometry-governed helimagnetic phase transition above the spin-flop field between vortex and onion states. The curvature-induced Dzyaloshinskii-Moriya interaction results in the spin-flop transition being of first- or second-order depending on the ring curvature. Spatial inhomogeneity of the Néel vector in the spin-flop phase generates weak ferromagnetic response in the plane perpendicular to the applied magnetic field. Our work contributes to the understanding of the physics of curvilinear antiferromagnets in magnetic fields and guides prospective experimental studies of geometrical effects relying on spin-chain-based nanomagnets.

cond-mat.mes-hall↗

arXiv2022

Circular stripe domains and cone state vortices in disk-shaped exchange coupled magnetic heterostructures

Vertically stacked exchange coupled magnetic heterostructures of cylindrical geometry can host complex noncolinear magnetization patterns. By tuning the interlayer exchange coupling between a layer accommodating magnetic vortex state and an out-of-plane magnetized layer, one can efficiently realize new topological chiral textures such as cone state vortices and circular stripe domains. We study how the number of circular stripes can be controlled by both the interlayer exchange coupling and the sample geometrical parameters. By varying geometrical parameters, a continuous phase transition between the homogeneous state, cone state vortex, circular stripe domains, and the imprinted vortex takes place, which is analysed by full scale micromagnetic simulations. The analytical description provides an intuitive pictures of the magnetization textures in each of these phases. The possibility to realize switching between different states allows for engineering magnetic textures with possible applications in spintronic devices.

cond-mat.mes-hall↗

arXiv2022

Impact of curvature-induced Dzyaloshinskii-Moriya interaction on magnetic vortex texture in spherical caps

Geometric curvature of nanoscale magnetic shells brings about curvature-induced anisotropy and Dzyaloshinskii-Moriya interaction (DMI). Here, we derive equations to describe the profile of the magnetic vortex state in a spherical cap. We demonstrate that the azimuthal component of magnetization acquires a finite tilt at the edge of the cap, which results in the increase of the magnetic surface energy. This is different compared to the case of a closed spherical shell, where symmetry of the texture does not allow any tilt of magnetization at the equator of the sphere. Furthermore, we analyze the size of the vortex core in a spherical cap and show that the presence of the curvature-induced DMI leads to the increase of the core size independent of the product of the circulation and polarity of the vortex. This is in contrast to the case of planar disks with intrinsic DMI, where the preferred direction of circulation as well as the decrease or increase of the size of vortex core is determined by the sign of the product of the circulation and polarity with respect to the sign of the constant of the intrinsic DMI.

cond-mat.mes-hall↗

arXiv2021

Nematic versus ferromagnetic shells: new insights in curvature-induced effects

Within the framework of continuum theory, we draw a parallel between ferromagnetic materials and nematic liquid crystals confined on curved surfaces, which are both characterized by local interaction and anchoring potentials. We show that the extrinsic curvature of the shell combined with the out-of-plane component of the director field gives rise to chirality effects. This interplay produces an effective energy term reminiscent of the chiral term in cholesteric liquid crystals, with the curvature tensor acting as a sort of anisotropic helicity. We discuss also how the different nature of the order parameter, a vector in ferromagnets and a tensor in nematics, yields different textures on surfaces with the same topology as the sphere. In particular, we show that the extrinsic curvature governs the ground state configuration on a nematic spherical shell, favouring two antipodal disclinations of charge +1 on small particles and four $+1/2$ disclinations of charge located at the vertices of a square inscribed in a great circle on larger particles.

cond-mat.soft↗

arXiv2021

Curvature-driven homogeneous Dzyaloshinskii-Moriya interaction and emergent weak ferromagnetism in anisotropic antiferromagnetic spin chains

Chiral antiferromagnets are currently considered for broad range of applications in spintronics, spin-orbitronics and magnonics. In contrast to the established approach relying on materials screening, the anisotropic and chiral responses of low-dimensional antifferromagnets can be tailored relying on the geometrical curvature. Here, we consider an achiral, anisotropic antiferromagnetic spin chain and demonstrate that these systems possess geometry-driven effects stemming not only from the exchange interaction but also from the anisotropy. Peculiarly, the anisotropy-driven effects are complementary to the curvature effects stemming from the exchange interaction and rather strong as they are linear in curvature. These effects are responsible for the tilt of the equilibrium direction of vector order parameters and the appearance of the homogeneous Dzyaloshinskii-Moriya interaction. The latter is a source of the geometry-driven weak ferromagnetism emerging in curvilinear antiferromagnetic spin chains. Our findings provide a deeper fundamental insight into the physics of curvilinear antiferromagnets beyond the $σ$-model and offer an additional degree of freedom in the design of spintronic and magnonic devices.

cond-mat.str-el↗

arXiv2021

Boundary conditions for the Néel order parameter in a chiral antiferromagnetic slab

Understanding of the interaction of antiferromagnetic solitons including domain walls and skyrmions with boundaries of chiral antiferromagnetic slabs is important for the design of prospective antiferromagnetic spintronic devices. Here, we derive the transition from spin lattice to micromagnetic nonlinear $σ$-model with the corresponding boundary conditions for a chiral cubic G-type antiferromagnet and analyze the impact of the slab boundaries and antisymmetric exchange (Dzyaloshinskii--Moriya interaction) on the vector order parameter. We apply this model to evaluate modifications of antiferromagnetic domain walls and skyrmions upon interaction with boundaries for different strengths of the antisymmetric exchange. Due to the presence of the antisymmetric exchange, both types of antiferromagnetic solitons become broader when approaching the boundary and transform to a mixed Bloch--Néel structure. Both textures feel the boundary at the distance of about 5 magnetic lengths. In this respect, our model provides design rules for antiferromagnetic racetracks, which can support bulk-like properties of solitons.

cond-mat.mes-hall↗

arXiv2020

Nanoscale mechanics of antiferromagnetic domain walls

Antiferromagnets offer remarkable promise for future spintronics devices, where antiferromagnetic order is exploited to encode information. The control and understanding of antiferromagnetic domain walls (DWs) - the interfaces between domains with differing order parameter orientations - is a key ingredient for advancing such antiferromagnetic spintronics technologies. However, studies of the intrinsic mechanics of individual antiferromagnetic DWs remain elusive since they require sufficiently pure materials and suitable experimental approaches to address DWs on the nanoscale. Here we nucleate isolated, 180° DWs in a single-crystal of Cr$_2$O$_3$, a prototypical collinear magnetoelectric antiferromagnet, and study their interaction with topographic features fabricated on the sample. We demonstrate DW manipulation through the resulting, engineered energy landscape and show that the observed interaction is governed by the DW's elastic properties. Our results advance the understanding of DW mechanics in antiferromagnets and suggest a novel, topographically defined memory architecture based on antiferromagnetic DWs.

cond-mat.mes-hall↗

arXiv2020

Curvilinear one-dimensional antiferromagnets

Antiferromagnets host exotic quasiparticles, support high frequency excitations and are key enablers of the prospective spintronic and spin-orbitronic technologies. Here, we propose a concept of a curvilinear antiferromagnetism where material responses can be tailored by a geometrical curvature without the need to adjust material parameters. We show that an intrinsically achiral one-dimensional (1D) curvilinear antiferromagnet behaves as a chiral helimagnet with geometrically tunable Dzyaloshinskii--Moriya interaction (DMI) and orientation of the Néel vector. The curvature-induced DMI results in the hybridization of spin wave modes and enables a geometrically-driven local minimum of the low frequency branch. This positions curvilinear 1D antiferromagnets as a novel platform for the realization of geometrically tunable chiral antiferromagnets for antiferromagnetic spin-orbitronics and fundamental discoveries in the formation of coherent magnon condensates in the momentum space.

cond-mat.mes-hall↗

arXiv2020

Unidirectional tilt of domain walls in equilibrium in biaxial stripes with Dzyaloshinskii-Moriya interaction

The orientation of a chiral magnetic domain wall in a racetrack determines its dynamical properties. In equilibrium, magnetic domain walls are expected to be oriented perpendicular to the stripe axis. We demonstrate the appearance of a unidirectional domain wall tilt in out-of-plane magnetized stripes with biaxial anisotropy and Dzyaloshinskii--Moriya interaction (DMI). The tilt is a result of the interplay between the in-plane easy-axis anisotropy and DMI. We show that the additional anisotropy and DMI prefer different domain wall structure: anisotropy links the magnetization azimuthal angle inside the domain wall with the anisotropy direction in contrast to DMI, which prefers the magnetization perpendicular to the domain wall plane. Their balance with the energy gain due to domain wall extension defines the equilibrium magnetization the domain wall tilting. We demonstrate that the Walker field and the corresponding Walker velocity of the domain wall can be enhanced in the system supporting tilted walls.

cond-mat.mes-hall↗

arXiv2019

Curvature induced magnonic crystal in nanowires

A new type of magnonic crystals, curvature induced ones, is realized in ferromagnetic nanowires with periodically deformed shape. A magnon band structure of such crystal is fully determined by its curvature: the developed theory is well confirmed by simulations. An application to nanoscale spintronic devises with the geometrically tunable parameters is proposed, namely, to filter elements.

cond-mat.mes-hall↗