arXiv subjects

Olga Kocharovskaya

Publications and source records attributed to Olga Kocharovskaya.

At least 19 recordsLinked to original sources

arXiv2026

Probing the Linewidth of the 12.4-keV $^{45}$Sc Isomeric Resonance in Solids by Nuclear Forward Scattering

The $^{45}$Sc transition from the nuclear ground state to the 12.389-keV isomer (lifetime 0.46~s) has an ultranarrow natural linewidth $Γ_{\ind{0}}\simeq 1.4$~feV, corresponding to a quality factor $\simeq 10^{19}$. This makes $^{45}$Sc a compelling candidate for nuclear-clock metrology, provided that coherence in solids can be maintained close to the natural limit. Here we investigate the linewidth and coherence properties of the $^{45}$Sc resonance in solids following resonant x-ray pumping. Using the European XFEL, we confirm persistence of the long-lived isomer excitation in a solid-state environment via time-delayed incoherent $K_{α,β}$ emission and observe a weak delayed elastic channel at 12.4~keV, from which we extract a partial internal-conversion coefficient $α_{K}=390(60)$. Time-domain nuclear forward scattering measurements in crystals of Sc, Sc$_2$O$_3$, ScN and ScAlMgO$_4$ at 20~K show no statistically significant coherent forward-scattering signal beyond $2$~ms; within the adopted linewidth-broadening model, we infer an effective broadening $ΔΓ\gtrsim 500\,Γ_{\ind{0}}$. These results provide the quantitative constraints on linewidth broadening in solid-state $^{45}$Sc with an intrinsic natural linewidth in the femto-electronvolt range thereby laying the groundwork for precision metrology in the X-ray regime and future nuclear-clock frequency references using $^{45}$Sc nuclear isomer.

quant-ph↗

arXiv2026

On Demand magnetic-Doppler nuclear frequency comb memory for hard X-ray photons

Nuclear quantum memories in the hard X-ray regime offer some key advantages over their optical counterparts, such as broader bandwidth and lower background noise. A Doppler frequency comb protocol has been theoretically proposed [X. Zhang \textit{et al.}, Phys. Rev. Lett. \textbf{123}, 250504 (2019)] and recently demonstrated experimentally [S. Velten \textit{et al.}, Sci. Adv. \textbf{10}, eadn9825 (2024)] for the storage and retrieval of X-ray photons. However, achieving on-demand retrieval remains challenging because of the requirement for precise and synchronous mechanical motion of multiple absorbers. We propose a hybrid, magnetic-Doppler nuclear frequency comb composed of Doppler-shifted resonant absorbers with lifted nuclear spin degeneracy, which expands the Doppler comb structure. By synchronously reversing the directions of both the magnetic fields and absorber velocities, the system achieves time-reversed phase evolution dynamics that allows for efficient on-demand photon retrieval with significantly reduced mechanical complexity.

quant-ph↗

arXiv2025

On-Demand Zeeman Nuclear Frequency Comb Quantum Memory

The emerging hard X-ray - nuclear interfaces offer unique potential advantages over traditional optical-atomic interfaces for room-temperature, solid-state quantum information processing, including lower background noise, tighter focusing, and exceptionally high resonance quality. Leveraging such interfaces, a major milestone was recently achieved with the first implementation of nuclear quantum memory in the hard X-ray range [S. Velten et al., Nuclear quantum memory for hard X-ray photon wave packets, Sci. Adv. 10, eadn9825 (2024)] using the Doppler frequency comb protocol. However, this approach relies on the synchronous mechanical motion of multiple nuclear absorbers, posing experimental challenges for on-demand photon retrieval. We propose an on-demand hard X-ray quantum memory based on reversing the direction of an external magnetic field in a single stationary solid-state nuclear absorber with sets of Zeeman sublevels. This scheme is exemplified by the quantum storage of an 1.41-$μ$s single photon wave packet at 6.2 keV for over 10 $μ$s in a $^{181}$Ta metallic foil, providing a feasible pathway for the first experimental demonstration of on-demand hard X-ray photon storage.

quant-ph↗

arXiv2021

Amplification of Elliptically Polarized Sub-Femtosecond Pulses in IR-Field-Dressed Neon-Like Active Medium of a Plasma-Based X-ray Laser

We propose a method for amplifying a train of sub-femtosecond pulses of circularly or elliptically polarized extreme ultraviolet (XUV) radiation constituted by high-order harmonics of an infrared (IR) laser field, in a neon-like active medium of a plasma-based X-ray laser, additionally irradiated with a replica of a fundamental frequency IR field. It is shown that the ellipticity of the pulses can be maintained or increased during the amplification process. The experimental implementation is suggested in an active medium of an X-ray laser based on neon-like Ti^{12+} ions irradiated by an IR laser field with a wavelength of 3.9 microns.

physics.optics↗

arXiv2021

Amplification and ellipticity enhancement of sub-femtosecond XUV pulses in IR-field-dressed neon-like active medium of a plasma-based X-ray laser

In [I.R. Khairulin et al., submitted to Phys. Rev. Lett.] we propose a method for amplifying a train of sub-femtosecond pulses of circularly or elliptically polarized extreme ultraviolet (XUV) radiation, constituted by high-order harmonics of an infrared (IR) laser field, in a neon-like active medium of a plasma-based X-ray laser, additionally irradiated with a replica of a fundamental frequency laser field used to generate harmonics, and show the possibility of maintaining or enhancing the ellipticity of high-harmonic radiation during its amplification. In the present paper we describe this process in detail both for a single harmonic component and a sub-femtosecond pulse train formed by a set of harmonics. We derive the analytical theory and describe both analytically and numerically the evolution of the high-harmonic field during its propagation through the medium. We discuss also the possibility of an experimental implementation of the suggested technique in an active medium of an X-ray laser based on neon-like Ti^{12+} ions irradiated by an IR laser field with a wavelength of 3.9 microns.

physics.optics↗

arXiv2020

Attosecond pulse formation in the "water window" range by optically dressed hydrogen-like plasma-based C5+ X-ray laser

In this paper, we present the analytical theory of attosecond pulse formation via optical modulation of an active medium of the hydrogen-like C5+ plasma-based X-ray laser at 3.4 nm wavelength in the "water window" range, taking into account a variation of the population inversion caused by radiative decay of the upper lasing states. We derive an analytical solution for the X-ray field amplified by an X-ray laser with time-dependent population inversion, which is simultaneously irradiated by a strong optical laser field, and use it to find the optimal conditions for the attosecond pulse formation from a narrowband seeding X-ray field. We show that the shape of pulses can be improved at the cost of reduced pulse peak intensity (i) via external attenuation of the resonant spectral component of the amplified X-ray field or (ii) by using a resonantly absorbing medium (the active medium of the X-ray laser after the change of sign of the population inversion) for the pulse formation. The results of the analytical theory are in a good agreement with the numerical solutions of the Maxwell-Bloch equations which account for the nonlinearity, as well as the amplified spontaneous emission, of the active medium. Both analytically and numerically we show the possibility to produce a train of attosecond pulses with sub-200 as duration and the peak intensity exceeding 10^12 W/cm^2 at the carrier wavelength 3.4 nm in the "water window" range, which makes them attractive for the biological and medical applications.

physics.optics↗

arXiv2019

Analytical theory of sub-fs pulse formation in a seeded hydrogen-like plasma-based X-ray laser dressed by an infrared field

We derive the analytical theory describing the process of sub-femtosecond pulse formation from a quasi-monochromatic seeding extreme ultraviolet (XUV) radiation, which propagates in active medium of a hydrogen-like plasma-based X-ray laser dressed by a strong infrared laser field. We discuss the ultimate capabilities and limitations of this process on the basis of the derived analytical solution and extensive numerical studies for the case of Li2+ plasma-based X-ray laser with a carrier wavelength 13.5nm. We analyze the role of plasma dispersion and find the optimal conditions for the formation of attosecond pulses with the highest contrast. Under the optimal conditions, the influence of amplified spontaneous emission from the active medium is negligible. The peak intensity of the produced XUV pulses can exceed 10^10-10^11 W/cm^2, while the duration of pulses varies in the range of 400-600 as.

physics.optics↗

arXiv2019

Observation of acoustically induced transparency for gamma-ray photons

We report an observation of a 148-fold suppression of resonant absorption of 14.4-keV photons from exp(-5.2) to exp(-0.2) with preservation of their spectral and temporal characteristics in an ensemble of the resonant two-level Fe-57 nuclei at room temperature. The transparency was induced via collective acoustic oscillations of nuclei. The proposed technique allows extending the concept of induced optical transparency to a hard x-ray/gamma-ray range and paves the way for acoustically controllable interface between x-ray/gamma-ray photons and nuclear ensembles, advancing the field of x-ray/gamma-ray quantum optics.

physics.optics↗

arXiv2019

Spectral control over $γ$-ray echo using a nuclear frequency comb system

Two kinds of spectral control over $γ$-ray echo using a nuclear frequency comb system are theoretically investigated. A nuclear frequency comb system is composed of multiple nuclear targets under magnetization (hyperfine splitting), mechanical motion (Doppler shift) or both, namely, moving and magnetized targets. In frequency domain the unperturbed single absorption line of $γ$-ray therefore splits into multiple lines with equal spacing and becomes a nuclear frequency comb structure. We introduce spectral shaping and dynamical splitting to the frequency comb structure respectively to optimize the use of a medium and to break the theoretical maximum of echo efficiency, i.e., 54\%. Spectral shaping scheme leads to the reduction of required sample resonant thickness for achieving high echo efficiency of especially a broadband input. Dynamical splitting method significantly advances the echo efficiency up to 67\% revealed by two equivalent nuclear frequency comb systems. We also show that using only few targets is enough to obtain good echo performance, which significantly eases the complexity of implementation. Our results extend quantum optics to 10keV regime and lay the foundation of the development of $γ$-ray memory.

quant-ph↗

arXiv2019

Attosecond Pulse Amplification in a Plasma-Based X-Ray Laser Dressed by an Infrared Laser Field

We suggest a technique to amplify a train of attosecond pulses, produced by high-harmonic generation (HHG) of an infrared (IR) laser field, in an active medium of a plasma-based X-ray laser. This technique is based on modulation of transition frequency of the X-ray laser by the same IR field, as used to generate the harmonics, via linear Stark effect, which results in redistribution of the resonant gain and simultaneous amplification of a wide set of harmonics in the incident field. We propose an experimental implementation of the suggested technique in active medium of C5+ ions at wavelength 3.4 nm in the "water window" range and show the possibility to amplify by two orders of magnitude a train of attosecond pulses with pulse duration down to 100 as. We show also a possibility to isolate a single attosecond pulse from the incident attosecond pulse train during its amplification in optically deep modulated medium.

physics.optics↗

arXiv2018

Nuclear quantum memory and time sequencing of a single $γ$ photon

A $γ$-ray-nuclear quantum interface is suggested as a new platform for quantum information processing, motivated by remarkable progresses in $γ$-ray quantum optics. The main advantages of a $γ$ photon over an optical photon lie in its almost perfect detectability and much tighter, potentially sub-angstrom, focusability. Nuclear ensembles hold important advantages over atomic ensembles in a unique combination of high nuclear density in bulk solids with narrow, lifetime-broadening Mössbauer transitions even at room temperature. This may lead to the densest long-lived quantum memories and the smallest size photon processors. Here we propose a technique for $γ$ photon quantum memory through a Doppler frequency comb, produced by a set of resonantly absorbing nuclear targets that move with different velocities. It provides a reliable storage, an on-demand generation, and a time sequencing of a single $γ$ photon. This scheme presents the first $γ$-photon-nuclear-ensemble interface opening a new direction of research in quantum information science.

quant-ph↗

arXiv2018

Light, the universe, and everything -- 12 Herculean tasks for quantum cowboys and black diamond skiers

The Winter Colloquium on the Physics of Quantum Electronics (PQE) has been a seminal force in quantum optics and related areas since 1971. It is rather mindboggling to recognize how the concepts presented at these conferences have transformed scientific understanding and human society. In January, 2017, the participants of PQE were asked to consider the equally important prospects for the future, and to formulate a set of questions representing some of the greatest aspirations in this broad field. The result is this multi-authored paper, in which many of the world's leading experts address the following fundamental questions: (1) What is the future of gravitational wave astronomy? (2) Are there new quantum phases of matter away from equilibrium that can be found and exploited - such as the time crystal? (3) Quantum theory in uncharted territory: What can we learn? (4) What are the ultimate limits for laser photon energies? (5) What are the ultimate limits to temporal, spatial, and optical resolution? (6) What novel roles will atoms play in technology? (7) What applications lie ahead for nitrogen-vacancy centers in diamond? (8) What is the future of quantum coherence, squeezing, and entanglement for enhanced superresolution and sensing? (9) How can we solve (some of) humanity's biggest problems through new quantum technologies? (10) What new understanding of materials and biological molecules will result from their dynamical characterization with free electron lasers? (11) What new technologies and fundamental discoveries might quantum optics achieve by the end of this century? (12) What novel topological structures can be created and employed in quantum optics?

quant-ph↗

arXiv2016

Quantum storage based on controllable frequency comb

We suggest an all-optical scheme for the storage, retrieval and processing of a single-photon wave packet through its off-resonant Raman interaction with a series of coherent control beams. These control beams, each with distinct carrier frequency, are distributed along the way of single-photon propagation, thus effectively forming a gradient absorption structure which can be controlled in various ways to achieve different single-photon processing functionalities. Such a controllable frequency comb is a hybrid of Raman, gradient echo memory (GEM) and atomic frequency comb (AFC) methods, therefore demonstrates many of their advantages all together in one.

quant-ph↗

arXiv2015

Application of the low finesse frequency comb for high resolution spectroscopy

High finesse frequency combs (HFC) with large ratio of the frequency spacing to the width of the spectral components have demonstrated remarkable results in many applications such as precision spectroscopy and metrology. We found that low finesse frequency combs having very small ratio of the frequency spacing to the width of the spectral components are more sensitive to the exact resonance with absorber than HFC. Our method is based on time domain measurements reviling oscillations of the radiation intensity after passing through an optically thick absorber. Fourier analysis of the oscillations allows to reconstruct the spectral content of the comb. If the central component of the incident comb is in exact resonance with the single line absorber, the contribution of the first sideband frequency into oscillations is exactly zero. We demonstrate this technique with gamma-photon absorbtion by Mössbauer nuclei providing the spectral resolution beyond the natural broadening.

physics.optics↗

arXiv2015

Conversion of recoilless gamma-radiation into a periodic sequence of ultrashort pulses in a set of dispersive and absorptive resonant media

An efficient technique to produce a periodic sequence of ultrashort pulses of recoilless gamma-radiation via its transmission through the optically thick vibrating resonant absorber was demonstrated recently [Nature, 508, 80 (2014)]. In this work we extend the theoretical analysis to the case of a set of multiple absorbers. We consider an analytical model describing the control of spectral content of a frequency modulated gamma-radiation by selective correction of amplitudes and initial phases of some spectral components, using, respectively, the resonant absorption or dispersion of nuclei. On the basis of the analytical solutions we determine the ultimate possibilities of the proposed technique.

physics.optics↗

arXiv2014

All optical quantum storage based on spatial chirp of the control field

We suggest an all-optical quantum memory scheme which is based on the off-resonant Raman interaction of a signal quantum field and a strong control field in a three-level atomic medium in the case, when the control field has a spatially varying frequency across the beam, called a spatial chirp. We show that the effect of such a spatial chirp is analogous to the effect of a controllable reversible inhomogeneous broadening (CRIB) of the atomic transition used in the gradient echo memory (GEM) scheme. However, the proposed scheme does not require temporal modulation of the control field or the atomic levels, and can be realized without additional electric or magnetic fields. It means that materials demonstrating neither linear Stark nor Zeeman effects can be used and/or materials which are placed in specific external fields remain undisturbed.

quant-ph↗

arXiv2014

Multimode cavity-assisted quantum storage via continuous phase matching control

A scheme for spatial multimode quantum memory is developed such that spatial-temporal structure of a weak signal pulse can be stored and recalled via cavity-assisted off-resonant Raman interaction with a strong angular-modulated control field in an extended $Λ$-type atomic ensemble. It is shown that effective multimode storage is possible when the Raman coherence spatial grating involves wave vectors with different longitudinal components relative to the paraxial signal field. The possibilities of implementing the scheme in the solid-state materials are discussed.

quant-ph↗

arXiv2013

Coherent Control of the Waveforms of Recoilless Gamma-Photons

An efficient method to coherently control the waveforms of gamma-photons has been proposed and experimentally realized. It is based on the resonant interaction of gamma-photons with an ensemble of nuclei with modulated frequency of the quantum transition. In particular, the temporal compression of an individual gamma-photon into coherent ultrashort pulse train has been demonstrated. The developed technique is expected to give a strong impetus on emerging fields of coherent and quantum gamma-optics, providing a basis for realization of the gamma-photon nuclear-ensemble interfaces and quantum interference effects at the nuclear gamma-ray transitions.

quant-ph↗