arXiv subjects
Publications and source records attributed to Olivier Dauchot.
We investigate the flow around an oscillating nearly-spherical particle at low, yet non-vanishing, Reynolds numbers, and the potential resulting locomotion. We analytically demonstrate that no net motion can arise up to order one in Re and order one in the asphericity parameter, regardless of the particle's shape. Therefore, geometry-induced acoustic streaming propulsion, if any, must arise at higher order.
The dynamics of an active walker in a harmonic potential is studied experimentally, numerically and theoretically. At odds with usual models of self-propelled particles, we identify two dynamical states for which the particle condensates at finite distance from the trap center. In the first state, also found in other systems, the particle points radially outward the trap, while diffusing along the azimuthal direction. In the second state, the particle performs circular orbits around the center of the trap. We show that self-alignment, taking the form of a torque coupling the particle orientation and velocity, is responsible for the emergence of this second dynamical state. The transition between the two states is controlled by the persistence of the particle orientation. At low inertia, the transition is continuous. For large inertia the transition is discontinuous and a coexistence regime with intermittent dynamics develops. The two states survive in the over-damped limit or when the particle is confined by a curved hard wall.
We experimentally and numerically study the structure and dynamics of a mono-disperse packing of spontaneously aligning self-propelled hard disks. The packings are such that their equilibrium counterparts form perfectly ordered hexagonal structures. Experimentally, we first form a perfect crystal in an hexagonal arena which respects the same crystalline symmetry. Frustration of the hexagonal order, obtained by removing a few particles, leads to the formation of a rapidly diffusing "droplet". Removing more particles, the whole system spontaneously forms a macroscopic sheared flow, while conserving an overall crystalline structure. This flowing crystalline structure, which we call a "rheo-crystal" is made possible by the condensation of shear along localized stacking faults. Numerical simulations very well reproduce the experimental observations and allow us to explore the parameter space. They demonstrate that the rheo-crystal is induced neither by frustration nor by noise. They further show that larger systems flow faster while still remaining ordered.
We propose a macroscopic realization of planar Brownian motion by vertically vibrated disks. We perform a systematic statistical analysis of many random trajectories of individual disks. The distribution of increments is shown to be almost Gaussian, with slight deviations at large increments caused by inter-disk collisions. The velocity auto-correlation function takes both positive and negative values at short lag times but rapidly vanishes. We compare the empirical and theoretical distributions of time averaged mean square displacements and discuss distinctions between its mean and mode. These well-controlled experimental data can serve for validating statistical tools developed for the analysis of single-particle trajectories in microbiology.
We present a novel, self-consistent and robust theoretical model to investigate elastic interactions between topological defects in liquid crystal shells. Accounting for the non-concentric nature of the shell in a simple manner, we are able to successfully and accurately explain and predict the positions of the defects, most relevant in the context of colloidal self-assembly. We calibrate and test our model on existing experimental data, and extend it to all newly observed defects configurations in chiral nematic shells. We perform new experiments to check further and confirm the validity of the present model. Moreover, we are able to obtain quantitative estimates of the energies of $+1$ or $+3/2$ disclination lines in cholesterics, whose intricate nature was only reported recently.
We investigate experimentally and numerically the defect configurations emerging when a cholesteric liquid crystal is confined to a spherical shell. We uncover a rich scenario of defect configurations, some of them non-existent in nematic shells, where new types of defects are stabilized by the helical ordering of the liquid crystal. In contrast to nematic shells, here defects are not simple singular points or lines, but have a large structured core. Specifically, we observe five different types of cholesteric shells. We study the statistical distribution of the different types of shells as a function of the two relevant geometrical dimensionless parameters of the system. By playing with these parameters, we are able to induce transitions between different types of shells. These transitions involve interesting topological transformations in which the defects recombine to form new structures. Surprisingly, the defects do not approach each other by taking the shorter distance route (geodesic), but by following intricate paths.
Analyzing the dynamics of a vibrated bi-dimensional packing of bidisperse granular discs below jamming, we provide evidences of a Gardner phase deep into the glass phase. To do so we perform several independent compression cycles within the same glass and show that the particles select different average vibrational positions at each cycle, while the neighborhood structure remains unchanged. We compute the mean square displacement as a function of the packing fraction and compare it with the average separation between the cages obtained for different compression cycles. Our results are fully compatible with recent numerical observations obtained for a mean field model of glass as well as for hard spheres in finite dimension. We also characterize the distribution of the cage order parameters. Here we note several differences from the numerical results, which could be attributed to activated processes and cage heterogeneities.
We propose a conservative two-dimensional particle model in which particles carry a continuous and classical spin. The model includes standard ferromagnetic interactions between spins of two different particles, and a nonstandard coupling between spin and velocity of the same particle inspired by the coupling observed in self-propelled hard discs. Because of this coupling Galilean invariance is broken and the conserved linear momentum associated to translation invariance is not proportional to the velocity of the center of mass. Also, the dynamics is not invariant under a global rotation of the spins alone. This, in principle, leaves room for collective motion and thus raises the question whether collective motion can arise in Hamiltonian systems. We study the statistical mechanics of such a system, and show that, in the fully connected (or mean-field) case, a transition to collective motion does exist in spite of momentum conservation. Interestingly, the velocity of the center of mass, which in the absence of Galilean invariance, is a relevant variable, also feeds back on the magnetization properties, as it acts as an external magnetic field that smoothens the transition. Molecular dynamics simulations of finite size systems indeed reveal a rich phase diagram, with a transition from a disordered to a homogeneous polar phase, but also more complex inhomogeneous phases with local order interrupted by topological defects.
We evidence critical fluctuations in the strain-rate of granular flows that are weakly vibrated. Strikingly, the critical point arises at {\em finite} values of the mean strain rate and vibration strength, far away from the yielding critical point at zero flow rate. We show that the global rheology, as well as the amplitude and correlation time of the fluctuations, are consistent with a mean-field, Landau like description, where strain rate and stress act as conjugated variables. We introduce a general model which captures the observed phenomenology, and argue that this type of critical behavior generically arises when self fluidization competes with friction.
We study cholesteric order in liquid crystal shells with planar degenerate anchoring. We observe that the bipolar and radial configurations intensively reported for bulk droplets have a higher degree of complexity when the liquid crystal is confined to a spherical shell. The bipolar configuration is replaced by a structure where the boojums are linked to a stack of disclination rings that spans the shell, while the radial configuration exhibits a double helix structure where two disclinations wind around each other. Our results confirm recent numerical simulations and highlight the complexity of the defect structures arising when cholesteric liquid crystals are confined to spherical geometries. We also show that the position of the boojums is only ruled by the shell geometry, independently of the cholesteric pitch. To understand quantitatively this behavior, we develop a simple yet insightful theoretical framework which captures the essence of the observed phenomenology. We also show that the transition between the two configurations is solely governed by the confinement ratio c = h/p, where h is the average shell thickness and p is the cholesteric pitch. Finally, we perform a dynamical study of this transition, and report a fascinating defect waltz due to a chemical Lehmann effect.
We study the spatially homogeneous phases of polar active particles in the low density limit, and specifically the transition from the isotropic phase to collective polar motion. We show that the fundamental quantity of interest for the stability of the isotropic phase is the forward component of the momentum change induced by binary scattering events. Building on the Boltzmann formalism, we introduce an ansatz for the one-particle distribution and derive a closed-form evolution equation for the order parameter. This approach yields a very intuitive and physically meaningful criterion for the destabilization of the isotropic phase, where the ansatz is exact. The criterion also predicts whether the transition is continuous or discontinuous, as illustrated in three different classes of models. The theoretical predictions are in excellent agreement with numerical results.
We study the effect of thermal fluctuations in the XY-model on a surface with non vanishing mean curvature and zero Gaussian curvature. Unlike Gaussian curvature that typically frustrates orientational order, the extrinsic curvature of the surface can act as a local field that promotes long range order at low temperature. We find numerically that the transition from the high temperature isotropic phase to the true long range ordered phase is characterized by critical exponents consistent with those of the flat space Ising model in two dimensions, up to finite size effects. Our results suggest a versatile strategy to achieve geometric control of liquid crystal order by suitable design of the underlying curvature of a substrate or bounding surface.
We investigate experimentally the mechanical response to shear of a 2D packing of grains across the jamming transition. First, we develop a dedicated experimental setup, together with tracking and photoelastic techniques in order to prepare the packing in a controlled fashion and to quantify the stress and strain tensors at the grain scale. Second, we install a inflating probe (a 2D "balloon"), which shears the packing with a cylindrical symmetry. We probe experimentally stresses and strains for strain amplitudes as low as $10^{-3}$ and for a range of packing fractions within $2\%$ variation around the jamming transition. We observe not only that shear strain induces shear stresses, but also normal stresses. Moreover, we show that both shear and normal stresses behave nonlinearly with the shear strain. Finally, we show by scaling analysis that the constitutive laws are controlled by the Jamming transition.
We show that low density homogeneous phases of self propelled hard disks exhibit a transition from isotropic to polar collective motion, albeit of a qualitatively distinct class from the Vicsek one. In the absence of noise, an abrupt discontinuous transition takes place between the isotropic phase and a fully polar absorbing state. Increasing the noise, the transition becomes continuous at a tri-critical point. We explain all our numerical findings in the framework of Boltzmann theory, on the basis of the binary scattering properties. We show that the qualitative differences observed between the present and the Vicsek model at the level of their phase behavior, take their origin in the complete opposite physics taking place during scattering events. We argue that such differences will generically hold for systems of self-propelled particles with repulsive short range interactions.
We study the problem of the transformation of a given reactant species into an immiscible product species, as they flow through a chemically active porous medium. We derive the equation governing the evolution of the volume fraction of the species -- in a one-dimensional macroscopic description --, identify the relevant dimensionless numbers, and provide simple models for capillary pressure and relative permeabilities, which are quantities of crucial importance when tackling multiphase flows in porous media. We set the domain of validity of our models and discuss the importance of viscous coupling terms in the extended Darcy's law. We investigate numerically the steady regime and demonstrate that the spatial transformation rate of the species along the reactor is non-monotonous, as testified by the existence of an inflection point in the volume fraction profiles. We obtain the scaling of the location of this inflection point with the dimensionless lengths of the problem. Eventually, we provide key elements for optimization of the reactor.
We report spontaneous motion in a fully bio-compatible system consisting of pure water droplets in an oil-surfactant medium of squalane and monoolein. Water from the droplet is solubilized by the reverse micellar solution, creating a concentration gradient of swollen reverse micelles around each droplet. The strong advection and weak diffusion conditions allow for the first experimental realization of spontaneous motion in a system of isotropic particles at sufficiently large Péclet number according to a straightforward generalization of a recently proposed mechanism. Experiments with a highly concentrated solution of salt instead of water, and tetradecane instead of squalane, confirm the above mechanism. The present swimming droplets are able to carry external bodies such as large colloids, salt crystals, and even cells.
We investigate experimentally the mechanical response of a monolayer of bi-disperse frictional grains to an inhomogeneous shear perturbation across the jamming transition. We inflate an intruder inside the packing and use photo-elasticity and tracking techniques to measure the induced shear strain and stresses at the grain scale. We quantify experimentally the constitutive relations for strain amplitudes as low as 0.001 and for a range of packing fractions within 2% variation around the jamming transition. At the transition strong nonlinear effects set in : both the shear modulus and the dilatancy shear-soften at small strain until a critical strain is reached where effective linearity is recovered. The dependencies of the critical strain and the associated critical stresses on the distance from jamming are extracted via scaling analysis. We check that the constitutive laws, when applied to the equations governing mechanical equilibrium, lead to the observed stress and strain profiles. These profiles exhibit a spatial crossover between an effective linear regime close to the inflater and the truly nonlinear regime away from it. The crossover length diverges at the jamming transition.
From the formation of animal flocks to the emergence of coordinate motion in bacterial swarms, at all scales populations of motile organisms display coherent collective motion. This consistent behavior strongly contrasts with the difference in communication abilities between the individuals. Guided by this universal feature, physicists have proposed that solely alignment rules at the individual level could account for the emergence of unidirectional motion at the group level. This hypothesis has been supported by agent-based simulations. However, more complex collective behaviors have been systematically found in experiments including the formation of vortices, fluctuating swarms, clustering and swirling. All these model systems predominantly rely on actual collisions to display collective motion. As a result, the potential local alignment rules are entangled with more complex, often unknown, interactions. The large-scale behavior of the populations therefore depends on these uncontrolled microscopic couplings. Here, we demonstrate a new phase of active matter. We reveal that dilute populations of millions of colloidal rollers self-organize to achieve coherent motion along a unique direction, with very few density and velocity fluctuations. Identifying the microscopic interactions between the rollers allows a theoretical description of this polar-liquid state. Comparison of the theory with experiment suggests that hydrodynamic interactions promote the emergence of collective motion either in the form of a single macroscopic flock at low densities, or in that of a homogenous polar phase at higher densities. Furthermore, hydrodynamics protects the polar-liquid state from the giant density fluctuations. Our experiments demonstrate that genuine physical interactions at the individual level are sufficient to set homogeneous active populations into stable directed motion.