arXiv subjects

Olle Eriksson

Publications and source records attributed to Olle Eriksson.

At least 19 recordsLinked to original sources

arXiv2026

Magnetic frustration and non-collinear textures in layered Gd magnets

Using scale-bridging simulations based on electronic structure theory and atomistic spin dynamics, we investigate the magnetic properties of skyrmionic GdRu$_2$Si$_2$ and GdRu$_2$Ge$_2$ layered rare-earth magnets and similar Gd-based compounds (GdAu$_2$Si$_2$, GdAu$_2$Ge$_2$, GdAg$_2$Si$_2$ and GdAg$_2$Ge$_2$). By studying the trends across this structural family, we confirm the importance of magnetic frustration and dipolar interactions for the stability of non-collinear and skyrmion phases. Furthermore, our calculations predict promising opportunities for chemical tuning of these magnets in terms of the balance between various exchange interactions and the character of the magnetic anisotropy. These changes lead to the formation of new types of skyrmions that are stable in a wide range of applied external magnetic field. In particular, we propose partial alkali-metal substitution of Gd in GdRu$_2$Si$_2$ leading to GdKRu$_4$Si$_4$, GdRbRu$_4$Si$_4$, GdCsRu$_4$Si$_4$ as well as GdYRu$_4$Si$_4$ compounds, and suggest that it is likely to result in an ordered layered structure, similarly to previously reported iron pnictides like CaKFe$_4$As$_4$.

cond-mat.mtrl-sci↗

arXiv2026

Energy Ordering from Nonlinear Quantum Dissipation

Energy-ordered occupation is deeply embedded in quantum physics, from the Aufbau principle governing the filling of electronic states in atoms and molecules to the emergence of low-energy configurations in quantum many-body systems. However, the dynamical mechanism by which a generic quantum state develops such an energy hierarchy remains a fundamental question. Here we show that such an energy hierarchy can emerge dynamically from nonlinear quantum dissipation. Rather than being imposed as a principle or generated through coupling to a thermal reservoir, an Aufbau-like ordering of energy levels emerges intrinsically under quantum Landau-Lifshitz-Gilbert dynamics from a generic initial mixed state. This convergence is a nontrivial consequence of Lyapunov monotonicity and instability of disordered population configurations. The resulting dynamics establish an intrinsic nonlinear mechanism for organizing density-matrix populations and provides a route toward selective preparation of low-energy subspaces. Numerical simulations confirm analytical predictions and illustrate convergence toward low-energy sectors.

quant-ph↗

arXiv2026

Exciton-induced magnons carrying orbital angular momentum in CrI3

Magnons are collective spin excitations that contain and transport spin angular momentum in magnetic materials. It has been suggested that they can also carry orbital angular momentum in analogy to the electronic motion around the nucleus. We explore the real-space topology of magnon wave-packets emanating from atomic-like excitons in the ferromagnetic insulator CrI3 and demonstrate the existence of orbital angular momentum in such wave-packets. We reveal that orbital angular momentum of magnons is nearly equal to their spin angular momentum and compensates the latter. This illustrates the existence of an unexplored internal angular momentum balance and demonstrates that the magnetization can be quenched without the need of angular momentum exchange with the lattice.

cond-mat.mtrl-sci↗

arXiv2026

Magnetic hopfions at room temperature

Hopfions are three-dimensional (3D) topological solitons predicted to exist in diverse magnetic systems, yet their practical utility has been largely restricted to cryogenic environments. Here, we overcome this temperature constraint by demonstrating stable magnetic hopfions in the chiral magnet Co8Zn8Mn4 at and above room temperature. Using a transmission electron microscope equipped for in situ optical excitation, we generate magnetic hopfions with femtosecond laser pulses. Long-term observations further reveal Brownian-like motion at room temperature and thermally activated collapse upon approaching the high-temperature regime. Together with micromagnetic simulations and homotopy group analysis, our experimental observations uncover the hopfion formation mechanism through the fusion of bimeron pairs. These findings establish room-temperature magnetic hopfions and provide a framework for their further studies under technologically relevant conditions.

cond-mat.mtrl-sci↗

arXiv2026

Topological Hall plateau in quasi-2D kagome magnet YMn$_6$Sn$_6$

We examine the impact of the Dzyaloshinskii-Moriya interaction (DMI) in kagome magnets and show that a predominantly planar DMI together with ferromagnetic exchange stabilizes a disordered skyrmion phase in quasi-two-dimensional (2D) YMn$_6$Sn$_6$. Within an ab initio framework combining density functional theory and spin-dynamics simulations, we generate realistic spin textures of disordered skyrmion and find that this phase persists for $B_{ext} < 0.5$ T, with a decreasing skyrmion size as magnetic field increases. We demonstrate the emergence of topological Hall plateau in the range $-0.5 \leq B_{ext} < 0.5$ T, driven by nearly uniform scalar spin chirality and the resulting constant real-space Berry curvature. This response is anti-symmetric with magnetic field while magnitude and sign of these plateau are determined by a complex interplay between Hund's coupling strength and chemical potential signifying the role of Dirac points and van Hove singularities. In addition, we reveal topological magnon excitations in the disordered skyrmion phase of quasi-2D YMn$_6$Sn$_6$.

cond-mat.mtrl-sci↗

arXiv2026

Ferroelectrical Switching as a Probe of Quantum Damping in Magnetic Spin Systems

While damped spin dynamics is important for the understanding of magnetic materials, clear signatures of \emph{quantum corrections} to the Gilbert damping mechanism remain elusive. We propose a route to distinguish quantum and classical Gilbert spin damping using ferroelectric control of a magnetic dimer. Ab initio calculations for dimers on ferroelectric substrates show that polarization reversal switches the inter-spin exchange between ferromagnetic and antiferromagnetic regimes. We formulate a magnetization-based diagnostic that relates magnetization traces to entanglement dynamics, which enables ferroelectrical on/off control of dimer entanglement. Material-informed quantum Landau-Lifshitz-Gilbert simulations illustrate how the signature of magnetization dynamics can, in principle, be used to infer the existence of quantum Gilbert spin damping. This minimal and non-volatile platform connects first-principles modeling to experimentally accessible observables and provides a starting point for voltage-controlled quantum entanglement in magnetic spin networks.

quant-ph↗

arXiv2026

Unraveling the symmetry of Al5C3N

The high-temperature ceramic compound Al5C3N with promising application usage belongs to the scarcely studied Al-C-N system. It was originally reported as an ordered compound in the non-centrosymmetric space group P63mc and described as a nanolaminate with an -Al2C-AlN-Al2C2- stacking sequence. The recently reported structural disorder in the related compound Al4SiC4 led us to question this proposed structure for Al5C3N and investigate the possibility of a disordered structure in the centrosymmetric space group P63/mmc. In the present work, we employed different synthesis routes to maximize the yield and quality of the desired phase, and applied a variety of techniques to probe the Al5C3N crystal structure. Our single-crystal X-ray diffraction analysis clearly indicates that the non-centrosymmetric space group P63mc must be rejected. From a joint refinement of single-crystal X-ray and powder neutron diffraction data, the occupancies of C and N were refined at two sites in P63/mmc resulting in the stacking sequence -Al2C-Al(C/N)-Al2(C/N)2-. Furthermore, DFT calculations show that a centrosymmetric disordered structure described in a supercell has the lowest energy, 0.2 eV per formula unit, relative to the previously reported P63mc structure. The calculated band structure shows both direct and indirect band gaps which lead to implications for the physical properties. Finally, STEM analysis provides additional evidence that the crystal structure of Al5C3N is better described in the centrosymmetric space group P63/mmc.

cond-mat.mtrl-sci↗

arXiv2026

Inequivalence of Landau-Lifshitz and Landau-Lifshitz-Gilbert dynamics for a single quantum spin

We examine the relation between the quantum Landau-Lifshitz equation ($q$-LL) [Phys. Rev. Lett. 110, 147201 (2013)] and quantum Landau-Lifshitz-Gilbert equation ($q$-LLG) [Phys. Rev. Lett. 133, 266704 (2024)]; two non-linear purity preserving master equations that extend classical atomistic spin dynamics into the quantum regime. While the classical LL and LLG counterparts for any number of spins are known to be equivalent, i.e., give identical spin trajectories up to a rescaling of the time parameter, the quantum formulations are equivalent only in certain cases, such as for pure states or for arbitrary single spin-$\frac{1}{2}$ states. Here, we demonstrate that this equivalence breaks down even at the level of a single spin, provided $s \geq 1$. Focusing on a spin-1 particle in an anisotropic crystal field, we show that the $q$-LL and $q$-LLG equations generate inequivalent time evolution. We introduce temporal rescaling misfits that quantify the inequivalence of the two types of dynamics. Although our results highlight fundamental differences in dissipation mechanisms encoded in these equations, the resulting trajectories remain qualitatively similar for this system.

quant-ph↗

arXiv2026

Ground-state selection via nonlinear quantum dissipation

Finding the ground state of complex quantum systems remains a central challenge in many-body physics, quantum chemistry, and combinatorial optimization, due to the exponential growth of the Hilbert-space dimension and the entangled structure of ground states. We show that quantum Landau--Lifshitz-Gilbert (QLLG) dynamics, proposed in [Phys. Rev. Lett. 133, 266704 (2024)], provides a physically realizable, real-time nonlinear mechanism that selectively suppresses excited-state components and drives the system toward the lowest-energy eigenstate contained in the initial state. Unlike purely numerical methods such as the imaginary-time projection method, QLLG combines coherent precession with dissipative suppression, enabling experimentally accessible ground-state preparation. For random initial states in the $N$-qubit Hilbert space of dimension $2^N$, convergence occurs in times scaling linearly with system size, $N$, and inversely with the spectral gap. We provide numerical simulations of our analytical results with a Hamiltonian describing an interacting spin chain with Heisenberg exchange and a Zeeman term. Our results identify nonlinear quantum dissipation as a powerful tool for real-time ground-state preparation in large quantum systems and quantum optimization.

quant-ph↗

arXiv2026

Electric-current-assisted nucleation of zero-field hopfion rings

Magnetic hopfions are three-dimensional topological solitons -- knotted, vortex-like spin configurations. In chiral magnets, hopfions can appear as isolated structures or they can be linked to skyrmion strings. Previous studies employed a sophisticated protocol and a special sample geometry to nucleate such hopfions linked to one or a few skyrmion strings. Here, we introduce an electric-current-assisted nucleation protocol that is simple and independent of the sample shape and size. The resulting hopfions exhibit extraordinary stability in the presence of both positive and negative magnetic fields, in perfect agreement with micromagnetic simulations. We also present a comprehensive framework for classifying hopfions, skyrmions, and merons by deriving the corresponding homotopy group.

cond-mat.mes-hall↗

arXiv2026

Mechanical control of magnetic exchange and response in GdRu$_2$Si$_2$: A computational study

We present a systematic computational study of the effect of uniaxial strain on the magnetic properties of GdRu$_2$Si$_2$, a centrosymmetric material known to host a field-induced skyrmion lattice (SkL). Using first-principles density functional theory, we first demonstrate the pronounced sensitivity of the exchange and anisotropy to specific structural distortions. These DFT-derived interactions are then integrated into a classical spin model to construct comprehensive magnetic phase diagrams under both compressive and tensile strain. Our key finding is that compressive strain ($\sim 2\%$) acts as an effective tuning parameter, substantially expanding the stability region of the $\vec Q_{100}$-driven topologically nontrivial phases. This results from the shifts in the critical magnetic fields and enhancement of the energy scale of the favored magnetic wave vector. In contrast, tensile strain induces a different magnetic ground-state by promoting a different magnetic ordering vector, $\vec Q_{110}$, leading to entirely distinct phase behavior. This work not only provides a quantitative understanding of the structural-magnetic coupling in GdRu$_2$Si$_2$ but also establishes strain engineering as a powerful approach to control and optimize topologically non-trivial magnetic phases in centrosymmetric magnets.

cond-mat.mtrl-sci↗

arXiv2025

New insights into the magnetism of DyCo$_{5}$

In this work, we present the first magnetization measurements of DyCo$_5$ single crystals in magnetic fields up to 14 T, spanning a temperature range up to 600 K. Our investigation reveals several unique features, including a significant magnetization anisotropy and an observed minimum in spontaneous magnetization near the compensation point, phenomena not previously reported. This work also uncovers the complex magnetic behavior of DyCo$_5$, with a pronounced interplay between the Dy and Co sublattices, each exhibiting distinct temperature-dependent magnetic properties. The combination of dynamical mean-field theory (DMFT), atomistic spin-dynamics (ASD) simulations, and the Effective Spin Model (ESM) for rare-earth compounds successfully explains the experimental data across both low and high temperatures. Our theoretical approach not only explains the observed magnetic anisotropy and the behavior near the compensation temperature but also successfully reproduces key experimental features such as the saturation behavior at high fields and the evolution of the magnetic moment at different temperatures.

cond-mat.mtrl-sci↗

arXiv2025

Topological Metal-Insulator Transition within the Ferromagnetic state

A major challenge in condensed matter physics is integrating topological phenomena with correlated electron physics to leverage both types of states for next-generation quantum devices. Metal-insulator transitions (MITs) are central to bridging these two domains while simultaneously serving as 'on-off' switches for electronic states. Here, we demonstrate how the prototypical material of K2Cr8O16 undergoes a ferromagnetic MIT accompanied by a change in band topology. Through inelastic x-ray and neutron scattering experiments combined with first-principles theoretical calculations, we demonstrate that this transition is not driven by a Peierls mechanism, given the lack of phonon softening. Instead, we establish the transition as a topological MIT within the ferromagnetic phase (topological-FM-MIT) with potential axionic properties, where electron correlations play a key role in stabilizing the insulating state. This work pioneers the discovery of a topological-FM-MIT and represents a fundamentally new class of topological phase transitions, revealing a unique pathway through which magnetism, topology, and electronic correlations interact.

cond-mat.str-el↗

arXiv2025

A configuration interaction approach to solve the Anderson impurity model; applications to elemental Ce

Accurate calculations of strongly correlated materials remain a formidable challenge in condensed matter physics, particularly due to the computational demand of conventional methods. This paper presents an efficient solver for dynamical mean field theory using configuration interaction (CI). The method is shown to have improved efficiency compared to traditional, exact diagonalization approaches. Hence, it provides an accessible, open-source alternative that can be executed on standard laptop computers or on supercomputers. The solver is demonstrated on cerium in the $\gamma$-, $\alpha$- and $\epsilon$-phases. An analysis of how the electronic structure of Ce evolves as function of lattice compression is made. It is argued that the electronic structure evolves from a localized nature of the 4f shell in $\gamma$-Ce to an essentially itinerant nature of the 4f shell of $\epsilon$-Ce. The transition between these two phases, as function of compression, can hence be seen as a Mott transition. However, this transition is intercepted by the strongly correlated $\alpha$-phase of elemental Ce, for which the 4f shell forms a Kondo singlet.

cond-mat.str-el↗

arXiv2025

Quantitative theory of magnetic properties of elemental praseodymium

Elemental Pr metal crystallizes in the double hexagonal close packed (dhcp) structure and is unique among rare-earth elements in featuring a localized partially filled 4f shell without ordered magnetism. Experimental evidence attributes this absence of magnetism to a singlet crystal-field (CF) ground state of the Pr 4f$^2$ configuration, which is energetically well isolated from excited magnetic doublets. Here, we construct a realistic effective magnetic Hamiltonian for dhcp Pr, by combining density-functional theory with dynamical mean-field theory, in the quasiatomic Hubbard-I approximation. Our calculations fully determine the CF potential and predict singlet CF ground states at both inequivalent sites of the dhcp lattice. The intersite exchange interactions, obtained from the magnetic force theorem, are found to be insufficient to close the CF gap to the magnetic doublets. Hence, ab-initio theory is demonstrated to explain the unusual, non-magnetic state of elemental Pr. Extending this analysis to the (0001) surface of Pr, we find that the singlet ground state remains robust preventing conventional magnetic orders. Nevertheless, the gap between the ground state and the lowest excited singlet is significantly reduced at the surface, opening the possibility for exotic two-dimensional multipolar orders to emerge within this two-singlet manifold.

cond-mat.str-el↗

arXiv2025

Linked skyrmions in shifted magnetic bilayer

Magnetic solitons have recently attracted significant attention due to their intricate physical properties and potential applications in information processing. The majority of the studies in this field, however, are focused on a particular type of solitons known as skyrmions, characterised by a unit topological charge. Here, we present a shifted magnetic bilayer that can demonstrate magnetic solitons with arbitrary large topological charges. These configurations, which we call linked skyrmions, consist of multiple skyrmions linked together with topological point defects. These topological point defects, termed as anti-aligned points, originate from the mutually orthogonal Dzyaloshinskii-Moriya interaction in two different layers. By tuning the interlayer exchange coupling and the external magnetic field, one can also achieve different ground states in this bilayer. Additionally, the system also demonstrates conventional skyrmion-bags and $k\pi$-skyrmions. Finally we propose a suitable material candidate where these magnetic configurations can be realised. Our findings, thus, can provide a way to achieve solitons with large topological charge and realise them in realistic systems.

cond-mat.mes-hall↗

arXiv2025

Hybrid micromagnetic and atomistic modeling of magnetization dynamics induced by engineered defects

This study presents a 3D version of multiscale approach for investigating magnetization dynamics in multiscale, hybrid micromagnetic-atomistic simulations. The present work introduces engineered discontinuities (i) a double-slit structure, which enables the study of domain wall and spin wave interference, and (ii) a tetrahedron shaped cluster of atoms with tunable anisotropy, which provides insights into how localized anisotropic perturbations influence domain wall pinning and skyrmion stability in fully three-dimensional (3D) hybrid simulations. We considered the dynamics of spin waves, domain walls, as well as 3D skyrmions, in the presence of these defects. The magnonic double-slit experiment demonstrates interference patterns analogous to electronic wave phenomena, offering potential applications in wave-based computing. Additionally, the results reveal the impact of the local anisotropy that leads to distinct transformations, including domain wall deformations, tubular and spherical structures, skyrmion annihilation, and breathing mode. The findings underscore the critical role of defect-induced anisotropic interactions in controlling domain wall motion, skyrmion topology, and spin wave propagation.

cond-mat.mtrl-sci↗

arXiv2025

Dynamical electronic correlation and chiral magnetism in van der Waals magnet Fe4GeTe2

Among the quasi-2D van der Waals magnetic systems, Fe4GeTe2 imprints a profound impact due to its near-room temperature ferromagnetic behaviour and the complex magnetothermal phase diagram exhibiting multiple phase transformations, as observed from magnetization and magnetotransport measurements. A complete analysis of these phase transformations in the light of electronic correlation and its impact on the underlying magnetic interactions remain unattended in the existing literature. Using first-principles methodologies, incorporating the dynamical nature of electron correlation, we have analysed the interplay of the direction of magnetization in the easy-plane and easy-axis manner with the underlying crystal symmetry, which reveals the opening of a pseudogap feature beyond the spin-reorientation transition (SRT) temperature. The impact of dynamical correlation on the calculated magnetic circular dichroism and x-ray absorption spectrum of the L-edge of the Fe atoms compared well with the existing experimental observations. The calculated intersite Heisenberg exchange interactions display a complicated nature, depending upon the pairwise interactions among the two inequivalent Fe sites, indicating a RKKY-like behaviour of the magnetic interactions. We noted the existence of significant anisotropic and antisymmetric exchanges interactions, resulting into a chirality in the magnetic behaviour of the system. Subsequent investigation of the dynamical aspects of magnetism in Fe4GeTe2 and the respective magnetothermal phase diagram reveal that the dynamical nature of spins and the decoupling of the magnetic properties for both sites of Fe is crucial to explain all the experimentally observed phase transformations.

cond-mat.other↗