arXiv subjects

Osip Schwartz

Publications and source records attributed to Osip Schwartz.

13 recordsLinked to original sources

arXiv2026

Probing the electromagnetic nonlinearity of vacuum with continuous-wave lasers

In classical electrodynamics, light waves propagating in vacuum do not interact. In quantum physics, however, photon-photon interactions are mediated by virtual particles, giving rise to the electromagnetic nonlinearity of vacuum (EMNV). A direct measurement of EMNV would test a long-standing prediction of quantum electrodynamics and constrain new physics models. Despite its fundamental significance and extensive efforts to detect it, free-space EMNV has not yet been directly measured in the laboratory. Here, we propose a tabletop all-optical measurement of EMNV based on resonantly enhanced four-wave mixing in focusing optical resonators with a circulating power of a few megawatts. As a key experimental step toward this measurement, we demonstrate a resonator reaching a circulating power of 2.5 MW, approaching the parameter range needed to detect EMNV at the level predicted by quantum electrodynamics.

physics.optics↗

arXiv2025

Spin Squeezing in Electron Microscopy

Quantum metrology experiments in atomic physics and quantum optics have demonstrated measurement accuracy beyond the shot-noise limit via multi-particle entanglement. At the same time, electron microscopy, an essential tool for high-resolution imaging of biological systems, is severely constrained in its signal-to-noise ratio (SNR) by shot noise, due to the dose limit imposed by electron beam-induced damage. Here, we show theoretically that spin squeezing, a form of quantum metrology based on entanglement, is a natural fit for improving the SNR in electron microscopy. We investigate the generation of the necessary entangled states through electron-electron Coulomb interactions and quantum non-demolition measurements. Our results connect the fields of quantum metrology and electron interferometry, paving the way toward electron microscopy with SNR beyond the shot-noise limit.

quant-ph↗

arXiv2021

A Quantum Klystron -- Controlling Quantum Systems with Modulated Electron Beams

Coherent control of quantum transitions -- indispensable in quantum technology -- generally relies on the interaction of quantum systems with electromagnetic radiation. Here, we theoretically demonstrate that the non-radiative electromagnetic near-field of a temporally modulated free-space electron beam can be utilized for coherent control of quantum systems. We show that such manipulation can be performed with only classical control over the electron beam itself, and is readily realizable with current technology. This approach may provide a pathway towards spectrally selective quantum control with nano-scale spatial resolution, harnessing the small de Broglie wavelength of electrons.

quant-ph↗

arXiv2020

High-Power Near-Concentric Fabry-Perot Cavity for Phase Contrast Electron Microscopy

Transmission electron microscopy (TEM) of vitrified biological macromolecules (cryo-EM) is limited by the weak phase contrast signal that is available from such samples. Using a phase plate would thus substantially improve the signal-to-noise ratio. We have previously demonstrated the use of a high-power Fabry-Perot cavity as a phase plate for TEM. We now report improvements to our laser cavity that allow us to achieve record continuous-wave intensities of over 450 GW/cm$^{2}$, sufficient to produce the optimal 90° phase shift for 300 keV electrons. In addition, we have performed the first cryo-EM reconstruction using a laser phase plate, demonstrating that the stability of this laser phase plate is sufficient for use during standard cryo-EM data collection.

physics.ins-det↗

arXiv2020

Observation of the relativistic reversal of the ponderomotive potential

The secular dynamics of a non-relativistic charged particle in an electromagnetic wave can be described by the ponderomotive potential. Although ponderomotive electron-laser interactions at relativistic velocities are important for emerging technologies from laser-based particle accelerators to laser-enhanced electron microscopy, the effects of special relativity on the interaction have only been studied theoretically. Here, we use a transmission electron microscope to measure the position-dependent phase shift imparted to a relativistic electron wave function when it traverses a standing laser wave. The kinetic energy of the electrons is varied between $80\,\mathrm{keV}$ and $300\,\mathrm{keV}$, and the laser standing wave has a continuous-wave intensity of $175\,\mathrm{GW/cm}^2$. In contrast to the non-relativistic case, we demonstrate that the phase shift depends on both the electron velocity and the wave polarization, confirming the predictions of a quasiclassical theory of the interaction. Remarkably, if the electron's speed is greater than $1/\sqrt{2}$ of the speed of light, the phase shift at the electric field nodes of the wave can exceed that at the antinodes. In this case there exists a polarization such that the phase shifts at the nodes and antinodes are equal, and the electron does not experience Kapitza-Dirac diffraction. Our results thus provide new capabilities for coherent electron beam manipulation.

physics.optics↗

arXiv2018

Attractive force on atoms due to blackbody radiation

Objects at finite temperature emit thermal radiation with an outward energy-momentum flow, which exerts an outward radiation pressure. At room temperature, a cesium atom scatters on average less than one of these blackbody radiation photons every 10^8 years. Thus, it is generally assumed that any scattering force exerted on atoms by such radiation is negligible. However, atoms also interact coherently with the thermal electromagnetic field. In this work, we measure an attractive force induced by blackbody radiation between a cesium atom and a heated, centimeter-sized cylinder which is orders of magnitude stronger than the outward directed radiation pressure. Using atom interferometry, we find that this force scales with the fourth power of the cylinder`s temperature. The force is in good agreement with that predicted from an ac Stark shift gradient of the atomic ground state in the thermal radiation field. This observed force dominates over both gravity and radiation pressure, and does so for a large temperature range.

physics.atom-ph↗

arXiv2016

Continuous 40 GW/cm$^2$ laser intensity in a near-concentric optical cavity

Manipulating free-space electron wave functions with laser fields can bring about new electron-optical elements for transmission electron microscopy. In particular, a Zernike phase plate would enable high-contrast imaging of soft matter, leading to new opportunities in structural biology and materials science. A Zernike plate can be implemented using a tight, intense CW laser focus that shifts the phase of the electron wave by the ponderomotive potential. Here, we use a near-concentric cavity to focus 7.5 kW of circulating laser power at 1064 nm into a 7 $μ$m waist, setting a record for CW laser intensity and establishing a pathway to ponderomotive phase contrast TEM.

physics.optics↗

arXiv2013

Cooperative Lamb shift in a quantum emitter array

Whenever several quantum light emitters are brought in proximity with one another, their interaction with common electromagnetic fields couples them, giving rise to cooperative shifts in their resonance frequency. Such collective line shifts are central to modern atomic physics, being closely related to superradiance on one hand and the Lamb shift on the other. Although collective shifts have been theoretically predicted more than fifty years ago, the effect has not been observed yet in a controllable system of a few isolated emitters. Here, we report a direct spectroscopic observation of the cooperative shift of an optical electric dipole transition in a system of up to eight Sr ions suspended in a Paul trap. We study collective resonance shift in the previously unexplored regime of far-field coupling, and provide the first observation of cooperative effects in an array of quantum emitters. These results pave the way towards experimental exploration of cooperative emission phenomena in mesoscopic systems.

quant-ph↗

arXiv2011

Shaped two-photon excitation deep inside scattering tissue

Light is the tool of the 21st century. New photosensitive tools offer the possibility to monitor and control neuronal activity from the sub-cellular to the integrative level. This ongoing revolution has motivated the development of new optical methods for light stimulation. Among them, it has been recently demonstrated that a promising approach is based on the use of wavefront shaping to generate optically confined extended excitation patterns. This was achieved by combining the technique of temporal focusing with different approaches for lateral light shaping including low numerical aperture Gaussian beams, holographic beams and beams created with the generalized phase contrast mthod. What is needed now is a precise characterization of the effect of scattering on hese different methods in order to extend their use for in depth excitation. Here we present a theoretical and experimental study on the effect of scattering on the propagation of wavefront shaped beams. Results from fixed and acute cortical slices show that temporally focused spatial patterns are extremely robust against the effects of scattering and this permits their three-dimensional confinement for depths up to 550 μm.

physics.optics↗

arXiv2011

Vectorial Phase Retrieval for Linear Characterization of Attosecond Pulses

The waveforms of attosecond pulses produced by high-harmonic generation carry information on the electronic structure and dynamics in atomic and molecular systems. Current methods for the temporal characterization of such pulses have limited sensitivity and impose significant experimental complexity. We propose a new linear and all-optical method inspired by widely-used multi-dimensional phase retrieval algorithms. Our new scheme is based on the spectral measurement of two attosecond sources and their interference. As an example, we focus on the case of spectral polarization measurements of attosecond pulses, relying on their most fundamental property -- being well confined in time. We demonstrate this method numerically reconstructing the temporal profiles of attosecond pulses generated from aligned $CO_2$ molecules.

physics.optics↗

arXiv2011

Fluorescence antibunching microscopy

Breaking the diffraction limit in microscopy by utilizing quantum properties of light has been the goal of intense research in the recent years. We propose a quantum superresolution technique based on non-classical emission statistics of fluorescent markers, routinely used as contrast labels for bio-imaging. The technique can be readily implemented using standard fluorescence microscopy equipment.

physics.optics↗

arXiv2010

Shot noise limited characterization of femtosecond light pulses

Probing the evolution of physical systems at the femto- or attosecond timescale with light requires accurate characterization of ultrashort optical pulses. The time profiles of such pulses are usually retrieved by methods utilizing optical nonlinearities, which require significant signal powers and operate in a limited spectral range\cite{Trebino_Review_of_Scientific_Instruments97,Walmsley_Review_09}. We present a linear self-referencing characterization technique based on time domain localization of the pulse spectral components, operated in the single-photon regime. Accurate timing of the spectral slices is achieved with standard single photon detectors, rendering the technique applicable in any spectral range from near infrared to deep UV. Using detection electronics with about $70$ ps response, we retrieve the temporal profile of a picowatt pulse train with $\sim10$ fs resolution, setting a new scale of sensitivity in ultrashort pulse characterization.

physics.optics↗

arXiv2010

Photodarkening of blinking quantum dots is not governed by Auger recombination

The observed intermittent light emission from colloidal semiconductor nanocrystals has long been associated with Auger recombination assisted quenching. We test this view by observing transient emission dynamics of CdSe/CdS/ZnS semiconductor nanocrystals using time-resolved photon counting. The size and intensity dependence of the observed decay dynamics are inconsistent with the those expected from Auger processes. Moreover, the data suggests that in the `off' state the quantum dot cycles in a three-step process: photoexcitation, rapid trapping and subsequent slow nonradiative decay.

cond-mat.mes-hall↗