arXiv subjects

Owen D. Miller

Publications and source records attributed to Owen D. Miller.

At least 55 records · Page 3Linked to original sources

arXiv2019

Scattering concentration bounds: Brightness theorems for waves

The brightness theorem---brightness is nonincreasing in passive systems---is a foundational conservation law, with applications ranging from photovoltaics to displays, yet it is restricted to the field of ray optics. For general linear wave scattering, we show that power per scattering channel generalizes brightness, and we derive power-concentration bounds for systems of arbitrary coherence. The bounds motivate a concept of "wave étendue" as a measure of incoherence among the scattering-channel amplitudes, and which is given by the rank of an appropriate density matrix. The bounds apply to nonreciprocal systems that are of increasing interest, and we demonstrate their applicability to maximal control in nanophotonics, for metasurfaces and waveguide junctions. Through inverse design, we discover metasurface elements operating near the theoretical limits.

physics.optics↗

arXiv2019

Limits to surface-enhanced Raman scattering near arbitrary-shape scatterers

The low efficiency of Raman spectroscopy can be overcome by placing the active molecules in the vicinity of scatterers, typically rough surfaces or nanostructures with various shapes. This surface-enhanced Raman scattering (SERS) leads to substantial enhancement that depends on the scatterer that is used. In this work, we find fundamental upper bounds on the Raman enhancement for arbitrary-shaped scatterers, depending only on its material constants and the separation distance from the molecule. According to our metric, silver is optimal in visible wavelengths while aluminum is better in the near-UV region. Our general analytical bound scales as the volume of the scatterer and the inverse sixth power of the distance to the active molecule. Numerical computations show that simple geometries fall short of the bounds, suggesting further design opportunities for future improvement. For periodic scatterers, we use two formulations to discover different bounds, and the tighter of the two always must apply. Comparing these bounds suggests an optimal period depending on the volume of the scatterer.

physics.optics↗

arXiv2019

High-NA Achromatic Metalenses by Inverse Design

We use inverse design to discover metalens structures that exhibit broadband, achromatic focusing across low, moderate, and high numerical apertures. We show that standard unit-cell approaches cannot achieve high-efficiency high-NA focusing, even at a single frequency, due to the incompleteness of the unit-cell basis, and we provide computational upper bounds on their maximum efficiencies. At low NA, our devices exhibit the highest theoretical efficiencies to date. At high NA -- of 0.9 with translation-invariant films and of 0.99 with "freeform" structures -- our designs are the first to exhibit achromatic high-NA focusing.

physics.optics↗

arXiv2019

Fundamental limits to near-field optical response, over any bandwidth

We develop an analytical framework to derive upper bounds to light--matter interactions in the optical near field, where applications ranging from spontaneous-emission amplification to greater-than-blackbody heat transfer show transformative potential. Our framework connects the classic complex-analytic properties of causal fields with newly developed energy-conservation principles, resulting in a new class of power--bandwidth limits. These limits demonstrate the possibility of orders-of-magnitude enhancement in near-field optical response with the right combination of material and geometry. At specific frequency and bandwidth combinations, the bounds can be closely approached by canonical plasmonic geometries, with the opportunity for new designs to emerge away from those frequency ranges. Embedded in the bounds is a material "figure of merit," which determines the maximum response of any material (metal/dielectric, bulk/2D, etc.), for any frequency and bandwidth. Our bounds on local density of states (LDOS) represent maximal spontaneous-emission enhancements, our bounds on cross density of states (CDOS) limit electromagnetic-field correlations, and our bounds on radiative heat transfer (RHT) represent the first such analytical rule, revealing fundamental limits relative to the classical Stefan--Boltzmann law.

physics.optics↗

arXiv2019

Maximal Spontaneous Photon Emission and Energy Loss from Free Electrons

Free electron radiation such as Cerenkov, Smith--Purcell, and transition radiation can be greatly affected by structured optical environments, as has been demonstrated in a variety of polaritonic, photonic-crystal, and metamaterial systems. However, the amount of radiation that can ultimately be extracted from free electrons near an arbitrary material structure has remained elusive. Here we derive a fundamental upper limit to the spontaneous photon emission and energy loss of free electrons, regardless of geometry, which illuminates the effects of material properties and electron velocities. We obtain experimental evidence for our theory with quantitative measurements of Smith--Purcell radiation. Our framework allows us to make two predictions. One is a new regime of radiation operation---at subwavelength separations, slower (nonrelativistic) electrons can achieve stronger radiation than fast (relativistic) electrons. The second is a divergence of the emission probability in the limit of lossless materials. We further reveal that such divergences can be approached by coupling free electrons to photonic bound states in the continuum (BICs). Our findings suggest that compact and efficient free-electron radiation sources from microwaves to the soft X-ray regime may be achievable without requiring ultrahigh accelerating voltages.

physics.optics↗

arXiv2018

Optimal nanoparticle forces, torques, and illumination fields

A universal property of resonant subwavelength scatterers is that their optical cross-sections are proportional to a square wavelength, $λ^2$, regardless of whether they are plasmonic nanoparticles, two-level quantum systems, or RF antennas. The maximum cross-section is an intrinsic property of the \emph{incident field}: plane waves, with infinite power, can be decomposed into multipolar orders with finite powers proportional to $λ^2$. In this Article, we identify $λ^2/c$ and $λ^3/c$ as analogous force and torque constants, derived within a more general quadratic scattering-channel framework for upper bounds to optical force and torque for any illumination field. This framework also solves the reverse problem: computing globally optimal "holographic" incident beams, for a fixed collection of scatterers. We analyze structures and incident fields that approach the bounds, which for wavelength-scale bodies show a rich interplay between scattering channels, and we show that spherically symmetric structures are forbidden from reaching the plane-wave force/torque bounds. This framework should enable optimal mechanical control of nanoparticles with light.

physics.optics↗

arXiv2017

Limits to the Optical Response of Graphene and 2D Materials

2D materials provide a platform for strong light--matter interactions, creating wide-ranging design opportunities via new-material discoveries and new methods for geometrical structuring. We derive general upper bounds to the strength of such light--matter interactions, given only the optical conductivity of the material, including spatial nonlocality, and otherwise independent of shape and configuration. Our material figure of merit shows that highly doped graphene is an optimal material at infrared frequencies, whereas single-atomic-layer silver is optimal in the visible. For quantities ranging from absorption and scattering to near-field spontaneous-emission enhancements and radiative heat transfer, we consider canonical geometrical structures and show that in certain cases the bounds can be approached, while in others there may be significant opportunity for design improvement. The bounds can encourage systematic improvements in the design of ultrathin broadband absorbers, 2D antennas, and near-field energy harvesters.

physics.optics↗

arXiv2017

General Theory of Spontaneous Emission Near Exceptional Points

We present a general theory of spontaneous emission at exceptional points (EPs)---exotic degeneracies in non-Hermitian systems. Our theory extends beyond spontaneous emission to any light--matter interaction described by the local density of states (e.g., absorption, thermal emission, and nonlinear frequency conversion). Whereas traditional spontaneous-emission theories imply infinite enhancement factors at EPs, we derive finite bounds on the enhancement, proving maximum enhancement of 4 in passive systems with second-order EPs and significantly larger enhancements (exceeding $400\times$) in gain-aided and higher-order EP systems. In contrast to non-degenerate resonances, EPs are associated with non-Lorentzian emission curves, leading to enhancements that scale polynomially with the resonance quality factor.

physics.optics↗

arXiv2017

Non-intuitive Computational Optimization of Illumination Patterns for Maximum Optical Force and Torque

This paper aims to maximize optical force and torque on arbitrary micro- and nano-scale objects using numerically optimized structured illumination. By developing a numerical framework for computer-automated design of 3d vector-field illumination, we demonstrate a 20-fold enhancement in optical torque per intensity over circularly polarized plane wave on a model plasmonic particle. The nonconvex optimization is efficiently performed by combining a compact cylindrical Bessel basis representation with a fast boundary element method and a standard derivative-free, local optimization algorithm. We analyze the optimization results for 2000 random initial configurations, discuss the tradeoff between robustness and enhancement, and compare the different effects of multipolar plasmon resonances on enhancing force and torque. All results are obtained using open-source computational software available online.

physics.optics↗

arXiv2016

Low-loss Plasmonic Dielectric Nanoresonators

Material losses in metals are a central bottleneck in plasmonics for many applications. Here we propose and theoretically demonstrate that metal losses can be successfully mitigated with dielectric particles on metallic films, giving rise to hybrid dielectric--metal resonances. In the far field, they yield strong and efficient scattering, beyond even the theoretical limits of all-metal and all-dielectric structures. In the near field, they offer high-Purcell-factor (${>}5000$), high-quantum-efficiency (${>}90\%$), and highly directional emission at visible and infrared wavelengths. Their quality factors can be readily tailored from plasmonic-like (${\sim}10$) to dielectric-like (${\sim}10^3$), with wide control over the individual resonant coupling to photon, plasmon, and dissipative channels. Compared with conventional plasmonic nanostructures, such resonances show robustness against detrimental nonlocal effects and provide higher field enhancement at extreme nanoscopic sizes and spacings. These hybrid resonances equip plasmonics with high efficiency, which has been the predominant goal since the field's inception.

physics.optics↗

arXiv2016

Silicon Color Filters for Light-Recycling Displays

We propose a set of silicon reflective transmission filters for light-recycling displays that are compatible with high-throughput nanofabrication technologies and have excellent angular stability.

physics.optics↗

arXiv2016

Perfect Single-Sided Radiation and Absorption without Mirrors

Highly directional radiation from photonic structures is important for many applications, including high power photonic crystal surface emitting lasers, grating couplers, and light detection and ranging devices. However, previous dielectric, few-layer designs only achieved moderate asymmetry ratios, and a fundamental understanding of bounds on asymmetric radiation from arbitrary structures is still lacking. Here, we show that breaking the 180$^\circ$ rotational symmetry of the structure is crucial for achieving highly asymmetric radiation. We develop a general temporal coupled-mode theory formalism to derive bounds on the asymmetric decay rates to the top and bottom of a photonic crystal slab for a resonance with arbitrary in-plane wavevector. Guided by this formalism, we show that infinite asymmetry is still achievable even without the need of back-reflection mirrors, and we provide numerical examples of designs that achieve asymmetry ratios exceeding $10^4$. The emission direction can also be rapidly switched from top to bottom by tuning the wavevector or frequency. Furthermore, we show that with the addition of weak material absorption loss, such structures can be used to achieve perfect absorption with single-sided illumination, even for single-pass absorption rates less than $0.5\%$ and without back-reflection mirrors. Our work provides new design principles for achieving highly directional radiation and perfect absorption in photonics.

physics.optics↗

arXiv2016

Giant frequency-selective near-field energy transfer in active--passive structures

We apply a fluctuation electrodynamics framework in combination with semianalytical (dipolar) approximations to study amplified spontaneous energy transfer (ASET) between active and passive bodies. We consider near-field energy transfer between semi-infinite planar media and spherical structures (dimers and lattices) subject to gain, and show that the combination of loss compensation and near-field enhancement (achieved by the proximity, enhanced interactions, and tuning of subwavelength resonances) in these structures can result in orders of magnitude ASET enhancements below the lasing threshold. We examine various possible geometric configurations, including realistic materials, and describe optimal conditions for enhancing ASET, showing that the latter depends sensitively on both geometry and gain, enabling efficient and tunable gain-assisted energy extraction from structured surfaces.

cond-mat.mes-hall↗

arXiv2016

Efficient, designable, and broad-bandwidth optical extinction via aspect-ratio-tailored silver nanodisks

Subwavelength resonators, ranging from single atoms to metallic nanoparticles, typically exhibit a narrow-bandwidth response to optical excitations. We computationally design and experimentally synthesize tailored distributions of silver nanodisks to extinguish light over broad and varied frequency windows. We show that metallic nanodisks are two-to-ten-times more efficient in absorbing and scattering light than common structures, and can approach fundamental limits to broadband scattering for subwavelength particles. We measure broadband extinction per volume that closely approaches theoretical predictions over three representative visible-range wavelength windows, confirming the high efficiency of nanodisks and demonstrating the collective power of computational design and experimental precision for developing new photonics technologies.

physics.optics↗

arXiv2016

Optically Thin Metallic Films for High-radiative-efficiency Plasmonics

Plasmonics enables deep-subwavelength concentration of light and has become important for fundamental studies as well as real-life applications. Two major existing platforms of plasmonics are metallic nanoparticles and metallic films. Metallic nanoparticles allow efficient coupling to far field radiation, yet their synthesis typically leads to poor material quality. Metallic films offer substantially higher quality materials, but their coupling to radiation is typically jeopardized due to the large momentum mismatch with free space. Here, we propose and theoretically investigate optically thin metallic films as an ideal platform for high-radiative-efficiency plasmonics. For far-field scattering, adding a thin high-quality metallic substrate enables a higher quality factor while maintaining the localization and tunability that the nanoparticle provides. For near-field spontaneous emission, a thin metallic substrate, of high quality or not, greatly improves the field overlap between the emitter environment and propagating surface plasmons, enabling high-Purcell (total enhancement > $10^4$), high-quantum-yield (> 50 %) spontaneous emission, even as the gap size vanishes (3$\sim$5 nm). The enhancement has almost spatially independent efficiency and does not suffer from quenching effects that commonly exist in previous structures.

physics.optics↗

arXiv2016

Fundamental limits to optical response in absorptive systems

At visible and infrared frequencies, metals show tantalizing promise for strong subwavelength resonances, but material loss typically dampens the response. We derive fundamental limits to the optical response of absorptive systems, bounding the largest enhancements possible given intrinsic material losses. Through basic conservation-of-energy principles, we derive geometry-independent limits to per-volume absorption and scattering rates, and to local-density-of-states enhancements that represent the power radiated or expended by a dipole near a material body. We provide examples of structures that approach our absorption and scattering limits at any frequency, by contrast, we find that common "antenna" structures fall far short of our radiative LDOS bounds, suggesting the possibility for significant further improvement. Underlying the limits is a simple metric, $|χ|^2 / \operatorname{Im} χ$ for a material with susceptibility $χ$, that enables broad technological evaluation of lossy materials across optical frequencies.

physics.optics↗

arXiv2015

Power--bandwidth limitations of an optical resonance

We present shape-independent upper limits to the power--bandwidth product for a single resonance in an optical scatterer, with the bound depending only on the material susceptibility. We show that quasistatic metallic scatterers can nearly reach the limits, and we apply our approach to the problem of designing $N$ independent, subwavelength scatterers to achieve flat, broadband response even if they individually exhibit narrow resonant peaks.

physics.optics↗

arXiv2015

Shape-Independent Limits to Near-Field Radiative Heat Transfer

We derive shape-independent limits to the spectral radiative heat-transfer rate between two closely spaced bodies, generalizing the concept of a black body to the case of near-field energy transfer. Through conservation of energy and reciprocity, we show that each body of susceptibility $χ$ can emit and absorb radiation at enhanced rates bounded by $|χ|^2 / \textrm{Im} χ$, optimally mediated by near-field photon transfer proportional to $1/d^2$ across a separation distance $d$. Dipole--dipole and dipole--plate structures approach restricted versions of the limit, but common large-area structures do not exhibit the material enhancement factor and thus fall short of the general limit. By contrast, we find that particle arrays interacting in an idealized Born approximation (i.e., neglecting multiple scattering) exhibit both enhancement factors, suggesting the possibility of orders-of-magnitude improvement beyond previous designs and the potential for radiative heat transfer to be comparable to conductive heat transfer through air at room temperature, and significantly greater at higher temperatures.

physics.optics↗