arXiv subjects

P. -G. Reinhard

Publications and source records attributed to P. -G. Reinhard.

At least 181 records · Page 10Linked to original sources

arXiv2005

Self-Consistent Separable Rpa Approach for Skyrme Forces: Axial Nuclei

The self-consistent separable RPA (random phase approximation) method is formulated for Skyrme forces with pairing. The method is based on a general self-consistent procedure for factorization of the two-body interaction. It is relevant for various density- and current-dependent functionals. The contributions of the time-even and time-odd Skyrme terms as well as of the Coulomb and pairing terms to the residual interaction are taken self-consistently into account. Most of the expression have a transparent analytical form, which makes the method convenient for the treatment and analysis. The separable character of the residual interaction allows to avoid diagonalization of high-rank RPA matrices and thus to minimize the calculation effort. The previous studies have demonstrated high numerical accuracy and efficiency of the method for spherical nuclei. In this contribution, the method is specified for axial nuclei. We provide systematic and detailed presentation of formalism and discuss different aspects of the model.

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arXiv2005

Practicable factorized TDLDA for arbitrary density- and current-dependent functionals

We propose a practicable method for describing linear dynamics of different finite Fermi systems. The method is based on a general self-consistent procedure for factorization of the two-body residual interaction. It is relevant for diverse density- and current-dependent functionals and, in fact, represents the self-consistent separable random-phase approximation (RPA), hence the name SRPA. SRPA allows to avoid diagonalization of high-rank RPA matrices and thus dwarfs the calculation expense. Besides, SRPA expressions have a transparent analytical form and so the method is very convenient for the analysis and treatment of the obtained results. SRPA demonstrates high numerical accuracy. It is very general and can be applied to diverse systems. Two very different cases, the Kohn-Sham functional for atomic clusters and Skyrme functional for atomic nuclei, are considered in detail as particular examples. SRPA treats both time-even and time-odd dynamical variables and, in this connection, we discuss the origin and properties of time-odd currents and densities in initial functionals. Finally, SRPA is compared with other self-consistent approaches for the excited states, including the coupled-cluster method.

physics.atm-clus↗

arXiv2005

Electronic excitations in atomic clusters: beyond dipole plasmon

Multipole electron modes beyond the Mie plasmon in atomic clusters are investigated within the time-dependent local density approximation theory (TDLDA). We consider the origin of the modes, their connection with basic cluster properties and possible routes of experimental observation. Particular attention is paid to infrared magnetic orbital modes, scissors and twist, and electric quadrupole mode. The scissors and twist modes determine orbital magnetism of clusters while the electric quadrupole mode provides direct access to the single electron spectra of the cluster. We examine two-photon processes (Raman scattering, stimulated emission pumping and stimulated adiabatic Raman passage) as the most promising tools for experimental investigation of the modes.

physics.atm-clus↗

arXiv2005

Two-Photon Excitation of Low-Lying Electronic Quadrupole States in Atomic Clusters

A simple scheme of population and detection of low-lying electronic quadrupole modes in free small deformed metal clusters is proposed. The scheme is analyzed in terms of the TDLDA (time-dependent local density approximation) calculations. As test case, the deformed cluster $Na^+_{11}$ is considered. Long-living quadrupole oscillations are generated via resonant two-photon (two-dipole) excitation and then detected through the appearance of satellites in the photoelectron spectra generated by a probe pulse. Femtosecond pump and probe pulses with intensities $I = 2\cdot 10^{10} - 2\cdot 10^{11} W/cm^2$ and pulse duration $T = 200 - 500$ fs are found to be optimal. The modes of interest are dominated by a single electron-hole pair and so their energies, being combined with the photoelectron data for hole states, allow to gather new information about mean-field spectra of valence electrons in the HOMO-LUMO region. Besides, the scheme allows to estimate the lifetime of electron-hole pairs and hence the relaxation time of electronic energy into ionic heat.

physics.atm-clus↗

arXiv2005

From finite nuclei to the nuclear liquid drop: leptodermous expansion based on the self-consistent mean-field theory

The parameters of the nuclear liquid drop model, such as the volume, surface, symmetry, and curvature constants, as well as bulk radii, are extracted from the non-relativistic and relativistic energy density functionals used in microscopic calculations for finite nuclei. The microscopic liquid drop energy, obtained self-consistently for a large sample of finite, spherical nuclei, has been expanded in terms of powers of A^{-1/3} (or inverse nuclear radius) and the isospin excess (or neutron-to-proton asymmetry). In order to perform a reliable extrapolation in the inverse radius, the calculations have been carried out for nuclei with huge numbers of nucleons, of the order of 10^6. The Coulomb interaction has been ignored to be able to approach nuclei of arbitrary sizes and to avoid radial instabilities characteristic of systems with very large atomic numbers. The main contribution to the fluctuating part of the binding energy has been removed using the Green's function method to calculate the shell correction. The limitations of applying the leptodermous expansion to actual nuclei are discussed. While the leading terms in the macroscopic energy expansion can be extracted very precisely, the higher-order, isospin-dependent terms are prone to large uncertainties due to finite-size effects.

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arXiv2005

Modeling Na clusters in Ar matrices

We present a microscopic model for Na clusters embedded in raregas matrices. The valence electrons of the Na cluster are described by time-dependent density-functional theory at the level of the local-density approximation (LDA). Particular attention is paid to the semi-classical picture in terms of Vlasov-LDA. The Na ions and Argon atoms are handled as classical particles whereby the Ar atoms carry two degrees of freedom, position and dipole polarization. The interaction between Na ions and electrons is mediated through local pseudo-potentials. The coupling to the Ar atoms is described by (long-range) polarization potentials and (short-range) repulsive cores. The ingredients are taken from elsewhere developed standards. A final fine-tuning is performed using the NaAr molecule as benchmark. The model is then applied to embedded systems Na8ArN. By close comparison with quantum-mechanical results, we explore the capability of the Vlasov-LDA to describe such embedded clusters. We show that one can obtain a reasonable description by appropriate adjustments in the fine-tuning phase of the model.

physics.atm-clus↗

arXiv2004

Time resolved fission in metal clusters

We explore from a theoretical point of view pump and probe (P&P) analysis for fission of metal clusters where probe pulses are generalized to allow for scanning various frequencies. We show that it is possible to measure the time the system needs to develop to scission. This is achieved by a proper choice of both delay and frequency of the probe pulse. A more detailed analysis even allows to access the various intermediate stages of the fission process.

cond-mat.other↗

arXiv2004

The Skyrme energy functional and low lying 2+ states in Sn, Cd and Te isotopes

We study the predictive power of Skyrme forces with respect to low lying quadrupole spectra along the chains of Sn, Cd, and Te isotopes. Excitation energies and B(E2) values for the lowest quadrupole states are computed from a collective Schroedinger equation which as deduced through collective path generated by constraint Skyrme-Hartree-Fock (SHF) plus self-consistent cranking for the dynamical response. We compare the results from four different Skyrme forces, all treated with two different pairing forces (volume versus density-dependent pairing). The region around the neutron shell closure N=82 is very sensitive to changes in the Skyrme while the mid-shell isotopes in the region N<82 depend mainly on the adjustment of pairing. The neutron rich isotopes are most sensitive and depend on both aspects.

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arXiv2004

Adjustment studies in self-consistent relativistic mean-field models

We investigate the influence of the adjustment procedure and the set of measured observables on the properties and predictive power of relativistic self-consistent mean-field models for the nuclear ground state. These studies are performed with the point-coupling variant of the relativistic mean-field model. We recommend optimal adjustment algorithms for the general two-part problem and we identify various trends and dependencies as well as deficiencies of current models. Consequences for model improvements are presented.

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arXiv2004

The two-proton shell gap in Sn isotopes

We present an analysis of two-proton shell gaps in Sn isotopes. As the theoretical tool we use self-consistent mean-field models, namely the relativistic mean-field model and the Skyrme-Hartree-Fock approach, both with two different pairing forces, a delta interaction (DI) model and a density-dependent delta interaction (DDDI). We investigate the influence of nuclear deformation as well as collective correlations and find that both effects contribute significantly. Moreover, we find a further significant dependence on the pairing force used. The inclusion of deformation plus correlation effects and the use of DDDI pairing provides agreement with the data.

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arXiv2004

Momentum distribution in heavy deformed nuclei: role of effective mass

The impact of nuclear deformation on the momentum distributions (MD) of occupied proton states in $^{238}$U is studied with a phenomenological Woods-Saxon (WS) shell model and the self-consistent Skyrme-Hartree-Fock (SHF) scheme. Four Skyrme parameterizations (SkT6, SkM*, SLy6, SkI3) with different effective masses are used. The calculations reveal significant deformation effects in the low-momentum domain of $K^π=1/2^{\pm}$ states, mainly of those lying near the Fermi surface. For other states, the deformation effect on MD is rather small and may be neglected. The most remarkable result is that the very different Skyrme parameterizations and the WS potential give about identical MD. This means that the value of effective mass, being crucial for the description of the spectra, is not important for the spatial shape of the wave functions and thus for the MD. In general, it seems that, for the description of MD at $0\le k \le 300$ MeV/c, one may use any single-particle scheme (phenomenological or self-consistent) fitted properly to the global ground state properties.

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arXiv2004

On the Isovector Channels in Relativistic Point Coupling Models within the Hartree and Hartree-Fock Approximations

We investigate the consequences of Fierz transformations acting upon the contact interactions for nucleon fields occurring in relativistic point coupling models in Hartree approximation, which yield the same models but in Hartree-Fock approximation instead. We find for four-fermion interactions occurring in two existing relativistic point coupling phenomenologies that whereas in Hartree the isovector-scalar strength, corresponding to delta-meson exchange, is unnaturally small, indicating a possible new symmetry, in Hartree-Fock it is instead comparable to the isovector-vector strength corresponding to rho-meson exchange, but the sum of the two isovector coupling constants appears to be preserved in both approaches. Furthermore, in Hartree-Fock approximation, both QCD-scaled isovector coupling constants are natural (dimensionless and of order 1) whereas in Hartree approximation only that of the isovector-vector channel is natural. This indicates that it is not necessary to search for a new symmetry and, moreover, that the role of the delta-meson should be reexamined.

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arXiv2004

Infrared electron modes in light deformed clusters

Infrared quadrupole modes (IRQM) of the valence electrons in light deformed sodium clusters are studied by means of the time-dependent local-density approximation (TDLDA). IRQM are classified by angular momentum components $λμ=$20, 21 and 22 whose $μ$ branches are separated by cluster deformation. In light clusters with a low spectral density, IRQM are unambiguously related to specific electron-hole excitations, thus giving access to the single-electron spectrum near the Fermi surface (HOMO-LUMO region). Most of IRQM are determined by cluster deformation and so can serve as a sensitive probe of the deformation effects in the mean field. The IRQM branch $λμ=$21 is coupled with the magnetic scissors mode, which gives a chance to detect the latter. We discuss two-photon processes, Raman scattering (RS), stimulated emission pumping (SEP), and stimulated adiabatic Raman passage (STIRAP), as the relevant tools to observe IRQM. A new method to detect the IRQM population in clusters is proposed.

physics.atm-clus↗

arXiv2004

Systematics of Fission Barriers in Superheavy Elements

We investigate the systematics of fission barriers in superheavy elements in the range Z = 108-120 and N = 166-182. Results from two self-consistent models for nuclear structure, the relativistic mean-field (RMF) model as well as the non-relativistic Skyrme-Hartree-Fock approach are compared and discussed. We restrict ourselves to axially symmetric shapes, which provides an upper bound on static fission barriers. We benchmark the predictive power of the models examining the barriers and fission isomers of selected heavy actinide nuclei for which data are available. For both actinides and superheavy nuclei, the RMF model systematically predicts lower barriers than most Skyrme interactions. In particular the fission isomers are predicted too low by the RMF, which casts some doubt on recent predictions about superdeformed ground states of some superheavy nuclei. For the superheavy nuclei under investigation, fission barriers drop to small values around Z = 110, N = 180 and increase again for heavier systems. For most of the forces, there is no fission isomer for superheavy nuclei, as superdeformed states are in most cases found to be unstable with respect to octupole distortions.

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arXiv2003

Low-energy quadrupole modes in deformed clusters

Properties of low-energy (infra-red) quadrupole modes (LEQM) of multipolarity $+AFw-lambda+AFw-mu =$20, 21 and 22 in deformed sodium clusters are studied within the Kohn-Sham LDA RPA approach. Possible manifestations of LEQM in stimulated Raman adiabatic passage (STIRAP) reaction are discussed. It is shown that, in free light clusters, where the low-energy spectrum is delute, LEQM can be unambiguously identified as particular electron-hole pairs. This gives a chance to reconstruct the mean field level scheme near the Fermi surface. Moreover, due to the connection with electric $+AFw-lambda+AFw-mu =$21 mode, the scissors mode can be detected. In heavy (supported) oblate clusters, LEQM are in general rather involved. Nevertheless, some interesting $+AFw-lambda+AFw-mu =$21 and 22 structures determined by specific deformation effects can be resolved. The origin of the structures is discussed in detail.

physics.atm-clus↗

arXiv2003

The nonrelativistic limit of the relativistic point coupling model

We relate the relativistic finite range mean-field model (RMF-FR) to the point-coupling variant and compare the nonlinear density dependence. From this, the effective Hamiltonian of the nonlinear point-coupling model in the nonrelativistic limit is derived. Different from the nonrelativistic models, the nonlinearity in the relativistic models automatically yields contributions in the form of a weak density dependence not only in the central potential but also in the spin-orbit potential. The central potential affects the bulk and surface properties while the spin-orbit potential is crucial for the shell structure of finite nuclei. A modification in the Skyrme-Hartree-Fock model with a density-dependent spin-orbit potential inspired by the point-coupling model is suggested.

nucl-th↗

arXiv2003

Generator Coordinate Truncations

We investigate the accuracy of several schemes to calculate ground-state correlation energies using the generator coordinate technique. Our test-bed for the study is the $sd$ interacting boson model, equivalent to a 6-level Lipkin-type model. We find that the simplified projection of a triaxial generator coordinate state using the $S_3$ subgroup of the rotation group is not very accurate in the parameter space of the Hamiltonian of interest. On the other hand, a full rotational projection of an axial generator coordinate state gives remarkable accuracy. We also discuss the validity of the simplified treatment using the extended Gaussian overlap approximation (top-GOA), and show that it works reasonably well when the number of boson is four or larger.

nucl-th↗

arXiv2003

Deformation effects in low-momentum distributions of heavy nuclei

Momentum distributions (MD) of deep hole proton states in $^{238}$U are studied paying particular attention to the influence of deformation. Two essentially different mean-field models, Woods-Saxon (WS) and Skyrme-Hartree-Fock with the SkM$^*$ force, are used. Noticeable deviations between the WS and SkM$^*$ results are found. They are mainly due to the difference in effective nucleon mass. In particular, SkM$^*$ gives much weaker deformation effects at low momenta than WS. It is shown that, in spite of the deformation mixing, MD at low momenta can serve for identification of $K^π=1/2^+$ hole states originating from $s_{1/2}$ spherical sub-shells. Moreover, following the WS calculations, the deformation results in additional $K^π=1/2^+$ states with strong $l=0$ contributions. A possibility to probe such states in knock-out experiments is discussed.

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