arXiv subjects

P. Adsley

Publications and source records attributed to P. Adsley.

At least 19 recordsLinked to original sources

arXiv2025

Refining the deep sub-barrier 12C+12C excitation function with STELLA

Purpose: We have investigated the cross section around the lowest direct coincident gamma-particle measurements, where previously only limits could be established with the aim of obtaining a detailed description of the excitation function. We have furthermore analysed the ratio of extreme decay branching into the first excited state of daughter nuclei with alpha or proton emission at relative kinetic energies where previous measurements are in disagreement with each other. Conclusions: Our findings in the astrophysics RoI support reaction-rate models with a lower average S-factor trend, that deviates significantly from standard extrapolations between 2.2 MeV and 2.6 MeV, for stellar carbon burning simulations of up to 25 Msol stars. Based on our data, an overall increase of the S-factor at deep subbarrier energy cannot be confirmed. The extremely low ratio of the branching into the first excited state with proton over alpha emission of ~ 2% at 3.23 MeV might indicate the presence of alpha cluster compound states in 24Mg. This highly favours {\alpha} emission with fundamental consequences in possible stellar carbon burning sites.

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arXiv2024

Large quadrupole deformation in $^{20}$Ne challenges rotor model and modern theory: urging for $\alpha$ clusters in nuclei

The spectroscopic quadrupole moment of the first excited state, $Q_{_S}(2^{+}_{1})$, at 1.634 MeV in $^{20}$Ne was determined from sensitive reorientation-effect Coulomb-excitation measurements using a heavy target and safe energies well below the Coulomb barrier. Particle-$\gamma$ coincidence measurements were collected at iThemba LABS with a digital data-acquisition system using the {\sc AFRODITE} array coupled to an annular, doubled-sided silicon detector. A precise value of $Q_{_S}(2^{+}_{1})=-0.22(2)$ eb was determined at backward angles in agreement with the only safe-energy measurement prior to this work, $Q_{_S}(2^{+}_{1})=-0.23(8)$ eb. This result adopts 1$\hbar\omega$ shell-model calculations of the nuclear dipole polarizability of the 2$^+_1$ state that contributes to the effective quadrupole interaction and determination of $Q_{_S}(2^{+}_{1})$. It disagrees, however, with the ideal rotor model for axially-symmetric nuclei by almost $3\sigma$. Larger discrepancies are computed by modern state-of-the-art calculations performed in this and prior work, including {\it ab initio} shell model with chiral effective interactions and the multi-reference relativistic energy density functional ({\sc MR-EDF}) model. The intrinsic nucleon density of the 2$^+_1$ state in $^{20}$Ne calculated with the {\sc MR-EDF} model illustrates the presence of $\alpha$ clustering, which explains the largest discrepancy with the rotor model found in the nuclear chart and motivates the explicit inclusion of $\alpha$ clustering for full convergence of $E2$ collective properties.

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arXiv2024

Understanding the total width of the $3_{1}^{-}$ state in $\mathrm{^{12}C}$

Recent measurements indicate that the previously established upper limit for the $γ$-decay branch of the $3_{1}^{-}$ resonance in $^{12}\textrm{C}$ at $E_{x} = 9.641(5)$ MeV may be incorrect. As a result, the $3_{1}^{-}$ resonance has been suggested as a significant resonance for mediating the triple-$α$ reaction at high temperatures above 2 GK. Accurate estimations of the $3_{1}^{-}$ contribution to the triple-$α$ reaction rate require accurate knowledge of not only the radiative width, but also the total width. In anticipation of future measurements to more accurately determine the $γ$-decay branch of the $3_{1}^{-}$ resonance, the objective of this work is to accurately determine the total width of the $3_{1}^{-}$ resonance. An evaluation was performed on all previous results considered in the current ENSDF average of 46(3) keV for the physical total width (FWHM) of the $3_{1}^{-}$ resonance in $^{12}\textrm{C}$. Significant unaccounted-for uncertainties and a misstated result were discovered in these previous results, leading to an invalid ENSDF average. In this work, the new global \textbf{R}-matrix analysis performed on direct-reaction data yields a formal total width of $Γ(E_{r}) = 46(2)$ keV and an observed total width of $Γ_{\textrm{obs}}(E_{r}) = 38(2)$ keV for the $3_{1}^{-}$ resonance. An observed total width of $Γ_{\textrm{obs}}(E_{r}) = 38(2)$ keV is recommended for the $3_{1}^{-}$ resonance in $\mathrm{^{12}C}$. This observed total width should be employed for future evaluations of the observed total radiative width for the $3_{1}^{-}$ resonance and its contribution to the high-temperature triple-$α$ reaction rate.

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arXiv2023

Proton-unbound states in $^{24}{\rm Al}$ relevant for the $^{23}{\rm Mg}(p,\gamma)$ reaction in novae

Background: The nucleosynthesis of several proton-rich nuclei is determined by radiative proton-capture reactions on unstable nuclei in nova explosions. One such reaction is $^{23}{\rm Mg}(p,\gamma)^{24}{\rm Al}$, which links the NeNa and MgAl cycles in oxygen-neon (ONe) novae. Purpose: To extract $^{23}{\rm Mg}(p,\gamma)$ resonance strengths from a study of proton-unbound states in $^{24}{\rm Al}$, produced via the $^{24}$Mg($^{3}$He,$t$) reaction. Methods: A beam of $^3 {\rm He}^{2+}$ ions at 50.7 MeV was used to produce the states of interest in $^{24}$Al. Proton-triton angular correlations were measured with a $K=600$ QDD magnetic spectrometer and a silicon detector array, located at iThemba LABS, South Africa. Results: We measured the excitation energies of the four lowest proton-unbound states in $^{24}$Al and place lower-limits on $\Gamma_p/\Gamma$ values for these four states. Together with shell-model calculations of partial gamma widths, the experimental data are also used to determine resonance strengths for the three lowest $^{23}{\rm Mg}(p,\gamma)^{24}{\rm Al}$ resonances. Conclusions: The energy of the dominant first $^{23}{\rm Mg}(p,\gamma)$ resonance is determined to be $E_{r} = 478 \pm 4$ keV, with a resonance strength $\omega \gamma = 19 \pm 9$ meV.

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arXiv2023

Searching for resonance states in $^{22}$Ne($p,γ$)$^{23}$Na

Background: Globular clusters show strong correlations between different elements, such as the well-known sodium-oxygen anticorrelation. One of the main sources of uncertainty in this anticorrelation is the $^{22}$Ne($p,γ$)$^{23}$Na reaction rate, due to the possible influence of an unobserved resonance state at $E_\mathrm{x} = 8862$ keV ($E_\mathrm{r, c.m.} = 68$ keV). The influence of two higher-lying resonance states at $E_\mathrm{x} = 8894$ and $9000$ keV has already been ruled out by direct $^{22}$Ne($p,γ$)$^{23}$Na measurementsPurpose: To study excited states in $^{23}$Na above the proton threshold to determine if the unconfirmed resonance states in $^{23}$Na exist. Methods: The non-selective proton inelastic scattering reaction at low energies was used to search for excited states in $^{23}$Na above the proton threshold. Protons scattered from various targets were momentum-analysed in the Q3D magnetic spectrograph at the Maier-Leibnitz Laboratorium, Munich, Germany. Results: The resonance states previously reported at $E_\mathrm{x} = 8862$, $8894$ and $9000$ keV in other experiments were not observed in the present experiment at any angle. This result, combined with other non-observations of these resonance states in most other experiments, results in a strong presumption against the existence of these resonance states. Conclusions: The previously reported resonance states at $E_\mathrm{x} = 8862$, $8894$ and $9000$ keV are unlikely to exist and should be omitted from future evaluations of the $^{22}$Ne($p,γ$)$^{23}$Na reaction rates. Indirect studies using low-energy proton inelastic scattering are a simple and yet exceptionally powerful tool in helping to constrain astrophysical reaction rates by providing non-selective information of the excited states of nuclei.

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arXiv2023

Fine structure of the isoscalar giant monopole resonance in $^{58}$Ni, $^{90}$Zr, $^{120}$Sn and $^{208}$Pb

Over the past two decades high energy-resolution inelastic proton scattering studies were used to gain an understanding of the origin of fine structure observed in the isoscalar giant quadrupole resonance (ISGQR) and the isovector giant dipole resonance (IVGDR). Recently, the isoscalar giant monopole resonance (ISGMR) in $^{58}$Ni, $^{90}$Zr, $^{120}$Sn and $^{208}$Pb was studied at the iThemba Laboratory for Accelerator Based Sciences (iThemba LABS) by means of inelastic $α$-particle scattering at very forward scattering angles (including $0\circ$). The good energy resolution of the measurement revealed significant fine structure of the ISGMR.~To extract scales by means of wavelet analysis characterizing the observed fine structure of the ISGMR in order to investigate the role of different mechanisms contributing to its decay width. Characteristic energy scales are extracted from the fine structure using continuous wavelet transforms. The experimental energy scales are compared to different theoretical approaches performed in the framework of quasiparticle random phase approximation (QRPA) and beyond-QRPA including complex configurations using both non-relativistic and relativistic density functional theory. All models highlight the role of Landau fragmentation for the damping of the ISGMR especially in the medium-mass region. Models which include the coupling between one particle-one hole (1p-1h) and two particle-two hole (2p-2h) configurations modify the strength distributions and wavelet scales indicating the importance of the spreading width. The effect becomes more pronounced with increasing mass number. Wavelet scales remain a sensitive measure of the interplay between Landau fragmentation and the spreading width in the description of the fine structure of giant resonances.

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arXiv2023

$^{138}{\rm Ba}(d,α)$ study of states in $^{136}{\rm Cs}$: Implications for new physics searches with xenon detectors

We used the $^{138}$Ba$(d,α)$ reaction to carry out an in-depth study of states in $^{136}$Cs, up to around 2.5~MeV. In this work, we place emphasis on hitherto unobserved states below the first $1^+$ level, which are important in the context of solar neutrino and fermionic dark matter (FDM) detection in large-scale xenon experiments. We identify for the first time candidate metastable states in $^{136}$Cs, which would allow a real-time detection of solar neutrino and FDM events in xenon detectors, with high background suppression. Our results are also compared with shell-model calculations performed with three Hamiltonians that were previously used to evaluate the nuclear matrix element (NME) for $^{136}$Xe neutrinoless double beta decay. We find that one of these Hamiltonians, which also systematically underestimates the NME compared to the others, dramatically fails to describe the observed low-energy $^{136}$Cs spectrum, while the other two show reasonably good agreement.

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arXiv2023

Isoscalar giant monopole strength in $^{58}$Ni, $^{90}$Zr, $^{120}$Sn and $^{208}$Pb

Inelastic $α$-particle scattering at energies of a few hundred MeV and very-forward scattering angles including $0^\circ$ has been established as a tool for the study of the isoscalar giant monopole (IS0) strength distributions in nuclei. An independent investigation of the IS0 strength in nuclei across a wide mass range was performed using the $0^\circ$ facility at iThemba Laboratory for Accelerator Based Sciences (iThemba LABS), South Africa, to understand differences observed between IS0 strength distributions in previous experiments performed at the Texas A\&M University (TAMU) Cyclotron Institute, USA and the Research Center for Nuclear Physics (RCNP), Japan. The isoscalar giant monopole resonance (ISGMR) was excited in $^{58}$Ni, $^{90}$Zr, $^{120}$Sn and $^{208}$Pb using $α$-particle inelastic scattering with $196$ MeV $α$ beam and scattering angles $θ_{\text{Lab}} = 0^\circ$ and $4^\circ$. The K$600$ magnetic spectrometer at iThemba LABS was used to detect and momentum analyze the inelastically scattered $α$ particles. The IS0 strength distributions in the nuclei studied were deduced with the difference-of-spectra (DoS) technique including a correction factor for the $4^\circ$ data based on the decomposition of $L > 0$ cross sections in previous experiments. IS0 strength distributions for $^{58}$Ni, $^{90}$Zr, $^{120}$Sn and $^{208}$Pb are extracted in the excitation-energy region $E_{\rm x} = 9 - 25$ MeV.Using correction factors extracted from the RCNP experiments, there is a fair agreement with their published IS0 results. Good agreement for IS0 strength in $^{58}$Ni is also obtained with correction factors deduced from the TAMU results, while marked differences are found for $^{90}$Zr and $^{208}$Pb.

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arXiv2022

Proton decays from $α$-unbound states in $^{22}$Mg and the $^{18}$Ne($α, p_{0}$)$^{21}$Na cross section

This paper examines the $^{18}$Ne($α, p_{0}$)$^{21}$Na cross-section relevant in X-ray bursts. The study was performed with the K600 magnetic spectrometer in coincidence with the CAKE, a silicon detector array, at iThemba LABS in Cape Town, South Africa. A 100-MeV proton beam was impinged on a $^{24}$Mg target to study the $^{24}$Mg($p,t$)$^{22}$Mg reaction. The triton ejectiles were momentum-analysed with the magnetic spectrometer and proton decays from the $^{22}$Mg recoil nucleus to the ground state of $^{21}$Na and various excited states thereof were detected with the CAKE. In doing so, we were able to compare our results to previous direct and indirect measurements of the $^{18}$Ne($α, p$)$^{21}$Na reaction.

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arXiv2022

PANDORA project: photo-nuclear reactions below $A=60$

Photo-nuclear reactions of light nuclei below a mass of $A=60$ are studied experimentally and theoretically by the PANDORA (Photo-Absorption of Nuclei and Decay Observation for Reactions in Astrophysics) project. Two experimental methods, virtual-photon excitation by proton scattering and real-photo absorption by a high-brilliance gamma-ray beam produced by laser Compton scattering, will be applied to measure the photo-absorption cross sections and the decay branching ratio of each decay channel as a function of the photon energy. Several nuclear models, e.g. anti-symmetrized molecular dynamics, mean-field type models, a large-scale shell model, and ab initio models, will be employed to predict the photo-nuclear reactions. The uncertainty in the model predictions will be evaluated from the discrepancies between the model predictions and the experimental data. The data and the predictions will be implemented in a general reaction calculation code TALYS . The results will be applied to the simulation of the photo-disintegration process of ultra-high-energy cosmic rays in inter-galactic propagation.

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arXiv2022

New measurement of the $E_{\mathrm{c.m.}}=323$ keV resonance in the $^{19}$F$($p,γ$)$^{20}$Ne reaction

At temperatures below 0.1 GK the $^{19}$F$(p,γ)^{20}$Ne reaction is the only breakout path out of the CNO cycle. Experimental studies of this reaction are challenging from a technical perspective due to copious $γ$-ray background from the far stronger $^{19}$F$(p,α)^{16}$O reaction channel. Here we present the first inverse kinematics study of the $^{19}$F$(p,γ)^{20}$Ne reaction, in which we measure the strength of the 323-keV resonance. We find a strength value of $ωγ= 3.3^{+1.1}_{-0.9}$ meV, which is a factor of two larger than the most recent previous study. The discrepancy is likely the result of a direct to ground state transition which previous studies were not sensitive to. We also observe the transition to the first $2^{-}$ state, which has not been observed for this resonance in previous studies. A new thermonuclear reaction rate is calculated and compared with the literature.

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arXiv2022

Constraints on key $^{17}$O($α,γ$)$^{21}$Ne resonances and impact on the weak s-process

The efficiency of the slow neutron-capture process in massive stars is strongly influenced by neutron-capture reactions on light elements. At low metallicity, $^{16}$O is an important neutron absorber, but the effectiveness of $^{16}$O as a light-element neutron poison is modified by competition between subsequent $^{17}$O$(α,n)^{20}$Ne and $^{17}$O$(α,γ)^{21}$Ne reactions. The strengths of key $^{17}$O$(α,γ)^{21}$Ne resonances within the Gamow window for core helium burning in massive stars are not well constrained by experiment. This work presents more precise measurements of resonances in the energy range $E_{c.m.} = 612 - 1319$ keV. We extract resonance strengths of $ωγ_{638} = 4.85\pm0.79$ $μ$eV, $ωγ_{721} = 13.0^{+3.3}_{-2.4}$ $μ$eV, $ωγ_{814} = 7.72\pm0.55$ meV and $ωγ_{1318} = 136\pm 13$ meV, for resonances at $E_{c.m.} =$ 638, 721, 814 and 1318 keV, respectively. We also report an upper limit for the 612 keV resonance of $ωγ<140$ neV ($95\%$ c.l.), which effectively rules out any significant contribution from this resonance to the reaction rate. From this work, a new $^{17}$O$(α,γ)^{21}$Ne thermonuclear reaction rate is calculated and compared to the literature. The effect of present uncertainties in the $^{17}$O$(α,γ)^{21}$Ne reaction rate on weak s-process yields are then explored using post-processing calculations based on a rotating $20M_{\odot}$ low-metallicity massive star. The resulting $^{17}$O$(α,γ)^{21}$Ne reaction rate is lower with respect to the pre-existing literature and found to enhance weak s-process yields in rotating massive star models.

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arXiv2022

The impact of $^{17}$O$+α$ reaction rate uncertainties on the s-process in rotating massive stars

Massive stars are crucial to galactic chemical evolution for elements heavier than iron. Their contribution at early times in the evolution of the Universe, however, is unclear due to poorly constrained nuclear reaction rates. The competing $^{17}$O($α,γ$)$^{21}$Ne and $^{17}$O($α,n$)$^{20}$Ne reactions strongly impact weak s-process yields from rotating massive stars at low metallicities. Abundant $^{16}$O absorbs neutrons, removing flux from the s-process, and producing $^{17}$O. The $^{17}$O($α,n$)$^{20}$Ne reaction releases neutrons, allowing continued s-process nucleosynthesis, if the $^{17}$O($α,γ$)$^{21}$Ne reaction is sufficiently weak. While published rates are available, they are based on limited indirect experimental data for the relevant temperatures and, more importantly, no uncertainties are provided. The available nuclear physics has been evaluated, and combined with data from a new study of astrophysically relevant $^{21}$Ne states using the $^{20}$Ne($d,p$)$^{21}$Ne reaction. Constraints are placed on the ratio of the ($α,n$)/($α,γ$) reaction rates with uncertainties on the rates provided for the first time. The new rates favour the ($α,n$) reaction and suggest that the weak s-process in rotating low-metallicity stars is likely to continue up to barium and, within the computed uncertainties, even to lead.

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arXiv2022

Horizons: Nuclear Astrophysics in the 2020s and Beyond

Nuclear Astrophysics is a field at the intersection of nuclear physics and astrophysics, which seeks to understand the nuclear engines of astronomical objects and the origin of the chemical elements. This white paper summarizes progress and status of the field, the new open questions that have emerged, and the tremendous scientific opportunities that have opened up with major advances in capabilities across an ever growing number of disciplines and subfields that need to be integrated. We take a holistic view of the field discussing the unique challenges and opportunities in nuclear astrophysics in regards to science, diversity, education, and the interdisciplinarity and breadth of the field. Clearly nuclear astrophysics is a dynamic field with a bright future that is entering a new era of discovery opportunities.

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arXiv2022

Evolution of the isoscalar giant monopole resonance in the Ca isotope chain

Two recent studies of the evolution of the isoscalar giant monopole resonance (ISGMR) within the calcium isotope chain report conflicting results. One study suggests that the monopole resonance energy, and thus the incompressibility of the nucleus $K_{A}$ increase with mass, which implies that $K_τ$, the asymmetry term in the nuclear incompressibility, has a positive value. The other study reports a weak decreasing trend of the energy moments, resulting in a generally accepted negative value for $K_τ$. An independent measurement of the central region of the ISGMR in the Ca isotope chain is provided to gain a better understanding of the origin of possible systematic trends. Inelastically scattered $α$ particles from a range of calcium targets ($\mathrm{^{40,42,44,48}Ca}$), observed at small scattering angles including 0$^\circ$, were momentum analyzed in the K600 magnetic spectrometer at iThemba LABS, South Africa. Monopole strengths spanning an excitation-energy range between 9.5 and 25.5 MeV were obtained using the difference-of-spectra (DoS) technique. The structure of the $E0$ strength distributions of $^{40,42,44}$Ca agrees well with the results from the previous measurement that supports a weak decreasing trend of the energy moments, while no two datasets agree in the case of $^{48}$Ca. Despite the variation in the structural character of $E0$ strength distribution from different studies, we find for all datasets that the moment ratios, calculated from the ISGMR strength in the excitation-energy range that defines the main resonance region, display at best only a weak systematic sensitivity to a mass increase. Different trends observed in the nuclear incompressibility are caused by contributions to the $E0$ strength outside of the main resonance region, and in particular for high excitation energies.

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arXiv2022

Multi-probe study of excited states in $\mathrm{^{12}C}$: disentangling the sources of monopole strength between the Hoyle state and $E_{x} = 13$ MeV

Knowledge of the low-lying monopole strength in $\mathrm{^{12}C}$, the Hoyle state in particular, is crucial for our understanding of both the astrophysically important $3α$ reaction and of $α$-particle clustering. The $\mathrm{^{12}C}(α, α^{\prime})\mathrm{^{12}C}$ and $\mathrm{^{14}C}(p, t)\mathrm{^{12}C}$ reactions were employed to populate states in $^{12}$C. A self-consistent, simultaneous analysis of the inclusive spectra with lineshapes was performed, which accounted for distortion due to nuclear dynamics and experimental effects. Clear evidence was found for excess monopole strength at $E_{x} \sim 9$ MeV, particularly in the $\mathrm{^{12}C}(α, α^{\prime})\mathrm{^{12}C}$ reaction at $0^{\circ}$. This additional strength cannot be reproduced by the previously established monopole states between $E_{x} = 7$ and 13 MeV. An additional $0^{+}$ state at $E_{x} \sim 9$ MeV yielded a significantly improved fit of the data and is the leading candidate for the predicted breathing-mode excitation of the Hoyle state. Alternatively, the results may suggest that a more sophisticated, physically motivated parameterization of the astrophysically important monopole strengths in $\mathrm{^{12}C}$ is required.

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arXiv2022

Investigating the predicted breathing-mode excitation of the Hoyle state

Knowledge of the low-lying monopole strength in $\mathrm{^{12}C}$ $-$ the Hoyle state in particular $-$ is crucial for our understanding of both the astrophysically important $3α$ reaction and of $α$-particle clustering. Multiple theoretical models have predicted a breathing mode of the Hoyle State at $E_{x} \approx 9$ MeV, corresponding to a radial in-phase oscillation of the underlying $α$ clusters. The $\mathrm{^{12}C}(α, α^{\prime})\mathrm{^{12}C}$ and $\mathrm{^{14}C}(p, t)\mathrm{^{12}C}$ reactions were employed to populate states in $^{12}$C in order to search for this predicted breathing mode. A self-consistent, simultaneous analysis of the inclusive spectra with R-matrix lineshapes, together with angular distributions of charged-particle decay, yielded clear evidence for excess monopole strength at $E_{x} \approx 9$ MeV which is highly collective. Reproduction of the experimentally observed inclusive yields using a fit, with consistent population ratios for the various broad states, required an additional source of monopole strength. The interpretation of this additional monopole resonance as the breathing-mode excitation of the Hoyle state would provide evidence supporting a $\mathcal{D}_{3h}$ symmetry for the Hoyle state itself. The excess monopole strength may complicate analysis of the properties of the Hoyle state, modifying the temperature dependence of the $3α$ rate at $T_{9} \gtrsim 2$ and ultimately, the predicted nucleosynthesis in explosive stars.

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arXiv2022

Experimental study of the $^{30}$Si($^{3}$He,$d$)$^{31}$P reaction and thermonuclear reaction rate of $^{30}$Si($p$,$γ$)$^{31}$P

[Background] Abundance anomalies in some globular clusters, such as the enhancement of potassium and the depletion of magnesium, can be explained in terms of an earlier generation of stars polluting the presently observed ones. It was shown that the potential range of temperatures and densities of the polluting sites depends on the strength of a few number of critical reaction rates. The reaction has been identified as one of these important reactions. [Purpose] The key ingredient for evaluating the thermonuclear reaction rate is the strength of the resonances which, at low energy, are proportional to their proton width. Therefore the goal of this work is to determine the proton widths of unbound 31P states. [Method] States in 31P were studied at the Maier-Leibnitz-Laboratorium using the one-proton transfer reaction. Deuterons were detected with the Q3D magnetic spectrometer. Angular distribution and spectroscopic factors were extracted for 27 states, and proton widths and resonance strengths were calculated for the unbound states. [Results] Several unbound states have been observed for the first time in a one-proton transfer reaction. Above 20 MK, the reaction rate is now entirely estimated from the observed properties of states. The reaction rate uncertainty from all resonances other than the resonance has been reduced down to less than a factor of two above that temperature. The unknown spin and parity of the resonance dominates the uncertainty in the rate in the relevant temperature range. [Conclusion] The remaining source of uncertainty on the reaction rate comes from the unknown spin and parity of the resonance which can change the reaction rate by a factor of ten in the temperature range of interest.

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