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P. Bourges

Publications and source records attributed to P. Bourges.

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Resonant Spin Excitation in an Overdoped High Temperature Superconductor

An inelastic neutron scattering study of overdoped Bi_2Sr_2CaCu_2O_{8+δ} $ (T_c = 83 K) has revealed a resonant spin excitation in the superconducting state. The mode energy is E_res=38 meV, significantly lower than in optimally doped Bi_2Sr_2CaCu_2O_{8+δ} (T_c = 91 K, E_ res =43 meV). This observation, which indicates a constant ratio E_res /k_B T_c \sim 5.4, helps resolve a long-standing controversy about the origin of the resonant spin excitation in high-temperature superconductors.

cond-mat.supr-con↗

Magnetic resonance peak and nonmagnetic impurities

Nonmagnetic Zn impurities are known to strongly suppress superconductivity. We review their effects on the spin excitation spectrum in $\rm YBa_2Cu_3O_{7}$, as investigated by inelastic neutron scattering measurements.

cond-mat.supr-con↗

The Spin Excitation Spectrum in Superconducting ${\bf YBa_2Cu_3O_{6.85}}$

A comprehensive inelastic neutron scattering study of magnetic excitations in the near-optimally doped high-temperature superconductor ${\rm YBa_{2}Cu_{3}O_{6.85}}$ is presented. The spin correlations in the normal state are commensurate with the crystal lattice, and the intensity is peaked around the wave vector characterizing the antiferromagnetic state of the insulating precursor ${\rm YBa_{2}Cu_{3}O_{6}}$. Profound modifications of the spin excitation spectrum appear abruptly below the superconducting transition temperature, $\rm T_C$, where a commensurate resonant mode and a set of weaker incommensurate peaks develop. The data are consistent with models based on an underlying two-dimensional Fermi surface that predict a continuous, downward dispersion relation connecting the resonant mode and the incommensurate excitations. The magnetic incommensurability in the ${\rm YBa_{2}Cu_{3}O_{6+x}}$ system is thus not simply related to that of another high temperature superconductor, ${\rm La_{2-x}Sr_xCuO_{4}}$, where incommensurate peaks persist well above $\rm T_C$. The temperature dependent incommensurability is difficult to reconcile with interpretations based on charge stripe formation in ${\rm YBa_{2}Cu_{3}O_{6+x}}$ near optimum doping.

cond-mat.supr-con↗

Spin Susceptibility in Underdoped $\bf YBa_2Cu_3O_{6+x}$

We report a comprehensive polarized and unpolarized neutron scattering study of the evolution of the dynamical spin susceptibility with temperature and doping in three underdoped single crystals of the \YBCO{6+x} high temperature superconductor: \YBCO{6.5} (Tc = 52 K), \YBCO{6.7} (Tc = 67 K), and \YBCO{6.85} (T_c = 87 K). Theoretical implications of these data are discussed, and a critique of recent attempts to relate the spin excitations to the thermodynamics of high temperature superconductors is given.

cond-mat.supr-con↗

Quantum Impurities and the Neutron Resonance Peak in ${\bf YBa_2 Cu_3 O_7}$: Ni versus Zn

The influence of magnetic (S=1) and nonmagnetic (S=0) impurities on the spin dynamics of an optimally doped high temperature superconductor is compared in two samples with almost identical superconducting transition temperatures: YBa$_2$(Cu$_{0.97}$Ni$_{0.03}$)$_3$O$_7$ (T$_c$=80 K) and YBa$_2$(Cu$_{0.99}$Zn$_{0.01}$)$_3$O$_7$ (T$_c$=78 K). In the Ni-substituted system, the magnetic resonance peak (which is observed at E$_r \simeq$40 meV in the pure system) shifts to lower energy with a preserved E$_r$/T$_c$ ratio while the shift is much smaller upon Zn substitution. By contrast Zn, but not Ni, restores significant spin fluctuations around 40 meV in the normal state. These observations are discussed in the light of models proposed for the magnetic resonance peak.

cond-mat.supr-con↗

Neutron Scattering from Magnetic Excitations in Bi_2 Sr_2 Ca_2 O_8+delta

Many physical properties of the copper oxide high temperature superconductors appear to defy the conventional (one-electron) theory of metals, and the development of new theories incorporating strong electron correlations is currently at the forefront of condensed matter physics. Inelastic neutron scattering provides incisive information about collective magnetic excitations that is required to guide this effort. Such measurements have thus far proven possible for only two of the many families of high temperature superconductors, La_{2-x} Sr_x CuO_4 and YBa_2 Cu_3 O_{6+x},because suitably large single crystals of other copper oxide compounds could not be grown. While the magnetic spectra of both materials bear certain similarities, there are also pronounced differences that have hampered a unified description of the spin dynamics in the copper oxides. In particular, a sharp resonant spin excitation dominates the spectrum in the superconducting state of YBa_2 Cu_3 O_{6+x}, but is not found in La_{2-x} Sr_x CuO_4. Here we report the discovery of a magnetic resonance peak in the superconducting state of a different copper oxide system, Bi_2 Sr_2 Ca Cu_2 O_{8+δ}, made possible by the synthesis of a sizable single crystal and modern neutron optics. This provides evidence of the generality of this unusual phenomenon among the copper oxides and greatly extends the empirical basis for its theoretical description.

cond-mat.supr-con↗

Evidence for incommensurate spin fluctuations in Sr_2RuO_4

We report first inelastic neutron scattering measurements in the normal state of Sr_2RuO_4 that reveal the existence of incommensurate magnetic spin fluctuations located at ${\bf q}_0=(\pm 0.6π/a, \pm 0.6π/a, 0)$. This finding confirms recent band structure calculations that have predicted incommensurate magnetic responses related to dynamical nesting properties of its Fermi surface.

cond-mat.supr-con↗

Linear dependence of peak width in $χ(\bq, ω)$ vs T_c for YBCO superconductors

It is shown that the momentum space width of the peak in the spin susceptibility, Im$χ(q,ω)$, is linearly proportional to the superconducting $T_c$: $T_c = \hbar v^*Δq$ with $\hbar v^* \simeq 35 meV$Å. This relation is similar to the linear relation between incommensurate peak splitting and $T_c$ in LaSrCuO superconductors, as first proposed by Yamada et al. (Phys. Rev. B 57, 6165, (1998)). The velocity $\hbar v^*$ is smaller than Fermi velocity or the spin-wave velocity of the parent compound and remains the same for a wide doping range. This result points towards strong similarities in magnetic state of YBCO and LaSrCuO.

cond-mat.supr-con↗

Effect of Nonmagnetic Impurities on the Magnetic Resonance Peak in YBa2Cu3O7

The magnetic excitation spectrum of a YBa_2 Cu_3 O_7 crystal containing 0.5% of nonmagnetic (Zn) impurities has been determined by inelastic neutron scattering. Whereas in the pure system a sharp resonance peak at E ~ 40 meV is observed exclusively below the superconducting transition temperature T_c, the magnetic response in the Zn-substituted system is broadened significantly and vanishes at a temperature much higher than T_c. The energy-integrated spectral weight observed near q = (pi,pi) increases with Zn substitution, and only about half of the spectral weight is removed at T_c.

cond-mat.supr-con↗

Superexchange coupling and spin susceptibility spectral weight in undoped monolayer cuprates

A systematic inelastic neutron scattering study of the superexchange interaction in three different undoped monolayer cuprates (La_2CuO_4, Nd_2CuO_4 and Pr_2CuO_4) has been performed using conventional triple axis technique. We deduce the in-plane antiferromagnetic (AF) superexchange coupling $J$ which actually presents no simple relation versus crystallographic parameters. The absolute spectral weight of the spin susceptibility has been obtained and it is found to be smaller than expected even when quantum corrections of the AF ground state are taken into account.

cond-mat.str-el↗