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P. C. Canfield

Publications and source records attributed to P. C. Canfield.

At least 271 records · Page 15Linked to original sources
arXiv2009

Competition and coexistence of antiferromagnetism and superconductivity in underdoped Ba(Fe0.953Co0.047)2As2

Neutron and x-ray diffraction studies show that the simultaneous first-order transition to an orthorhombic and antiferromagnetic (AFM) ordered state in BaFe2As2 splits into two transitions with Co doping. For Ba(Fe0.953Co0.047)2As2, a tetragonal-orthorhombic transition occurs at TS = 60 K, followed by a second-order transition to AFM order at TN = 47 K. Superconductivity (SC) occurs in the orthorhombic state below TC = 15 K and coexists with AFM. Below TC, the static Fe moment is reduced and a 4 meV spin gap develops indicating competition between coexisting SC and AFM order.

cond-mat.supr-con↗
arXiv2009

Non-exponential London penetration depth in RFeAsO$_{0.9}$F$_{0.1}$ (R=La,Nd) single crystals

The superconducting penetration depth, $λ(T)$, has been measured in RFeAsO$_{0.9}$F$_{0.1}$ (R=La,Nd) single crystals (R-1111). In Nd-1111, we find an upturn in $λ(T)$ upon cooling and attribute it to the paramagnetism of the Nd ions, similar to the case of the electron-doped cuprate Nd-Ce-Cu-O. After the correction for paramagnetism, the London penetration depth variation is found to follow a power-law behavior, $Δλ_L(T)\propto T^{2}$ at low temperatures. The same $T^2$ variation of $λ(T)$ was found in non-magnetic La-1111 crystals. Analysis of the superfluid density and of penetration depth anisotropy over the full temperature range is consistent with two-gap superconductivity. Based on this and on our previous work, we conclude that both the RFeAsO (1111) and BaFe$_2$As$_2$ (122) families of pnictide superconductors exhibit unconventional two-gap superconductivity.

cond-mat.supr-con↗
arXiv2009

Resistivity Anisotropy of $AE$Fe$_2$As$_2$ ($AE$ =Ca, Sr, Ba): direct versus Montgomery technique measurements

The anisotropy of electrical resistivity was measured in parent compounds of the iron-arsenic high temperature superconductors, AEFe2As2 with Alkali Earth elements AE=Ca,Sr, Ba. Measurements were performed using both the Montgomery technique and direct resistivity measurements on samples cut along principal crystallographic directions. The anisotropy ratio γ_ρ=ρ_c/ρ_a is well below 10 for all compounds in the whole temperature range studied (4 to 300 K), in notable contrast to previous reports. The anisotropy at room temperature increases from about 2 in Ca, to about 4 in Sr and Ba. In all compounds the resistivity ratio decreases on cooling through the structural/antiferromagnetic transition temperature T_{SM}, with the change mainly coming from stronger variation in ρ_a as compared with ρ_c. This suggests that the transitions stronger affect the two-dimensional parts of the Fermi surface. We compare our experimental observations with band structure calculations, and find similar trend in the evolution of anisotropy with the size of AE ion. Our results show that the electronic structure of the iron pnictides has large contribution from three-dimensional areas of the Fermi surface.

cond-mat.supr-con↗
arXiv2009

Point contact Andreev reflection spectroscopy of superconducting energy gaps in 122-type family of iron pnictides

A brief overview of the superconducting energy gap studies on 122-type family of iron pnictides is given. It seems that the situation in the hole-doped Ba1-xKxFe2As2 is well resolved. Most of the measurements including the presented here point-contact Andreev reflection spectra agree on existence of multiple nodeless gaps in the excitation spectrum of this multiband system. The gaps have basically two sizes - the small one with a strength up to the BCS weak coupling limit and the large one with a very strong coupling with 2Delta/kTc ~ 6 - 8. In the electron doped Ba(Fe1-xCox)2As2 the most of the experiments including our point contact measurements reveal in quite broadened spectra only a single gap with a strong coupling strength. The high precision ARPES measurements on this system identified two gaps but very close to each other, both showing a strong coupling with 2Delta/kTc ~ 5 and 6, respectively.

cond-mat.supr-con↗
arXiv2009

Non-exponential London penetration depth in Ba$_{1-}$K$_{x}$Fe$_{2}$As$_{2}$ single crystals

We have studied the in- and out-of-plane magnetic penetration depths in the hole- doped iron based superconductor Ba$_{1-x}$K$_{x}$Fe$_{2}$As$_{2}$ ($T_{c}\approx$ 30K). The study was performed on single crystals grown from different fluxes and we find that the results are nearly the same. The in-plane London penetration depth $λ_{ab}$ does not show exponential saturation at low temperature, as would be expected from a fully gapped superconductor. Instead, $λ_{ab}(T)$ shows a power-law behavior, $λ\propto T^{n}$ ($n\approx 2$), down to $T\approx 0.02 T_{c}$, similar to the electron doped Ba(Fe$_{1-x}$Co$_{x}$)$_{2}$As$_{2}$. The penetration depth anisotropy $γ_λ=λ_{c}(T)/λ_{ab}(T)$ increases upon cooling, opposite to the trend observed in the anisotropy of the upper critical field, $γ_ξ=H_{c2}^{\perp c}(0)/H_{c2}^{\parallel c}(0)$. These are universal characteristics of both the electron and hole doped 122 systems, suggesting unconventional superconductivity. The behavior of the in-plane superfluid density $ρ_{ab}(T)$ is discussed in light of existing theoretical models proposed for the iron pnictides superconductors.

cond-mat.supr-con↗
arXiv2009

Electronic structure of CaFe2As2: Contribution of itinerant Fe 3d-states to the Fermi Level

We present density functional theory (DFT) calculations and a full set of X-ray spectra (resonant inelastic X-ray scattering and X-ray photoelectron spectra) measurements of single crystal CaFe2As2. The experimental valence band spectra are consistent with our DFT calculations. Both theory and experiment show that the Fe 3d-states dominate the Fermi level and hybridize with Ca 3d-states. The simple shape of Xray photoelectron (XPS) Fe 2p-core level spectrum (without any satellite structure typical for correlated systems) suggests itinerant character of the Fe 3d-electrons. Based on the similarity of the calculated and experimental Fe 3d-states distribution in LaOFeAs and CaFe2As2 we conclude that superconductivity in the FeAs-systems can be described within a minimal model, taking into account only Fe 3d-bands close to the Fermi level.

cond-mat.supr-con↗
arXiv2009

Doping dependent Irreversible Magnetic Properties of Ba(Fe1-xCox)2As2 Single Crystals

We discuss the irreversible magnetic properties of self-flux grown Ba(Fe1-xCox)2As2 single crystals for a wide range of concentrations covering the whole phase diagram from the underdoped to the overdoped regime, x=0.038, 0.047, 0.058, 0.071, 0.074, 0.10, 0.106 and 0.118. Samples were characterized by a magneto-optical method and show excellent spatial uniformity of the superconducting state. The overall behavior closely follows classical Bean model of the critical state. The field-dependent magnetization exhibits second peak at a temperature and doping - dependent magnetic field, Hp. The evolution of this fishtail feature with doping is discussed. Magnetic relaxation is time-logarithmic and unusually fast. Similar to cuprates, there is an apparent crossover from collective elastic to plastic flux creep above Hp. At high fields, the field dependence of the relaxation rate becomes doping independent. We discuss our results in the framework of the weak collective pinning and show that vortex physics in iron-based pnictide crystals is much closer to high-Tc cuprates than to conventional s-wave (including MgB2) superconductors.

cond-mat.supr-con↗
arXiv2009

Anisotropic London Penetration Depth and Superfluid Density in Single Crystals of Iron-based Pnictide Superconductors

In- and out-of-plane magnetic penetration depths were measured in three iron-based pnictide superconducting systems. All studied samples of both 122 systems show a robust power-law behavior, $λ(T) T^n$, with the sample-dependent exponent n=2-2.5, which is indicative of unconventional pairing. This scenario could be possible either through scattering in a $s_{\pm }$ state or due to nodes in the superconducting gap. In the Nd-1111 system, the interpretation of data may be obscured by the magnetism of rare-earth ions. The overall anisotropy of the pnictide superconductors is small. The 1111 system is about two times more anisotropic than the 122 system. Our data and analysis suggest that the iron-based pnictides are complex superconductors in which a multiband three-dimensional electronic structure and strong magnetic fluctuations play important roles.

cond-mat.supr-con↗
arXiv2009

Structural, magnetic and superconducting phase transitions in CaFe2As2 under ambient and applied pressure

At ambient pressure CaFe2As2 has been found to undergo a first order phase transition from a high temperature, tetragonal phase to a low temperature orthorhombic / antiferromagnetic phase upon cooling through T ~ 170 K. With the application of pressure this phase transition is rapidly suppressed and by ~ 0.35 GPa it is replaced by a first order phase transition to a low temperature collapsed tetragonal, non-magnetic phase. Further application of pressure leads to an increase of the tetragonal to collapsed tetragonal phase transition temperature, with it crossing room temperature by ~ 1.7 GPa. Given the exceptionally large and anisotropic change in unit cell dimensions associated with the collapsed tetragonal phase, the state of the pressure medium (liquid or solid) at the transition temperature has profound effects on the low temperature state of the sample. For He-gas cells the pressure is as close to hydrostatic as possible and the transitions are sharp and the sample appears to be single phase at low temperatures. For liquid media cells at temperatures below media freezing, the CaFe2As2 transforms when it is encased by a frozen media and enters into a low temperature multi-crystallographic-phase state, leading to what appears to be a strain stabilized superconducting state at low temperatures.

cond-mat.supr-con↗
arXiv2009

Probing fractal magnetic domains on multiple length scales in Nd2Fe14B

Using small-angle neutron scattering, we demonstrate that the complex magnetic domain patterns at the surface of Nd2Fe14B, revealed by quantitative Kerr and Faraday microscopy, propagate into the bulk and exhibit structural features with dimensions down to 6 nm, the domain wall thickness. The observed fractal nature of the domain structures provides an explanation for the anomalous increase in the bulk magnetization of Nd2Fe14B below the spin-reorientation transition. These measurements open up a rich playground for studies of fractal structures in highly anisotropic magnetic systems.

cond-mat.mtrl-sci↗
arXiv2009

Evidence for two-gap superconductivity in (Ba,K)Fe_2As_2 by directional point contact Andreev reflection spectroscopy

Directional point-contact Andreev-reflection spectroscopy measurements on the Ba$_{0.55}$K$_{0.45}$Fe$_2$As$_2$ single crystals are presented. The spectra show significant differences when measured in the $ab$ plane in comparison with those measured in the $c$ direction of the crystal. In the latter case only a reduced point-contact conductance around zero bias has been revealed persisting well above $T_c$ and probably related to the structural and magnetic transitions in the system. Within the $ab$ plane two superconducting energy gaps are detected below $T_c$. Here a reduced conductance above $T_c$ could also be found. The fits of the $ab$-plane data to the superconducting s-wave two-gap model indicate that the smaller gap has a size below the BCS value while the large gap reveals much higher coupling strength.

cond-mat.supr-con↗
arXiv2009

The Absence of Superconductivity in Single Phase CaFe2As2 under Hydrostatic Pressure

Recent high-pressure studies found that superconductivity can be achieved under very low pressure in the parent iron arsenide compound CaFe2As2, although details of the sharpness and temperature of transitions vary between liquid medium and gas medium measurements. To better understand this issue, we performed high-pressure susceptibility and transport studies on CaFe2As2, using helium as the pressure medium. The signatures of the transitions to the low-temperature orthorhombic and collapsed tetragonal phase remained exceptionally sharp and no signature of bulk superconductivity was found under our hydrostatic conditions. Our results suggest that phase separation and superconductivity in CaFe2As2 are induced by non-hydrostatic conditions associated with the frozen liquid media.

cond-mat.supr-con↗
arXiv2009

Thermal expansion and anisotropic pressure derivatives of T_c in Ba(Fe_{1-x}Co_x)_2As_2 single crystals

Heat capacity and anisotropic thermal expansion was measured for Ba(Fe_{1-x}Co_x)_2As_2 (x = 0, 0.038, 0.074) single crystals. Thermal expansion is anisotropic and, in tetragonal phase, is significantly higher along the c-axis. Previously reported phase transitions, including possibly split structural and magnetic for x = 0.038 are clearly seen in both measurements. Uniaxial pressure derivatives of the superconducting transition temperature inferred from the Ehrenfest relation have opposite signs for in-plane and c-axis pressures for both Ba(Fe_{0.962}Co_{0.038})_2As_2 and Ba(Fe_{0.926}Co_{0.074})_2As_2, with the opposite sign of this anisotropy.

cond-mat.supr-con↗
arXiv2008

Anisotropy of the Optimally-Doped Iron Pnictide Superconductor Ba(Fe0.926Co0.074)2As2

Anisotropies of electrical resistivity, upper critical field, London penetration depth and critical currents have been measured in single crystals of the optimally doped iron pnictide superconductor Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$, $x$=0.074 and $T_c \sim$23 K. The normal state resistivity anisotropy was obtained by employing both the Montgomery technique and direct measurements on samples cut along principal crystallographic directions. The ratio $γ_ρ = ρ_c /ρ_a$ is about 4$\pm$1 just above $T_c$ and becomes half of that at room temperature. The anisotropy of the upper critical field, $γ_{H} = H_{c2,ab} /H_{c2,c} $, as determined from specific heat measurements close to $T_c$, is in the range of 2.1 to 2.6, depending on the criterion used. A comparable low anisotropy of the London penetration depth, $γ_λ=λ_{c}/λ_{ab}$, was recorded from TDR measurements and found to persist deep into the superconducting state. An anisotropy of comparable magnitude was also found in the critical currents, $γ_j=j_{c,ab}/j_{c,c}$, as determined from both direct transport measurements ($\sim$1.5) and from the analysis of the magnetization data ($\sim$3). Overall, our results show that iron pnictide superconductors manifest anisotropies consistent with essentially three-dimensional intermetallic compound and bear little resemblance to cuprates.

cond-mat.supr-con↗
arXiv2008

Vortex studies in superconducting Ba(Fe0.93Co0.07)2As2

We present small-angle neutron scattering (SANS) and Bitter decoration studies of the superconducting vortices in Ba(Fe$_{0.93}$Co$_{0.07}$)$_2$As$_2$}. A highly disordered vortex configuration is observed at all measured fields, and is attributed to strong pinning. This conclusion is supported by the absence of a Meissner rim in decoration images obtained close to the sample edge. The field dependence of the magnitude of the SANS scattering vector indicates vortex lattice domains of (distorted) hexagonal symmetry, consistent with the decoration images which show primarily 6-fold coordinated vortex domains. An analysis of the scattered intensity shows that this decreases much more rapidly than expected from estimates of the upper critical field, consistent with the large degree of disorder.

cond-mat.supr-con↗
arXiv2008

Suppression of antiferromagnetic spin fluctuations in the collapsed tetragonal phase of CaFe2As2

Inelastic neutron scattering measurements of CaFe2As2 under applied hydrostatic pressure show that the antiferromagnetic spin fluctuations observed in the ambient pressure, paramagnetic, tetragonal (T) phase are strongly suppressed, if not absent, in the collapsed tetragonal (cT) phase. These results are consistent with a quenched Fe moment in the cT phase and the strong decrease in resistivity observed upon crossing the boundary from the T to cT phase. The suppression or absence of static antiferromagnetic order and dynamic spin fluctuations in the non-superconducting cT phase supports the notion of a coupling between spin fluctuations and superconductivity in the iron arsenides.

cond-mat.supr-con↗
arXiv2008

Upper and lower critical fields in NdFeAs(O,F) single crystals : a study by Hall probe magnetization and specific heat

The upper and lower critical fields have been deduced from specific heat and Hall probe magnetization measurements in non-optimally doped NdFeAs(O,F) single crystals ($T_c \sim 32-35$K). The anisoptropy of the penetration depth ($Γ_λ$) is temperature independent and on the order of $4.0 \pm 1.5$. Similarly specific heat data lead an anisotropy of the coherence lenght $Γ_ξ\sim 5.5 \pm 1.5$ close to $T_c$. Our results suggest the presence of rather large thermal fluctuations and to the existence of a vortex liquid phase over a broad temperature range ($\sim 5$K large at 2T).

cond-mat.supr-con↗