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P. C. Canfield

Publications and source records attributed to P. C. Canfield.

422 records · Page 24Linked to original sources

Unconventional electronic Raman spectra of borocarbide superconductors

Borocarbide superconductors, which are thought to be conventional BCS-type superconductors, are not so conventional in several electronic Raman properties. Anisotropic gap-like features and finite scattering strength below the gap were observed for the $R$Ni$_2$B$_2$C ($R$ = Lu, Y) systems in our previous study. The effects of Co-doping on the 2$Δ$ gap-like features and the finite scattering strength below and above the gap are studied in $R$ = Lu (B = B$^{11}$) system. In superconducting states, Co-doping strongly suppresses the 2$Δ$ peak in both B$_{2g}$ and B$_{1g}$ symmetries. Raman cross-section calculation which includes inelastic scattering shows a relatively good fit to the features above the 2$Δ$ peak, while it does not fully account for the features below the peak.

cond-mat.supr-con↗

Interdependence of magnetism and superconductivity in the borocarbide TmNi2B2C

We have discovered a new antiferromagnetic phase in TmNi2B2C by neutron diffraction. The ordering vector is Q_A = (0.48,0,0) and the phase appears above a critical in-plane magnetic field of 0.9 T. The field was applied in order to test the assumption that the zero-field magnetic structure at Q_F = (0.094,0.094,0) would change into a c-axis ferromagnet if superconductivity were destroyed. We present theoretical calculations which show that two effects are important: A suppression of the ferromagnetic component of the RKKY exchange interaction in the superconducting phase, and a reduction of the superconducting condensation energy due to the periodic modulation of the moments at the wave vector Q_A.

cond-mat↗

Nesting properties and anisotropy of the Fermi surface of LuNi$_{2}$B$_{2}$C

The rare earth nickel borocarbides, with the generic formula $R$Ni$_{2}$B$_{2}$C, have recently been shown to display a rich variety of phenomena. Most striking has been the competition between, and even coexistence of, antiferromagnetism and superconductivity. We have measured the Fermi surface (FS) of LuNi$_{2}$B$_{2}$C, and shown that it possesses nesting features capable of explaining some of the phenomena experimentally observed. In particular, it had previously been conjectured that a particular sheet of FS is responsible for the modulated magnetic structures manifest in some of the series. We report the first direct experimental observation of this sheet.

cond-mat↗

Heat Capacity Measurements in Pulsed Magnetic Fields

The new NHMFL 60T quasi-continuous magnet produces a flat-top field for a period of 100 ms at 60 Tesla, and for longer time at lower fields, e.g. 0.5 sec at 35 Tesla. We have developed for the first time the capability to measure heat capacity at very high magnetic fields in the NHMFL 60 T quasi-continuous magnet at LANL, using a probe built out of various plastic materials. The field plateau allows us to utilize a heat-pulse method to obtain heat capacity data. Proof-of-principle heat capacity experiments were performed on a variety of correlated electron systems. Both magnet performance characteristics and physical properties of various materials studied hold out a promise of wide application of this new tool.

cond-mat.str-el↗

Magnetic Field Dependence of the Low-Temperature Specific Heat in PrInAg_2: Support for a Non-Magnetic Heavy-Fermion Ground State

In order to elucidate the nature of the ground state in the heavy-electron system PrInAg_2, we measured its specific heat for temperatures between 60 mK and 2 K in magnetic fields up to 9 T. The peak maximum of the low temperature anomaly in the specific heat (interpreted as Kondo anomaly) shifts from 0.42 K at zero field to 0.45 K at 6 T, and to 0.5 K at 9 T. The data at 3 T (after subtracting the low temperature tail due to a Schottky anomaly) is practically indistinguishable from the zero field data. A low temperature nuclear Schottky anomaly from a hyperfine enhancement of the Pr nuclei was observed in field. Both enhanced hyperfine interaction and the insensitivity of the specific heat anomaly to fields support the hypothesis that the Kondo effect in this system has a non-magnetic origin.

cond-mat.str-el↗

Muon Spin Relaxation and Nonmagnetic Kondo State in PrInAg_2

Muon spin relaxation experiments have been carried out in the Kondo compound PrInAg_2. The zero-field muon relaxation rate is found to be independent of temperature between 0.1 and 10 K, which rules out a magnetic origin (spin freezing or a conventional Kondo effect) for the previously-observed specific heat anomaly at \sim0.5 K. The low-temperature muon relaxation is quantitatively consistent with nuclear magnetism including hyperfine enhancement of the ^{141}Pr nuclear moment. This is strong evidence against a Pr^{3+} electronic magnetic moment, and for the Γ_3 crystalline-electric-field-split ground state required for a nonmagnetic route to heavy-electron behavior. The data imply the existence of an exchange interaction between neighboring Pr^{3+} ions of the order of 0.2 K in temperature units, which should be taken into account in a complete theory of a nonmagnetic Kondo effect in PrInAg_2.

cond-mat.str-el↗

Vortex Response and Critical Fields observed via rf penetration depth measurements on the superconductor YNi_2B_2C

Measurements of the rf penetration depth λ(T,H,θ) are used to study the superconducting order parameter, vortex dynamics in the mixed state and delineate critical fields in the borocarbide superconductor YNi_2B_2C. The lower critical field has an anomalous T dependence, H_{c1}(T)=1.12[1-(T/T_c)] kOe, which is however consistent with independent superfluid density measurements at microwave frequencies. The vortex response is dominated by viscous flux flow, indicative of extremely weak pinning, and is parametrized by a field scale H_{c2,eff}. The angular dependence of the vortex contribution λ(θ) is in good agreement with the Coffey-Clem model. Structure is seen in the depairing transition in the vicinity of the upper critical field, with the existence of well-defined critical fields H_{c2a}, H_{c2b} and H_{c2c}, with the vortex field scale H_{c2,eff} closest to H_{c2b}. Overall the measurements indicate that YNi_2B_2C has a rich and unusual field dependence of its transport parameters.

supr-con↗

Microwave Properties of Borocarbide Superconductors LnNi2B2C (Ln = Y, Er, Tm, Ho)

We report measurements of the microwave surface impedance of the borocarbide family of superconductors LnNi2B2C (Ln=Y, Er, Tm, Ho). The experiments enable direct measurements of the superfluid density, and are particularly sensitive to the influence of magnetic pairbreaking. In HoNi2B2C the antiferromagnetic transition is clearly observed at zero field, and leads to a drastic reduction of the superfluid density, which recovers at lower temperatures. In ErNi2B2C the antiferromagnetic transition is not seen in zero field data. Magnetic effects are responsible for anomalies in the low temperature surface impedance below approximately 4K in HoNi2B2C and TmNi2B2C. The temperature dependence of the microwave impedance disagrees with simple BCS calculations.

supr-con↗