SearcharxivSearch

arXiv subjects

P. Choudhury

Publications and source records attributed to P. Choudhury.

10 recordsLinked to original sources

Vortex dynamics and second magnetization peak in PrFeAsO$_{0.60}$F$_{0.12}$ superconductor

We have studied the vortex dynamics in the PrFeAsO$_{0.60}$F$_{0.12}$ superconducting sample by dc magnetization and dynamic magnetization-relaxation rate $(Q)$ measurements. The field dependence of the superconducting irreversible magnetization $M_s$ reveals a second magnetization peak or fishtail effect. The large value of $Q$ is an indication of moderate vortex motion and relatively weak pinning energy. Data analysis based on the generalized inversion scheme suggests that the vortex dynamics can be described by the collective pinning model. The temperature dependence of the critical current is consistent with the pinning due to the spatial variation in the mean free path near a lattice defect ($δl$ pinning). The temperature and field dependence of $Q$ indicates a crossover from elastic to plastic vortex creep with increasing temperature and magnetic field. Finally, we have constructed the vortex phase diagram based on the present data.

cond-mat.supr-con

Fe-spin reorientation in PrFeAsO : Evidences from resistivity and specific heat studies

We report the magnetic field dependence of resistivity ($ρ$) and specific heat ($C$) for the non-superconducting PrFeAsO compound. Our study shows a hitherto unobserved anomaly at $T_{SR}$ in the resistivity and specific heat data which arises as a result of the interplay of antiferromagnetic (AFM) Pr and Fe sublattices. Below the AFM transition temperature ($T_N^{\rm{Pr}}$), Pr moment orders along the crystallographic c axis and its effect on the iron subsystem causes a reorientation of the ordered inplane Fe moments in a direction out of the $ab$ plane. Application of magnetic field introduces disorder in the AFM Pr sublattice, which, in turn, reduces the out-of-plane Pr-Fe exchange interaction responsible for Fe spin reorientation. Both in $ρ$($T$) and $d(C/T)/dT$ curves, the peak at $T_{SR}$ broadens with the increase of $H$ due to the introduction of the disorder in the AFM Pr sublattice by magnetic field. In $ρ$($T$) curve, the peak shifts towards lower temperature with $H$ and disappears above 6 T while in $d(C/T)/dT$ curve the peak remains visible up to 14 T. The broadening of the anomaly at $T_N^{\rm{Pr}}$ in $C(T)$ with increasing $H$ further confirms that magnetic field induces disorder in the AFM Pr sublattice.

cond-mat.str-el

Multiferroic coupling in nanoscale BiFeO3

Using the results of x-ray and neutron diffraction experiments, we show that the ferroelectric polarization, in ~22 nm particles of BiFeO3, exhibits a jump by ~30% around the magnetic transition point T_N (~635 K) and a suppression by ~7% under 5T magnetic field at room temperature (<<T_N). These results confirm presence of strong multiferroic coupling even in nanoscale BiFeO3 and thus could prove to be quite useful for applications based on nanosized devices of BiFeO3.

cond-mat.mtrl-sci

The magnetization of PrFeAsO$_{0.60}$F$_{0.12} sueprconductor

The magnetization of the PrFeAsO$_{0.60}$F$_{0.12}$ polycrystalline sample has been measured as functions of temperature and magnetic field $(H)$. The observed total magnetization is the sum of a superconducting irreversible magnetization ($M_s$) and a paramagnetic magnetization ($M_p$). Analysis of dc susceptibility $χ(T)$ in the normal state shows that the paramagnetic component of magnetization comes from the Pr$^{+3}$ magnetic moments. The intragrain critical current density $(J_L)$ derived from the magnetization measurement is large. The $J_L(H)$ curve displays a second peak which shifts towards the high-field region with decreasing temperature. In the low-field region, a plateau up to a field $H^*$ followed by a power law $H^{-5/8}$ behavior of $J_L(H)$ is the characteristic of the strong pinning. A vortex phase diagram for the present superconductor has been obtained from the magnetization and resistivity data.

cond-mat.supr-con

Quantm Magnetoresistance of the PrFeAsO oxypnictides

We report the observation of an unusual $B$ dependence of transverse magnetoresistance (MR) in the PrFeAsO, one of the parent compound of pnictide superconductors. Below the spin density wave transition, MR is large, positive and increases with decreasing temperature. At low temperatures, MR increases linearly with $B$ up to 14 T. For $T$$\geq$40 K, MR vs $B$ curve develops a weak curvature in the low-field region which indicates a crossover from $B$ linear to $B^2$ dependence as $B$$\rightarrow$0. The $B$ linear MR originates from the Dirac cone states and has been explained by the quantum mechanical model proposed by Abrikosov.

cond-mat.supr-con

Particle size dependence of magnetization and non-centrosymmetry in nanoscale BiFeO3

The saturation magnetization (M_s), antiferromagnetic transition point (T_N), and the off-center displacements of Bi and Fe ions have been measured as a function of particle size in nanoscale BiFeO3. T_N decreases down to ~550 K for particles of size ~5 nm from ~653 K in bulk while M_s rises by more than an order of magnitude. Analysis of crystallographic structure from Rietveld refinement of x-ray diffraction patterns shows significant rise in off-center displacements of Bi (del_Bi) and Fe (del_Fe) ions within a unit cell with the decrease in particle size. The net unit-cell polarization P_S too, is found to be larger in nanoscale regime.

cond-mat.mtrl-sci

Resistivity saturation in PrFeAsO$_{1-x}$F$_y$ superconductor: An evidence of strong electron-phonon coupling

We have measured the resistivity of PrFeAsO$_{1-x}$F$_y$ samples over a wide range of temperature in order to elucidate the role of electron-phonon interaction on normal- and superconducting-state properties. The linear T dependence of $ρ$ above 170 K followed by a saturationlike behavior at higher temperature is a clear signature of strong electron-phonon coupling. From the analysis of T dependence of $ρ$, we have estimated several normal-state parameters useful for understanding the origin of superconductivity in this system. Our results suggest that Fe-based oxypnictides are phonon mediated BCS superconductors like Chevrel phases and A15 compounds.

cond-mat.supr-con

Normal-state transport properties of PrFeAsO$_{1-x}$F$_y$ superconductor

We have synthesized oxygen-deficient fluorine-doped samples of nominal composition PrFeAsO$_{1-x}$F$_y$ to study the normal and superconducting state properties. Resistivity of undoped PrFeAsO exhibits a strong anomaly at around 155 K due to the spin-density-wave instability. Fluorine doping ($x$=0.4, $y$=0.12) suppresses this magnetic instability and drives the system to the superconducting ground state with superconducting onset temperature 50 K. The behavior of normal-state resistivity changes from $T^2$-like to $T$-linear to sublinear in $T$ with increasing temperature indicating that both electron-electron interaction and electron-phonon interaction are strong. From the analysis of $T$ dependence of $ρ$, we have estimated the electron-phonon coupling strength ($λ$) to be quite large (1.3).

cond-mat.supr-con

Ferromagnetism in nanoscale BiFeO3

A remarkably high saturation magnetization of ~0.4mu_B/Fe along with room temperature ferromagnetic hysteresis loop has been observed in nanoscale (4-40 nm) multiferroic BiFeO_3 which in bulk form exhibits weak magnetization (~0.02mu_B/Fe) and an antiferromagnetic order. The magnetic hysteresis loops, however, exhibit exchange bias as well as vertical asymmetry which could be because of spin pinning at the boundaries between ferromagnetic and antiferromagnetic domains. Interestingly, like in bulk BiFeO_3, both the calorimetric and dielectric permittivity data in nanoscale BiFeO_3 exhibit characteristic features at the magnetic transition point. These features establish formation of a true ferromagnetic-ferroelectric system with a coupling between the respective order parameters in nanoscale BiFeO_3.

cond-mat.mtrl-sci

Perturbative expansion using variational phonon basis for Holstein model

A simple variational displacement phonon basis, obtained through the modified Lang-Firsov (MLF) transformation, is proposed to study the Holstein model.This phonon basis contains only one variational parameter, but capable of describing lattice distortions at distant sites from the charge carrier. Perturbation method based on this MLF basis is employed to calculate the single-electron ground-state energy and static charge-lattice deformation correlation as a function of electron-phonon coupling. The energy obtained up to the second-order perturbation within this approach agrees well with the available numerical results for the entire range of coupling strength.

cond-mat