SearcharxivSearch

arXiv subjects

P. Chudzinski

Publications and source records attributed to P. Chudzinski.

17 recordsLinked to original sources

Anisotropic fully-gapped superconductivity in quasi-one-dimensional Li$_{0.9}$Mo$_6$O$_{17}$

Superconductivity in quasi-one-dimensional Li$_{0.9}$Mo$_6$O$_{17}$ emerges from an exotic, non-metallic normal state that exhibits signatures of Tomonaga-Luttinger liquid behavior, emergent symmetry and excitonic order. The high upper critical field, $H_{c2}$, in Li$_{0.9}$Mo$_6$O$_{17}$ suggests that that the favored pairing state is spin-triplet in nature. Here, we report measurements of the magnetic penetration depth down to $0.08\,\mathrm{K}$ ($T/T_c \lesssim 0.04$) and the specific heat down to $0.4\,\mathrm{K}$ ($T/T_c \lesssim 0.2$), and show that they are consistent with a moderately-coupled, fully-gapped superconducting state with marked gap anisotropy and a minimum ($\Delta_{\rm min} \simeq 0.4\,k_{\mathrm{B}}T_c$) occurring over a very narrow region in $k$-space. Combined with knowledge of $H_{c2}$, these measurements support the presence of a nodeless and possibly odd-parity spin-triplet superconducting order parameter in Li$_{0.9}$Mo$_6$O$_{17}$.

cond-mat.supr-con

Non-equilibrium Floquet steady states of time-periodic driven Luttinger liquids

Time-periodic driving facilitates a wealth of novel quantum states and quantum engineering. The interplay of Floquet states and strong interactions is particularly intriguing, which we study using time-periodic fields in a one-dimensional quantum gas, modeled by a Luttinger liquid with periodically changing interactions. By developing a time-periodic operator algebra, we are able to solve and analyze the complete set of non-equilibrium steady states in terms of a Floquet-Bogoliubov ansatz and known analytic functions. Complex valued Floquet eigenenergies occur when multiples of driving frequency approximately match twice the dispersion energy, which correspond to resonant states. In experimental systems of Lieb-Liniger bosons we predict a change from powerlaw correlations to dominant collective density wave excitations at the corresponding wave numbers as the frequency is lowered below a characteristic cut-off.

cond-mat.quant-gas

Parameters of Tomonaga-Luttinger liquid in a quasi-1D material with Coulomb interactions

In this work we derive a new scheme to calculate Tomonaga-Luttinger liquid (TLL) parameters and holon (charge modes) velocities in a quasi-1D material that consists of two-leg ladders coupled through Coulomb interactions. Firstly, we obtain an analytic formula for electron-electron interaction potential along the conducting axis for a generalized charge distribution in a plane perpendicular to it. In the second step we introduce many-body screening that is present in a quasi-1D material. To this end we propose a new approximation for the charge susceptibility. Based on this we are able to find the TLL's parameters and velocities. We then show how to use these to validate the experimental ARPES data measured recently in p-polarization in $NbSe_3$. Although we focus our study on this specific material it is applicable for any quasi-1D system that consists of two-leg ladders as basic units.

cond-mat.str-el

Can 1D topological states explain the extraordinary thermoelectric properties of Bi 2 Te 3 ? An exact analytical solution in the Tomonaga-Luttinger liquids (TLLs) framework

Topological insulators are frequently also one of the best known thermoelectric materials. It has been recently discovered that in 3D topological insulators each skew dislocation can host a pair of 1D topological states a helical TLL. We derive exact analytical formulas for thermoelectric Seebeck coefficient in TLL and investigate up to what extent one can ascribe the outstanding thermoelectric properties of Bi 2 Te 3 to these 1D topological states. To this end we take a model of a dense dislocation network and find an analytic formula for an overlap between 1D (the TLL) and 3D electronic states. Our study is applicable to a weakly n-doped Bi 2 Te 3 but also to a broader class of nano-structured materials with artificially created 1D systems. Furthermore, our results can be used at finite frequency settings e.g. to capture transport activated by photo-excitations.

cond-mat.str-el

Anharmonic coupling between electrons and TO phonons in the vicinity of ferroelectric quantum critical point

We explore a novel coupling mechanism of electrons with the transverse optical (TO) phonon branch in a regime when the TO mode becomes highly anharmonic and drives the ferroelectric phase transition. We show that this anharmonicity, which leads to a collective motion of ions, is able to couple electronic and lattice displacement fields. An effective correlated electron-ion dynamics method is required to capture the effect of the onset of the local electric polarization due to this collective behavior close to the quantum critical point. We identify an intermediate temperature range where an emergent phonon drag may contribute substantially to thermoelectric conductivity in this regime. We find that, under optimal conditions, this extra contribution may be larger than values achieved so far in the benchmark material, PbTe. In the last part we make a case for the importance of our results in the generic problem of anharmonic electron-lattice dynamics.

cond-mat.str-el

Why it is so hard to detect Luttinger liquids in ARPES?

The problem of photoemission from a quasi-1D material is studied. We identify two issues that play a key role in the detection of gapless Tomonaga-Luttinger liquid (TLL) phase. Firstly, we show how a disorder -- backward scattering as well as forward scattering component, is able to significantly obscure the TLL states, hence the initial state of ARPES. Secondly, we investigate the photo-electron propagation towards a sample's surface. We focus on the scattering path operator contribution to the final state of ARPES. We show that, in the particular conditions set by the 1D states, one can derive exact analytic solution for this intermediate stage of ARPES. The solution shows that for particular energies of incoming photons the intensity of photo-current may be substantially reduced. Finally, we put together the two aspects (the disorder and the scattering path operator) to show the full, disruptive force of any inhomogeneities on the ARPES amplitude.

cond-mat.str-el

Emerging one-dimensionality from self-organization of electrons in NbSe$_3$

Materials where the electron filling is close to commensurate filling provide one of the great challenges in materials science. Several proposals of unconventional orderings, where the electronic liquid self-organizes into components with distinct properties, were recently put forward, in particular in cuprates and pnictides where electronic nematic orders have been observed. The electrons self-organization is expected to yield complex intra and inter unit cell patterns, and a reduction of dimensionality. Nevertheless, an unambiguous experimental proof of such complex orders, namely the direct observation of distinct dispersions, is still missing. Here we report a Nano Angle Resolved Photo-emission Spectroscopy (Nano-ARPES) study of NbSe$_3$, a material that has been considered a paradigm of charge order. The new data (Fig.1) invalidate the canonical picture of imperfect nesting and reveals the emergence of a novel order. The electrons self-organization uncovers the one-dimensional (1D) physics hidden in a material which naively should be the most 3D of all columnar chalcogenides.

cond-mat.str-el

Slow quenches in XXZ spin-chains -- the role of Galilean invariance breaking

We study a XXZ spin-chain in a gapless Tomonaga-Luttinger liquid (TLL) phase with time dependent anisotropy of spin exchange interactions. To begin we focus on a linear ramp of $J_z$, starting at XX point and slowly increasing towards the anti-ferromagnetic Heisenberg point. Although the problem of a linear ramp in the TLL has been recently under intense scrutiny in a perturbative \emph{g-ology} framework, an aspect that has been overlooked so far is the role of the Galilean invariance breaking. We find that, although the differential equation that needs to be solved to find time evolution of the system is substantially more complicated, in some cases exact analytic solutions can be given. We obtain them for the linear ramp in the limit of small $J_z$ as well as $J_z\rightarrow 1$, and for such protocols that are tailored to keep the Galilean invariance breaking term constant for every $J_z$. We point out the features of dynamics during the quench that stays unaltered, and those that need to be taken with care when Galilean invariance breaking is present. We are able to deduce that it is the shape of the propagating front that is affected in the most pronounced way.

cond-mat.str-el

Multi-orbital physics in lithium-molybdenum purple-bronze: going beyond paradigm

We investigate the role of inter-orbital fluctuations in the low energy physics of a quasi-1D material - lithium molybdenum purple bronze (LMO). It is an exceptional material that may provide us a long sought realization of a Tomonaga-Luttinger liquid (TLL) physics, but its behaviour at temperatures of the order of $T^*\approx 30$K remains puzzling despite numerous efforts. Here we make a conjecture that the physics around $T^*$ is dominated by multi-orbital excitations. Their properties can be captured using an excitonic picture. Using this relatively simple model we compute fermionic Green's function in the presence of excitons. We find that the spectral function is broadened with a Gaussian and its temperature dependence acquires an extra $T^1$ factor. Both effects are in perfect agreement with experimental findings. We also compute the resistivity for temperatures above and below critical temperature $T_o$. We explain an upturn of the resistivity at 28K and interpret the suppression of this extra component of resistivity when a magnetic field is applied along the conducting axis. Furthermore, in the framework of our model, we qualitatively discuss and consistently explain other experimentally detected peculiarities of purple bronze: the breaking of Wiedmann-Franz law and the magnetochromatic behaviour.

cond-mat.str-el

Resonant plasmon-phonon coupling and its role in magneto-thermoelectricity in bismuth

Using diagrammatic methods we derive an effective interaction between a low energy collective movement of fermionic liquid (acoustic plasmon) and acoustic phonon. We show that the coupling between the plasmon and the lattice has a very non-trivial, resonant structure. When real and imaginary parts of the acoustic plasmon's velocity are of the same order as the phonon's velocity, the resonance qualitatively changes the nature of phonon-drag. In the following we study how magneto-thermoelectric properties are affected. Our result suggests that the novel mechanism of energy transfer between electron liquid and crystal lattice can be behind the huge Nernst effect in bismuth.

cond-mat.str-el

Luttinger liquid theory of purple bronze $Li_{0.9}Mo_6O_{17}$ in the charge regime

Molybdenum purple bronze Li$_{0.9}$Mo$_{6}$O$_{17}$ is an exceptional material known to exhibit one dimensional (1D) properties for energies down to a few meV. This fact seems to be well established both in experiments and in band structure theory. We use the unusual, very 1-dimensional band dispersion obtained in \emph{ab-initio} DFT-LMTO band calculations as our starting point to study the physics emerging below 300meV. A dispersion perpendicular to the main dispersive direction is obtained and investigated in detail. Based on this, we derive an effective low energy theory within the Tomonaga Luttinger liquid (TLL) framework. We estimate the strength of the possible interactions and from this deduce the values of the TLL parameters for charge modes. Finally we investigate possible instabilities of TLL by deriving renormalization group (RG) equations which allow us to predict the size of potential gaps in the spectrum. While $2k_F$ instabilities strongly suppress each other, the $4k_F$ instabilities cooperate, which paves the way for a possible CDW at the lowest energies. The aim of this work is to understand the experimental findings, in particular the ones which are certainly lying within the 1D regime. We discuss the validity of our 1D approach and further perspectives for the lower energy phases.

cond-mat.str-el

Effects of thermal- and spin- fluctuations on the band structure of purple bronze Li$_2$Mo$_{12}$O$_{34}$

The band structures of ordered and thermally disordered Li$_2$Mo$_{12}$O$_{34}$ are calculated by use of ab-initio DFT-LMTO method. The unusual, very 1-dimensional band dispersion obtained in previous band calculations is confirmed for the ordered structure, and the overall band structure agrees reasonably with existing photoemission data. Dispersion and bandstructure perpendicular to the main dispersive direction is obtained. A temperature dependent band broadening is calculated from configurations with thermal disorder of the atomic positions within the unit cell. This leads a band broadening of the two bands at the Fermi energy which can become comparable to their energy separation. The bands are particularly sensitive to in-plane movements of Mo sites far from the Li-sites, where the density-of-states is highest. The latter fact makes the effect of Li vacancies on the two bands relatively small. Spin-polarized band results for the ordered structure show a surprisingly large exchange enhancement on the high DOS Mo sites. Consequences for spin fluctuations associated with a cell doubling along the conducting direction are discussed.

cond-mat.str-el

Collective excitations and low temperature transport properties of bismuth

We examine the influence of collective excitations on the transport properties (resistivity, magneto- optical conductivity) for semimetals, focusing on the case of bismuth. We show, using an RPA approximation, that the properties of the system are drastically affected by the presence of an acoustic plasmon mode, consequence of the presence of two types of carriers (electrons and holes) in this system. We found a crossover temperature T* separating two different regimes of transport. At high temperatures T > T* we show that Baber scattering explains quantitatively the DC resistivity experiments, while at low temperatures T < T* interactions of the carriers with this collective mode lead to a T^5 behavior of the resistivity. We examine other consequences of the presence of this mode, and in particular predict a two plasmon edge feature in the magneto-optical conductivity. We compare our results with the experimental findings on bismuth. We discuss the limitations and extensions of our results beyond the RPA approximation, and examine the case of other semimetals such as graphite or 1T-TiSe_2.

cond-mat.str-el

Spin rotational symmetry breaking by orbital current patterns in two-leg ladders.

We investigate the physical consequences of orbital current patterns (OCP) in doped two-leg Cu-O Hubbard ladders. The internal symmetry of the pattern, in the case of the ladder structure, differs slightly from that suggested so far for cuprates. We focus on this OCP and look for measurable signatures of its existence. We compute the magnetic field produced by the OCP at each lattice site, and estimate its value in view of a possible experimental detection. Using a renormalization group (RG) analysis, we determine the changes that are caused by the SU(2) spin-rotational symmetry breaking which occurs when the OCP is present in the ground state phase diagram. The most signifcant one is an in-plane SDW gap opening in an otherwise critical phase, at intermediate dopings. We estimate the value of this gap, give an analytic expression for the correlation functions and examine some of the magnetic properties of this new phase which can be revealed in measurements. We compute the conductance in the presence of a single impurity, using an RG analysis. A discussion of the various sources of SU(2) symmetry breaking underscores the specificity of the OCP induced effects.

cond-mat.str-el

Influence of non-magnetic impurities on hole doped two-leg Cu-O Hubbard ladders

We study the influence of non magnetic impurities on the phase diagram of doped two-leg Hubbard Cu-O ladders. In the absence of impurities this system posseses d-wave superconducting states and orbital current states depending on the doping. A single, strong, scatterer modifies its environment locally and this effect is assessed using a renormalization group analysis. At high doping, disorder causes intraband instabilities and at low doping it promotes interband instabilities. In the former case, we extend the boundary conformal field theory method, developed in the context of single chains, to handle the ladder problem, and we find exact closed-form analytical expressions for the correlation functions. This allows us to compute experimentally measurable local quantities such as the nuclear magnetic resonance line broadenings and scanning tunnelling microscope profiles. We also discuss the low doping regime where Kondo physics is at play, making qualitative predictions about its nature. Insight into collective effects is also given in the many weak impurities case, based on an RG approach. In this regime, one sees the interplay between interactions and disorder. We emphasize the influence of the O atoms on disorder effects both for the single- and for the many-defect situations.

cond-mat.str-el

Orbital current patterns in doped two-leg Cu-O Hubbard ladders

In the weak coupling limit, we investigate two-leg ladders with a unit cell containing both Cu and O atoms, as a function of doping. For purely repulsive interactions, using bosonization, we find significant differences with the single orbital case: a completely massless quantum critical regime is obtained for a finite range of carrier concentration. In a broad region of the phase diagram the ground state consists of a pattern of orbital currents plus a density wave. NMR properties of the Cu and O nuclei are presented for the various phases.

cond-mat.str-el

Phase diagram of hole doped two-leg Cu-O ladders

In the weak coupling limit, we establish the phase diagram of a two-leg ladder with a unit cell containing both Cu and O atoms, as a function of doping. We use bosonization and design a specific RG procedure to handle the additional degrees of freedom. Significant differences are found with the single orbital case; for purely repulsive interactions, a completely massless quantum critical region is obtained at intermediate carrier concentrations (well inside the bands) where the ground state consists of an incommensurate pattern of orbital currents plus a spin density wave (SDW) structure.

cond-mat.str-el