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P. D. O'Malley

Publications and source records attributed to P. D. O'Malley.

At least 19 recordsLinked to original sources

Neutron dynamics in the fusion of neutron-rich O ions with $^{12}$C

The fusion excitation function for $^{21}$O + $^{12}$C was measured for the first time and compared to the fusion of less neutron-rich isotopes. The impact of valence neutrons in the d$_{5/2}$ shell on the fusion excitation function is examined. The experimental data manifest a clear dependence of the extracted barrier height, V$_B$, and barrier position, R$_B$ on neutron excess. To assess the role of dynamics the experimental data are compared with both density constrained frozen Hartree Fock (DCFHF) and density constrained time-dependent Hartree Fock (DCTDHF) theories.

nucl-ex

Offline Commissioning of the St. Benedict Gas Catcher

Precision measurements of $β$ decay transitions offer a promising channel through which the Standard Model (SM) can be probed. There is currently an ongoing effort to increase the precision on measurements of $\mathcal{F}t$-values for superallowed $β$ decay transitions between mirror nuclides. These allow for a determination of $V_{ud}$ which is complementary to that obtained from pure Fermi $0^+ \rightarrow 0^+$ transitions. The Superallowed Transition BEta-NEutrino Decay Ion Coincidence Trap (St. Benedict), under construction at the Nuclear Science Laboratory (NSL) at the University of Notre Dame, seeks to measure the Fermi-to-Gamow-Teller mixing ratio for transitions between mirror nuclei in order to expand the list of nuclides from which $V_{ud}$ can be extracted. Production and selection of the species of interest will be done in-flight, using the \textit{TwinSol} magnetic separator system. The first element of St. Benedict will be a large volume gas catcher which will thermalize radioactive ion beams for low energy delivery to the rest of the system. Offline commissioning of this gas catcher has been completed using an internal potassium source, and the device demonstrated a transport efficiency upwards of 95\% for pressures of 66 mbar and lower.

physics.ins-det

Off-line Commissioning of the St. Benedict Radio Frequency Quadrupole Ion Guide

The Superallowed Transition Beta-Neutrino Decay Ion Coincidence Trap (St. Benedict) is currently under construction at the Nuclear Science Laboratory (NSL) of the University of Notre Dame. It aims to measure the beta-neutrino angular correlation parameter for superallowed mixed mirror beta decay transitions. Measurements of this kind offer unique insight into the electroweak part of the Standard Model through tests of unitarity of the Cabibbo-Kobayashi-Maskawa (CKM) matrix. St. Benedict is comprised of several beam-manipulating components including a radio frequency quadrupole (RFQ) ion guide. This ion guide features an off-line source at $90^\circ$ to the beam path for testing and calibration of downstream components once St. Benedict is online. Off-line commissioning of the ion guide demonstrated a transport efficiency greater than 95% for ions coming from the upstream RF carpet chamber. When taking ions from the $90^\circ$ off-line source a lower efficiency of 60% was obtained.

physics.ins-det

Off-line Commissioning of the St. Benedict Radiofrequency Quadrupole Cooler-Buncher

The St. Benedict ion trapping system, which aims to measure the $β-ν$ angular correlation parameter in superallowed-mixed mirror transitions, is under construction at the University of Notre Dame. These measurements will provide much-needed data to improve the accuracy of the $V_{ud}$ element of the CKM matrix. One of the major components of this system is the radio frequency quadrupole cooler-buncher, which is necessary to create low-emittance ion bunches for injection into the measurement Paul trap. The off-line commissioning of the cooler-buncher, using a potassium ion source, determined that the device could produce cooled ion bunches characterized by a 50-ns full-width-half-maximum time width. The commissioning results also determined the trapping efficiency to be 93(1)$\%$ and the trapping half-life to be 20.0(5) s.

physics.ins-det

$^{28}$Al Half-life Measurement and the negative mirror asymmetry between the $^{28}$Al($β^-$)$^{28m}$Si and $^{28}$P($β^+$)$^{28m}$Si decays

In the past, the mirror asymmetry parameter has been proposed as a probing mechanism for the presence of beyond the Standard Model second-class currents in nuclear beta decay transitions. However, this was hindered by large uncertainties in the required nuclear structure correction terms. Recently, a new calculation of these corrections attempted, but could not fully explain the negative mirror asymmetry between the $^{28}$Al($β^-$)$^{28m}$Si and $^{28}$P($β^+$)$^{28m}$Si decays. To put the mirror asymmetry parameter on a more solid footing, the half-life of $^{28}$Al was measured for the first time using a radioactive ion beam at the Nuclear Science Laboratory of the University of Notre Dame. The new result, $t_{1/2}=$134.432(34) s, is consistent with most of the past data except for one highly discrepant measurement. The new mirror asymmetry parameter of -3.5(10)$\%$ obtained still does not agree with nuclear structure calculations.

nucl-ex

The Beta-decay Paul Trap Mk IV: Design and commissioning

The Beta-decay Paul Trap is an open-geometry, linear trap used to measure the decays of $^8$Li and $^8$B to search for a tensor contribution to the weak interaction. In the latest $^8$Li measurement of Burkey et al. (2022), $β$ scattering was the dominant experimental systematic uncertainty. The Beta-decay Paul Trap Mk IV reduces the prevalence of $β$ scattering by a factor of 4 through a redesigned electrode geometry and the use of glassy carbon and graphite as electrode materials. The trap has been constructed and successfully commissioned with $^8$Li in a new data campaign that collected 2.6 million triple coincidence events, an increase in statistics by 30% with 4 times less $β$ scattering compared to the previous $^8$Li data set.

physics.ins-det

Structure Studies of $^{13}\text{Be}$ from the $^{12}$Be(d,p) reaction in inverse kinematics on a solid deuteron target

The low-lying structure of $^{13}$Be has remained an enigma for decades. Despite numerous experimental and theoretical studies, large inconsistencies remain. Being both unbound, and one neutron away from $^{14}$Be, the heaviest bound beryllium nucleus, $^{13}$Be is difficult to study through simple reactions with weak radioactive ion beams or more complex reactions with stable-ion beams. Here, we present the results of a study using the $^{12}$Be(d,p)$^{13}$Be reaction in inverse kinematics using a 9.5~MeV per nucleon $^{12}$Be beam from the ISAC-II facility. The solid deuteron target of IRIS was used to achieve an increased areal thickness compared to conventional deuterated polyethylene targets. The Q-value spectrum below -4.4~MeV was analyzed using a Bayesian method with GEANT4 simulations. A three-point angular distribution with the same Q-value gate was fit with a mixture of $s$- and $p$-wave, $s$- and $d$-wave, or pure $p$-wave transfer. The Q-value spectrum was also compared with GEANT simulations obtained using the energies and widths of states reported in four previous works. It was found that our results are incompatible with works that revealed a wide $5/2^+$ resonance but shows better agreement with ones that reported a narrower width.

nucl-ex

First direct measurement constraining the $^{34}$Ar($α$,p)$^{37}$K reaction cross section for mixed hydrogen and helium burning in accreting neutron stars

The rate of the final step in the astrophysical $α$p-process, the $^{34}$Ar($α$,\textit{p})$^{37}$K reaction, suffers from large uncertainties due to lack of experimental data, despite having a considerable impact on the observable light curves of x-ray bursts and the composition of the ashes of hydrogen and helium burning on accreting neutron stars. We present the first direct measurement constraining the $^{34}$Ar($α$,p)$^{37}$K reaction cross section, using the Jet Experiments in Nuclear Structure and Astrophysics (JENSA) gas jet target. The combined cross section for the $^{34}$Ar,Cl($α$,p)$^{37}$K,Ar reaction is found to agree well with Hauser-Feshbach predictions. The $^{34}$Ar($α$,2p)$^{36}$Ar cross section, which can be exclusively attributed to the $^{34}$Ar beam component, also agrees to within the typical uncertainties quoted for statistical models. This indicates the applicability of the statistical model for predicting astrophysical ($α$,p) reaction rates in this part of the $α$p process, in contrast to earlier findings from indirect reaction studies indicating orders-of-magnitude discrepancies. This removes a significant uncertainty in models of hydrogen and helium burning on accreting neutron stars.

nucl-ex

Remeasuring the anomalously enhanced $B(E2; 2^+ \rightarrow 1^+)$ in $^8\mathrm{Li}$

The large reported $E2$ strength between the $2^+$ ground state and $1^+$ first excited state of $\isotope[8]{Li}$, $B(E2; 2^+ \rightarrow 1^+)= 55(15)\,e^2\fm^4$, presents a puzzle. Unlike in neighboring $A=7\text{--}9$ isotopes, where enhanced $E2$ strengths may be understood to arise from deformation as rotational in-band transitions, the $2^+\rightarrow1^+$ transition in $^8$Li cannot be understood in any simple way as a rotational in-band transition. Moreover, the reported strength exceeds \textit{ab initio} predictions by an order of magnitude. In light of this discrepancy, we revisited the Coulomb excitation measurement of this strength, now using particle-$γ$ coincidences, yielding a revised $B(E2; 2^+ \rightarrow 1^+)$ of $19(^{+7}_{-6})(2)$~e$^2$fm$^4$. We explore how this value compares to what might be expected in the limits of rotational models. While the present value is about a factor of three smaller than previously reported, it remains anomalously enhanced.

nucl-ex

Obtaining high resolution excitation functions with an active thick-target approach and validating them with mirror nuclei

Measurement of fusion excitation functions for stable nuclei has largely been restricted to nuclei with significant natural abundance. Typically, to investigate neighboring nuclei with low natural abundance has required obtaining isotopically enriched material. This restriction often limits the ability to perform such measurements. We report the measurement of a high quality fusion excitation function for a $^{17}$O beam produced from unenriched material with 0.038\% natural abundance. The measurement is enabled by using an active thick-target approach and the accuracy of the result is validated using its mirror nucleus $^{17}$F and resonances. The result provides important information about the average fusion cross-section for the oxygen isotopic chain as a function of neutron excess.

nucl-ex

TriSol: a major upgrade of the TwinSol RNB facility

We report here on the recent upgrade of the TwinSol radioactive nuclear beam (RNB) facility at the University of Notre Dame. The new TriSol system includes a magnetic dipole to provide a second beamline and a third solenoid which acts to reduce the size of the radioactive beam on target.

physics.acc-ph

Neutron transfer reactions on the ground state and isomeric state of a 130Sn beam

The structure of nuclei around the neutron-rich nucleus 132Sn is of particular interest due to the vicinity of the Z = 50 and N = 82 shell closures and the r-process nucleosynthetic path. Four states in 131Sn with a strong single-particle-like component have previously been studied via the (d,p) reaction, with limited excitation energy resolution. The 130Sn(9Be,8Be)131Sn and 130Sn(13C,12C)131Sn single-neutron transfer reactions were performed in inverse kinematics at the Holifield Radioactive Ion Beam Facility using particle-gamma coincidence spectroscopy. The uncertainties in the energies of the single-particle-like states have been reduced by more than an order of magnitude using the energies of gamma rays. The previous tentative Jpi values have been confirmed. Decays from high-spin states in 131Sn have been observed following transfer on the isomeric component of the 130Sn beam. The improved energies and confirmed spin-parities of the p-wave states important to the r-process lead to direct-semidirect cross-sections for neutron capture on the ground state of 130Sn at 30 keV that are in agreement with previous analyses. A similar assessment of the impact of neutron-transfer on the isomer would require significant nuclear structure and reaction theory input. There are few measurements of transfer reaction on isomers, and this is the first on an isomer in the 132Sn region.

nucl-ex

Use of Bayesian Optimization to Understand the Structure of Nuclei

Monte Carlo simulations are widely used in nuclear physics to model experimental systems. In cases where there are significant unknown quantities, such as energies of states, an iterative process of simulating and fitting is often required to describe experimental data. We describe a Bayesian approach to fitting experimental data, designed for data from a $^{12}$Be(d,p) reaction measurement, using simulations made with GEANT4. Q-values from the $^{12}$C(d,p) reaction to well-known states in $^{13}$C are compared with simulations using BayesOpt. The energies of the states were not included in the simulation to reproduce the situation for $^{13}$Be where the states are poorly known. Both cases had low statistics and significant resolution broadening owing to large proton energy losses in the solid deuterium target. Excitation energies of the lowest three excited states in $^{13}$C were extracted to better than 90 keV, paving a way for extracting information on $^{13}$Be.

physics.comp-ph

MuSIC@Indiana: an effective tool for accurate measurement of fusion with low-intensity radioactive beams

The design, construction, and characterization of the Multi-Sampling Ionization Chamber, MuSIC@Indiana, are described. This detector provides efficient and accurate measurement of the fusion cross-section at near-barrier energies. The response of the detector to low-intensity beams of $^{17,18}$O, $^{19}$F, $^{23}$Na, $^{24,26}$Mg, $^{27}$Al, and $^{28}$Si at E$_{lab}$ = 50-60 MeV was examined. MuSIC@Indiana was commissioned by measuring the $^{18}$O+$^{12}$C fusion excitation function for 11 $<$ E$_{cm}$ $<$ 20 MeV using CH$_{4}$ gas. A simple, effective analysis cleanly distinguishes proton capture and two-body scattering events from fusion on carbon. With MuSIC@Indiana, measurement of 15 points on the excitation function for a single incident beam energy is achieved. The resulting excitation function is shown to be in good agreement with literature data

physics.ins-det

The Notre-Dame Cube: An active-target time-projection chamber for radioactive beam experiments and detector development

Active-target detectors have the potential to address the difficulties associated with the low intensities of radioactive beams. We have developed an active-target detector, the Notre Dame Cube (ND-Cube), to perform experiments with radioactive beams produced at $\mathit{TwinSol}$ and to aid in the development of active-target techniques. Various aspects of the ND-Cube and its design were characterized. The ND-Cube was commissioned with a $^{7}$Li beam for measuring $^{40}$Ar + $^{7}$Li fusion reaction cross sections and investigating $^{7}$Li($α$,$α$)$^{7}$Li scattering events. The ND-Cube will be used to study a range of reactions using light radioactive ions produced at low energy.

physics.ins-det

Determination of hexadecapole ($β_{4}$) deformation of the light-mass nucleus $^{24}$Mg using quasi-elastic measurement

Quasi-elastic scattering measurements have been performed using $^{16}$O and $^{24}$Mg projectiles off $^{90}$Zr at energies around the Coulomb barrier. Experimental data have been analyzed in the framework of coupled channels (CC) calculations using the code CCFULL. The quasi-elastic scattering excitation function and derived barrier distribution for $^{16}$O + $^{90}$Zr reaction are well reproduced by the CC calculations using the vibrational coupling strengths for $^{90}$Zr reported in the literature. Using these vibrational coupling strengths, a Bayesian analysis is carried out for $^{24}$Mg + $^{90}$Zr reaction. The $β_{2}$ and $β_{4}$ values for $^{24}$Mg are determined to be $+0.43 \pm 0.02$ and $ - 0.11 \pm 0.02$, respectively. The $β_{2}$ parameter determined in the present work is in good agreement with results obtained using inelastic scattering probes. The hexadecapole deformation of $^{24}$Mg has been measured very precisely for the first time. Present results establish that quasi-elastic scattering could provide a useful probe to determine the ground state deformation of atomic nuclei.

nucl-ex

New $γ$-ray Transitions Observed in $^{19}$Ne with Implications for the $^{15}$O($α$,$γ$)$^{19}$Ne Reaction Rate

The $^{15}$O($α$,$γ$)$^{19}$Ne reaction is responsible for breakout from the hot CNO cycle in Type I x-ray bursts. Understanding the properties of resonances between $E_x = 4$ and 5 MeV in $^{19}$Ne is crucial in the calculation of this reaction rate. The spins and parities of these states are well known, with the exception of the 4.14- and 4.20-MeV states, which have adopted spin-parities of 9/2$^-$ and 7/2$^-$, respectively. Gamma-ray transitions from these states were studied using triton-$γ$-$γ$ coincidences from the $^{19}$F($^{3}$He,$tγ$)$^{19}$Ne reaction measured with GODDESS (Gammasphere ORRUBA Dual Detectors for Experimental Structure Studies) at Argonne National Laboratory. The observed transitions from the 4.14- and 4.20-MeV states provide strong evidence that the $J^π$ values are actually 7/2$^-$ and 9/2$^-$, respectively. These assignments are consistent with the values in the $^{19}$F mirror nucleus and in contrast to previously accepted assignments.

nucl-ex

Key $^{19}$Ne states identified affecting $γ$-ray emission from $^{18}$F in novae

Detection of nuclear-decay $γ$ rays provides a sensitive thermometer of nova nucleosynthesis. The most intense $γ$-ray flux is thought to be annihilation radiation from the $β^+$ decay of $^{18}$F, which is destroyed prior to decay by the $^{18}$F($p$,$α$)$^{15}$O reaction. Estimates of $^{18}$F production had been uncertain, however, because key near-threshold levels in the compound nucleus, $^{19}$Ne, had yet to be identified. This Letter reports the first measurement of the $^{19}$F($^{3}$He,$tγ$)$^{19}$Ne reaction, in which the placement of two long-sought 3/2$^+$ levels is suggested via triton-$γ$-$γ$ coincidences. The precise determination of their resonance energies reduces the upper limit of the rate by a factor of $1.5-17$ at nova temperatures and reduces the average uncertainty on the nova detection probability by a factor of 2.1.

nucl-ex