arXiv subjects

P. Dey

Publications and source records attributed to P. Dey.

11 recordsLinked to original sources

arXiv2025

Competition between the neutron-proton pair break-ups delineating the level structure of 202Po

High-spin spectroscopic study of $^{202}$Po ($Z$ = 84, $N$ = 118) has been carried out using the $^{195}$Pt($^{12}$C, 5n)$^{202}$Po fusion-evaporation reaction. An extended level scheme has been proposed up to an excitation energy of $E_x\approx$ 8 MeV and angular momentum of 27$\hbar$, with the addition of 57 newly observed $\gamma$-ray transitions, along with the revisions in the placement of 8 already known transitions and the multipolarities of 4 of these transitions. The energy of the unobserved 8$^+ \rightarrow 6^+$ transition has been proposed to be 9.0(5) keV, which resolves the uncertainty in the excitation energy of the levels above the 6$^{+}$ state. Three new sequences of $M1$ transitions have also been identified in the high excitation energy regime and included in the proposed level scheme. The large-scale shell model calculations for $Z>82$ and $N<126$ valence space have been carried out using PBPOP interaction which explained the overall level scheme for both the positive and negative parity states. The calculations successfully reproduced the purity of the proton $\pi h_{9/2}$ dominated $8^+$ isomeric state, and also explained the missing $E2$ decay of the ${12}^+$ isomeric state in terms of changing nucleonic configurations.

nucl-ex↗

arXiv2024

In-beam $\gamma-$spectroscopy of the transitional nucleus $^{217}$Ac

High-spin states in the transitional $^{217}$Ac nucleus are established up to 3.8 MeV excitation energy and $I^{\pi} =$ 41/2$^+$ with the addition of around 20 new transitions. The structure of the yrast and near-yrast states below the 29/2$^+$ isomer is revisited. The inconsistencies in the level schemes reported earlier are resolved. The level structure above the 29/2$^+$ isomer is established for the first time. Large-basis shell-model calculations with the KHPE interaction are performed to compare the experimentally observed level energies with the theoretical predictions. A comparison with the systematics of the N = 128 isotones suggests that the yrast structures result from a weak coupling of the odd proton to the even-even 216Ra core, which is consistent with the shell-model configurations. Furthermore, alpha decay of the 29/2$^+$ isomer is revisited and the decay scheme established from this work is discussed in the framework of the shell model.

nucl-ex↗

arXiv2024

Computation of Electrical Conductivities of Aqueous Electrolyte Solutions: Two Surfaces , One Property

In this work, we have computed electrical conductivities at ambient conditions of aqueous NaCl and KCl solutions by using the Einstein-Helfand equation. Common force fields (charge q = 1 e) do not reproduce the experimental values of electrical conductivities, viscosities and diffusion coefficients. Recently, we proposed the idea of using different charges to describe the Potential Energy Surface (PES) and the Dipole Moment Surface (DMS). In this work, we implement this concept. The equilibrium trajectories required to evaluate electrical conductivities (within linear response theory) were obtained by using scaled charges (with the value q = 0.75 e ) to describe the PES. The potential parameters were those of the Madrid-Transport force field, which describe accurately viscosities and diffusion coefficients of these ionic solutions. However, integer charges were used to compute the conductivities (thus describing the DMS). The basic idea is that although the scaled charge describes the ion-water interaction better, the integer charge reflects the value of the charge that is transported due to the electric field. The agreement obtained with experiments is excellent, as for the first time electrical conductivities (and the other transport properties) of NaCl and KCl electrolyte solutions are described with high accuracy for the whole concentration range up to their solubility limit. Finally, we propose an easy way to obtain a rough estimate of the actual electrical conductivity of the potential model under consideration using the approximate Nernst-Einstein equation, which neglects correlations between different ions.

physics.chem-ph↗

arXiv2018

Detection of thermodynamic "valley noise" in monolayer semiconductors: access to intrinsic valley relaxation timescales

Together with charge and spin degrees of freedom, many new 2D materials also permit information to be encoded in an electron's valley degree of freedom - that is, in particular momentum states in the material's Brillouin zone. With a view towards future generations of valley-based (opto)electronic technologies, the intrinsic timescales of scattering and relaxation between valleys therefore represent fundamental parameters of interest. Here we introduce and demonstrate an entirely passive, noise-based approach for exploring intrinsic valley dynamics in atomically-thin transition-metal dichalcogenide (TMD) semiconductors. Exploiting the valley-specific optical selection rules in monolayer TMDs, we use optical Faraday rotation to detect, under conditions of strict thermal equilibrium, the stochastic thermodynamic fluctuations of the valley polarization in a Fermi sea of resident carriers. Frequency spectra of this spontaneous "valley noise" reveal narrow Lorentzian lineshapes and therefore long exponentially-decaying intrinsic valley relaxation. Moreover, the valley noise signals are shown to validate both the relaxation times and the spectral dependence of conventional (perturbative) pump-probe measurements. These results provide a viable route toward quantitative measurements of intrinsic valley dynamics, free from any external perturbation, pumping, or excitation.

cond-mat.mes-hall↗

arXiv2018

Superradiant coupling effects in transition-metal dichalcogenides

Cooperative effects allow for fascinating characteristics in light-matter interacting systems. Here, we study naturally occurring superradiant coupling in a class of quasi-two-dimensional, layered semiconductor systems. We perform optical absorption experiments of the lowest exciton for transition-metal dichalcogenides with different numbers of atomic layers. We examine two representative materials, MoSe$_2$ and WSe$_2$, using incoherent broadband white light. The measured transmission at the A exciton resonance does not saturate for optically thick samples consisting of hundreds of atomic layers, and the transmission varies nonmonotonously with the layer number. A self-consistent microscopic calculation reproduces the experimental observations, clearly identifying superradiant coupling effects as the origin of this unexpected behavior.

cond-mat.mes-hall↗

arXiv2017

Gate controlled spin-valley locking of resident carriers in WSe2 monolayers

Using time-resolved Kerr rotation, we measure the spin/valley dynamics of resident electrons and holes in single charge-tunable monolayers of the archetypal transition-metal dichalcogenide (TMD) semiconductor WSe2. In the n-type regime, we observe long (70 ns) polarization relaxation of electrons that is sensitive to in-plane magnetic fields $B_y$, indicating spin relaxation. In marked contrast, extraordinarily long (2 microsecond) polarization relaxation of holes is revealed in the p-type regime, that is unaffected by $B_y$, directly confirming long-standing expectations of strong spin-valley locking of holes in the valence band of monolayer TMDs. Supported by continuous-wave Kerr spectroscopy and Hanle measurements, these studies provide a unified picture of carrier polarization dynamics in monolayer TMDs, which can guide design principles for future valleytronic devices.

cond-mat.mes-hall↗

arXiv2017

Ab initio explanation of disorder and off-stoichiometry in Fe-Mn-Al-C kappa carbides

Carbides play a central role for the strength and ductility in many materials. Simulating the impact of these precipitates on the mechanical performance requires the knowledge about their atomic configuration. In particular, the C content is often observed to substantially deviate from the ideal stoichiometric composition. In the present work, we focus on Fe-Mn-Al-C steels, for which we determined the composition of the nano-sized kappa carbides (Fe,Mn)3AlC by atom probe tomography (APT) in comparison to larger precipitates located in grain boundaries. Combining density functional theory with thermodynamic concepts, we first determine the critical temperatures for the presence of chemical and magentic disorder in these carbides. Secondly, the experimentally observed reduction of the C content is explained as a compromise between the gain in chemical energy during partitioning and the elastic strains emerging in coherent microstructures.

cond-mat.mtrl-sci↗

arXiv2013

The muon anomalous magnetic moment in the Randall-Sundrum model

We calculate the anomalous magnetic moment of the muon in the minimal Randall-Sundrum model with standard model fields in five-dimensional (5D) warped space and a brane-localized Higgs. We use a fully 5D framework to compute the one-loop matching coefficients of the effective theory at the electroweak scale. The extra contribution to the anomalous magnetic moment from the model-independent gauge-boson exchange contributions Δa_μis approximately 8.8*10^-11 (1TeV/T)^2, where 1/T denotes the location of the TeV brane in conformal coordinates, and is related to the mass of the lowest gauge boson KK excitation, which is roughly 2.5T. The result constitutes the first complete determination of the gauge-boson contribution to g-2 and is robust against the variation of the bulk fermion masses and 5D Yukawa coupling. We also determine the strongly model-parameter dependent effect of Higgs-exchange diagrams.

hep-ph↗

arXiv2013

Crossover from injection to tunneling conduction mode and associated magneto-resistance in a single $Fe_{3}O_{4}$(111)/$Alq_{3}$/Co spin-valve device

We demonstrate interface energy level engineering, exploiting the modification in energy band structure across Verwey phase transition of $Fe_{3}O_{4}$ electrode, in a $Fe_{3}O_{4}$(111)/$Alq_{3}$/Co vertical spin-valve (SV) device. Experimental results on device characteristics I-V) study exhibit a transition in conduction mode from carrier injection to tunneling across Verwey transition temperature ($T_{V}$) of $Fe_{3}O_{4}$ electrode. Both giant magneto-resistance (GMR) and tunneling MR (TMR) have been observed in a single SV device as a function of temperature, below and above $T_{V}$, respectively. Appearance of GMR, accompanied by injection limited natural Schottky-like I-V characteristics, provide evidences of spin injection at electrode/$Alq_{3}$ interface and transport through molecular orbitals in this SV device. Features of TMR exhibit significant differences from that of GMR. This is due to the dominant hyperfine-field interaction in the multi-step tunneling regime. We have achieved room-temperature SV operation in our device. A phenomenological model for device operation has been proposed to explain the transition in the conduction mode and associated MR features across $T_{V}$. We propose that the tuning of charge gap at Fermi level across Verwey transition due to charge ordering on the octahedral iron sites of $Fe_{3}O_{4}$ results in a corresponding tuning of conduction mode causing this unique cross over from GMR to TMR in this ferrite-based organic SV.

cond-mat.mes-hall↗

arXiv2007

Enhanced grain surface effect on magnetic properties of nanometric La0.7Ca0.3MnO3 manganite : Evidence of surface spin freezing of manganite nanoparticles

We have investigated the effect of nanometric grain size on magnetic properties of single phase, nanocrystalline, granular La0.7Ca0.3MnO3 (LCMO) sample. We have considered core-shell structure of our LCMO nanoparticles, which can explain its magnetic properties. From the temperature dependence of field cooled (FC) and zero-field cooled (ZFC) dc magnetization (DCM), the magnetic properties could be distinguished into two regimes: a relatively high temperature regime T > 40 K where the broad maximum of ZFC curve (at T = Tmax) is associated with the blocking of core particle moments, whereas the sharp maximum (at T = TS) is related to the freezing of surface (shell) spins. The unusual shape of M (H) loop at T = 1.5 K, temperature dependent feature of coercive field and remanent magnetization give a strong support of surface spin freezing that are occurring at lower temperature regime (T < 40 K) in this LCMO nanoparticles. Additionally, waiting time (tw) dependence of ZFC relaxation measurements at T = 50 K show weak dependence of relaxation rate [S(t)] on tw and dM/dln(t) following a logarithmic variation on time. Both of these features strongly support the high temperature regime to be associated with the blocking of core moments. At T = 20 K, ZFC relaxation measurements indicates the existence of two different types of relaxation processes in the sample with S(t) attaining a maximum at the elapsed time very close to the wait time tw = 1000 sec, which is an unequivocal sign of glassy behavior. This age-dependent effect convincingly establish the surface spin freezing of our LCMO nanoparticles associated with a background of superparamagnetic (SPM) phase of core moments.

cond-mat.mtrl-sci↗

arXiv2006

Direct evidence of random field effect on magnetic ordering of La_(0.5)Gd_(0.2)Sr_(0.3)MnO_(3) manganite system

We report direct experimental evidence of the effect of quenched random field on magnetic ordering of La_(0.5)Gd_(0.2)Sr_(0.3)MnO_(3) manganites system. We demonstrate magnetic measurements providing serious evidence to support that quenched random field of Gd divides the system in finite size clusters which undergo cluster-glass like freezing. The size or concentration of these clusters is found to be closely related to the effect of random field, which in turn is a function of applied field.

cond-mat.str-el↗