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P. E. Jönsson

Publications and source records attributed to P. E. Jönsson.

17 recordsLinked to original sources
arXiv2012

Finite-size effects in amorphous Fe90Zr10/Al75Zr25 multilayers

The thickness dependence of the magnetic properties of amorphous Fe90Zr10 layers has been explored using Fe90Zr10/Al75Zr25 multilayers. The Al75Zr25 layer thickness is kept at 40 Å, while the thickness of the Fe90Zr10 layers is varied between 5 and 20 Å. The thickness of the Al75Zr25 layers is sufficiently large to suppress any significant interlayer coupling. Both the Curie temperature and the spontaneous magnetization decrease non-linearly with decreasing thickness of the Fe90Zr10 layers. No ferromagnetic order is observed in the multilayer with 5 Å Fe90Zr10 layers. The variation of the Curie temperature $T_c$ with the Fe90Zr10 layer thickness $t$ is fitted with a finite-size scaling formula $[1-\Tc(t)/\Tc(\infty)]=[(t-t')/t_0]^{-λ}$, yielding $λ=1.2$, and a critical thickness $t'=6.5$ Å, below which the Curie temperature is zero.

cond-mat.mtrl-sci↗
arXiv2007

Absence of Conventional Spin-Glass Transition in the Ising Dipolar System LiHo_xY_{1-x}F_4

The magnetic properties of single crystals of LiHo_xY_{1-x}F_4 with x=16.5% and x=4.5% were recorded down to 35 mK using a micro-SQUID magnetometer. While this system is considered as the archetypal quantum spin glass, the detailed analysis of our magnetization data indicates the absence of a phase transition, not only in a transverse applied magnetic field, but also without field. A zero-Kelvin phase transition is also unlikely, as the magnetization seems to follow a non-critical exponential dependence on the temperature. Our analysis thus unmasks the true, short-ranged nature of the magnetic properties of the LiHo_xY_{1-x}F_4 system, validating recent theoretical investigations suggesting the lack of phase transition in this system.

cond-mat.dis-nn↗
arXiv2007

Electron Correlation Driven Heavy-Fermion Formation in LiV2O4

Optical reflectivity measurements were performed on a single crystal of the d-electron heavy-fermion (HF) metal LiV2O4. The results evidence the highly incoherent character of the charge dynamics for all temperatures above T^* \approx 20 K. The spectral weight of the optical conductivity is redistributed over extremely broad energy scales (~ 5 eV) as the quantum coherence of the charge carriers is recovered. This wide redistribution is, in sharp contrast to f-electron Kondo lattice HF systems, characteristic of a metallic system close to a correlation driven insulating state. Our results thus reveal that strong electronic correlation effects dominate the low-energy charge dynamics and heavy quasiparticle formation in LiV2O4. We propose the geometrical frustration, which limits the extension of charge and spin ordering, as an additional key ingredient of the low-temperature heavy-fermion formation in this system.

cond-mat.str-el↗
arXiv2005

Dynamical breakdown of the Ising spin-glass order under a magnetic field

The dynamical magnetic properties of an Ising spin glass Fe$_{0.55}$Mn$_{0.45}$TiO$_3$ are studied under various magnetic fields. Having determined the temperature and static field dependent relaxation time $τ(T;H)$ from ac magnetization measurements under a dc bias field by a general method, we first demonstrate that these data provide evidence for a spin-glass (SG) phase transition only in zero field. We next argue that the data $τ(T;H)$ of finite $H$ can be well interpreted by the droplet theory which predicts the absence of a SG phase transition in finite fields.

cond-mat.dis-nn↗
arXiv2004

Spin Glasses: A Ghost Story

Extensive experimental and numerical studies of the non-equilibrium dynamics of spin glasses subjected to temperature or bond perturbations have been performed to investigate chaos and memory effects in selected spin glass systems. Temperature shift and cycling experiments were performed on the strongly anisotropic Ising-like system {\ising} and the weakly anisotropic Heisenberg-like system {\AgMn}, while bond shift and cycling simulations were carried out on a 4 dimensional Ising Edwards-Anderson spin glass. These spin glass systems display qualitatively the same characteristic features and the observed memory phenomena are found to be consistent with predictions from the ghost domain scenario of the droplet scaling model.

cond-mat.mtrl-sci↗
arXiv2004

Aging and Memory Effects in Superparamagnets and Superspin Glasses

Many dense magnetic nanoparticle systems exhibit slow dynamics which is qualitatively indistinguishable from that observed in atomic spin glasses and its origin is attributed to dipole interactions among particle moments (or superspins). However, even in dilute nanoparticle systems where the dipole interactions are vanishingly small, slow dynamics is observed and is attributed solely to a broad distribution of relaxation times which in turn comes from that of the anisotropy energy barriers. To clarify characteristic differences between the two types of slow dynamics, we study a simple model of a non-interacting nanoparticle system (a superparamagnet) analytically as well as ferritin (a superparamagnet) and a dense Fe-N nanoparticle system (a superspin glass) experimentally. It is found that superparamagnets in fact show aging (a waiting time dependence) of the thermoremanent-magnetization as well as various memory effects. We also find some dynamical phenomena peculiar only to superspin glasses such as the flatness of the field-cooled magnetization below the critical temperature and memory effects in the zero-field-cooled magnetization. These dynamical phenomena are qualitatively reproduced by the random energy model, and are well interpreted by the so-called droplet theory in the field of the spin-glass study.

cond-mat.dis-nn↗
arXiv2004

Absence of rejuvenation in a Superspin Glass

Effects of temperature changes on the nonequilibrium spin-glass dynamics of a strongly interacting ferromagnetic nanoparticle system (superspin glass) are studied. In contrary to atomic spin glasses, strong cooling rate effects are observed, and no evidence for temperature-chaos is found. The flip time of a magnetic moment is much longer than that of an atomic spin and hence much shorter time scales are probed within the experimental time window for a superspin glass than for an atomic spin glass. Within a real space picture the cumulative aging observed for the superspin glass can be explained considering that all investigated length scales are shorter than the temperature-chaos overlap length. The transient relaxation, observed in experiments after temperature changes, can be understood as the adjustment of thermally active droplets, which is mutatis mutandis the Kovacs effect observed in most glassy systems.

cond-mat.dis-nn↗
arXiv2004

Comment on "Memory Effects in an Interacting Magnetic Nanoparticle System"

In Phys. Rev. Lett. 91 167206 (2003), Sun et al. study memory effects in an interacting nanoparticle system with specific temperature and field protocols. The authors claim that the observed memory effects originate from spin-glass dynamics and that the results are consistent with the hierarchical picture of the spin-glass phase. In this comment, we argue their claims premature by demonstrating that all their experimental curves can be reproduced qualitatively using only a simplified model of isolated nanoparticles with a temperature dependent distribution of relaxation times.

cond-mat.dis-nn↗
arXiv2002

Strong rejuvenation in a chiral-glass superconductor

The glassy paramagnetic Meissner phase of a Bi$_2$Sr$_2$CaCu$_2$O$_x$ superconductor ($x$ = 8.18) is investigated by squid magnetometry, using ``dc-memory'' experiments employed earlier to study spin glasses. The temperature dependence of the zero-field-cooled and thermo-remanent magnetization is recorded on re-heating after specific cooling protocols, in which single or multiple halts are performed at constant temperatures. The 'spin' states equilibrated during the halts are retrieved on re-heating. The observed memory and rejuvenation effects are similar to those observed in Heisenberg-like spin glasses.

cond-mat.mtrl-sci↗
arXiv2002

Domain growth by isothermal aging in 3d Ising and Heisenberg spin glasses

Non-equilibrium dynamics of three dimensional model spin glasses - the Ising system Fe$_{0.50}$Mn$_{0.50}$TiO$_3$ and the Heisenberg like system Ag(11 at% Mn) - has been investigated by measurements of the isothermal time decay of the low frequency ac-susceptibility after a quench from the paramagnetic to the spin glass phase. It is found that the relaxation data measured at different temperatures can be scaled according to predictions from the droplet scaling model, provided that critical fluctuations are accounted for in the analyzes.

cond-mat.dis-nn↗
arXiv2002

Symmetrical Temperature-Chaos Effect with Positive and Negative Temperature Shifts in a Spin Glass

The aging in a Heisenberg-like spin glass Ag(11 at% Mn) is investigated by measurements of the zero field cooled magnetic relaxation at a constant temperature after small temperature shifts $|ΔT/T_g| < 0.012$. A crossover from fully accumulative to non-accumulative aging is observed, and by converting time scales to length scales using the logarithmic growth law of the droplet model, we find a quantitative evidence that positive and negative temperature shifts cause an equivalent restart of aging (rejuvenation) in terms of dynamical length scales. This result supports the existence of a unique overlap length between a pair of equilibrium states in the spin glass system.

cond-mat.dis-nn↗
arXiv2001

Thermodynamic perturbation theory for dipolar superparamagnets

Thermodynamic perturbation theory is employed to derive analytical expressions for the equilibrium linear susceptibility and specific heat of lattices of anisotropic classical spins weakly coupled by the dipole-dipole interaction. The calculation is carried out to the second order in the coupling constant over the temperature, while the single-spin anisotropy is treated exactly. The temperature range of applicability of the results is, for weak anisotropy (A/kT << 1), similar to that of ordinary high-temperature expansions, but for moderately and strongly anisotropic spins (A/kT > 1) it can extend down to the temperatures where the superparamagnetic blocking takes place (A/kT \sim 25), provided only the interaction strength is weak enough. Besides, taking exactly the anisotropy into account, the results describe as particular cases the effects of the interactions on isotropic (A = 0) as well as strongly anisotropic (A \to \infty) systems (discrete orientation model and plane rotators).

cond-mat.mtrl-sci↗
arXiv2001

Fragility of the spin-glass-like collective state to a magnetic field in an interacting Fe-C nanoparticle system

The effect of applied magnetic fields on the collective nonequilibrium dynamics of a strongly interacting Fe-C nanoparticle system has been investigated. It is experimentally shown that the magnetic aging diminishes to finally disappear for fields of moderate strength. The field needed to remove the observable aging behavior increases with decreasing temperature. The same qualitative behavior is observed in an amorphous metallic spin glass (Fe_{0.15}Ni_{0.85})_{75}P_{16}B_6Al_3.

cond-mat.mtrl-sci↗
arXiv2001

Memory and chaos in an Ising spin glass

The non-equilibrium dynamics of the model 3d-Ising spin glass - Fe$_{0.55}$Mn$_{0.45}$TiO$_3$ - has been investigated from the temperature and time dependence of the zero field cooled magnetization recorded under certain thermal protocols. The results manifest chaos, rejuvenation and memory features of the equilibrating spin configuration that are very similar to those observed in corresponding studies of the archetypal RKKY spin glass Ag(Mn). The sample is rapidly cooled in zero magnetic field, and the magnetization recorded on re-heating. When a stop at constant temperature $T_s$ is made during the cooling, the system evolves toward its equilibrium state at this temperature. The equilibrated state established during the stop becomes frozen in on further cooling and is retrieved on re-heating. The memory of the aging at $T_s$ is not affected by a second stop at a lower temperature $T'_s$. Reciprocally, the first equilibration at $T_s$ has no influence on the relaxation at $T'_s$, as expected within the droplet model for domain growth in a chaotic landscape.

cond-mat.mtrl-sci↗
arXiv2001

Relaxation time of weakly interacting superparamagnets

The relaxation time of weakly interacting classical spins is calculated by introducing the averages of the local dipolar field, obtained by thermodynamic perturbation theory, in a rigorous expression for the single-spin thermoactivation rate in a weak but arbitrarily oriented field. At low temperatures the non-trivial dependence of the superparamagnetic blocking on the damping coefficient, numerically found by Berkov and Gorn, is reproduced by our model and interpreted in terms of the deviations from uniaxial anisotropy associated to the transversal component of the dipolar field acting on each spin.

cond-mat.mtrl-sci↗