arXiv subjects

P. G. LaBarre

Publications and source records attributed to P. G. LaBarre.

6 recordsLinked to original sources

arXiv2022

Neutron Scattering Study of Fluctuating and Static Spin Correlations in the Anisotropic Spin Glass Fe$_2$TiO$_5$

The anisotropic spin glass transition, in which spin freezing is observed only along the c-axis in pseudobrookite Fe$_2$TiO$_5$, has long been perplexing because the Fe$^{3+}$ moments (d$^5$) are expected to be isotropic. Recently, neutron diffraction demonstrated that surfboard-shaped antiferromagnetic nanoregions coalesce above the glass transition temperature, T$_g$ $\approx$ 55 K, and a model was proposed in which the freezing of the fluctuations of the surfboards' magnetization leads to the anisotropic spin glass state. Given this new model, we have carried out high resolution inelastic neutron scattering measurements of the spin-spin correlations to understand the temperature dependence of the intra-surfboard spin dynamics on neutron (picosecond) time-scales. Here, we report on the temperature-dependence of the spin fluctuations measured from single crystal Fe$_2$TiO$_5$. Strong quasi-elastic magnetic scattering, arising from intra-surfboard correlations, is observed well above T$_g$. The spin fluctuations possess a steep energy-wave vector relation and are indicative of strong exchange interactions, consistent with the large Curie-Weiss temperature. As the temperature approaches T$_g$ from above, a shift in spectral weight from inelastic to elastic scattering is observed. At various temperatures between 4 K and 300 K, a characteristic relaxation rate of the fluctuations is determined. Despite the freezing of the majority of the spin correlations, an inelastic contribution remains even at base temperature, signifying the presence of fluctuating intra-surfboard spin correlations to at least T/T$_g$ $\approx$ 0.1 consistent with a description of Fe$_2$TiO$_5$ as a hybrid between conventional and geometrically frustrated spin glasses.

cond-mat.dis-nn↗

arXiv2022

The Geometrically Frustrated Spin Glass (Fe1-pGap)2TiO5

The unusual anisotropy of the spin glass transition in the pseudobrookite system Fe$_2$TiO$_5$ has been interpreted as arising from an induced, van der Waals-like, interaction among magnetic clusters. Here we present susceptibility ($χ$) and specific heat data (C) for Fe2TiO5 diluted with non-magnetic Ga, (Fe$_{1-p}$Ga$_p$)$_2$TiO$_5$, for disorder parameter p = 0, 0.11, and 0.42, and elastic neutron scattering data for p = 0.20. A uniform suppression of T{_g} is observed upon increasing p, along with a value of $χ(T_g)$ that increases as T$_g$ decreases, i.e. $dχ(T_g)/dT_g< 0$. We also observe C(T) $\propto$ T$^2$ in the low temperature limit. The observed behavior places (Fe$_{1-p}$Ga$_p$)$_2$TiO$_5$ in the category of a strongly geometrically frustrated spin glass.

cond-mat.dis-nn↗

arXiv2022

Magnetoquantum Oscillations in the Specific Heat of a Topological Kondo Insulator

Surprisingly, magnetoquantum oscillations (MQO) characteristic of a metal with a Fermi surface have been observed in measurements of the topological Kondo insulator SmB6. As these MQO have only been observed in measurements of magnetic torque (dHvA) and not in measurements of magnetoresistance (SdH), a debate has arisen as to whether the MQO are an extrinsic effect arising from rare-earth impurities, defects, and/or aluminum inclusions or an intrinsic effect revealing the existence of charge-neutral excitations. We report here the first observation of magnetoquantum oscillations in the low-temperature specific heat of SmB6. The observed frequencies and their angular dependence for these flux-grown samples are consistent with previous results based on magnetic torque for SmB6 but the inferred effective masses are significantly larger than previously reported. Such oscillations can only be observed if the MQO are of bulk thermodynamic origin; the measured magnetic-field dependent oscillation amplitude and effective mass allow us to rule out suggestions of an extrinsic, aluminium inclusion-based origin for the MQO.

cond-mat.str-el↗

arXiv2022

Observation of Quantum Oscillations in The Low Temperature Specific Heat of SmB$_6$

We report measurements of the low-temperature specific heat of Al-flux-grown samples of SmB$_6$ in magnetic fields up to 32 T. Quantum oscillations periodic in $1/H$ are observed between 8 and 32 T at selected angles between [001] and [111]. The observed frequencies and their angular dependence are consistent with previous magnetic torque measurements of SmB$_6$ but the effective masses inferred from Lifshitz-Kosevich theory are significantly larger and closer to those inferred from zero-field specific heat. Our results are thus consistent with a bulk density of states origin for the oscillations.

cond-mat.str-el↗

arXiv2020

Fluctuation-Induced Interactions and the Spin Glass Transition in $Fe_2TiO_5$

We investigate the spin-glass transition in the strongly frustrated well-known compound $Fe_2TiO_5$. A remarkable feature of this transition, widely discussed in the literature, is its anisotropic properties: the transition manifests itself in the magnetic susceptibly only along one axis, despite $Fe^{3+}$ $d^5$ spins having no orbital component. We demonstrate, using neutron scattering, that below the transition temperature $T_g = 55 K$, $Fe_2TiO_5$ develops nanoscale surfboard shaped antiferromagnetic regions in which the $Fe^{3+}$ spins are aligned perpendicular to the axis which exhibits freezing. We show that the glass transition may result from the freezing of transverse fluctuations of the magnetization of these regions and we develop a mean-field replica theory of such a transition, revealing a type of magnetic van der Waals effect.

cond-mat.dis-nn↗

arXiv2019

Evidence for Undoped Weyl Semimetal Charge Transport in $Y_{2}Ir_{2}O_{7}$

Weyl fermions scattering from a random Coulomb potential are predicted to exhibit resistivity versus temperature $ρ\space α\space T^{-4}$ in a single particle model. Here we show that, in closed environment-grown polycrystalline samples of $Y_{2}Ir_{2}O_{7}$, $ρ= ρ_{0} T^{-4}$ over four orders of magnitude in $ρ$. While the measured prefactor, $ρ_{0}$, is obtained from the model using reasonable materials parameters, the $T^{-4}$ behavior extends far beyond the model's range of applicability. In particular, the behavior extends into the low-temperature, high-resistivity region where the Ioffe-Regel parameter, $k_{T} \ell \ll 2π$. Strong on-site Coulomb correlations, instrumental for predicting a Weyl semimetal state in $Y_{2}Ir_{2}O_{7}$, are the possible origin of such "bad" Weyl semimetal behavior.

cond-mat.str-el↗