arXiv subjects

P. Hartogh

Publications and source records attributed to P. Hartogh.

At least 19 recordsLinked to original sources

arXiv2026

New 12C/13C and 14N/15N isotopic ratio measurements in Jupiter's stratosphere revealed by ALMA

The collision of comet SL9 with Jupiter in 1994 changed the chemical composition of the Jovian stratosphere for decades. New molecules were detected minutes after the impacts (HCN, CO, CS, etc.) and some are still present today. They were deposited in the stratosphere at pressures lower than 0.1 mbar and were most probably formed by shock-induced chemistry recombining Jovian and cometary material. However, the question of the origin of these molecules is still not completely understood. One way to address this open question is to determine the isotopic composition of the new molecules. Isotopic ratios have long been measured in the Solar System. They present a variety of values depending on the object or the molecule and therefore trace different reservoirs of material. Derivations of carbon and nitrogen isotopic ratios in HCN four years after SL9 showed atypical depletions in the heavier isotopes that had never been observed before in the Solar System. These results suggested an unusual cometary composition or an unknown fractionation mechanism in the hot and shocked air parcels. We aim to measure carbon and nitrogen isotopic ratios in HCN to shed light on the puzzling results of 1998. With Atacama Large Millimeter/submillimeter Array data from 2017 and radiative-transfer calculations, we derived the abundance of two HCN isotopologues, H13CN and HC15N, at pressures probed from 0.03 to 1.8 mbar. We find 12C/13C = $73\pm5$ and 14N/15N = $245\pm29$, respectively (0.76-0.87) and (0.80-1.00) times the terrestrial references, and (0.69-0.87) and (0.42-0.70) times the solar-Jovian bulk values. In contrast to the strong depletions reported in 1998, our values are instead compatible with an enrichment in the heavier isotopes relative to the Jovian bulk. We interpret these enrichments as the direct signature of the cometary contribution in HCN and/or as 23 years of chemical evolution.

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arXiv2023

A Collection of German Science Interests in the Next Generation Very Large Array

The Next Generation Very Large Array (ngVLA) is a planned radio interferometer providing unprecedented sensitivity at wavelengths between 21 cm and 3 mm. Its 263 antenna element array will be spatially distributed across North America to enable both superb low surface brightness recovery and sub-milliarcsecond angular resolution imaging. The project was developed by the international astronomy community under the lead of the National Radio Astronomy Observatory (NRAO), and is anticipated to be built between 2027 and 2037. Two workshops have been held in 2022 and 2023 with the goal to discuss and consolidate the scientific interests in the ngVLA within the German astronomical community. This community paper constitutes a collection of 48 science ideas which the German community aims to pursue with the ngVLA in the 2030s. This is not a complete list and the ideas are not developed at the level of a "Science Book", such that the present document is mainly meant provide a basis for further discussion within the community. As such, additional contributions are welcome, and will be considered for inclusion in future revisions.

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arXiv2023

Cometary surface dust layers built out of millimetre-scale aggregates: dependence of modelled cometary gas production on the layer transport properties

The standard approach to obtaining knowledge about the properties of the surface layer of a comet from observations of gas production consists of two stages. First, various thermophysical models are used to calculate gas production for a few sets of parameters. Second, a comparison of observations and theoretical predictions is performed. This approach is complicated because the values of many model characteristics are known only approximately. Therefore, it is necessary to investigate the sensitivity of the simulated outgassing to variations in the properties of the surface layer. This problem was recently considered by us for aggregates up to tens of microns in size. For millimetre-size aggregates, a qualitative extension of the method used to model the structural characteristics of the layer is required. It is also necessary to study the role of radiative thermal conductivity, which may play an important role for such large particles. We investigated layers constructed from large aggregates and having various thicknesses and porosity and evaluated the effective sublimation of water ice at different heliocentric distances. For radiative conductivity, approximate commonly used models and the complicated model based on the Dense Medium Radiative Transfer theory were compared. It was shown that for millimetre-size aggregates careful consideration of the radiative thermal conductivity is required since this mechanism of energy transfer may change the resulting gas productivity by several times. We demonstrate that our model is more realistic for an evolved comet than simple models parameterising the properties of the cometary surface layer, yet maintains comparable computational complexity.

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arXiv2022

Moonraker -- Enceladus Multiple Flyby Mission

Enceladus, an icy moon of Saturn, possesses an internal water ocean and jets expelling ocean material into space. Cassini investigations indicated that the subsurface ocean could be a habitable environment having a complex interaction with the rocky core. Further investigation of the composition of the plume formed by the jets is necessary to fully understand the ocean, its potential habitability, and what it tells us about Enceladus' origin. Moonraker has been proposed as an ESA M-class mission designed to orbit Saturn and perform multiple flybys of Enceladus, focusing on traversals of the plume. The proposed Moonraker mission consists of an ESA-provided platform, with strong heritage from JUICE and Mars Sample Return, and carrying a suite of instruments dedicated to plume and surface analysis. The nominal Moonraker mission has a duration of 13.5 years. It includes a 23-flyby segment with 189 days allocated for the science phase, and can be expanded with additional segments if resources allow. The mission concept consists in investigating: i) the habitability conditions of present-day Enceladus and its internal ocean, ii) the mechanisms at play for the communication between the internal ocean and the surface of the South Polar Terrain, and iii) the formation conditions of the moon. Moonraker, thanks to state-of-the-art instruments representing a significant improvement over Cassini's payload, would quantify the abundance of key species in the plume, isotopic ratios, and physical parameters of the plume and the surface. Such a mission would pave the way for a possible future landed mission.

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arXiv2022

Water, hydrogen cyanide, carbon monoxide, and dust production from distant comet 29P/Schwassmann-Wachmann 1

29P/Schwassmann-Wachmann 1 is a distant Centaur/comet, showing persistent CO-driven activity and frequent outbursts. We used the Herschel space observatory in 2010, 2011, and 2013 to observe H$_2$O and NH$_3$ and to image the dust coma. Observations with the IRAM 30 m were undertaken in 2007, 2010, 2011, and 2021 to monitor the CO production rate and to search for HCN. Modeling was performed to constrain the size of the sublimating icy grains and to derive the dust production rate. HCN is detected for the first time in comet 29P (at 5$\sigma$ in the line area). H$_2$O is detected as well, but not NH$_3$. H$_2$O and HCN line shapes differ strongly from the CO line shape, indicating that these two species are released from icy grains. CO production rates are in the range (2.9-5.6) $\times$ 10$^{28}$ s$^{-1}$ (1400--2600 kg s$^{-1}$). A correlation between the CO production rate and coma brightness is observed, as is a correlation between CO and H$_2$O production. The correlation obtained between the excess of CO production and excess of dust brightness with respect to the quiescent state is similar to that established for the continuous activity of comet Hale-Bopp. The measured $Q$(H$_2$O)/$Q$(CO) and $Q$(HCN)/$Q$(CO) production rate ratios are 10.0 $\pm$ 1.5 % and 0.12 $\pm$ 0.03 %, respectively, averaging the April-May 2010 measurements ($Q$(H$_2$O) = (4.1 $\pm$ 0.6) $\times$ 10$^{27}$ s$^{-1}$, $Q$(HCN) = (4.8 $\pm$ 1.1) $\times$ 10$^{25}$ s$^{-1}$). We derive three independent and similar values of the effective radius of the nucleus, $\sim$ 31 $\pm$ 3 km. The inferred dust mass-loss rates during quiescent phases are in the range 30-120 kg s$^{-1}$, indicating a dust-to-gas mass ratio $<$ 0.1 during quiescent activity. We conclude that strong local heterogeneities exist on the surface of 29P, with quenched dust activity from most of the surface, but not in outbursting regions.

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arXiv2021

Ground-based HCN submillimetre measurements in Titan's atmosphere: an intercomparison with Herschel observations

The aim of this study is to measure the vertical distribution of HCN on Titan's stratosphere using ground-based submm observations acquired quasi-simultaneously with the Herschel ones. This allows us to perform a consistency check between space and ground-based observations and to build a reference mean HCN vertical profile in Titan's stratosphere. Using APEX and IRAM 30-m, we obtained the spectral emission of HCN (4-3) and (3-2) lines. We applied a line-by-line radiative transfer code to calculate the synthetic spectra of HCN, and a retrieval algorithm based on optimal estimation to retrieve the temperature and HCN distributions. Our derived HCN abundance profiles are consistent with an increase from 40 ppb at ~100 km to 4 ppm at ~200 km, which is an altitude region where the HCN signatures are sensitive. We also demonstrate that the retrieved HCN distribution is sensitive to the data information. Comparisons between our results and the values from Herschel show similar abundance distributions, with maximum differences of 2.5 ppm ranging between 100 and 300 km. These comparisons also allow us to inter-validate both data sets and indicate reliable and consistent measurements. The inferred abundances are also consistent with the distribution in previous observational studies, with the profiles from ALMA, Cassini/CIRS, and SMA (the latest ones below ~230 km). Our HCN profile is also comparable to photochemical models by Krasnopolsky (2014) and Vuitton et al. (2019) below 230 km and consistent with that of Loison et al. (2015) above 250 km. However, it appears to show large differences with respect to the estimates by Loison et al. (2015), Dobrijevic & Loison (2018), and Lora et al. (2018) below 170 km, and by Dobrijevic & Loison (2018) and Lora et al. (2018) above 400 km, although they are similar in shape. We conclude that these particular photochemical models need improvement.

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arXiv2021

First direct measurement of auroral and equatorial jets in the stratosphere of Jupiter

Context. The tropospheric wind pattern in Jupiter consists of alternating prograde and retrograde zonal jets with typical velocities of up to 100 m/s around the equator. At much higher altitudes, in the ionosphere, strong auroral jets have been discovered with velocities of 1-2 km/s. There is no such direct measurement in the stratosphere of the planet. Aims. In this paper, we bridge the altitude gap between these measurements by directly measuring the wind speeds in Jupiter's stratosphere. Methods. We use the Atacama Large Millimeter/submillimeter Array's very high spectral and angular resolution imaging of the stratosphere of Jupiter to retrieve the wind speeds as a function of latitude by fitting the Doppler shifts induced by the winds on the spectral lines. Results. We detect for the first time equatorial zonal jets that reside at 1 mbar, i.e. above the altitudes where Jupiter's Quasi-Quadrennial Oscillation occurs. Most noticeably, we find 300-400 m/s non-zonal winds at 0.1 mbar over the polar regions underneath the main auroral ovals. They are in counter-rotation and lie several hundreds of kilometers below the ionospheric auroral winds. We suspect them to be the lower tail of the ionospheric auroral winds. Conclusions. We detect directly and for the first time strong winds in Jupiter's stratosphere. They are zonal at low-to-mid latitudes and non-zonal at polar latitudes. The wind system found at polar latitudes may help increase the effciency of chemical complexification by confining the photochemical products in a region of large energetic electron precipitation.

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arXiv2020

Origins Space Telescope: From First Light to Life -- ESA Voyage 2050 White Paper

The Origins Space Telescope (Origins) is one of four science and technology definition studies selected by National Aeronautics and Space Administration (NASA) in preparation of the 2020 Astronomy and Astrophysics Decadal survey in the US. Origins will trace the history of our origins from the time dust and heavy elements permanently altered the cosmic landscape to present-day life. It is designed to answer three major science questions: How do galaxies form stars, make metals, and grow their central supermassive black holes from reionization? How do the conditions for habitability develop during the process of planet formation? Do planets orbiting M-dwarf stars support life? Origins operates at mid- to far-infrared wavelengths from ~2.8 to 588 μm, is more than 1000 times more sensitive than prior far-IR missions due to its cold (~4.5 K) aperture and state-of-the-art instruments.

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arXiv2020

18-year long monitoring of the evolution of H2O vapor in the stratosphere of Jupiter with the Odin space telescope

Comet Shoemaker-Levy 9 impacted Jupiter in July 1994, leaving its stratosphere with several new species, among them water vapor (H2O). With the aid of a photochemical model H2O can be used as a dynamical tracer in the jovian stratosphere. In this paper, we aim at constraining vertical eddy diffusion (Kzz) at the levels where H2O resides. We monitored the H2O disk-averaged emission at 556.936 GHz with the Odin space telescope between 2002 and 2019, covering nearly two decades. We analyzed the data with a combination of 1D photochemical and radiative transfer models to constrain vertical eddy diffusion in the stratosphere of Jupiter. The Odin observations show us that the emission of H2O has an almost linear decrease of about 40% between 2002 and 2019.We can only reproduce our time series if we increase the magnitude of Kzz in the pressure range where H2O diffuses downward from 2002 to 2019, i.e. from ~0.2 mbar to ~5 mbar. However, this modified Kzz is incompatible with hydrocarbon observations. We find that, even if allowance is made for the initially large abundances of H2O and CO at the impact latitudes, the photochemical conversion of H2O to CO2 is not sufficient to explain the progressive decline of the H2O line emission, suggestive of additional loss mechanisms. The Kzz we derived from the Odin observations of H2O can only be viewed as an upper limit in the ~0.2 mbar to ~5 mbar pressure range. The incompatibility between the interpretations made from H2O and hydrocarbon observations probably results from 1D modeling limitations. Meridional variability of H2O, most probably at auroral latitudes, would need to be assessed and compared with that of hydrocarbons to quantify the role of auroral chemistry in the temporal evolution of the H2O abundance since the SL9 impacts. Modeling the temporal evolution of SL9 species with a 2D model would be the next natural step.

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arXiv2019

Herschel map of Saturn's stratospheric water, delivered by the plumes of Enceladus

Context. The origin of water in the stratospheres of Giant Planets has been an outstanding question ever since its first detection by ISO some 20 years ago. Water can originate from interplanetary dust particles, icy rings and satellites and large comet impacts. Analysis of Herschel Space Observatory observations have proven that the bulk of Jupiter's stratospheric water was delivered by the Shoemaker-Levy 9 impacts in 1994. In 2006, the Cassini mission detected water plumes at the South Pole of Enceladus, placing the moon as a serious candidate for Saturn's stratospheric water. Further evidence was found in 2011, when Herschel demonstrated the presence of a water torus at the orbital distance of Enceladus, fed by the moon's plumes. Finally, water falling from the rings onto Saturn's uppermost atmospheric layers at low latitudes was detected during the final orbits of Cassini's end-of-mission plunge into the atmosphere. Aims. In this paper, we use Herschel mapping observations of water in Saturn's stratosphere to identify its source. Methods. Several empirical models are tested against the Herschel-HIFI and -PACS observations, which were collected on December 30, 2010, and January 2nd, 2011 (respectively). Results. We demonstrate that Saturn's stratospheric water is not uniformly mixed as a function of latitude, but peaking at the equator and decreasing poleward with a Gaussian distribution. We obtain our best fit with an equatorial mole fraction 1.1 ppb and a half-width at half-maximum of 25°, when accounting for a temperature increase in the two warm stratospheric vortices produced by Saturn's Great Storm of 2010-2011. Conclusions. This work demonstrates that Enceladus is the main source of Saturn's stratospheric water.

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arXiv2019

3D analysis of spatial resolution of MIRO/Rosetta measurements at 67P/CG

The MIRO instrument's remote sensing capability is integral in constraining water density, temperature and velocity fields in the coma of 67P/Churyumov-Gersimenko. Our aim is to quantify the contribution to the water density from all facets inside and outside the field-of-view (FOV) of MIRO, in both, nadir and limb geometries. This information is crucial for understanding the MIRO derived coma production rates and their relation to the nucleus characteristics, and inherent spatial resolution of the data. This study relies on a detailed 3D nucleus shape model, illumination conditions and the pointing information of the viewing geometry. With these parameters, we can evaluate the relative contribution of water density originating from facets directly inside the MIRO beam as well outside of the beam as a function of distance along the MIRO line-of-sight. We also calculate the ratio of in-beam versus out-of-beam number density. We demonstrate that despite the rather small MIRO field-of-view there is only a small fraction of molecules that originate from facets within the MIRO beam. This is true for nadir, but also translated into the limb observing geometry. The MIRO instrument cannot discriminate active from non-active regions directly from observations. This study also suggests that the beam averaged solar incidence angle, local time and mean normal vectors are not necessary related to molecules within the MIRO beam. These results also illustrate why the 1D spherical Haser model can be applied with relative success for analyzing the MIRO data (and generally any Rosetta measurements). The future possibilities of constraining gas activity distribution on the surface should use 3D codes extracting information from the MIRO spectral line shapes which contain additional information. The presented results are in fact applicable to all relevant instruments onboard Rosetta.

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arXiv2019

Constraining spatial pattern of early activity of comet 67P/C-G with 3D modeling of the MIRO observations

Our aim is to investigate early activity (July 2014) of 67P/CG with 3D coma and radiative transfer modeling of MIRO measurements, accounting for nucleus shape, illumination, and orientation of the comet. We investigate MIRO line shape information for spatial distribution of water activity on the nucleus during the onset of activity. During this period we show that MIRO line shape have enough information to clearly isolate contribution from Hapi and Inhotep independently, and compare it to the nominal case of activity from the entire illuminated surface. We also demonstrate that spectral line shapes differ from the 1D model for different viewing geometries and coma conditions relevant to this study. Specifically, line shapes are somewhat sensitive to the location of the terminator in the coma. At last, fitting the MIRO observations we show that the Imhotep region (possible extended source of H$_{2}$O due to CO$_{2}$ activity) contributes only a small fraction of the total number of water molecules into MIRO beam in the early activity. On the other hand, a strong enhancement of water activity from the Hapi region seems required to fit the MIRO line shapes. This is consistent with earlier Rosetta results. Nevertheless, within the assumption of our coma and surface boundary conditions, we cannot get a reasonable fit to all MIRO mapping observations in July 2014, which may illustrate that a more sophisticated coma model or more accurate temperature/velocity distribution is needed.

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arXiv2017

Tensile Strength of 67P/Churyumov-Gerasimenko Nucleus Material from Overhangs

We directly measure twenty overhanging cliffs on the surface of comet 67P/Churyumov-Gerasimenko extracted from the latest shape model and estimate the minimum tensile strengths needed to support them against collapse under the comet's gravity. We find extremely low strengths of around one Pa or less (one to five Pa, when scaled to a metre length). The presence of eroded material at the base of most overhangs, as well as the observed collapse of two features and implied previous collapse of another, suggests that they are prone to failure and that true material strengths are close to these lower limits (although we only consider static stresses and not dynamic stress from, for example, cometary activity). Thus, a tensile strength of a few pascals is a good approximation for the tensile strength of 67P's nucleus material, which is in agreement with previous work. We find no particular trends in overhang properties with size, over the $\sim10-100$ m range studied here, or location on the nucleus. There are no obvious differences, in terms of strength, height or evidence of collapse, between the populations of overhangs on the two cometary lobes, suggesting that 67P is relatively homogenous in terms of tensile strength. Low material strengths are supportive of cometary formation as a primordial rubble pile or by collisional fragmentation of a small (tens of km) body.

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arXiv2017

Thermal fracturing on comets. Applications to 67P/Churyumov-Gerasimenko

We simulate the stresses induced by temperature changes in a putative hard layer near the surface of comet 67P/Churyumov--Gerasimenko with a thermo-viscoelastic model. Such a layer could be formed by the recondensation or sintering of water ice (and dust grains), as suggested by laboratory experiments and computer simulations, and would explain the high compressive strength encountered by experiments on board the Philae lander. Changes in temperature from seasonal insolation variation penetrate into the comet's surface to depths controlled by the thermal inertia, causing the material to expand and contract. Modelling this with a Maxwellian viscoelastic response on a spherical nucleus, we show that a hard, icy layer with similar properties to Martian permafrost will experience high stresses: up to tens of MPa, which exceed its material strength (a few MPa), down to depths of centimetres to a metre. The stress distribution with latitude is confirmed qualitatively when taking into account the comet's complex shape but neglecting thermal inertia. Stress is found to be comparable to the material strength everywhere for sufficient thermal inertia ($\gtrsim50$ J m$^{-2}$ K$^{-1}$ s$^{-1/2}$) and ice content ($\gtrsim 45\%$ at the equator). In this case, stresses penetrate to a typical depth of $\sim0.25$ m, consistent with the detection of metre-scale thermal contraction crack polygons all over the comet. Thermal fracturing may be an important erosion process on cometary surfaces which breaks down material and weakens cliffs.

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arXiv2017

Scientific rationale for Uranus and Neptune in situ explorations

The ice giants Uranus and Neptune are the least understood class of planets in our solar system but the most frequently observed type of exoplanets. Presumed to have a small rocky core, a deep interior comprising ~70% heavy elements surrounded by a more dilute outer envelope of H2 and He, Uranus and Neptune are fundamentally different from the better-explored gas giants Jupiter and Saturn. Because of the lack of dedicated exploration missions, our knowledge of the composition and atmospheric processes of these distant worlds is primarily derived from remote sensing from Earth-based observatories and space telescopes. As a result, Uranus's and Neptune's physical and atmospheric properties remain poorly constrained and their roles in the evolution of the Solar System not well understood. Exploration of an ice giant system is therefore a high-priority science objective as these systems (including the magnetosphere, satellites, rings, atmosphere, and interior) challenge our understanding of planetary formation and evolution. Here we describe the main scientific goals to be addressed by a future in situ exploration of an ice giant. An atmospheric entry probe targeting the 10-bar level, about 5 scale heights beneath the tropopause, would yield insight into two broad themes: i) the formation history of the ice giants and, in a broader extent, that of the Solar System, and ii) the processes at play in planetary atmospheres. The probe would descend under parachute to measure composition, structure, and dynamics, with data returned to Earth using a Carrier Relay Spacecraft as a relay station. In addition, possible mission concepts and partnerships are presented, and a strawman ice-giant probe payload is described. An ice-giant atmospheric probe could represent a significant ESA contribution to a future NASA ice-giant flagship mission.

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arXiv2017

The European Far-Infrared Space Roadmap

The European Far-Infrared (FIR) Space Roadmap focuses on fundamental, yet still unresolved, astrophysical questions that can only be answered through a far-infrared space mission and gives an overview of the technology required to answer them. The document discusses topics ranging from Solar System and Planet Formation, Our Galaxy and nearby Galaxies and Distant Galaxies and Galaxy Evolution. The FIR Roadmap was open to comments from the wider astronomical community following a presentation during EWASS 2016.

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arXiv2014

Herschel observations of gas and dust in comet C/2006 W3 (Christensen) at 5 AU from the Sun

We aimed to measure the H2O and dust production rates in C/2006 W3 (Christensen) with the Herschel Space Observatory at a heliocentric distance of ~ 5 AU. We have searched for emission in the H2O and NH3 ground-state rotational transitions at 557 GHz and 572 GHz, simultaneously, with HIFI onboard Herschel on UT 1.5 September 2010. Photometric observations of the dust coma in the 70 and 160 μm channels were acquired with the PACS instrument on UT 26.5 August 2010. A tentative 4-σ H2O line emission feature was found in the spectra obtained with the HIFI wide-band and high-resolution spectrometers, from which we derive a water production rate of $2.0(5) \times 10^{27}$ molec. s$^{-1}$. A 3-σ upper limit for the ammonia production rate of <$1.5 \times 10^{27}$ molec. s$^{-1}$ is obtained taking into account the contribution from all hyperfine components. The blueshift of the water line detected by HIFI suggests preferential emission from the subsolar point. However, it is also possible that water sublimation occurs in small ice-bearing grains that are emitted from an active region on the nucleus surface at a speed of ~ 0.2 km s$^{-1}$. The dust thermal emission was detected in the 70 and 160 μm filters, with a more extended emission in the blue channel. The dust production rates, obtained for a dust size distribution index that explains the fluxes at the photocenters of the PACS images, lie in the range 70-110 kg s$^{-1}$. Scaling the CO production rate measured post-perihelion at 3.20 and 3.32 AU, these values correspond to a dust-to-gas production rate ratio in the range 0.3-0.4. The dust production rates derived in August 2010 are roughly one order of magnitude lower than in September 2009, suggesting that the dust-to-gas production rate ratio remained approximately constant during the period when the activity became increasingly dominated by CO outgassing.

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arXiv2014

Searches for HCl and HF in comets 103P/Hartley 2 and C/2009 P1 (Garradd) with the Herschel space observatory

HCl and HF are expected to be the main reservoirs of fluorine and chlorine wherever hydrogen is predominantly molecular. They are found to be strongly depleted in dense molecular clouds, suggesting freeze-out onto grains in such cold environments. We can then expect that HCl and HF were also the major carriers of Cl and F in the gas and icy phases of the outer solar nebula, and were incorporated into comets. We aimed to measure the HCl and HF abundances in cometary ices as they can provide insights on the halogen chemistry in the early solar nebula. We searched for the J(1-0) lines of HCl and HF at 626 and 1232 GHz, respectively, using the HIFI instrument on board the Herschel Space Observatory. HCl was searched for in comets 103P/Hartley 2 and C/2009 P1 (Garradd), whereas observations of HF were conducted in comet C/2009 P1. In addition, observations of H$_2$O and H$_2^{18}$O lines were performed in C/2009 P1 to measure the H$_2$O production rate. Three lines of CH$_3$OH were serendipitously observed in the HCl receiver setting. HCl is not detected, whereas a marginal (3.6-$σ$) detection of HF is obtained. The upper limits for the HCl abundance relative to water are 0.011% and 0.022%, for 103P and C/2009 P1, respectively, showing that HCl is depleted with respect to the solar Cl/O abundance by a factor more than 6$^{+6}_{-3}$ in 103P, where the error is related to the uncertainty in the chlorine solar abundance. The marginal HF detection obtained in C/2009 P1 corresponds to an HF abundance relative to water of (1.8$\pm$0.5) $\times$ 10$^{-4}$, which is approximately consistent with a solar photospheric F/O abundance. The observed depletion of HCl suggests that HCl was not the main reservoir of chlorine in the regions of the solar nebula where these comets formed. HF was possibly the main fluorine compound in the gas phase of the outer solar nebula.

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