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P. Knüppel

Publications and source records attributed to P. Knüppel.

3 recordsLinked to original sources

Spectroscopy of Wigner crystal polarons in an atomically thin semiconductor

Strongly interacting electrons in two-dimensional systems can spontaneously break translational symmetry, forming a periodic Wigner crystal. Although these crystals have been realized in several platforms, experimental studies of their collective many-body excitations in the absence of a magnetic field remain an outstanding challenge. Here, we access this regime optically by uncovering Wigner crystal polarons: novel light-matter excitations arising from the dressing of excitons by collective excitations of the Wigner crystal. These hybrid quasiparticles manifest as new optical resonances in cryogenic reflectance spectra of a charge-tunable WSe$_2$ monolayer, appearing concurrently with previously identified exciton umklapp transitions. In contrast to the latter, the energies of Wigner crystal polarons are governed not only by the electronic lattice constant but also by their hybridization with attractive exciton-polarons, whose strength is controlled by electronic interactions. These novel many-body excitations provide an optical interface to the spin state of the Wigner crystal, which as we demonstrate, can be controlled both magnetically and optically. Our work establishes layered materials as a unique platform for exploring dynamical impurity dressing by strongly correlated electronic orders.

cond-mat.mes-hall

Spin Reversal of a Quantum Hall Ferromagnet at a Landau Level Crossing

When Landau levels (LLs) become degenerate near the Fermi energy in the quantum Hall regime, interaction effects can drastically modify the electronic ground state. We study the quantum Hall ferromagnet formed in a two-dimensional hole gas around the LL filling factor $ν=1$ in the vicinity of a LL crossing in the heave-hole valence band. Cavity spectroscopy in the strong-coupling regime allows us to optically extract the two-dimensional hole gas' spin polarization. By analyzing this polarization as a function of hole density and magnetic field, we observe a spin flip of the ferromagnet. Furthermore, the depolarization away from $ν=1$ accelerates close to the LL crossing. This is indicative of an increase in the size of Skyrmion excitations as the effective Zeeman energy vanishes at the LL crossing.

cond-mat.str-el

Shubnikov-de Haas oscillations in optical conductivity of monolayer MoSe$_2$

We report polarization-resolved resonant reflection spectroscopy of a charge-tunable atomically-thin valley semiconductor hosting tightly bound excitons coupled to a dilute system of fully spin- and valley-polarized holes in the presence of a strong magnetic field. We find that exciton-hole interactions manifest themselves in hole-density dependent, Shubnikov-de Haas-like oscillations in the energy and line broadening of the excitonic resonances. These oscillations are evidenced to be precisely correlated with the occupation of Landau levels, thus demonstrating that strong interactions between the excitons and Landau-quantized itinerant carriers enable optical investigation of quantum-Hall physics in transition metal dichalcogenides.

cond-mat.mes-hall