arXiv subjects

P. Krüger

Publications and source records attributed to P. Krüger.

At least 19 recordsLinked to original sources

arXiv2025

Quantum magnetic imaging of current density in lithium-ion batteries

The projected rapid growth of battery cell production over the next decade demands advanced diagnostic tools for quality control, ageing prediction, and recycling. Most existing techniques lack the spatial and temporal resolution required to capture internal electrochemical processes non-invasively. Here, we present magnetic imaging of current densities in battery cells, a sensitive quantum-magnetometry method that uses optically pumped magnetometers (OPMs) to perform real-time imaging of internal dynamics in open-circuit configuration. We demonstrate this approach for monitoring relaxation processes in 6000 mA h lithium-ion cells following pulsed discharges across a range of pulse durations and currents as well as states of charge. The measurement results are benchmarked against superconducting-quantum-interference-device (SQUID) magnetometry and validated with three-dimensional finite element simulations. Equivalent circuit models are employed to interpret the relaxation profiles, revealing spatially resolved features and transient magnetic-field signatures that are inaccessible with complementary non-invasive techniques such as electrochemical impedance spectroscopy (EIS). This work establishes OPM-based magnetic imaging of battery current density as a powerful diagnostic tool with potential impact on cell development, manufacturing quality assurance, and second-life assessment.

quant-ph↗

arXiv2024

Photoelectron diffraction of twisted bilayer graphene

Photoelectron diffraction (PED) is a powerful spectroscopic technique that combines elemental resolution with a high sensitivity to the local atomic arrangement at crystal surfaces, thus providing unique fingerprints of selected atomic sites in matter. Stimulated by the rapid innovation in the development of various analysis methods for probing the atomic and electronic structures of van der Waals (vdW) heterostructures of two-dimensional materials, we present a theoretical assessment of the capacity of PED for extracting structural properties such as stacking, twist angles and interlayer distances. We provide a complete description of PED for the benchmark vdW heterostructure bilayer graphene (BLG), by calculating and analyzing the PED of BLG in Bernal and AA-stacking as well as twisted BLG for a wide range of the twist angle.

cond-mat.mtrl-sci↗

arXiv2023

Quantum gas-enabled direct mapping of active current density in percolating networks of nanowires

Electrically percolating nanowire networks are amongst the most promising candidates for next-generation transparent electrodes. Scientific interest in these materials stems from their intrinsic current distribution heterogeneity, leading to phenomena like percolating pathway re-routing and localized self-heating, which can cause irreversible damage. Without an experimental technique to resolve the current distribution, and an underpinning nonlinear percolation model, one relies on empirical rules and safety factors to engineer these materials. We introduce Bose-Einstein microscopy to address the long-standing problem of imaging active current flow in 2D materials. We report on improvement of the performance of this technique, whereby observation of dynamic redistribution of current pathways becomes feasible. We show how this, combined with existing thermal imaging methods, eliminates the need for assumptions between electrical and thermal properties. This will enable testing and modelling individual junction behaviour and hotspot formation. Investigating both reversible and irreversible mechanisms will contribute to the advancement of devices with improved performance and reliability.

physics.app-ph↗

arXiv2021

Signature of spin-resolved quantum point contact in p-type trilayer WSe$_{2}$ van der Waals heterostructure

In this study, the electrostatically induced quantum confinement structure, quantum point contact, has been realized in p-type trilayer tungsten diselenide-based van der Waals heterostructure with modified van der Waals contact method with degenerately doped transition metal dichalcogenide crystals. Clear quantized conductance and pinch-off state through the one-dimensional confinement were observed by dual-gating of split gate electrodes and top gate. Conductance plateaus were observed at step of 0.5 $\times$ 2e$^{2}$/h at zero and high magnetic field in addition to quarter plateaus at a finite bias voltage condition indicating the signature of spin-polarized quantum point contact realization.

cond-mat.mes-hall↗

arXiv2021

Using graphene conductors to enhance the functionality of atom-chips

We show that the performance and functionality of atom-chips can be transformed by using graphene-based van der Waals heterostructures to overcome present limitations on the lifetime of the trapped atom cloud and on its proximity to the chip surface. Our analysis involves Green-function calculations of the thermal (Johnson) noise and Casimir-Polder atom-surface attraction produced by the atom-chip. This enables us to determine the lifetime limitations produced by spin-flip, tunneling and three-body collisional losses. Compared with atom-chips that use thick metallic conductors and substrates, atom-chip structures based on two-dimensional materials reduce the minimum attainable atom-surface separation to a few 100 nm and increase the lifetimes of the trapped atom clouds by orders of magnitude so that they are limited only by the quality of the background vacuum. We predict that atom-chips with two-dimensional conductors will also reduce spatial fluctuations in the trapping potential originating from imperfections in the conductor patterns. These advantages will enhance the performance of atom-chips for quantum sensing applications and for fundamental studies of complex quantum systems.

quant-ph↗

arXiv2019

Additively manufactured ultra-high vacuum chamber below $10^{-10}$ mbar

Metal-based additive manufacturing (AM) represents a paradigm change in engineering and production methods across multiple industries and sectors. AM methods enable mass reduction and performance optimisation well beyond that achievable via conventional manufacturing, thereby impacting significantly on aerospace and space technologies. Technologies relying on high and ultra-high vacuum (UHV), such as x-ray photo-electron spectroscopy, photo-sensors, cameras and cryostats, could also benefit greatly from AM. Despite recent advances in AM processing of metals, additively manufactured UHV chambers have so far not been achieved. Reducing the mass of UHV equipment is particularly critical for the development of portable cold atom systems, which are expected to underpin the next generation of sensing and timekeeping technologies and to allow novel space-based sensors for fundamental research. We demonstrate here an additively manufactured UHV chamber reaching a pressure below $10^{-10}$ mbar, enabling a cloud of cold $^{85}$Rb atoms to be trapped - the starting point for many precision timekeeping and sensing devices. The chamber is manufactured from aluminium alloy AlSi10Mg by laser powder bed fusion and has a mass of less than a third of a commercially-available equivalent. Outgassing analysis based on mass spectrometry was performed and it was demonstrated that even without active pumping the system remains in the $10^{-9}$ mbar regime for up to 48 hours.

quant-ph↗

arXiv2017

3D-printed components for quantum devices

Recent advances in the preparation, control and measurement of atomic gases have led to new insights into the quantum world and unprecedented metrological sensitivities, e.g. in measuring gravitational forces and magnetic fields. The full potential of applying such capabilities to areas as diverse as biomedical imaging, non-invasive underground mapping, and GPS-free navigation can only be realised with the scalable production of efficient, robust and portable devices. Here we introduce additive manufacturing as a production technique of quantum device components with unrivalled design freedom, providing a step change in efficiency, compactness and facilitating systems integration. As a demonstrator we present a compact ultracold atom source using less than ten milliwatts power to produce large samples of cold rubidium gases in an ultrahigh vacuum environment. This disruptive technology opens the door to drastically improved integrated structures, which will further reduce power consumption, size and assembly complexity in scalable series manufacture of bespoke quantum devices.

quant-ph↗

arXiv2015

Superfluid flow above the critical velocity

Superfluidity and superconductivity have been studied widely since the last century in many different contexts ranging from nuclear matter to atomic quantum gases. The rigidity of these systems with respect to external perturbations results in frictionless motion for superfluids and resistance-free electric current in superconductors. This peculiar behaviour is lost when external perturbations overcome a critical threshold, i.e. above a critical magnetic field or a critical current for superconductors. In superfluids, such as liquid helium or ultracold gases, the corresponding quantities are critical rotation rate and critical velocity, respectively. Enhancing the critical values is of great fundamental and practical value. Here we demonstrate that superfluidity can be achieved for flow above the critical velocity through quantum interference induced resonances. This has far reaching consequences for the fundamental understanding of superfluidity and superconductivity and opens up new application possibilities in quantum metrology, e.g. in rotation sensing.

cond-mat.quant-gas↗

arXiv2015

Scattering of matter-waves in spatially inhomogeneous environments

We study scattering of quasi one-dimensional matter-waves at an interface of two spatial domains, one with repulsive and one with attractive interatomic interactions. It is shown that the incidence of a Gaussian wavepacket from the repulsive to the attractive region gives rise to generation of a soliton train. More specifically, the number of emergent solitons can be controlled e.g. by the variation of the amplitude or the width of the incoming wavepacket. Furthermore, we study the reflectivity of a soliton incident from the attractive region to the repulsive one. We find the reflection coefficient numerically and employ analytical methods, that treat the soliton as a particle (for moderate and large amplitudes) or a quasi-linear wavepacket (for small amplitudes), to determine the critical soliton momentum - as function of the soliton amplitude - for which total reflection is observed.

cond-mat.quant-gas↗

arXiv2015

Data quality monitoring in the presence of aerosols and other adverse atmospheric conditions with H.E.S.S

Cherenkov telescope experiments, such as H.E.S.S., have been very successful in astronomical observations in the very-high-energy (VHE; E $>$ 100 GeV) regime. As an integral part of the detector, such experiments use Earth's atmosphere as a calorimeter. For the calibration and energy determination, a standard model atmosphere is assumed. Deviations of the real atmosphere from the model may therefore lead to an energy misreconstruction of primary gamma rays. To guarantee satisfactory data quality with respect to difficult atmospheric conditions, several atmospheric data quality criteria are implemented in the H.E.S.S. software. These quantities are sensitive to clouds and aerosols. Here, the Cherenkov transparency coefficient will be presented. It is a new monitoring quantity that is able to measure long-term changes in the atmospheric transparency. The Cherenkov transparency coefficient derives exclusively from Cherenkov data and is quite hardware-independent. Furthermore, its positive correlation with independent satellite measurements, performed by the Multi-angle Imaging SpectroRadiometer (MISR), will be presented.

astro-ph.IM↗

arXiv2014

AtmoHEAD 2013 workshop / Atmospheric Monitoring for High-Energy Astroparticle Detectors

A 3-day international workshop on atmospheric monitoring and calibration for high-energy astroparticle detectors, with a view towards next-generation facilities. The atmosphere is an integral component of many high-energy astroparticle detectors. Imaging atmospheric Cherenkov telescopes and cosmic-ray extensive air shower detectors are the two instruments driving the rapidly evolving fields of very-high- and ultra-high-energy astrophysics. In these instruments, the atmosphere is used as a giant calorimeter where cosmic rays and gamma rays deposit their energy and initiate EASs; it is also the medium through which the resulting Cherenkov light propagates. Uncertainties in real-time atmospheric conditions and in the fixed atmospheric models typically dominate all other systematic errors. With the improved sensitivity of upgraded IACTs such as H.E.S.S.-II and MAGIC-II and future facilities like the Cherenkov Telescope Array (CTA) and JEM-EUSO, statistical uncertainties are expected to be significantly reduced, leaving the atmosphere as the limiting factor in the determination of astroparticle spectra. Varying weather conditions necessitate the development of suitable atmospheric monitoring to be integrated in the overall instrument calibration, including Monte Carlo simulations. With expertise distributed across multiple collaborations and scientific domains, an interdisciplinary workshop is being convened to advance progress on this critical and timely topic.

astro-ph.IM↗

arXiv2013

Impact of aerosols and adverse atmospheric conditions on the data quality for spectral analysis of the H.E.S.S. telescopes

The Earth's atmosphere is an integral part of the detector in ground-based imaging atmospheric Cherenkov telescope (IACT) experiments and has to be taken into account in the calibration. Atmospheric and hardware-related deviations from simulated conditions can result in the mis-reconstruction of primary particle energies and therefore of source spectra. During the eight years of observations with the High Energy Stereoscopic System (H.E.S.S.) in Namibia, the overall yield in Cherenkov photons has varied strongly with time due to gradual hardware aging, together with adjustments of the hardware components, and natural, as well as anthropogenic, variations of the atmospheric transparency. Here we present robust data selection criteria that minimize these effects over the full data set of the H.E.S.S. experiment and introduce the Cherenkov transparency coefficient as a new atmospheric monitoring quantity. The influence of atmospheric transparency, as quantified by this coefficient, on energy reconstruction and spectral parameters is examined and its correlation with the aerosol optical depth (AOD) of independent MISR satellite measurements and local measurements of atmospheric clarity is investigated.

astro-ph.IM↗

arXiv2013

First-principles calculations of spin and angle-resolved resonant photoemission spectra of Cr(110) surfaces at the 2$p$ - 3$d$ resonance

A first principles approach for spin and angle resolved resonant photoemission is developed within multiple scattering theory and applied to a Cr(110) surface at the 2$p$-3$d$ resonance. The resonant photocurrent from this non ferromagnetic system is found to be strongly spin polarized by circularly polarized light, in agreement with experiments on antiferromagnetic and magnetically disordered systems. By comparing the antiferromagnetic and Pauli-paramagnetic phases of Cr, we explicitly show that the spin polarization of the photocurrent is independent of the existence of local magnetic moments, solving a long-standing debate on the origin of such polarization. New spin polarization effects are predicted for the paramagnetic phase even with unpolarized light, opening new directions for full mapping of spin interactions in macroscopically non magnetic or nanostructured systems.

cond-mat.str-el↗

arXiv2011

Atom chips with two-dimensional electron gases: theory of near surface trapping and ultracold-atom microscopy of quantum electronic systems

We show that current in a two-dimensional electron gas (2DEG) can trap ultracold atoms $<1 μ$m away with orders of magnitude less spatial noise than a metal trapping wire. This enables the creation of hybrid systems, which integrate ultracold atoms with quantum electronic devices to give extreme sensitivity and control: for example, activating a single quantized conductance channel in the 2DEG can split a Bose-Einstein condensate (BEC) for atom interferometry. In turn, the BEC offers unique structural and functional imaging of quantum devices and transport in heterostructures and graphene.

cond-mat.quant-gas↗

arXiv2010

Weakly interacting Bose gas in the one-dimensional limit

We prepare a chemically and thermally one-dimensional (1d) quantum degenerate Bose gas in a single microtrap. We introduce a new interferometric method to distinguish the quasicondensate fraction of the gas from the thermal cloud at finite temperature. We reach temperatures down to $kT\approx 0.5\hbarω_\perp$ (transverse oscillator eigenfrequency $ω_\perp$) when collisional thermalization slows down as expected in 1d. At the lowest temperatures the transverse momentum distribution exhibits a residual dependence on the line density $n_{1d}$, characteristic for 1d systems. For very low densities the approach to the transverse single particle ground state is linear in $n_{1d}$.

cond-mat.quant-gas↗

arXiv2009

Zone-plate focusing of Bose-Einstein condensates for atom optics and erasable high-speed lithography of quantum electronic components

We show that Fresnel zone plates, fabricated in a solid surface, can sharply focus atomic Bose-Einstein condensates that quantum reflect from the surface or pass through the etched holes. The focusing process compresses the condensate by orders of magnitude despite inter-atomic repulsion. Crucially, the focusing dynamics are insensitive to quantum fluctuations of the atom cloud and largely preserve the condensates' coherence, suggesting applications in passive atom-optical elements, for example zone plate lenses that focus atomic matter waves and light at the same point to strengthen their interaction. We explore transmission zone-plate focusing of alkali atoms as a route to erasable and scalable lithography of quantum electronic components in two-dimensional electron gases embedded in semiconductor nanostructures. To do this, we calculate the density profile of a two-dimensional electron gas immediately below a patch of alkali atoms deposited on the surface of the nanostructure by zone-plate focusing. Our results reveal that surface-induced polarization of only a few thousand adsorbed atoms can locally deplete the electron gas. We show that, as a result, the focused deposition of alkali atoms by existing zone plates can create quantum electronic components on the 50 nm scale, comparable to that attainable by ion beam implantation but with minimal damage to either the nanostructure or electron gas.

cond-mat.quant-gas↗

arXiv2009

An optical lattice on an atom chip

Optical dipole traps and atom chips are two very powerful tools for the quantum manipulation of neutral atoms. We demonstrate that both methods can be combined by creating an optical lattice potential on an atom chip. A red-detuned laser beam is retro-reflected using the atom chip surface as a high-quality mirror, generating a vertical array of purely optical oblate traps. We load thermal atoms from the chip into the lattice and observe cooling into the two-dimensional regime where the thermal energy is smaller than a quantum of transverse excitation. Using a chip-generated Bose-Einstein condensate, we demonstrate coherent Bloch oscillations in the lattice.

physics.atom-ph↗

arXiv2006

Adiabatic radio frequency potentials for the coherent manipulation of matter waves

Adiabatic dressed state potentials are created when magnetic sub-states of trapped atoms are coupled by a radio frequency field. We discuss their theoretical foundations and point out fundamental advantages over potentials purely based on static fields. The enhanced flexibility enables one to implement numerous novel configurations, including double wells, Mach-Zehnder and Sagnac interferometers which even allows for internal state-dependent atom manipulation. These can be realized using simple and highly integrated wire geometries on atom chips.

physics.atom-ph↗