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P. Krogstrup

Publications and source records attributed to P. Krogstrup.

At least 19 recordsLinked to original sources

Spin-split superconductivity in spin-orbit coupled hybrid nanowires with ferromagnetic barriers

We report transport studies of hybrid Josephson junctions based on semiconducting InAs nanowires with fully overlapping epitaxial ferromagnetic insulator EuS and superconducting Al partial shells. Current-biased measurements reveal a hysteretic superconducting window with a sizable supercurrent near the coercive field of the ferromagnetic insulator, accompanied by multiple Andreev reflections. Tunneling spectroscopy shows a superconducting gap characterized by three peaks, which we attribute to tunneling between exchange-split superconductors. A theoretical model reproduces the observed features and indicates that spin mixing, driven by sizable spin-orbit coupling, is essential to their formation. Our results demonstrate proximity-induced superconductivity through a ferromagnetic insulator and establish a new platform for exploring spin-triplet pairing.

cond-mat.mes-hall

Ground state phase diagram and "parity flipping'' microwave transitions in a gate-tunable Josephson Junction

We probed a gate-tunable InAs nanowire Josephson weak link by coupling it to a microwave resonator. Tracking the resonator frequency shift when the weak link is close to pinch-off, we observe that the ground state of the latter alternates between a singlet and a doublet when varying either the gate voltage or the superconducting phase difference across it. The corresponding microwave absorption spectra display lines that approach zero energy close to the singlet-doublet boundaries, suggesting parity flipping transitions, which are in principle forbidden in microwave spectroscopy and expected to arise only in tunnel spectroscopy. We tentatively interpret them by means of an ancillary state isolated in the junction acting as a reservoir for individual electrons.

cond-mat.mes-hall

Supercurrent transport through 1$e$-periodic full-shell Coulomb islands

We experimentally investigate supercurrent through Coulomb islands, where island and leads are fabricated from semiconducting nanowires with fully surrounding superconducting shells. Applying flux along the wire yields a series of destructive Little-Parks lobes with reentrant supercurrent. We find Coulomb blockade with 2$e$ peak spacing in the zeroth lobe and 1$e$ average spacing, with regions of significant even-odd modulation, in the first lobe. Evolution of Coulomb-peak amplitude through the first lobe is consistent with a theoretical model of supercurrent carried predominantly by zero-energy states in the leads and the island.

cond-mat.mes-hall

Integrated bioelectronic proton-gated logic elements utilizing nanoscale patterned Nafion

A central endeavour in bioelectronics is the development of logic elements to transduce and process ionic to electronic signals. Motivated by this challenge, we report fully monolithic, nanoscale logic elements featuring n- and p-type nanowires as electronic channels that are proton-gated by electron-beam patterned Nafion. We demonstrate inverter circuits with state-of-the-art ion-to-electron transduction performance giving DC gain exceeding 5 and frequency response up to 2 kHz. A key innovation facilitating the logic integration is a new electron-beam process for patterning Nafion with linewidths down to 125 nm. This process delivers feature sizes compatible with low voltage, fast switching elements. This expands the scope for Nafion as a versatile patternable high-proton-conductivity element for bioelectronics and other applications requiring nanoengineered protonic membranes and electrodes.

physics.app-ph

Microwave spectroscopy of interacting Andreev spins

Andreev bound states are fermionic states localized in weak links between superconductors which can be occupied with spinful quasiparticles. Microwave experiments using superconducting circuits with InAs/Al nanowire Josephson junctions have recently enabled probing and coherent manipulation of Andreev states but have remained limited to zero or small fields. Here we use a flux-tunable superconducting circuit in external magnetic fields up to 1T to perform spectroscopy of spin-polarized Andreev states up to ~250 mT, beyond which the spectrum becomes gapless. We identify singlet and triplet states of two quasiparticles occupying different Andreev states through their dispersion in magnetic field. These states are split by exchange interaction and couple via spin-orbit coupling, analogously to two-electron states in quantum dots. We also show that the magnetic field allows to drive a direct spin-flip transition of a single quasiparticle trapped in the junction. Finally, we measure a gate- and field-dependent anomalous phase shift of the Andreev spectrum, of magnitude up to approximately $0.7\pi$. Our observations demonstrate new ways to manipulate Andreev states in a magnetic field and reveal spin-polarized triplet states that carry supercurrent.

cond-mat.mes-hall

Supercurrent reversal in ferromagnetic hybrid nanowire Josephson junctions

We report supercurrent transport measurements in hybrid Josephson junctions comprised of semiconducting InAs nanowires with epitaxial ferromagnetic insulator EuS and superconducting Al coatings. The wires display a hysteretic superconducting window close to the coercivity, away from zero external magnetic field. Using a multi-interferometer setup, we measure the current-phase relation of multiple magnetic junctions and find an abrupt switch between $\pi$ and 0 phases within the superconducting window. We attribute the 0-$\pi$ transition to the discrete flipping of the EuS domains and provide a qualitative theory showing that a sizable exchange field can polarize the junction and lead to the supercurrent reversal. Both $0$ and $\pi$ phases can be realized at zero external field by demagnetizing the wire.

cond-mat.supr-con

Electrostatic control of quasiparticle poisoning in a hybrid semiconductor-superconductor island

The performance of superconducting devices is often degraded by the uncontrolled appearance and disappearance of quasiparticles, a process known as poisoning. We demonstrate electrostatic control of quasiparticle poisoning in the form of single-charge tunneling across a fixed barrier onto a Coulomb island in an InAs/Al hybrid nanowire. High-bandwidth charge sensing was used to monitor charge occupancy of the island across Coulomb blockade peaks, where tunneling rates were maximal, and Coulomb valleys, where tunneling was absent. Electrostatic gates changed on-peak tunneling rates by two orders of magnitude for a barrier with fixed normal-state resistance, which we attribute to gate dependence of the size and softness of the induced superconducting gap on the island, corroborated by separate density-of-states measurements. Temperature and magnetic field dependence of tunneling rates are also investigated.

cond-mat.mes-hall

Parity switching in a full-shell superconductor-semiconductor nanowire qubit

The rate of charge-parity switching in a full-shell superconductor-semiconductor nanowire qubit is measured by directly monitoring the dispersive shift of a readout resonator. At zero magnetic field, the measured switching time scale $T_P$ is on the order of 100 ms. Two-tone spectroscopy data post-selected on charge-parity is demonstrated. With increasing temperature or magnetic field, TP is at first constant, then exponentially suppressed, consistent with a model that includes both non-equilibrium and thermally activated quasiparticles. As TP is suppressed, qubit lifetime T1 also decreases. The long $T_P\sim 0.1$ s at zero field is promising for future development of qubits based on hybrid nanowires.

cond-mat.mes-hall

Signatures of interactions in the Andreev spectrum of nanowire Josephson junctions

We performed microwave spectroscopy of an InAs nanowire between superconducting contacts implementing a finite-length, multi-channel Josephson weak link. Certain features in the spectra, such as the splitting by spin-orbit interactions of the transition lines among Andreev states, have been already understood in terms of non-interacting models. However, we identify here additional transitions, which evidence the presence of Coulomb interactions. By combining experimental measurements and model calculations, we reach a qualitative understanding of these very rich Andreev spectra.

cond-mat.mes-hall

Microwave susceptibility observation of interacting many-body Andreev states

Electrostatic charging affects the many-body spectrum of Andreev states, yet its influence on their microwave properties has not been elucidated. We developed a circuit quantum electrodynamics probe that, in addition to transition spectroscopy, measures the microwave susceptibility of different states of a semiconductor nanowire weak link with a single dominant (spin-degenerate) Andreev level. We found that the microwave susceptibility does not exhibit a particle-hole symmetry, which we qualitatively explain as an influence of Coulomb interaction. Moreover, our state-selective measurement reveals a large, $\pi$-phase shifted contribution to the response common to all many-body states which can be interpreted as arising from a phase-dependent continuum in the superconducting density of states.

cond-mat.mes-hall

Dynamical polarization of the fermion parity in a nanowire Josephson junction

Josephson junctions in InAs nanowires proximitized with an Al shell can host gate-tunable Andreev bound states. Depending on the bound state occupation, the fermion parity of the junction can be even or odd. Coherent control of Andreev bound states has recently been achieved within each parity sector, but it is impeded by incoherent parity switches due to excess quasiparticles in the superconducting environment. Here, we show that we can polarize the fermion parity dynamically using microwave pulses by embedding the junction in a superconducting LC resonator. We demonstrate polarization up to 94% $\pm$ 1% (89% $\pm$ 1%) for the even (odd) parity as verified by single shot parity-readout. Finally, we apply this scheme to probe the flux-dependent transition spectrum of the even or odd parity sector selectively, without any post-processing or heralding.

cond-mat.mes-hall

Evidence for spin-polarized bound states in semiconductor-superconductor-ferromagnetic insulator islands

We report Coulomb blockade transport studies of semiconducting InAs nanowires grown with epitaxial superconducting Al and ferromagnetic insulator EuS on overlapping facets. Comparing experiment to a theoretical model, we associate cotunneling features in even-odd bias spectra with spin-polarized Andreev levels. Results are consistent with zero-field spin splitting exceeding the induced superconducting gap. Energies of subgap states are tunable on either side of zero via electrostatic gates.

cond-mat.mes-hall

Coherent manipulation of an Andreev spin qubit

Two promising architectures for solid-state quantum information processing are electron spins in semiconductor quantum dots and the collective electromagnetic modes of superconducting circuits. In some aspects, these two platforms are dual to one another: superconducting qubits are more easily coupled but are relatively large among quantum devices $(\sim\mathrm{mm})$, while electrostatically-confined electron spins are spatially compact ($\sim \mathrm{\mu m}$) but more complex to link. Here we combine beneficial aspects of both platforms in the Andreev spin qubit: the spin degree of freedom of an electronic quasiparticle trapped in the supercurrent-carrying Andreev levels of a Josephson semiconductor nanowire. We demonstrate coherent spin manipulation by combining single-shot circuit-QED readout and spin-flipping Raman transitions, finding a spin-flip time $T_S = 17~\mathrm{\mu s}$ and a spin coherence time $T_{2E}=52~\mathrm{ns}$. These results herald a new spin qubit with supercurrent-based circuit-QED integration and further our understanding and control of Andreev levels -- the parent states of Majorana zero modes -- in semiconductor-superconductor heterostructures.

cond-mat.mes-hall

Magnetic-Field-Compatible Superconducting Transmon Qubit

We present a hybrid semiconductor-based superconducting qubit device which remains coherent at magnetic fields up to 1 T. The qubit transition frequency exhibits periodic oscillations with magnetic field, consistent with interference effects due to the magnetic flux threading the cross section of the proximitized semiconductor nanowire junction. As induced superconductivity revives, additional coherent modes emerge at high magnetic fields, which we attribute to the interaction of the qubit and low-energy Andreev states.

cond-mat.mes-hall

Electronic properties of InAs/EuS/Al hybrid nanowires

We study the electronic properties of InAs/EuS/Al heterostructures as explored in a recent experiment [S. Vaitiekenas \emph{et al.}, Nat. Phys. (2020)], combining both spectroscopic results and microscopic device simulations. In particular, we use angle-resolved photoemission spectroscopy to investigate the band bending at the InAs/EuS interface. The resulting band offset value serves as an essential input to subsequent microscopic device simulations, allowing us to map the electronic wave function distribution. We conclude that the magnetic proximity effects at the Al/EuS as well as the InAs/EuS interfaces are both essential to achieve topological superconductivity at zero applied magnetic field. Mapping the topological phase diagram as a function of gate voltages and proximity-induced exchange couplings, we show that the ferromagnetic hybrid nanowire with overlapping Al and EuS layers can become a topological superconductor within realistic parameter regimes, and that the topological phase can be optimized by external gating. Our work highlights the need for a combined experimental and theoretical effort for faithful device simulation.

cond-mat.mes-hall

Andreev Modes from Phase Winding in a Full-shell Nanowire-based Transmon

We investigate transmon qubits made from semiconductor nanowires with a fully surrounding superconducting shell. In the regime of reentrant superconductivity associated with the destructive Little-Parks effect, numerous coherent transitions are observed in the first reentrant lobe, where the shell carries 2{\pi} winding of superconducting phase, and are absent in the zeroth lobe. As junction density was increased by gate voltage, qubit coherence was suppressed then lost in the first lobe. These observations and numerical simulations highlight the role of winding-induced Andreev states in the junction.

cond-mat.mes-hall

Quantum-Dot Parity Effects in Trivial and Topological Josephson Junctions

An odd-occupied quantum dot in a Josephson junction can flip transmission phase, creating a {\pi}-junction. When the junction couples topological superconductors, no phase flip is expected. We investigate this and related effects in a full-shell hybrid interferometer, using gate voltage to control dot-junction parity and axial magnetic flux to control the transition from trivial to topological superconductivity. Enhanced zero-bias conductance and critical current for odd parity in the topological phase reflects hybridization of the confined spin with zero-energy modes in the leads.

cond-mat.mes-hall

A Parity-Protected Superconductor-Semiconductor Qubit

Coherence of superconducting qubits can be improved by implementing designs that protect the parity of Cooper pairs on superconducting islands. Here, we introduce a parity-protected qubit based on voltage-controlled semiconductor nanowire Josephson junctions, taking advantage of the higher harmonic content in the energy-phase relation of few-channel junctions. A symmetric interferometer formed by two such junctions, gate-tuned into balance and frustrated by a half-quantum of applied flux, yields a cos(2{\phi}) Josephson element, reflecting coherent transport of pairs of Cooper pairs. We demonstrate that relaxation of the qubit can be suppressed tenfold by tuning into the protected regime.

cond-mat.mes-hall