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P. Lalanne

Publications and source records attributed to P. Lalanne.

At least 19 recordsLinked to original sources

A dressed polarizability framework for interface-coupled meta-atoms and large-scale metasurfaces

The modeling of large collections of interacting meta-atoms remains a central challenge in photonics because it requires the simultaneous treatment of complex scatterer geometries, multiple scattering, and heterogeneous environments. Here, we introduce the dressed Global Polarizability Matrix (dGPM), a reduced-order electromagnetic framework in which complex meta-atoms are represented by compact scattering operators that explicitly incorporate the influence of nearby interfaces. The dGPM accurately reconstructs near- and far-field electromagnetic responses for interface-coupled structures, including geometries beyond the practical applicability of conventional T-matrix approaches. The framework naturally combines interface-coupled and free-space scatterers within a unified multiple-scattering formalism and enables simulations of large ordered and disordered metasurfaces. More broadly, the dGPM extends operator-based electromagnetic modeling to heterogeneous photonic environments while preserving a compact scatterer-based representation, providing an efficient framework for the simulation and design of large-scale photonic systems.

physics.optics

Modal analysis of electromagnetic resonators: MAN software expansion to 2D materials and coupled systems

This work presents an updated version of the previously released freeware MAN (Modal Analysis of Nanoresonators) [Comput Phys Commun 284, 108627 (2023)], a software package designed to efficiently compute and normalize quasinormal modes (QNMs) and to use them for the analysis of the optical response of electromagnetic resonators. This release substantially extends the capabilities of the original software through three major developments. First, it introduces dedicated models and numerical tools for resonators incorporating two-dimensional materials, including graphene, using a surface-conductivity formulation. Second, it implements a coupled-QNM formalism that computes the complex coupling coefficients between resonator modes directly from the QNMs of the individual resonators. Unlike conventional coupled-mode theory, where these coefficients are often introduced phenomenologically or determined by fitting, MAN evaluates them rigorously from first principles. Third, it provides post-processing tools that determine the Fano parameters governing extinction spectra directly from the computed QNM field distributions. Together, these advances broaden the range of nanophotonic systems accessible to MAN while providing new tools for the quantitative interpretation of complex resonant phenomena.

physics.optics

Disordered Optical Metasurfaces: Basics, Properties, and Applications

Optical metasurfaces are conventionally viewed as organized flat arrays of photonic or plasmonic nanoresonators, also called metaatoms. These metasurfaces are typically highly ordered and fabricated with precision using expensive tools. However, the inherent imperfections in large-scale nanophotonic devices, along with recent advances in bottom-up nanofabrication techniques and design strategies, have highlighted the potential benefits of incorporating disorder to achieve specific optical functionalities. This review offers an overview of the key theoretical, numerical, and experimental aspects related to the exploration of disordered optical metasurfaces. It introduces fundamental concepts of light scattering by disordered metasurfaces and outlines theoretical and numerical methodologies for analyzing their optical behavior. Various fabrication techniques are discussed, highlighting the types of disorder they deliver and their achievable precision level. The review also explores critical applications of disordered optical metasurfaces, such as light manipulation in thin film materials and the design of structural colors and visual appearances. Finally, the article offers perspectives on the burgeoning future research in this field. Disordered optical metasurfaces offer a promising alternative to their ordered counterparts, often delivering unique functionalities or enhanced performance. They present a particularly exciting opportunity in applications demanding large-scale implementation, such as sustainable renewable energy systems, as well as aesthetically vibrant coatings for luxury goods and architectural designs.

physics.optics

Minireview on Disordered Optical Metasurfaces

The use of coherent wave phenomena to enhance device performance is a cornerstone of modern optics. In juxtaposition to (locally) periodic metasurfaces, their disordered counterparts exhibit an interplay of destructive and constructive interferences occurring at the same spatial and spectral frequencies. This attribute provides disordered metasurfaces with a remarkable degree of flexibility, setting them apart from the constraints of periodic arrangements. Hereafter, we provide a concise overview of the cutting-edge developments and offer insights into the forthcoming research in this dynamic field.

physics.optics

Tailoring iridescent visual appearance with disordered resonant metasurfaces

The nanostructures of natural species offer beautiful visual appearances with saturated and iridescent colors and the question arises whether we can reproduce or even create new appearances with man-made metasurfaces. However, harnessing the specular and diffuse light scattered by disordered metasurfaces to create attractive and prescribed visual effects is currently inaccessible. Here, we present an interpretive, intuitive and accurate modal-based tool that unveils the main physical mechanisms and features defining the appearance of colloidal disordered monolayers of resonant meta-atoms deposited on a reflective substrate. The model shows that the combination of plasmonic and Fabry-Perot resonances offers uncommon iridescent visual appearances, differing from those classically observed with natural nanostructures or thin-film interferences. We highlight an unusual visual effect exhibiting only two distinct colors and theoretically investigate its origin. The approach can be useful in the design of visual appearance with easy-to-make and universal building blocks having a large resilience to fabrication imperfections, and potential for innovative coatings and fine-art applications.

physics.optics

Modal analysis of electromagnetic resonators: user guide for the MAN program

All electromagnetic systems, in particular resonators or antennas, have resonances with finite lifetimes. The associated eigenstates, also called quasinormal modes, are essentially non-Hermitian and determine the optical responses of the system. We introduce MAN (Modal Analysis of Nanoresonators), a software with many open scripts, which computes and normalizes the quasinormal modes of virtually any electromagnetic resonator, be it composed of dispersive, anisotropic, or non-reciprocal materials. MAN reconstructs the scattered field in the basis formed by the quasinormal modes of the resonator and provides a transparent interpretation of the physics. The software is implemented in MATLAB and has been developed over the past ten years. MAN features many toolboxes that illustrate how to use the software for various emblematic computations in low and high frequency regimes. A specific effort has been devoted to interface the solver with the finite-element software COMSOL Multiphysics. However, MAN can also be used with other frequency-domain numerical solvers. This article introduces the program, summarizes the relevant theoretical background. MAN includes a comprehensive set of classical models and toolboxes that can be downloaded from the web.

physics.comp-ph

Normalization, orthogonality and completeness of quasinormal modes of open systems: the case of electromagnetism

The scattering of electromagnetic waves by resonant systems is determined by the excitation of quasinormal modes (QNMs), i.e., the eigenmodes of the system. This Review addresses three fundamental concepts in relation with the representation of the scattered field as a superposition of the excited QNMs: normalization, orthogonality, and completeness. Orthogonality and normalization enable a straightforward assessment of the QNM excitation strength for any incident wave. Completeness guaranties that the scattered field can be faithfully expanded into the QNM basis. These concepts are non-trivial for non-conservative (non-Hermitian) systems and have driven many theoretical developments since initial studies in the 70's. Yet, owing to recent achievements, they are not easily grasped from the extensive and scattered literature, especially for newcomers in the field. After recalling fundamental results obtained in early studies on the completeness of the QNM basis for simple resonant systems, we review recent achievements and debates on the normalization, clarify under which circumstances the QNM basis is complete, and highlight the concept of QNM regularization with complex coordinate transform.

quant-ph

Mapping Complex Mode Volumes with Cavity Perturbation Theory

Microcavities and nanoresonators are characterized by their quality factors Q and mode volumes V. While Q is unambiguously defined, there are still questions on V and in particular on its complex-valued character, whose imaginary part is linked to the non-Hermitian nature of open systems. Helped by cavity perturbation theory and near field experimental data, we clarify the physics captured by the imaginary part of V and show how a mapping of the spatial distribution of both the real and imaginary parts can be directly inferred from perturbation measurements. This result shows that the mathematically abstract complex mode volume in fact is directly observable.

physics.optics

Quasinormal mode solvers for resonators with dispersive materials

Optical resonators are widely used in modern photonics. Their spectral response and temporal dynamics are fundamentally driven by their natural resonances, the so-called quasinormal modes (QNMs), with complex frequencies. For optical resonators made of dispersive materials, the QNM computation requires solving a nonlinear eigenvalue problem. This rises a difficulty that is only scarcely documented in the literature. We review our recent efforts for implementing efficient and accurate QNM-solvers for computing and normalizing the QNMs of micro- and nano-resonators made of highly-dispersive materials. We benchmark several methods for three geometries, a two-dimensional plasmonic crystal, a two-dimensional metal grating, and a three-dimensional nanopatch antenna on a metal substrate, in the perspective to elaborate standards for the computation of resonance modes.

physics.comp-ph

Anomalous light absorption around subwavelength apertures in metal films

In this work, we study the heat dissipated at metal surfaces by the electromagnetic field scattered by isolated subwavelength apertures in metal screens. In contrast to our common belief that the intensity of waves created by local sources should decrease with the distance from the sources, we reveal that the dissipated heat at the surface remains constant over a broad spatial interval of a few tens of wavelengths. This behavior which occurs for noble metals at near infrared wavelengths is observed with nonintrusive thermoreflectance measurements and is analyzed with an analytical model which underlines the intricate role played by quasi-cylindrical waves in the phenomenon. Additionally, computational results reveal that the absorption plateau is an intrinsic property that occurs for a large variety of topologies, irrespective of aperture shapes.

physics.optics

Broadband and efficient diffraction

Surface topography dictates the deterministic functionality of diffraction by a surface. In order to maximize the efficiency with which a diffractive optical component, such as a grating or a diffractive lens, directs light into a chosen order of diffraction, it is necessary that it be "blazed". The efficiency of most diffractive optical components reported so far varies with the wavelength, and blazing is achieved only at a specific nominal energy, the blaze wavelength. The existence of spurious light in undesirable orders represents a severe limitation that prevents using diffractive components in broadband systems. Here we experimentally demonstrate that broadband blazing over almost one octave can be achieved by combining advanced optical design strategies and artificial dielectric materials that offer dispersion chromatism much stronger than those of conventional bulk materials. The possibility of maintaining an efficient funneling of the energy into a specific order over a broad spectral range may empower advanced research to achieve greater control over the propagation of light, leading to more compact, efficient and versatile optical components.

physics.optics

Theory of the Spontaneous Emission in Photonic and Plasmonic Nanoresonators

We provide a self-consistent electromagnetic theory of the coupling between dipole emitters and dissipative nanoresonators. The theory that relies on the concept of quasi-normal modes with complex frequencies provides an accurate closed-form expression for the electromagnetic local density of states (LDOS) of any photonic or plasmonic resonator with strong radiation leakage, absorption and material dispersion. It represents a powerful tool to calculate and conceptualize the electromagnetic response of systems that are governed by a small number of resonance modes. We use the formalism to revisit Purcell's factor. The new formula substantially differs from the usual one; in particular, it predicts that a spectral detuning between the emitter and the resonance does not necessarily result in a Lorentzian response in the presence of dissipation. Comparisons with fully-vectorial numerical calculations for plasmonic nanoresonators made of gold nanorods evidence the high accuracy of the predictions achieved by our semi-analytical treatment.

cond-mat.mes-hall

Theory of fishnet negative-index optical metamaterials

We theoretically study fishnet metamaterials at optical frequencies. In contrast to earlier works, we provide a microscopic description by tracking the transversal and longitudinal flows of energy through the fishnet mesh composed of intersecting subwavelength plasmonic waveguides. The analysis is supported by a semi-analytical model based on surface-plasmon coupled-mode equations, which provides accurate formulas for the fishnet refractive index, including the real-negative and imaginary parts. The model simply explains how the surface plasmons couple at the waveguide intersections and it shines new light on the fishnet negative-index paradigm at optical frequencies. Extension of the theory for loss-compensated metamaterials with gain media is also presented.

physics.optics

Decomposing the scattered field of two-dimensional metaatoms into multipole contributions

We introduce a technique to decompose the scattered near field of two-dimensional arbitrary metaatoms into its multipole contributions. To this end we expand the scattered field upon plane wave illumination into cylindrical harmonics as known from Mie theory. By relating these cylin- drical harmonics to the field radiated by Cartesian multipoles, the contribution of the lowest order electric and magnetic multipoles can be identified. Revealing these multipoles is essential for the design of metamaterials because they largely determine the character of light propagation. In par- ticular, having this information at hand it is straightforward to distinguish between effects that result either from the arrangement of the metaatoms or from their particular design.

physics.optics

Difference between penetration and damping lengths in photonic crystal mirrors

Different mirror geometries in two-dimensional photonic crystal slabs are studied with fully-vectorial calculations. We compare their optical properties and, in particular, we show that, for heterostructure mirrors, the penetration length associated with the delay induced by distributed reflection is not correlated to the characteristic damping length of the electromagnetic energy distribution in the mirror. This unexpected result evidences that the usual trade-off between short damping lengths and large penetration lengths that is classically encountered in distributed Bragg reflectors can be overcome with carefully designed photonic crystal structures.

cond-mat.other

A microscopic view of the electromagnetic properties of sub-wavelength metallic surfaces

We review the properties of the surface waves that are scattered by two-dimensional sub-wavelength indentations on metallic surfaces. We show that two distinct waves are involved, a surface plasmon polariton (SPP) and a quasi-cylindrical wave (quasi-CW). We discuss the main characteristics of these waves, their damping characteristic lengths and their relative excitation weights as a function of the separation distance from the indentation and as a function of the metal conductivity. In particular we show that derive a closed-form expression for the quasi-CW, which clarifies its physical origin and its main properties. We further present an intuitive microscopic model, which explains how the elementary SPPs and quasi-CWs exchange their energies by multiple-scattering to build up a rich variety of near- and far-field optical effects.

cond-mat.other

Theory of surface plasmon generation at nanoslit apertures

In this letter, we study the scattering of light by a single subwavelength slit in a metal screen. In contrast to previous theoretical works, we provide a microscopic description of the scattering process by emphasizing the generation of surface plasmons at the slit apertures. The analysis is supported by a rigorous formalism based on a normal-mode-decomposition technique and by a semi-analytical model which provides accurate formulae for the plasmonic generation strengths. The generation is shown to be fairly efficient for metals with a low conductivity, like gold in the visible regime. Verification of the theory is also shown by comparison with recent experimental data [H.F. Schouten et al., Phys. Rev. Lett. 94, 053901 (2005)].

physics.optics