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P. Lodahl

Publications and source records attributed to P. Lodahl.

At least 19 recordsLinked to original sources

A photonic source with half-a-GHz single-photon flux

Advanced optical quantum technologies demands high quality quantum light generation at very high rates. Here, we report on a deterministic single-photon source that simultaneously combines high excitation rates with high system efficiency to reach over 500 MHz of in-fibre single-photon flux. The source delivers optical power of over 100 pW, as is measured with an off-the-shelf powermeter, enabling a simple and direct way of determining the single-photon source fiber efficiency.

quant-ph

Deterministic quantum dot single-photon sources: operational principles and state-of-the-art specifications

Non-classical states of light play a fundamental role in quantum technology. From photonic quantum computers and simulators, to quantum communication and sensing, quantum states of light enable performing tasks that may outperform their best classical counterparts. Semiconductor quantum dots embedded in photonic nanostructures offer the most advanced classes of quantum light sources. Importantly, the underlying physics processes determining device performance are today fully understood, and dedicated engineering projects are currently advancing these sources towards real-world quantum technology applications. We review the performance of deterministic single-photon sources based on quantum dots in photonic crystal waveguides, the approach with the highest performance specs since it intrinsically combines suppression of leaky modes and Purcell enhancement to slow-light waveguide mode. Furthermore, we present prototype data from sources that today are commercially available and with performance metrics approaching the ideal.

physics.optics

Wafer-Scale Epitaxial Modulation of Quantum Dot Density

Precise control of the properties of semiconductor quantum dots (QDs) is vital for creating novel devices for quantum photonics and advanced opto-electronics. Suitable low QD-density for single QD devices and experiments are challenging to control during epitaxy and are typically found only in limited regions of the wafer. Here, we demonstrate how conventional molecular beam epitaxy (MBE) can be used to modulate the density of optically active QDs in one- and two- dimensional patterns, while still retaining excellent quality. We find that material thickness gradients during layer-by-layer growth result in surface roughness modulations across the whole wafer. Growth on such templates strongly influences the QD nucleation probability. We obtain density modulations between 1 and 10 QDs/$μm^{2}$ and periods ranging from several millimeters down to at least a few hundred microns. This novel method is universal and expected to be applicable to a wide variety of different semiconductor material systems. We apply the method to enable growth of ultra-low noise QDs across an entire 3-inch semiconductor wafer.

cond-mat.mtrl-sci

Quantum Networks with Deterministic Spin-Photon Interfaces

We consider how recent experimental progress on deterministic solid state spin-photon interfaces enable the construction of a number of key elements of quantum networks. After reviewing some of the recent experimental achievements, we discuss their integration into Bell state analyzers, quantum non-demolition detection, and photonic cluster state generation. Finally, we outline how these elements can be used for long-distance entanglement generation and quantum key distribution in a quantum network.

quant-ph

Single-photon superradiance from a quantum dot

We report on the observation of single-photon superradiance from an exciton in a semiconductor quantum dot. The confinement by the quantum dot is strong enough for it to mimic a two-level atom, yet sufficiently weak to ensure superradiance. The electrostatic interaction between the electron and the hole comprising the exciton gives rise to an anharmonic spectrum, which we exploit to prepare the superradiant quantum state deterministically with a laser pulse. We observe a five-fold enhancement of the oscillator strength compared to conventional quantum dots. The enhancement is limited by the base temperature of our cryostat and may lead to oscillator strengths above 1000 from a single quantum emitter at optical frequencies.

cond-mat.mes-hall

Optical refrigeration with coupled quantum wells

Refrigeration of a solid-state system with light has potential applications for cooling small-scale electronics and photonics. We show theoretically that two coupled semiconductor quantum wells are efficient cooling media for optical refrigeration because they support long-lived indirect electron-hole pairs. Thermal excitation of these pairs to distinct higher-energy states with faster radiative recombination allows an efficient escape channel to remove thermal energy from the system. This allows reaching much higher cooling efficiencies than with single quantum wells. From band-diagram calculations along with an experimentally realistic level scheme we calculate the cooling efficiency and cooling yield of different devices with coupled quantum wells embedded in a suspended nanomembrane. The dimension and composition of the quantum wells allow optimizing either of these quantities, which cannot, however, be maximized simultaneously. Quantum-well structures with electrical control allow tunability of carrier lifetimes and energy levels so that the cooling efficiency can be optimized over time as the thermal population decreases due to the cooling.

cond-mat.mes-hall

Single-photon nonlinear optics with a quantum dot in a waveguide

Strong nonlinear interactions between photons enable logic operations for both classical and quantum-information technology. Unfortunately, nonlinear interactions are usually feeble and therefore all-optical logic gates tend to be inefficient. A quantum emitter deterministically coupled to a propagating mode fundamentally changes the situation, since each photon inevitably interacts with the emitter, and highly correlated many-photon states may be created . Here we show that a single quantum dot in a photonic-crystal waveguide can be utilized as a giant nonlinearity sensitive at the single-photon level. The nonlinear response is revealed from the intensity and quantum statistics of the scattered photons, and contains contributions from an entangled photon-photon bound state. The quantum nonlinearity will find immediate applications for deterministic Bell-state measurements and single-photon transistors and paves the way to scalable waveguide-based photonic quantum-computing architectures.

quant-ph

Photon Sorting, Efficient Bell Measurements and a Deterministic CZ Gate using a Passive Two-level Nonlinearity

Although the strengths of optical non-linearities available experimentally have been rapidly increasing in recent years, significant challenges remain to using such non-linearities to produce useful quantum devices such as efficient optical Bell state analysers or universal quantum optical gates. Here we describe a new approach that avoids the current limitations by combining strong non-linearities with active Gaussian operations in efficient protocols for Bell state analysers and Controlled-Sign gates.

quant-ph

Efficient out-coupling of high-purity single photons from a coherent quantum dot in a photonic-crystal cavity

We demonstrate a single-photon collection efficiency of $(44.3\pm2.1)\%$ from a quantum dot in a low-Q mode of a photonic-crystal cavity with a single-photon purity of $g^{(2)}(0)=(4\pm5)\%$ recorded above the saturation power. The high efficiency is directly confirmed by detecting up to $962\pm46$ kilocounts per second on a single-photon detector on another quantum dot coupled to the cavity mode. The high collection efficiency is found to be broadband, as is explained by detailed numerical simulations. Cavity-enhanced efficient excitation of quantum dots is obtained through phonon-mediated excitation and under these conditions, single-photon indistinguishability measurements reveal long coherence times reaching $0.77\pm0.19$ ns in a weak-excitation regime. Our work demonstrates that photonic crystals provide a very promising platform for highly integrated generation of coherent single photons including the efficient out-coupling of the photons from the photonic chip.

quant-ph

Near-unity coupling efficiency of a quantum emitter to a photonic-crystal waveguide

A quantum emitter efficiently coupled to a nanophotonic waveguide constitutes a promising system for the realization of single-photon transistors, quantum-logic gates based on giant single-photon nonlinearities, and high bit-rate deterministic single-photon sources. The key figure of merit for such devices is the $β$-factor, which is the probability for an emitted single photon to be channeled into a desired waveguide mode. We report on the experimental achievement of $β= 98.43 \pm 0.04\%$ for a quantum dot coupled to a photonic-crystal waveguide, corresponding to a single-emitter cooperativity of $η= 62.7 \pm 1.5$. This constitutes a nearly ideal photon-matter interface where the quantum dot acts effectively as a 1D "artificial" atom, since it interacts almost exclusively with just a single propagating optical mode. The $β$-factor is found to be remarkably robust to variations in position and emission wavelength of the quantum dots. Our work demonstrates the extraordinary potential of photonic-crystal waveguides for highly efficient single-photon generation and on-chip photon-photon interaction.

quant-ph

Influence of multi-electronic states on few-quantum-dot nanolasers

We present an experimental and theoretical study on the gain mechanism in a photonic-crystal-cavity nanolaser with embedded quantum dots. From time-resolved measurements at low excitation power we find that four excitons are coupled to the cavity. At high excitation power we observe a smooth low-threshold transition from spontaneous emission to lasing. Before lasing emission sets in, however, the excitons are observed to saturate, and the gain required for lasing originates rather from multi-electronic transitions, which give rise to a broad emission background. We compare the experiment to a model of quantum-dot microcavity lasers and find that the number of emitters feeding the cavity must greatly exceed four, which confirms that the gain is provided by multi-electronic states. Our results are consistent with theoretical predictions.

cond-mat.mes-hall

Microscopic theory of indistinguishable single-photon emission from a quantum dot coupled to a cavity: The role of non-Markovian phonon-induced decoherence

We study the fundamental limit on single-photon indistinguishability imposed by decoherence due to phonon interactions in semiconductor quantum dot-cavity QED systems. Employing an exact diagonalization approach we find large differences compared to standard methods. An important finding is that short-time non-Markovian effects limit the maximal attainable indistinguishability. The results are explained using a polariton picture that yields valuable insight into the phonon-induced dephasing dynamics.

cond-mat.mes-hall

Cooperative Fluorescence from a Strongly Driven Dilute Cloud of Atoms

We investigate cooperative fluorescence in a dilute cloud of strongly driven two-level emitters. Starting from the Heisenberg equations of motion, we compute the first-order scattering corrections to the saturation of the excited-state population and to the resonance-fluorescence spectrum, which both require going beyond the state-of-the-art linear-optics approach to describe collective phenomena. A dipole blockade is observed due to long range dipole-dipole coupling that vanishes at stronger driving fields. Furthermore, we compute the inelastic component of the light scattered by a cloud of many atoms and find that the Mollow triplet is affected by cooperativity. In a lobe around the forward direction, the inelastic Mollow triplet develops a spectral asymmetry, observable under experimental conditions.

physics.atom-ph

Quantitative analysis of quantum dot dynamics and emission spectra in cavity quantum electrodynamics

We present detuning-dependent spectral and decay-rate measurements to study the difference between spectral and dynamical properties of single quantum dots embedded in micropillar and photonic-crystal cavities. For the micropillar cavity, the dynamics is well described by the dissipative Jaynes-Cummings model, while systematic deviations are observed for the emission spectra. The discrepancy for the spectra is attributed to coupling of other exciton lines to the cavity and interference of different propagation paths towards the detector of the fields emitted by the quantum dot. In contrast, quantitative information about the system can readily be extracted from the dynamical measurements. In the case of photonic crystal cavities we observe an anti crossing in the spectra when detuning a single quantum dot through resonance, which is the spectral signature of strong coupling. However, time-resolved measurements reveal that the actual coupling strength is significantly smaller than anticipated from the spectral measurements and that the quantum dot is rather weakly coupled to the cavity. We suggest that the observed Rabi splitting is due to cavity feeding by other quantum dots and/or multiexcition complexes giving rise to collective emission effects.

quant-ph

Quantifying the intrinsic amount of fabrication disorder in photonic-crystal waveguides from optical far-field intensity measurements

Residual disorder due to fabrication imperfections has important impact in nanophotonics where it may degrade device performance by increasing radiation loss or spontaneously trap light by Anderson localization. We propose and demonstrate experimentally a method of quantifying the intrinsic amount of disorder in state-of-the-art photonic-crystal waveguides from far-field measurements of the Anderson-localized modes. This is achieved by comparing the spectral range that Anderson localization is observed to numerical simulations and the method offers sensitivity down to ~ 1 nm.

physics.optics

Measuring the effective phonon density of states of a quantum dot

We employ detuning-dependent decay-rate measurements of a quantum dot in a photonic-crystal cavity to study the influence of phonon dephasing in a solid-state quantum-electrodynamics experiment. The experimental data agree with a microscopic non-Markovian model accounting for dephasing from longitudinal acoustic phonons, and identifies the reason for the hitherto unexplained difference between non-resonant cavity feeding in different nanocavities. From the comparison between experiment and theory we extract the effective phonon density of states experienced by the quantum dot. This quantity determines all phonon dephasing properties of the system and is found to be described well by a theory of bulk phonons.

cond-mat.mes-hall

Microscopic theory of phonon-induced effects on semiconductor quantum dot decay dynamics in cavity QED

We investigate the influence of the electron-phonon interaction on the decay dynamics of a quantum dot coupled to an optical microcavity. We show that the electron-phonon interaction has important consequences on the dynamics, especially when the quantum dot and cavity are tuned out of resonance, in which case the phonons may add or remove energy leading to an effective non-resonant coupling between quantum dot and cavity. The system is investigated using two different theoretical approaches: (i) a second-order expansion in the bare phonon coupling constant, and (ii) an expansion in a polaron-photon coupling constant, arising from the polaron transformation which allows an accurate description at high temperatures. In the low temperature regime we find excellent agreement between the two approaches. An extensive study of the quantum dot decay dynamics is performed, where important parameter dependencies are covered. We find that in general the electron-phonon interaction gives rise to a greatly increased bandwidth of the coupling between quantum dot and cavity. At low temperature an asymmetry in the quantum dot decay rate is observed, leading to a faster decay when the quantum dot has a larger energy than to the cavity. We explain this as due to the absence of phonon absorption processes. Furthermore, we derive approximate analytical expressions for the quantum dot decay rate, applicable when the cavity can be adiabatically eliminated. The expressions lead to a clear interpretation of the physics and emphasizes the important role played by the effective phonon density, describing the availability of phonons for scattering, in quantum dot decay dynamics. Based on the analytical expressions we present the parameter regimes where phonon effects are expected to be important. Also, we include all technical developments in appendices.

cond-mat.mes-hall

Extraction of optical Bloch modes in a photonic-crystal waveguide

We perform phase-sensitive near-field scanning optical microscopy on photonic-crystal waveguides. The observed intricate field patterns are analyzed by spatial Fourier transformations, revealing several guided TE- and TM-like modes. Using the reconstruction algorithm proposed by Ha, et al. (Opt. Lett. 34 (2009)), we decompose the measured two-dimensional field pattern in a superposition of propagating Bloch modes. This opens new possibilities to study specific modes in near-field measurements. We apply the method to study the transverse behavior of a guided TE-like mode, where the mode extends deeper in the surrounding photonic crystal when the band edge is approached.

physics.optics