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P. M. Kadletz

Publications and source records attributed to P. M. Kadletz.

3 recordsLinked to original sources

Evaluation of a method for time-of-flight, wavelength and distance calibration for neutron scattering instruments by means of a mini-chopper and standard neutron monitors

Accurate conversion of neutron time-of-flight (TOF) to wavelength, and its uncertainty, is of fundamental importance to neutron scattering measurements. Especially in cases where instruments are highly configurable, the determination of the absolute wavelength after any change must always be performed. Inspired by the manner with which neutron spectrometers determine the absolute wavelength, we evaluate for the first time, in the author's knowledge, a commonly used method for converting TOF to neutron wavelength, the distance of a monitor from the source of neutrons and we analytically calculate the uncertainty contributions that limit the precision of the conversion. The method was evaluated at the V20 test beamline at the Helmholtz Zentrum Berlin (HZB), emulating the ESS source with a pulse of 2.86 ms length and 14 Hz repetition rate, by using a mini-chopper operated at 140 Hz, beam monitors (BMs) and data acquisition infrastructure. The mini-chopper created well-defined neutron pulses and the BM was placed at two positions, enabling the average wavelength of each of the pulses created to be determined. The used experimental setup resulted in absolute wavelength determination at the monitor positions with a $δλ_{mean} / λ_{mean}$ of $\sim$1.8% for $λ>4$ Å. With a modest increase of the distance between the reference monitor positions a $δλ_{mean} / λ_{mean}$ of below 0.5% can be achieved. Further improvements are possible by using a thinner monitor, smaller chopper disc openings and a higher rotational speed chopper. The method requires only two neutron measurements and doesn't necessitate the use of crystals or complex fitting, and could constitute a suitable addition to imaging, diffraction, reflectometers and small angle neutron scattering instruments, at spallation sources, that do not normally utilise fast choppers.

physics.ins-det

Spectroscopic Neutron Imaging for Resolving Hydrogen Dynamics Changes in Battery Electrolytes

We present spectroscopic neutron imaging (SNI), a bridge between imaging and scattering techniques, for the analysis of hydrogenated molecules in lithium-ion cells. The scattering information of CHn-based organic solvents and electrolytes was mapped in two-dimensional space by investigating the wavelength-dependent property of hydrogen atoms through time-of-flight imaging. Our investigation demonstrates a novel approach to detect physical and chemical changes in hydrogenated liquids, which extends, but not limits, the use of SNI to relevant applications in electrochemical devices, e.g., the study of electrolytes in Li-ion batteries.

cond-mat.mtrl-sci

Time- and energy-resolved effects in the boron-10 based Multi-Grid and helium-3 based thermal neutron detectors

The boron-10 based Multi-Grid detector is being developed as an alternative to helium-3 based neutron detectors. At the European Spallation Source, the detector will be used for time-of-flight neutron spectroscopy at cold to thermal neutron energies. The objective of this work is to investigate fine time- and energy-resolved effects of the Multi-Grid detector, down to a few $μ$eV, while comparing it to the performance of a typical helium-3 tube. Furthermore, it is to characterize differences between the detector technologies in terms of internal scattering, as well as the time reconstruction of ~ $μ$s short neutron pulses. The data were taken at the Helmholtz Zentrum Berlin, where the Multi-Grid detector and a helium-3 tube were installed at the ESS test beamline, V20. Using a Fermi-chopper, the neutron beam of the reactor was chopped into a few tens of $μ$s wide pulses before reaching the detector, located a few tens of cm downstream. The data of the measurements show an agreement between the derived and calculated neutron detection efficiency curve. The data also provide fine details on the effect of internal scattering, and how it can be reduced. For the first time, the chopper resolution was comparable to the timing resolution of the Multi-Grid detector. This allowed a detailed study of time- and energy resolved effects, as well as a comparison with a typical helium-3 tube.

physics.ins-det