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P. M. R. Brydon

Publications and source records attributed to P. M. R. Brydon.

At least 37 records · Page 2Linked to original sources

General theory of robustness against disorder in multi-band superconductors

We investigate the influence of general forms of disorder on the robustness of superconductivity in multiband materials. Specifically, we consider a general two-band system where the bands arise from an orbital degree of freedom of the electrons. Within the Born approximation, we show that the interplay of the spin-orbital structure of the normal-state Hamiltonian, disorder scattering, and superconducting pairing potentials can lead to significant deviations from the expected robustness of the superconductivity. This can be conveniently formulated in terms of the so-called "superconducting fitness". In particular, we verify a key role for unconventional $s$-wave states, permitted by the spin-orbital structure and which may pair electrons that are not time-reversed partners. To exemplify the role of Fermi surface topology and spin-orbital texture, we apply our formalism to the candidate topological superconductor Cu$_x$Bi$_2$Se$_3$, for which only a single band crosses the Fermi energy, as well as models of the iron pnictides, which possess multiple Fermi pockets.

cond-mat.supr-con↗

Field-induced transition from even to odd parity superconductivity in CeRh$_2$As$_2$

We report the discovery of two-phase unconventional superconductivity in CeRh$_2$As$_2$. Using thermodynamic probes, we establish that the superconducting critical field of its high-field phase is as high as 14 T, remarkable in a material whose transition temperature is 0.26 K. Furthermore, a $c$-axis field drives a transition between two different superconducting phases. In spite of the fact that CeRh$_2$As$_2$ is globally centrosymmetric, we show that local inversion-symmetry breaking at the Ce sites enables Rashba spin-orbit coupling to play a key role in the underlying physics. More detailed analysis identifies the transition from the low- to high-field states to be associated with one between states of even and odd parity.

cond-mat.supr-con↗

Distortional weak-coupling instability of Bogoliubov Fermi surfaces

Centrosymmetric multiband superconductors which break time-reversal symmetry generically have two-dimensional nodes, i.e., Fermi surfaces of Bogoliubov quasiparticles. We show that the coupling of the electrons to the lattice always leads to a weak-coupling instability of such a state towards spontaneous breaking of inversion symmetry at low temperatures. This instability is driven by a Cooper logarithm in the internal energy but the order parameter is not superconducting but distortional. We present a comprehensive symmetry analysis and introduce a measure that allows to compare the strengths of competing distortional instabilities. Moreover, we discuss the instability using an effective single-band model. This framework reveals a duality mapping of the effective model which maps the distortional order parameter onto a superconducting one, providing a natural explanation for the Cooper logarithm and the weak-coupling nature of the instability. Finally, we consider the possibility of a pair-density wave state when inversion symmetry is broken. We find that it can indeed exist but does not affect the instability itself.

cond-mat.supr-con↗

Origin of the anomalous Hall effect in two-band chiral superconductors

We consider the origin of the anomalous Hall effect in a general model of a clean two-band chiral superconductor. Within the Kubo formalism we derive an analytic expression for the high-frequency ac Hall conductivity valid close to the critical temperature. This expression involves two distinct gauge-invariant time-reversal-odd bilinear (TROB) functions involving the pairing potential and its Hermitian conjugate. We argue that the existence of at least one of these TROBs generically implies a nonzero ac Hall conductivity. The TROBs allow us to clarify the roles of intra- and interband pairing, and provide a straightforward criterion for a superconducting state to exhibit the anomalous Hall effect. We briefly exemplify our results with model calculations for a chiral $p$-wave pairing state in strontium ruthenate and a chiral $d$-wave pairing state on the honeycomb lattice.

cond-mat.supr-con↗

Topological band and superconductivity in UTe$_2$

UTe$_2$ has recently been found to be a likely spin-triplet superconductor that exhibits evidence for chiral Majorana edge states. A characteristic structural feature of UTe$_2$ is inversion-symmetry related pairs of U atoms, forming rungs of ladders. Here we show how each rung's two sublattice degrees of freedom play a key role in understanding the electronic structure and the origin of superconductivity. In particular, we show that DFT+$U$ calculations generically reveal a topological band that originates from a band inversion associated with $5f$ electrons residing on these rung sublattice degrees of freedom. Furthermore, we show that a previously identified strong ferromagnetic interaction within a U-U rung leads to a pseudospin-triplet superconducting state that can account for a non-zero polar Kerr angle, observed magnetic field-temperature phase diagrams, and nodal Weyl fermions. Our analysis may also be relevant for other U-based superconductors.

cond-mat.supr-con↗

Stabilizing Even-Parity Chiral Superconductivity in Sr$_2$RuO$_4$

Strontium ruthenate (Sr$_2$RuO$_4$) has long been thought to host a spin-triplet chiral $p$-wave superconducting state. However, the singletlike response observed in recent spin-susceptibility measurements casts serious doubts on this pairing state. Together with the evidence for broken time-reversal symmetry and a jump in the shear modulus $c_{66}$ at the superconducting transition temperature, the available experiments point towards an even-parity chiral superconductor with $k_z(k_x\pm ik_y)$-like $E_g$ symmetry, which has consistently been dismissed based on the quasi-two-dimensional electronic structure of Sr$_2$RuO$_4$. Here, we show how the orbital degree of freedom can encode the two-component nature of the $E_g$ order parameter, allowing for a local orbital-antisymmetric spin-triplet state that can be stabilized by on-site Hund's coupling. We find that this exotic $E_g$ state can be energetically stable once a complete, realistic three-dimensional model is considered, within which momentum-dependent spin-orbit coupling terms are key. This state naturally gives rise to Bogoliubov Fermi surfaces.

cond-mat.supr-con↗

Robustness of unconventional $s$-wave superconducting states against disorder

We investigate the robustness against disorder of superconductivity in multiband systems where the fermions have four internal degrees of freedom. This permits unconventional $s$-wave pairing states, which may transform nontrivially under crystal symmetries. Using the self-consistent Born approximation, we develop a general theory for the effect of impurities on the critical temperature, and find that the presence of these novel $s$-wave channels significantly modifies the conclusions of single-band theories. We apply our theory to two candidate topological superconductors, YPtBi and Cu$_x$Bi$_2$Se$_3$, and show that the novel $s$-wave states display an enhanced resilience against disorder, which extends to momentum-dependent pairing states with the same crystal symmetry. The robustness of the $s$-wave states can be quantified in terms of their superconducting fitness, which can be readily evaluated for model systems.

cond-mat.supr-con↗

Bogoliubov Fermi surfaces stabilized by spin-orbit coupling

It was recently understood that centrosymmetric multiband superconductors that break time-reversal symmetry generically show Fermi surfaces of Bogoliubov quasiparticles. We investigate the thermodynamic stability of these Bogoliubov Fermi surfaces in a paradigmatic model. To that end, we construct the mean-field phase diagram as a function of spin-orbit coupling and temperature. It confirms the prediction that a pairing state with Bogoliubov Fermi surfaces can be stabilized at moderate spin-orbit coupling strengths. The multiband nature of the model also gives rise to a first-order phase transition, which can be explained by the competition of intra- and interband pairing and is strongly affected by cubic anisotropy. For the state with Bogoliubov Fermi surfaces, we also discuss experimental signatures in terms of the residual density of states and the induced magnetic order. Our results show that Bogoliubov Fermi surfaces of experimentally relevant size can be thermodynamically stable.

cond-mat.supr-con↗

Loop currents and anomalous Hall effect from time-reversal symmetry-breaking superconductivity on the honeycomb lattice

We study a tight-binding model on the honeycomb lattice of chiral $d$-wave superconductivity that breaks time-reversal symmetry. Due to its nontrivial sublattice structure, we show that it is possible to construct a gauge-invariant time-reversal-odd bilinear of the pairing potential. The existence of this bilinear reflects the sublattice polarization of the pairing state. We show that it generates persistent loop current correlations around each lattice site and opens a topological mass gap at the Dirac points, resembling Haldane's model of the anomalous quantum Hall effect. In addition to the usual chiral $d$-wave edge states, there also exist electron-like edge resonances due to the topological mass gap. We show that the presence of loop-current correlations directly leads to a nonzero intrinsic ac Hall conductivity, which produces the polar Kerr effect without an external magnetic field. Similar results also hold for the nearest-neighbor chiral $p$-wave pairing. We briefly discuss the relevance of our results to superconductivity in twisted bilayer graphene.

cond-mat.supr-con↗

Bogoliubov Fermi surfaces: General theory, magnetic order, and topology

We present a comprehensive theory for Bogoliubov Fermi surfaces in inversion-symmetric superconductors which break time-reversal symmetry. A requirement for such a gap structure is that the electrons posses internal degrees of freedom apart from the spin (e.g., orbital or sublattice indices), which permits a nontrivial internal structure of the Cooper pairs. We develop a general theory for such a pairing state, which we show to be nonunitary. A time-reversal-odd component of the nonunitary gap product is found to be essential for the appearance of Bogoliubov Fermi surfaces. These Fermi surfaces are topologically protected by a $\mathbb{Z}_2$ invariant. We examine their appearance in a generic low-energy effective model and then study two specific microscopic models supporting Bogoliubov Fermi surfaces: a cubic material with a $j=3/2$ total-angular-momentum degree of freedom and a hexagonal material with distinct orbital and spin degrees of freedom. The appearance of Bogoliubov Fermi surfaces is accompanied by a magnetization of the low-energy states, which we connect to the time-reversal-odd component of the gap product. We additionally calculate the surface spectra associated with these pairing states and demonstrate that the Bogoliubov Fermi surfaces are characterized by additional topological indices. Finally, we discuss the extension of phenomenological theories of superconductors to include Bogoliubov Fermi surfaces, and identify the time-reversal-odd part of the gap product as a composite order parameter which is intertwined with superconductivity.

cond-mat.supr-con↗

Resilient nodeless $d$-wave superconductivity in monolayer FeSe

Monolayer FeSe exhibits the highest transition temperature among the iron based superconductors and appears to be fully gapped, seemingly consistent with $s$-wave superconductivity. Here, we develop a theory for the superconductivity based on coupling to fluctuations of checkerboard magnetic order (which has the same translation symmetry as the lattice). The electronic states are described by a symmetry based ${\bf k}\cdot {\bf p}$-like theory and naturally account for the states observed by angle resolved photoemission spectroscopy. We show that a prediction of this theory is that the resultant superconducting state is a fully gapped, nodeless, $d$-wave state. This state, which would usually have nodes, stays nodeless because, as seen experimentally, the relevant spin-orbit coupling term has an energy scale smaller than the superconducting gap.

cond-mat.supr-con↗

Inflated nodes and surface states in superconducting half-Heusler compounds

Two topics of high current interest in the field of unconventional superconductivity are non-centrosymmetric superconductors and multiband superconductivity. Half-Heusler superconductors such as YPtBi exemplify both. In this paper, we study bulk and surface states in nodal superconducting phases of the half-Heusler compounds, belonging to the $A_1$ ($s+p$-like) and $T_2$ ($k_zk_x+ik_zk_y$-like) irreducible representations of the point group. These two phases preserve and break time-reversal symmetry, respectively. For the $A_1$ case, we find that flat surface bands persist in the multiband system. In addition, the system has dispersive surface bands with zero-energy crossings forming Fermi arcs, which are protected by mirror symmetries. For the $T_2$ case, there is an interesting coexistence of point and line nodes, known from the single-band case, with Bogoliubov Fermi surfaces (two-dimensional nodes). There are no flat-band surface states, as expected, but dispersive surface bands with Fermi arcs exist. If these arcs do not lie in high-symmetry planes, they are split by the antisymmetric spin-orbit coupling so that their number is doubled compared to the inversion-symmetric case.

cond-mat.supr-con↗

Bogoliubov Fermi surfaces in superconductors with broken time-reversal symmetry

It is commonly believed that in the absence of disorder or an external magnetic field, there are three possible types of superconducting excitation gaps: the gap is nodeless, it has point nodes, or it has line nodes. Here, we show that for an even-parity nodal superconducting state which spontaneously breaks time-reversal symmetry, the low-energy excitation spectrum generally does not belong to any of these categories, instead it has extended Bogoliubov Fermi surfaces. These Fermi surfaces can be visualized as two-dimensional surfaces generated by "inflating" point or line nodes into spheroids or tori, respectively. These inflated nodes are topologically protected from being gapped by a $\mathbb{Z}_2$ invariant, which we give in terms of a Pfaffian. We also show that superconducting states possessing these Fermi surfaces can be energetically stable. A crucial ingredient in our theory is that more than one band is involved in the pairing, since all candidate materials for even-parity superconductivity with broken time-reversal symmetry are multiband systems, we expect these $\mathbb{Z}_2$-protected Fermi surfaces to be ubiquitous.

cond-mat.supr-con↗

Pairing of j=3/2 fermions in half-Heusler superconductors

We theoretically consider the superconductivity of the topological half-Heusler semimetals YPtBi and LuPtBi. We show that pairing occurs between j=3/2 fermion states, which leads to qualitative differences from the conventional theory of pairing between j=1/2 states. In particular, this permits Cooper pairs with quintet or septet total angular momentum, in addition to the usual singlet and triplet states. Purely on-site interactions can generate s-wave quintet time-reversal symmetry-breaking states with topologically nontrivial point or line nodes. These local s-wave quintet pairs reveal themselves as d-wave states in momentum space. Furthermore, due to the broken inversion symmetry in these materials, the s-wave singlet state can mix with a p-wave septet state, again with topologically-stable line nodes. Our analysis lays the foundation for understanding the unconventional superconductivity of the half-Heuslers.

cond-mat.supr-con↗

Conductance spectroscopy of topological superconductor wire junctions

We study the zero-temperature transport properties of one-dimensional normal-superconductor (NS) junctions with topological superconductors across their topological transitions. Working within the Blonder-Tinkham-Klapwijk (BTK) formalism generalized for topological NS junctions, we analytically calculate the differential conductance for tunneling into two models of a topological superconductor: a spinless intrinsic $p$-wave superconductor and a spin-orbit-coupled $s$-wave superconductor in a Zeeman field. In both cases we verify that the zero-bias conductance is robustly quantized at $2e^2/h$ in the topological regime, while it takes nonuniversal values in the non-topological phase. The conductance spectra in the topological state develops a peak at zero bias for certain parameter regimes, with the peak width controlled by the strength of spin-orbit coupling and barrier transparency.

cond-mat.mes-hall↗

Bound states of a ferromagnetic wire in a superconductor

We consider the problem of bound states in strongly anisotropic ferromagnetic impurities in a superconductor, motivated by recent experiments that claim to observe Majorana modes at the ends of ferromagnetic wires on a superconducting substrate [S. Nadj-Perge et al., Science 346, 602 (2014)]. Generalizing the successful theory of bound states of spherically symmetric impurities, we consider a wire-like potential using both analytical and numerical approaches. We find that away from the ends of the wire the bound states form bands with pronounced van Hove singularities, giving rise to subgap peaks in the local density of states. For sufficiently strong magnetization of the wire, we show that this process generically produces a sharp peak at zero energy in the local density of states near the ends of the wire. This zero-energy peak has qualitative similarities to the claimed signature of a Majorana mode observed in the aforementioned experiment.

cond-mat.supr-con↗

Substrate-induced Majorana renormalization in topological nanowires

We theoretically consider the substrate-induced Majorana localization length renormalization in nanowires in contact with a bulk superconductor in the strong tunnel-coupled regime, showing explicitly that this renormalization depends strongly on the transverse size of the one-dimensional nanowires. For metallic (e.g. Fe on Pb) or semiconducting (e.g. InSb on Nb) nanowires, the renormalization effect is found to be very strong and weak respectively because the transverse confinement size in the two situations happens to be 0.5nm (metallic nanowire) and 20nm (semiconducting nanowire). Thus, the Majorana localization length could be very short (long) for metallic (semiconducting) nanowires even for the same values of all other parameters (except for the transverse wire size). We also show that any tunneling conductance measurements in such nanowires, carried out at temperatures and/or energy resolutions comparable to the induced superconducting energy gap, cannot distinguish between the existence of the Majorana modes or ordinary subgap fermionic states since both produce very similar broad and weak peaks in the subgap tunneling conductance independent of the localization length involved. Only low temperature (and high resolution) tunneling measurements manifesting sharp zero bias peaks can be considered to be signatures of Majorana modes in topological nanowires.

cond-mat.supr-con↗

Surface instability in nodal noncentrosymmetric superconductors

We study the stability of topologically protected zero-energy flat bands at the surface of nodal noncentrosymmetric superconductors, accounting for the alteration of the gap near the surface. Within a selfconsistent mean-field theory, we show that the flat bands survive in a broad temperature range below the bulk transition temperature. There is a second transition at a lower temperature, however, below which the system spontaneously breaks time-reversal symmetry. The surface bands are shifted away from zero energy and become weakly dispersive. Simultaneously, a spin polarization and an equilibrium charge current develop in the surface region.

cond-mat.supr-con↗