arXiv subjects

P. M. S. Monteiro

Publications and source records attributed to P. M. S. Monteiro.

3 recordsLinked to original sources

arXiv2022

Determining the Proximity Effect Induced Magnetic Moment in Graphene by Polarized Neutron Reflectivity and X-ray Magnetic Circular Dichroism

We report the magnitude of the induced magnetic moment in CVD-grown epitaxial and rotated-domain graphene in proximity with a ferromagnetic Ni film, using polarized neutron reflectivity (PNR) and X-ray magnetic circular dichroism (XMCD). The XMCD spectra at the C K-edge confirms the presence of a magnetic signal in the graphene layer and the sum rules give a magnetic moment of up to $\sim\,0.47\,μ$_B/C atom induced in the graphene layer. For a more precise estimation, we conducted PNR measurements. The PNR results indicate an induced magnetic moment of $\sim$ 0.53 $μ$_B/C atom at 10 K for rotated graphene and $\sim$ 0.38 $μ$_B/C atom at 10 K for epitaxial graphene. Additional PNR measurements on graphene grown on a non-magnetic Ni_9Mo_1 substrate, where no magnetic moment in graphene is measured, suggest that the origin of the induced magnetic moment is due to the opening of the graphene's Dirac cone as a result of the strong C pz-3d hybridization.

cond-mat.mes-hall↗

arXiv2021

Table-like magnetocaloric effect and enhanced refrigerant capacity in EuO1-δ thin films

An approach to adjusting the conduction band population for tuning the magnetic and magnetocaloric response of EuO1-δ thin films through control of oxygen vacancies (δ = 0, 0.025, and 0.09) is presented. The films each showed a paramagnetic to ferromagnetic transition around 65 K, with an additional magnetic ordering transition at higher temperatures in the oxygen deficient samples. All transitions are observed to be of second order. A maximum magnetic entropy change of 6.4 J/kg K over a field change of 2 T with a refrigerant capacity of 223 J/kg was found in the sample with δ = 0, and in all cases the refrigerant capacities of the thin films under study were found to exceed that reported for bulk EuO. Adjusting the oxygen content was shown to produce table-like magnetocaloric effects, desirable for ideal Ericsson-cycle magnetic refrigeration. These films are thus excellent candidates for small-scale magnetic cooling technology in the liquid nitrogen temperature range.

cond-mat.mtrl-sci↗

arXiv2010

Spin configurations in hard-soft coupled bilayer systems: from rigid magnet to exchange spring transitions

We investigate equilibrium properties of an exchange-spring magnetic system constituted of a soft layer (e.g. Fe) of a given thickness on top of a hard magnetic layer (e.g. FePt). The magnetization profile M(z) as a function of the atomic position ranging from the bottom of the hard layer to the top of the soft layer is obtained in two cases with regard to the hard layer: i) in the case of a rigid interface (the FePt layer is a single layer), the profile is obtained analytically as the exact solution of a sine-Gordon equation with Cauchy's boundary conditions. Additional numerical simulations also confirm this result. Asymptotic expressions of M(z) show a linear behavior near the bottom and the top of the soft layer. In addition, a critical value of the number of atomic planes in the soft layer, that is necessary for the onset of spin deviations, is obtained in terms of the anisotropy and exchange coupling between the adjacent plane in the soft layer. ii) in the case of a relaxed interface (the FePt layer is a multilayer), the magnetization profile is obtained numerically for various Fe and FePt films thicknesses and applied field.

cond-mat.mtrl-sci↗