arXiv subjects

P. Morfouace

Publications and source records attributed to P. Morfouace.

At least 37 records · Page 2Linked to original sources

arXiv2021

Energy Dependence of Prompt Fission Neutron Multiplicity in the $^{239}$Pu($n,f$) Reaction

Accurate multiplicities of prompt fission neutrons emitted in neutron-induced fission on a large energy range are essential for fundamental and applied nuclear physics. Measuring them to high precision for radioactive fissioning nuclides remains, however, an experimental challenge. In this work, the average prompt-neutron multiplicity emitted in the 239Pu(n,f) reaction was extracted as a function of the incident-neutron energy, over the range 1-700~MeV, with a novel technique, which allowed to minimize and correct for the main sources of bias and thus achieve unprecedented precision. At low energies, our data validate for the first time the ENDF/B-VIII.0 nuclear data evaluation with an independent measurement and reduce the evaluated uncertainty by up to $60\%$. This work opens up the possibility of precisely measuring prompt fission neutron multiplicities on highly radioactive nuclei relevant for an essential component of energy production world-wide.

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arXiv2021

Reaction Losses of Charged Particles in CsI(Tl) crystals

To efficiently detect energetic light charged particles, it is common to use arrays of energy-loss telescopes involving two or more layers of detection media. As the energy of the particles increases, thicker layers are usually needed. However, carrying out measurements with thick-telescopes may require corrections for the losses due to nuclear reactions induced by the incident particles on nuclei within the detector and for the scattering of incident particles out of the detector, without depositing their full energy in the active material. In this paper, we develop a method for measuring such corrections and determine the reaction and out-scattering losses for data measured with the silicon-CsI(Tl) telescopes of the newly developed HiRA10 array. The extracted efficiencies are in good agreement with model predictions using the GEANT4 reaction loss algorithm for Z=1 and Z=2 isotopes. After correcting for the HiRA10 geometry, a general function that describes the efficiencies from the reaction loss in CsI(Tl) crystals as a function of range is obtained.

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arXiv2021

Evaluation of the $^{35}$K($p$,$γ$)$^{36}$Ca reaction rate using the $^{37}$Ca($p$,$d$)$^{36}$Ca transfer reaction

A recent sensitivity study has shown that the $^{35}$K$(p,γ)^{36}$Ca reaction is one of the ten $(p,γ)$ reaction rates that could significantly impact the shape of the calculated X-ray burst light curve. In this work, we propose to reinvestigate the $^{35}$K$(p,γ)^{36}$Ca reaction rate, as well as related uncertainties, by determining the energies and decay branching ratios of $^{36}$Ca levels, within the Gamow window, in the 0.5 to 2 GK X-ray burst temperature range. These properties were studied using the one neutron pick-up transfer reaction $^{37}$Ca$(p,d)^{36}$Ca in inverse kinematics using a radioactive beam of $^{37}$Ca at 48 MeV nucleon$^{-1}$. The experiment performed at GANIL, used the liquid Hydrogen target CRYPTA, the MUST2 detector array for the detection of the light charged particles and a zero degree detection system for the outgoing heavy ions. The atomic mass of $^{36}$Ca is confirmed and new resonances have been proposed together with their proton decay branching ratios. This spectroscopic information, used in combination with recent theoretical predictions for the $γ$-width, were used to calculate the $^{35}$K$(p,γ)^{36}$Ca reaction rate. The recommended rate of the present work was obtain within a uncertainty factor of 2 at 1 sigma. This is consistent, with the previous estimate in the X-ray burst temperature range. A large increase of the reaction rate was found at higher temperatures due to two newly discovered resonances. The $^{35}$K$(p,γ)^{36}$Ca thermonuclear reaction rate is now well constrained by the present work in a broad range of temperatures. Our results show that the $^{35}$K$(p,γ)^{36}$Ca reaction does not affect the shape of the X-ray burst light curve, and that it can be removed from the list of the few influential proton radiative captures reactions having a strong impact on the light curve.

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arXiv2021

Using spin alignment of inelastically-excited fast beams to make spin assignments: the spectroscopy of 13O as a test case

Excited states in 13O were investigated using inelastic scattering of an E/A=69.5-MeV 13O beam off of a 9Be target. The excited states were identified in the invariant-mass spectra of the decay products. Both single proton and sequential two-proton decays of the excited states were examined. For a number of the excited states, the protons were emitted with strong anisotropy where emissions transverse to the beam axis are favored. The measured proton-decay angular distributions were compared to predictions from distorted-wave born-approximation (DWBA) calculations of the spin alignment which was shown to be largely independent of the excitation mechanism. The deduced $^{13}$O level scheme is compared to ab initio no-core shell model with continuum (NCSMC) predictions. The lowest-energy excited states decay isotropically consistent with predictions of strong proton 1s1/2 structure. Above these states in the level scheme, we observed a number of higher-spin states not predicted within the model. Possibly these are associated with rotational bands built on deformed cluster configurations predicted by antisymmetrized molecular dynamics (AMD) calculations. The spin alignment mechanism is shown to be useful for making spin assignments and may have widespread use.

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arXiv2021

Persistence of the ${Z=28}$ shell gap in ${A=75}$ isobars: Identification of a possible ${(1/2^-)}$ $μ$s isomer in ${^{75}}$Co and $β$ decay to ${^{75}}$Ni

Background: The evolution of shell structure around doubly magic exotic nuclei is of great interest in nuclear physics and astrophysics. In the `southwest' region of $^{78}$Ni, the development of deformation might trigger a major shift in our understanding of explosive nucleosynthesis. To this end, new spectroscopic information on key close-lying nuclei is very valuable. Purpose: We intend to measure the isomeric and $β$ decay of $^{75}$Co, with one-proton and two-neutron holes relative to $^{78}$Ni, to access new nuclear structure information in $^{75}$Co and its $β$-decay daughters $^{75}$Ni and $^{74}$Ni. Methods: The nucleus $^{75}$Co is produced in relativistic in-flight fission reactions of $^{238}$U at the Radioactive Ion Beam Factory in the RIKEN Nishina Center. Its isomeric and $β$ decay are studied exploiting the BigRIPS and EURICA setups. Results: We obtain partial $β$-decay spectra for $^{75}$Ni and $^{74}$Ni, and report a new isomeric transition in $^{75}$Co. The energy [$E_γ=1914(2)$ keV] and half-life [$t_{1/2}=13(6)$ $μ$s] of the delayed $γ$ ray lend support for the existence of a $J^π=(1/2^-)$ isomeric state at 1914(2) keV. A comparison with PFSDG-U shell-model calculations provides a good account for the observed states in $^{75}$Ni, but the first calculated $1/2^-$ level in $^{75}$Co, a prolate $K=1/2$ state, is predicted about 1 MeV below the observed $(1/2^-)$ level. Conclusions: The spherical-like structure of the lowest-lying excited states in $^{75}$Ni is proved. In the case of $^{75}$Co, the results suggest that the dominance of the spherical configurations over the deformed ones might be stronger than expected below $^{78}$Ni. Further experimental efforts to discern the nature of the $J^π=(1/2^-)$ isomer are necessary.

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arXiv2021

Neutron-proton pairing in the N=Z radioactive fp-shell nuclei 56Ni and 52Fe probed by pair transfer

The isovector and isoscalar components of neutron-proton pairing are investigated in the N=Z unstable nuclei of the \textit{fp}-shell through the two-nucleon transfer reaction (p,$^3$He) in inverse kinematics. The combination of particle and gamma-ray detection with radioactive beams of $^{56}$Ni and $^{52}$Fe, produced by fragmentation at the GANIL/LISE facility, made it possible to carry out this study for the first time in a closed and an open-shell nucleus in the \textit{fp}-shell. The transfer cross-sections for ground-state to ground-state (J=0$^+$,T=1) and to the first (J=1$^+$,T=0) state were extracted for both cases together with the transfer cross-section ratios $σ$(0$^+$,T=1) /$σ$(1$^+$,T=0). They are compared with second-order distorted-wave born approximation (DWBA) calculations. The enhancement of the ground-state to ground-state pair transfer cross-section close to mid-shell, in $^{52}$Fe, points towards a superfluid phase in the isovector channel. For the "deuteron-like" transfer, very low cross-sections to the first (J=1$^+$,T=0) state were observed both for \Ni\phe\, and \Fe\phe\, and are related to a strong hindrance of this channel due to spin-orbit effect. No evidence for an isoscalar deuteron-like condensate is observed.

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arXiv2021

Probing the Symmetry Energy with the Spectral Pion Ratio

Many neutron star (NS) properties, such as the proton fraction within a NS, reflect the symmetry energy contributions to the Equation of State that dominate when neutron and proton densities differ strongly. To constrain these contributions at supra-saturation densities, we measure the spectra of charged pions produced by colliding rare isotope tin (Sn) beams with isotopically enriched Sn targets. Using ratios of the charged pion spectra measured at high transverse momenta, we deduce the slope of the symmetry energy to be $42 < L < 117$ MeV. This value is slightly lower but consistent with the $L$ values deduced from a recent measurement of the neutron skin thickness of $^{208}$Pb.

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arXiv2021

Probing nuclear forces beyond the nuclear drip line: The cases of $^{16}$F and $^{15}$F

The unbound proton-rich nuclei $^{16}$F and $^{15}$F are investigated experimentally and theoretically. Several experiments using the resonant elastic scattering method were performed at GANIL with radioactive beams to determine the properties of the low lying states of these nuclei. Strong asymmetry between $^{16}$F-$^{16}$N and $^{15}$F-$^{15}$C mirror nuclei is observed. The strength of the $nucleon-nucleon$ effective interaction involving the loosely bound proton in the $s_{1/2}$ orbit is significantly modified with respect to their mirror nuclei $^{16}$N and $^{15}$C. The reduction of the effective interaction is estimated by calculating the interaction energies with a schematic zero-range force. It is found that, after correcting for the effects due to changes in the radial distribution of the single-particle wave functions, the mirror symmetry of the $n-p$ interaction is preserved between $^{16}$F and $^{16}$N, while a difference of 63\% is measured between the $p-p$ versus $n-n$ interactions in the second excited state of $^{15}$F and $^{15}$C nuclei. Several explanations are proposed.

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arXiv2020

Symmetry energy investigation with pion production from Sn+Sn systems

In the past two decades, pions created in the high density regions of heavy ion collisions have been predicted to be sensitive at high densities to the symmetry energy term in the nuclear equation of state, a property that is key to our understanding of neutron stars. In a new experiment designed to study the symmetry energy, the multiplicities of negatively and positively charged pions have been measured with high accuracy for central $^{132}$Sn+$^{124}$Sn, $^{112}$Sn+$^{124}$Sn, and $^{108}$Sn+$^{112}$Sn collisions at $E/A=270~\mathrm{MeV}$ with the S$π$RIT Time Projection Chamber. While the uncertainties of individual pion multiplicities are measured to 4\%, those of the charged pion multiplicity ratios are measured to 2\%. We compare these data to predictions from seven major transport models. The calculations reproduce qualitatively the dependence of the multiplicities and their ratios on the total neutron to proton number in the colliding systems. However, the predictions of the transport models from different codes differ too much to allow extraction of reliable constraints on the symmetry energy from the data. This finding may explain previous contradictory conclusions on symmetry energy constraints obtained from pion data in Au+Au system. These new results call for better understanding of the differences among transport codes, and new observables that are more sensitive to the density dependence of the symmetry energy.

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arXiv2020

Low-lying single-particle structure of 17C and the N = 14 sub-shell closure

The first investigation of the single-particle structure of the bound states of 17C, via the d(16C, p) transfer reaction, has been undertaken. The measured angular distributions confirm the spin-parity assignments of 1/2+ and 5/2+ for the excited states located at 217 and 335 keV, respectively. The spectroscopic factors deduced for these states exhibit a marked single-particle character, in agreement with shell model and particle-core model calculations, and combined with their near degeneracy in energy provide clear evidence for the absence of the N = 14 sub-shell closure. The very small spectroscopic factor found for the 3/2+ ground state is consistent with theoretical predictions and indicates that the ν1d3/2 strength is carried by unbound states. With a dominant l = 0 valence neutron configuration and a very low separation energy, the 1/2+ excited state is a one-neutron halo candidate.

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arXiv2020

Bayesian Analysis of the $^{70}$Zn$(d, ^3\!\text{He}) ^{69}$Cu Transfer Reaction

Transfer reactions provide information about the single-particle nature of nuclear levels. In particular, the differential cross sections from these measurements are sensitive to the angular momentum of the transferred particle and the spectroscopic factor of the populated level. However, the process of extracting these properties is subject to uncertainties, both from experimental and theoretical sources. By integrating the distorted wave Born approximation into a Bayesian model, we propagate these uncertainties through to the spectroscopic factors and orbital angular momentum values. We use previously reported data of the proton pickup reaction $^{70}$Zn$(d, ^3\!\text{He}) ^{69}$Cu as an example. By accounting for uncertainties in the experimental data, optical model parameters, and reaction mechanism, we find that the extracted spectroscopic factors for low lying states of $^{69}$Cu are subject to large, asymmetric uncertainties ranging from $35 \%$ to $108 \%$. Additionally, Bayesian model comparison is employed to assign probabilities to each of the allowed angular momentum transfers. This method confirms the assignments for many states, but suggests that the data for a state lying at $3.70$ MeV is better characterized by an $\ell = 3$ transfer, rather than the previously reported $\ell = 2$.

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arXiv2020

Scission configuration of $^{239}$U from yields and kinetic information of fission fragments

The simultaneous measurement of the isotopic fission-fragment yields and fission-fragment velocities of $^{239}$U has been performed for the first time. The $^{239}$U fissioning system was produced in one-neutron transfer reactions between a $^{238}$U beam at 5.88 MeV/nucleon and a $^{9}$Be target. The combination of inverse kinematics at low energy and the use of the VAMOS++ spectrometer at the GANIL facility allows the isotopic identification of the full fission-fragment distribution and their velocity in the reference frame of the fissioning system. The proton and neutron content of the fragments at scission, their total kinetic and total excitation energy, as well as the neutron multiplicity were determined. Information from the scission point configuration is obtained from these observables and the correlation between them. The role of the octupole-deformed proton and neutron shells in the fission-fragment production is discussed.

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arXiv2020

Particle decays of levels in $^{11,12}$N and $^{12}$O investigated with the invariant-mass method

Particle-decaying states of the light nuclei $^{11,12}$N and $^{12}$O were studied using the invariant-mass method. The decay energies and intrinsic widths of a number of states were measured, and the momentum correlations of three-body decaying states were considered. A second 2$p$-decaying 2$^+$ state of $^{12}$O was observed for the first time, and a higher energy $^{12}$O state was observed in the 4$p$+2$α$ decay channel. This 4$p$+2$α$ channel also contains contributions from fission-like decay paths, including $^6$Be$_{g.s.}$+$^{6}$Be$_{g.s.}$. Analogs to these states in $^{12}$O were found in $^{12}$N in the 2$p$+$^{10}$B and 2$p$+$α$+$^6$Li channels. The momentum correlations for the prompt 2$p$ decay of $^{12}$O$_{g.s.}$ were found to be nearly identical to those of $^{16}$Ne$_{g.s.}$, and the correlations for the new 2$^+$ state were found to be consistent with sequential decay through excited states in $^{11}$N. The momentum correlations for the 2$^+_1$ state in $^{12}$O provide a new value for the $^{11}$N ground-state energy. The states in $^{12}$N/$^{12}$O that belong to the $A$=12 isobaric sextet do not deviate from the quadratic isobaric multiplet mass equation (IMME) form.

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arXiv2019

Prompt Fission Neutrons in the $^{239}$Pu($n,f$) Reaction

Prompt fission neutron spectra from $^{239}$Pu($n,f$) were measured for incident neutron energies from $0.7$ to $700\,$MeV at the Weapons Neutron Research facility (WNR) of the Los Alamos Neutron Science Center. A newly designed high-efficiency fission chamber was coupled to the highly segmented Chi-Nu array to detect neutrons emitted in fission events. The double time-of-flight technique was used to deduce the incident-neutron energies from the spallation target and the outgoing-neutron energies from the fission chamber. Prompt fission neutron spectra (PFNS) were measured with respect to $^{252}$Cf spontaneous fission down to $200\,$keV and up to about $12\,$MeV for all the incident neutron energies with typical uncertainties well below $2\%$ up to about $10\,$MeV outgoing-neutron energy. The general trend of PFNS is well reproduced by JEFF3.3 and ENDF-B\VIII.0 evaluations. Discrepancies were however observed for the low-energy part of the spectra, where evaluations overestimate the number of emitted neutrons. Neutron multiplicities and average kinetic energies as a function of incident-neutron energy are obtained experimentally with reported uncertainties below $0.4\%$. Neutron multiplicities disagree with some older datasets above $6\,$ MeV, indicating the need of using a high-efficiency fission detector, which does not bias the data. The measured mean kinetic energies agree with the most recent data. Evaluations fairly reproduce the trend, but fail to reproduce the experimental values within their uncertainties.

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arXiv2019

First direct measurement of isotopic fission-fragment yields of $^{239}$U

A direct and complete measurement of isotopic fission-fragment yields of $^{239}$U has been performed for the first time. The $^{239}$U fissioning system was produced with an average excitation energy of 8.3 MeV in one-neutron transfer reactions between a $^{238}$U beam and a $^{9}$Be target at Coulomb barrier energies. The fission fragments were detected and isotopically identified using the VAMOS++ spectrometer at the GANIL facility. This measurement allows to directly evaluate the fission models at excitation energies of fast neutrons, relevant for next-generation nuclear reactors. The present data, in agreement with model calculations, do not support the recently reported anomaly in the fission-fragment yields of $^{239}$U and confirm the persistence of spherical shell effects in the Sn region at excitation energies exceeding the fission barrier by few MeV.

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arXiv2019

Normal and intruder configurations in $^{34}$Si populated in the $β^-$ decay of $^{34}$Mg and $^{34}$Al

The structure of $^{34}$Si was studied through $γ$ spectroscopy separately in the $β^-$ decays of $^{34}$Mg and $^{34}$Al at the ISOLDE facility of CERN. Different configurations in $^{34}$Si were populated independently from the two recently identified $β$-decaying states in $^{34}$Al having spin-parity assignments $J^π= 4^-$ dominated by the normal configuration $π(d_{5/2})^{-1} \otimes ν(f_{7/2})$ and $J^π= 1^+$ by the intruder configuration $π(d_{5/2})^{-1} \otimes ν(d_{3/2})^{-1}(f_{7/2})^{2}$. The paper reports on spectroscopic properties of $^{34}$Si such as an extended level scheme, spin and parity assignments based on log($ft$) values and $γ$-ray branching ratios, absolute $β$ feeding intensities and neutron emission probabilities. A total of 11 newly identified levels and 26 transitions were added to the previously known level scheme of $^{34}$Si. Large scale shell-model calculations using the {\sc sdpf-u-mix} interaction, able to treat higher order intruder configurations, are compared with the new results and conclusions are drawn concerning the predictive power of {\sc sdpf-u-mix}, the $N=20$ shell gap, the level of mixing between normal and intruder configurations for the 0$_1^+$, 0$_2^+$ and 2$_1^+$ states and the absence of triaxial deformation in $^{34}$Si.

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arXiv2019

Constraining the symmetry energy with heavy-ion collisions and Bayesian analyses

Efficiency corrected single ratios of neutron and proton spectra in central $^{112}$Sn+$^{112}$Sn and $^{124}$Sn+$^{124}$Sn collisions at 120 MeV/u are combined with double ratios to provide constraints on the density and momentum dependencies of the isovector mean-field potential. Bayesian analyses of these data reveal that the isoscalar and isovector nucleon effective masses, $m_s^* - m_v^*$ are strongly correlated. The linear correlation observed in $m_s^* - m_v^*$ yields a nearly independent constraint on the effective mass splitting $Δm_{np}^*= (m_n^*-m_p^*)/m_N = -0.05_{-0.09}^{+0.09}δ$. The correlated constraint on the standard symmetry energy, $S_0$ and the slope, $L$ at saturation density yields the values of symmetry energy $S(ρ_s)=16.8_{-1.2}^{+1.2}$ MeV at a sensitive density of $ρ_s/ρ_0 = 0.43_{-0.05}^{+0.05}$.

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arXiv2019

Non-linearity effects on the light-output calibration of light charged particles in CsI(Tl) scintillator crystals

The light output produced by light ions (Z<=4) in CsI(Tl) crystals is studied over a wide range of detected energies (E<=300 MeV). Energy-light calibration data sets are obtained with the 10 cm crystals in the recently upgraded High-Resolution Array (HiRA10). We use proton recoil data from 40,48Ca + CH2 at 28 MeV/u, 56.6 MeV/u, 39 MeV/u and 139.8 MeV/u and data from a dedicated experiment with direct low-energy beams. We also use the punch through points of p, d, and t particles from 40,48Ca + 58,64Ni, 112,124Sn collisions reactions at 139.8 MeV/u. Non-linearities, arising in particular from Tl doping and light collection efficiency in the CsI crystals, are found to significantly affect the light output and therefore the calibration of the detector response for light charged particles, especially the hydrogen isotopes. A new empirical parametrization of the hydrogen light output, L(E,Z=1,A), is proposed to account for the observed effects. Results are found to be consistent for all 48 CsI(Tl) crystals in a cluster of 12 HiRA10 telescopes.

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