arXiv subjects

P. Moroshkin

Publications and source records attributed to P. Moroshkin.

10 recordsLinked to original sources

arXiv2018

Zero-phonon lines in the spectra of dysprosium atoms in superfluid helium

We present an experimental study of a zero-phonon line (ZPL) in the absorption spectrum of Dy atoms solvated in superfluid He. The dopants reside in nanometer-sized spherical cavities known as atomic bubbles. We observe a temperature-dependent broadening of ZPL in the absorption spectrum. The effect is attributed to the scattering of thermal phonons on the atomic bubble that leads to the dephasing of the Dy transition dipole. The extrapolated ZPL intrinsic spectral width at zero temperature is 2300 times larger than the natural linewidth in a free atom. This can be assigned to a fast radiationless quenching of the upper state of the studied transition.

physics.chem-ph↗

arXiv2018

Dynamics of fine particles due to quantized vortices on the surface of superfluid $^4$He

Peculiar dynamics of a free surface of the superfluid 4He has been observed experimentally with a newly established technique utilizing a number of electrically charged fine metal particles trapped electrically at the surface by Moroshkin et al. They have reported that some portion of the particles exhibit some irregular motions and suggested the existence of quantized vortices interacting with the metal particles. We have conducted calculations with the vortex filament model, which turns out to support the idea of the vortex-particle interactions. The observed anomalous metal particle motions are roughly categorized into two types; (1) circular motions with specific frequencies, and (2) quasi-linear oscillations. The former ones seem to be explained once we consider a vertical vortex filament whose edges are terminated at the bottom and at a particle trapped at the surface. Although it is not yet clear whether all the anomalous motions are due to the quantum vortices, the vortices seem to play important roles for the motions.

cond-mat.other↗

arXiv2018

Dynamics of the vortex-particle complexes bound to the free surface of superfluid helium

We present an experimental and theoretical study of the 2D dynamics of electrically charged nanoparticles trapped under a free surface of superfluid helium in a static vertical electric field. We focus on the dynamics of particles driven by the interaction with quantized vortices terminating at the free surface. We identify two types of particle trajectories and the associated vortex structures: vertical linear vortices pinned at the bottom of the container and half-ring vortices travelling along the free surface of the liquid.

cond-mat.other↗

arXiv2007

Dependence of Resonant Absorption Linewidth on Atomic Vapour Column Thickness for D1 Line of Cs Atoms Confined in Nano-Cell

A new nano-cell with smoothly varying longitudinal thickness of the atomic vapour layer L in the range of 350 - 5100 nm allowing to study the resonant absorption of D1 and D2 lines of Cs atoms for thicknesses changing from L = Lambda/2 to L = 6 Lambda with the step of Lambda/2 (Lambda = 852 nm or 894 nm are the resonant laser wavelengths) and for different intensities is developed. It is revealed that for low laser intensities there is narrowing of the resonant absorption spectrum for the thicknesses L = (2n + 1)Lambda/2 (where n is an integer) up to L = 7Lambda /2 and broadening of the spectrum for L = n Lambda. For relatively high laser intensity (>1 mW/cm2), velocity selective optical pumping/saturated resonances of a reduced absorption (with the line-width close to the natural one), and centred on the hyperfine transitions occur when L = n Lambda. The possible application of these resonance peaks is given. The developed theoretical model describes well the experiment.

physics.atom-ph↗

arXiv2007

Saturated absorption spectroscopy: elimination of crossover resonances by use of a nanocell

It is demonstrated that velocity selective optical pumping/saturation resonances of reduced absorption in a Rb vapor nanocell with thickness \textit{L=} $λ$, 2$λ$, and 3$λ$ (resonant wavelength $λ$ = 780 nm) allow the complete elimination of crossover (CO) resonances. We observe well pronounced resonances corresponding to the F$_{g}=3$ $\to $ F$_{e}=2,3,4$ hyperfine transitions of the $^{85}$Rb D$_{2}$ line with linewidths close to the natural width. A small CO resonance located midway between F$_{g}=3$ $\to $ F$_{e}=3$ and F$_{g}=3$ $\to$ F$_{e}=4$ transitions appears only for \textit{L} = 4$λ$. The D$_{2}$ line ($λ$ = 852 nm) in a Cs nanocell exhibits a similar behavior. From the amplitude ratio of the CO and VSOP resonances it is possible to determine the thickness of the column of alkali vapor in the range of 1 - 1000 $μ$m. The absence of CO resonances for nanocells with $L \sim λ$ is attractive for frequency reference application and for studying transitions between Zeeman sublevels in external magnetic fields.

physics.class-ph↗

arXiv2006

Reconciliation of experimental and theoretical electric tensor polarizabilities of the cesium ground state

We present a new theoretical analysis of the strongly suppressed F- and M-dependent Stark shifts of the Cs ground state hyperfine structure. Our treatment uses third order perturbation theory including off-diagonal hyperfine interactions not considered in earlier treatments. A numerical evaluation of the perturbation sum using bound states up to n=200 yields ground state tensor polarizabilities which are in good agreement with experimental values, thereby bridging the 40-year-old gap between experiments and theory. We have further found that the tensor polarizabilities of the two ground state hyperfine manifolds have opposite signs, in disagreement with an earlier derivation. This sign error has a direct implication for the precise evaluation of the blackbody radiation shift in primary frequency standards.

physics.atom-ph↗

arXiv2006

Spectroscopy of Rb$_{2}$ dimers in solid $^{4}$He

We present experimental and theoretical studies of the absorption, emission and photodissociation spectra of Rb$_{2}$ molecules in solid helium. We have identified 11 absorption bands of Rb$_{2}$. All laser-excited molecular states are quenched by the interaction with the He matrix. The quenching results in efficient population of a metastable (1)$^{3}Π_{u}$ state, which emits fluorescence at 1042 nm. In order to explain the fluorescence at the forbidden transition and its time dependence we propose a new molecular exciplex Rb$_{2}(^{3}Π_{u})$He$_{2}$. We have also found evidence for the formation of diatomic bubble states following photodissociation of Rb$_{2}$.

physics.atom-ph↗

arXiv2006

Stark effect of the cesium ground state: electric tensor polarizability and shift of the clock transition frequency

We present a theoretical analysis of the Stark effect in the hyperfine structure of the cesium ground-state. We have used third order perturbation theory, including diagonal and off-diagonal hyperfine interactions, and have identified terms which were not considered in earlier treatments. A numerical evaluation using perturbing levels up to n=18 yields new values for the tensor polarizability $α_2(6S_{1/2})$ and for the Stark shift of the clock transition frequency in cesium. The polarizabilities are in good agreement with experimental values, thereby removing a 40-year-old discrepancy. The clock shift value is in excellent agreement with a recent measurement, but in contradiction with the commonly accepted value used to correct the black-body shift of primary frequency standards.

physics.atom-ph↗

arXiv2006

Rb*He_n exciplexes in solid 4_He

We report the observation of emission spectra from Rb*He_n exciplexes in solid 4He. Two different excitation channels were experimentally identified, viz., exciplex formation via laser excitation to the atomic 5P3/2 and to the 5P1/2 levels. While the former channel was observed before in liquid helium, on helium nanodroplets and in helium gas by different groups, the latter creation mechanism occurs only in solid helium or in gaseous helium above 10 Kelvin. The experimental results are compared to theoretical predictions based on the extension of a model, used earlier by us for the description of Cs*He_n exciplexes. We also report the first observation of fluorescence from atomic rubidium in solid helium, and discuss striking differences between the spectroscopic feature of Rb-He and Cs-He systems.

physics.atom-ph↗

arXiv2004

Discovery of dumbbell-shaped Cs*He_n exciplexes in solid He 4

We have observed several new spectral features in the fluorescence of cesium atoms implanted in the hcp phase of solid helium following laser excitation to the 6$^{2}$P states. Based on calculations of the emission spectra using semiempirical Cs-He pair potentials the newly discovered lines can be assigned to the decay of specific Cs*He$_{n}$ exciplexes: an apple-shaped Cs$(AΠ_{3/2})$He$_{2}$ and a dumbbell-shaped Cs$(AΠ_{1/2}) $He$_{n}$ exciplex with a well defined number $n$ of bound helium atoms. While the former has been observed in other enviroments, it was commonly believed that exciplexes with $n>2$ might not exist. The calculations suggest Cs$(AΠ_{1/2}) $He$_{6}$ to be the most probable candidate for that exciplex, in which the helium atoms are arranged on a ring around the waist of the dumbbell shaped electronic density distribution of the cesium atom.

physics.atm-clus↗