arXiv subjects

P. O. Kapralov

Publications and source records attributed to P. O. Kapralov.

5 recordsLinked to original sources

arXiv2024

Asymmetric Faraday effect caused by a break of spatial symmetry

It is widely known that the magneto-optical Faraday effect is linear in magnetization, and therefore the Faraday angles for the states with opposite magnetizations are of opposite sign but equal in modulus. Here we demonstrate that under certain spatial symmetry-breaking conditions, an asymmetric Faraday effect (AFE) arises, meaning that the Faraday angles for opposite magnetic states differ not only in sign but in absolute value as well. Experimental investigations of AFE are performed in a one-dimensional all-garnet magnetophotonic crystal, where AFE appears in the vicinity of the cavity resonance for an oblique incidence of light with an inclined light polarization plane. The magnitude of the observed asymmetry between Faraday rotations for the two opposite magnetizations is very large and reaches 30$\%$ of the absolute value of the Faraday effect. We confirm the generality of the suggested effect by the numerical analysis of several different configurations in which AFE arises. The discovered AFE is of prime importance for nanoscale magnonics and optomagnetism.

physics.optics↗

arXiv2022

Birefringence-mediated enhancement of the magneto-optical activity in anisotropic magnetic crystals

Optical anisotropy is usually treated as an unfavorable condition for the magneto-optical measurements since it is known to diminish the Faraday rotation concerning the case of the isotropic medium. Here we show that the situation could be quite opposite: a phenomenon of birefringence mediated enhancement of the magneto-optical activity appears if the incident light polarization and angle of incidence are set properly. The present study relies on the experimental, analytical, and numerical studies of iron borate $\mathrm{FeBO_3}$ crystals. We demonstrate a significant increase of the magneto-optical activity resulting in nearly $100\%$ magneto-optical light modulation magnitude. The approach applies to other types of birefringent crystals with the magneto-optical response that makes it crucial for various practical applications, including magneto-optical microscopy, pump-probe studies, and others.

physics.optics↗

arXiv2021

Valley polarization of trions in monolayer MoSe$_2$ interfaced with bismuth iron garnet

Interfacing atomically thin van der Waals semiconductors with magnetic substrates enables additional control on their intrinsic valley degree of freedom and provides a promising platform for the development of novel valleytronic devices for information processing and storage. Here we study circularly polarized photoluminescence in heterostructures of monolayer MoSe$_2$ and thin films of ferrimagnetic bismuth iron garnet. We observe strong emission from charged excitons with negative valley polarization, which switches sign with increasing temperature, and demonstrate contrasting response to left and right circularly polarized excitation, associated with finite out-of-plane magnetization in the substrate. We propose a theoretical model accounting for magnetization-induced imbalance of charge carriers in the two valleys of MoSe$_2$, as well as for valley-switching scattering from B to A excitons and fast formation of trions with extended valley relaxation times, which shows excellent agreement with the experimental data. Our results provide new insights into valley physics in 2D semiconductors interfaced with magnetic substrates.

cond-mat.mes-hall↗

arXiv2020

Non-rotational mechanism of polarization in alcohols

Chemical polarity governs various mechanical, chemical and thermodynamic properties of dielectrics. Polar liquids have been amply studied, yet the basic mechanisms underpinning their dielectric properties remain not fully understood, as standard models following Debye's phenomenological approach do not account for quantum effects and cannot aptly reproduce the full dc-up-to-THz spectral range. Here, using the illustrative case of monohydric alcohols, we show that deep tunneling and the consequent intermolecular separation of excess protons and "proton-holes" in the polar liquids govern their static and dynamic dielectric properties on the same footing. We performed systematic ultrabroadband (0-10 THz) spectroscopy experiments with monohydric alcohols of different (0.4-1.6 nm) molecular lengths, and show that the finite lifetime of molecular species, and the proton-hole correlation length are the two principle parameters responsible for the dielectric response of all the studied alcohols across the entire frequency range. Our results demonstrate that a quantum non-rotational intermolecular mechanism drives the polarization in alcohols while the rotational mechanism of molecular polarization plays a secondary role, manifesting itself in the sub-terahertz region only.

physics.chem-ph↗

arXiv2020

Nanophotonic structures with optical surface modes for tunable spin current generation

Heat generated by spin currents in spintronics-based devices is typically much less than that generated by charge current flows in conventional electronic devices. However, the conventional approaches for excitation of spin currents based on spin-pumping and spin Hall effect are limited in efficiency which restricts their application for viable spintronic devices. We propose a novel type of photonic-crystal (PC) based structures for efficient and tunable optically-induced spin current generation via the Spin Seebeck and inverse spin Hall effects. It is experimentally demonstrated that optical surface modes localized at the PC surface covered by ferromagnetic layer and materials with giant spin-orbit coupling (SOC) notably increase the efficiency of the optically-induced spin current generation and provides its tunability by modifying light wavelength or angle of incidence. Up to 100% of the incident light power can be transferred to heat within the SOC layer and, therefore, to spin current. Importantly, high efficiency becomes accessible even for ultra-thin SOC layers. Moreover, surface patterning of the PC-based spintronic nanostructure allows local generation of spin currents at the pattern scales rather than diameter of the laser beam.

cond-mat.mes-hall↗