arXiv subjects

P. Padhan

Publications and source records attributed to P. Padhan.

17 recordsLinked to original sources

arXiv2014

Raman spectra and Magnetization of all-ferromagnetic superlattices grown on (110) oriented SrTiO3

Superlattices consist of two ferromagnets La0.7Sr0.3MnO3(LSMO)and SrRuO3(SRO) were grown in (110)-orientation on SrTiO3(STO) substrates. The x-ray diffraction and Raman spectra of these superlattices show the presence of in-plane compressive strain and orthorhombic structure of less than 4 u.c. thick LSMO spacer,respectively. Magnetic measurements reveal several features including reduced magnetization, enhanced coercivity, antiferromagnetic coupling, and switching from antiferromagnetic to ferromagnetic coupling with magnetic field orientations. These magnetic properties are explained by the observed orthorhombic structure of spacer LSMO in Raman scattering which occurs due to the modification in the stereochemistry of Mn at the interfaces of SRO and LSMO.

cond-mat.mtrl-sci↗

arXiv2012

Electronic structure and optical band gap of CoFe2O4 thin films

Electronic structure and optical band gap of CoFe2O4 thin films grown on (001) oriented LaAlO3 have been investigated. Surprisingly, these films show additional Raman modes at room temperature as compared to a bulk spinel structure. The splitting of Raman modes is explained by considering the short-range ordering of Co and Fe cations in octahedral site of spinel structure. In addition, an expansion of band-gap is observed with the reduction of film thickness, which is explained by the quantum size effect and misfit dislocation. Such results provide interesting insights for the growth of spinel phases.

cond-mat.mtrl-sci↗

arXiv2010

Magnetocaloric effect and improved relative cooling power in (La0.7Sr0.3MnO3/SrRuO3) superlattices

Magnetic properties of a series of (La0.7Sr0.3MnO3/SrRuO3) superlattices, where the SrRuO3 layer thickness is varying, are examined. A room-temperature magnetocaloric effect is obtained owing to the finite size effect which reduces the TC of La0.7Sr0.3MnO3 layers. While the working temperature ranges are enlarged,, -DeltaSmax values remains similar to the values in polycrystalline La0.7Sr0.3MnO3. Consequently, the relative cooling powers are significantly improved, the microscopic mechanism of which is related to the effect of the interfaces at La0.7Sr0.3MnO3/SrRuO3 and higher nanostructural disorder. This study indicates that artificial oxide superlattices/multilayers might provide an alternative pathway in searching for efficient room-temperature magnetic refrigerators for (nano)microscale systems.

cond-mat.mtrl-sci↗

arXiv2010

Tunable magnetic interaction at the atomic scale in oxide heterostructures

We report on a systematic study of a number of structurally identical but chemically distinct transition metal oxides in order to determine how the material-specific properties such as the composition and the strain affect the properties at the interface of heterostructures. Our study considers a series of structures containing two layers of ferromagnetic SrRuO3, with antiferromagnetic insulating manganites sandwiched in between. The results demonstrate how to control the strength and relative orientation of interfacial ferromagnetism in correlated electron materials by means of valence state variation and substrate-induced strain, respectively.

cond-mat.mtrl-sci↗

arXiv2010

Anisotropic magnetocaloric effect in all-ferromagnetic (La0.7Sr0.3MnO3/SrRuO3) superlattices

We exploit the magnetic interlayer coupling in La0.7Sr0.3MnO3/SrRuO3 superlattices to realize a crossover between inverse and conventional magnetic entropy changes. Our data reveal a strong anisotropic nature of the magnetocaloric effect due to the magnetic anisotropy of the superlattice. Therefore, artificial superlattices built from ferromagnetic materials that can be used to alter the magnetic structure as well as the magnetic anisotropy, could also be utilized for tuning the magnetocaloric properties, which may open a constructive approach for magnetic refrigeration applications.

cond-mat.mtrl-sci↗

arXiv2007

Anomalous exchange coupling in transition-metal-oxide based superlattices with antiferromagnetic spacer layers

A direct correlation is seen between the coercive field (HC) and the magnetic-field-dependent resistivity (MR) in SrMnO3/SrRuO3 superlattices of perpendicular magnetic anisotropy. The magnetoresistance shows a sharp jump at Hc for in-plane current and the out-of-plane magnetic field. Both HC and high-field MR also oscillate with the thickness of the SrMnO3 spacer layers separating the metallic ruthenate. Since the spacer in these superlattices has no mobile carriers to facilitate an oscillatory coupling, we attribute the observed behavior to the spin-polarized quantum tunneling of electrons between the ferromagnetic layers and antiferromagnetically ordered t2g spins of SrMnO3.

cond-mat.str-el↗

arXiv2006

Antiferromagnetic coupling and enhanced magnetization in all-ferromagnetic superlattices

The structural and magnetic properties of a series of superlattices consisting of two ferromagnetic metals La$_{0.7}$Sr$_{0.3}$MnO$_3$ (LSMO) and SrRuO$_3$ (SRO) grown on (001) oriented SrTiO$_3$ are studied. Superlattices with a fixed LSMO layer thickness of 20 unit cells (u.c.) and varying SRO layer thickness show a sudden drop in magnetization on cooling through temperature where both LSMO and SRO layers are ferromagnetic. This behavior suggests an antiferromagnetic coupling between the layers. In addition, the samples having thinner SRO layers (n \TEXTsymbol{<} 6) exhibit enhanced saturation magnetization at 10 K. These observations are attributed to the possible modification in the stereochemistry of the Ru and Mn ions in the interfacial region.

cond-mat.mtrl-sci↗

arXiv2005

Effect of electric/magnetic field on pinned/biased moments at the interfaces of magnetic superlattices

We have observed the pinned/biased moments in the superlattices consisting of ferromagnetic (FM) SrRuO3 (SRO) and antiferromagnetic (AFM) SrMnO3 (SMO)bilayer. The alternate stacking of SRO and SMO leading to a low field positive magnetoresistance with enhanced hysteretic field dependent magnetoresistance under the application of the out-of-plane magnetic field. We attribute these effects to the observed biased/pinned magnetic moments in the SRO layer in the vicinity of the interfaces. In addition, the biased/pinned moments can be oriented under the application of either the out-of-plane magnetic field or a combination of out-of-plane magnetic field and in-plane electric field. These results will bring new insights in the understanding of the coupling at the AFM/FM interface which can be useful for creating new exotic phenomena at the interfaces of the multilayer.

cond-mat.str-el↗

arXiv2005

Effect of strain on the electrical transport and magnetization of the epitaxial Pr0.5Ca0.5MnO3/La0.5Ca0.5MnO3/ Pr0.5Ca0.5MnO3 trilayer structures

Epitaxial trilayer structures consisting of two antifferomagnetic charge/orbital order insulators Pr0.5Ca0.5MnO3 (PCMO) and La0.5Ca0.5MnO3 (LCMO) are grown on (001)-oriented SrTiO3 and LaAlO3 substrates. In this trilayer series, a thin film of LCMO with various thicknesses is sandwiched between the two fixed thicknesses of PCMO. These samples show a Curie temperature with a hysteretic field dependent magnetization at 10 K, although the individual compounds are antiferromagnetic. The zero field electronic transport of all samples on LAO shows thermally activated behavior, while the thermally activated behavior is suppressed and a metal-like transport is appearing for the samples on STO as the LCMO layer thickness increases above 10 unit cell. We have discussed these magnetic and transport properties of the trilayer structures on STO and LAO by the interfacial effect due to the stabilized CO state and the vibration mode of Jahn-Teller distortion.

cond-mat.mtrl-sci↗

arXiv2005

Direct observation of pinned/biased moments in magnetic superlattices

We report the \QTR{it}{pinned/biased} \QTR{it}{moment} in the superlattices consisting of ferromagnetic (FM) SrRuO$_3$ and antiferromgnetic (AFM) SrMnO$_3$. This superlattice system shows anisotropy and oriented pinning/biasing in the field-cooled (FC) hysteresis loop. The in-plane cooling-field provides antiferromagnetic orientations while out-of-plane cooling-field provides ferromagnetic orientations to the pinned/biased moments. The spacer layer thickness, strength and orientation of magnetic field, cooling field, and driving current influence the pinning strength. We propose that the magnetic structure is a repetition of $AFM/Pin/FM$($Free$)/$Pin$ unit below a critical field to explain its magnetic and transport properties. The transport behavior is discussed using the spin-dependent conduction.

cond-mat.str-el↗

arXiv2005

Ferromagnetism and metal-like transport in antiferromagnetic insulator heterostructures

Strained Pr$_{0.5}$Ca$_{0.5}$MnO$_3$/La$_{0.5}$Ca$_{0.5}$MnO$_3$/Pr$_{0.5}$Ca$_{0.5}$MnO $_3$ trilayers were grown on (001)-SrTiO$_3$ substrates using the pulsed-laser deposition technique. The coupling at the interfaces of several trilayers has been investigated from magnetization and electronic transport experiments. An increase of La$_{0.5}$Ca$_{0.5}$MnO$_3$ layer thickness induces a magnetic ordering in the strain layers and at the interfaces leading to ferromagnetic behavior and enhanced coercivity, while resistivity shows metal-like behaviors. These effects are not observed in the parent compounds, which are antiferromagnetic insulators, opening a path, to induce artificially some novel properties.

cond-mat.mtrl-sci↗

arXiv2005

Anisotropic pinned/biased magnetization in $SrRuO_3/SrMnO_3$ superlattices

The exchange coupling at the interfaces of magnetic superlattices consisting of ferromagnetic $SrRuO_3$ and antiferromagnetic $SrMnO_3$ grown on (001) oriented $SrTiO_3$ is studied with in-plane and out-of-plane orientations, with respect to the substrate plane, of the cooling magnetic field. The magnetization of the in-plane, field cooled hysteresis loop is lower than the corresponding in-plane zero-field-cooled hysteresis loop. The out-of-plane field cooled hysteresis loop is shifted, from the origin, along the graphical magnetization axis. We attribute this irreversible rotation of the moment to the pinning/biasing of spin in the $SrRuO_3$ layer in the vicinity of interfaces by the antiferromagnetic $SrMnO_3$ layer.

cond-mat.mtrl-sci↗

arXiv2005

Exchange coupling induced antiferromagnetic-ferromagnetic transition in $Pr_{0.5}Ca_{0.5}MnO_3/La_{0.5}Ca_{0.5}MnO_3$ superlattices

Superlattices built from two antiferromagnetic (AFM) charge/orbital order compounds, $Pr_{0.5}Ca_{0.5}MnO_3$ and $La_{0.5}Ca_{0.5}MnO_3$, have been studied as the thickness of $La_{0.5}Ca_{0.5}MnO_3$ ($LCMO$) varied. High structural quality thin films were obtained on $LaAlO_3$ substrates using the pulsed laser deposition technique. An antiferromagnetic-to-ferromagnetic transition, in addition to an enhancement of the coercivity, are observed as the $LCMO$ layer thickness increases. The small shift in the origin of the field-cooled hysteresis loop along the field axis indicates the presence of ferromagnetic and antiferromagnetic phases in the superlattices. We attribute these features to the AFM spin fluctuations at the $Pr_{0.5}Ca_{0.5}MnO_3/La_{0.5}Ca_{0.5}MnO_3$ interfaces resulting from the strain effects.

cond-mat.str-el↗

arXiv2004

Magnetotransport properties of ferromagnetic Pr0.85Ca0.15MnO3/ferroelectric Ba0.6Sr0.4TiO3 superlattice films

Artificial superlattices designed with ferromagnetic Pr0.85Ca0.15MnO3 insulating layer and ferroelectric Ba0.6Sr0.4TiO3 layer were grown on (100) SrTiO3 substrates. The magnetotransport properties were measured with the current perpendicular to the plane geometry. An increase in magnetoresistance (MR), with no significant low field effect, was observed as the number of ferroelectric Ba0.6Sr0.4TiO3 layer thickness increases even up to 9 unit cells. For example, the superlattice [(Pr0.85Ca0.15MnO3)10(Ba0.6Sr0.4TiO3)9]25 shows 35 % MR at 100 K, though the Pr0.85Ca0.15MnO3 film was a robust insulator with negligible MR even at high applied magnetic field. This observed large MR cannot be explained by simple interfacial ferromagnetism or by the tunneling magnetoresistance. One possible explanation could be the effect due to the ferroelectric spacer layer and the associated magnetoelectric coupling.

cond-mat.str-el↗

arXiv2004

Current-induced metallic behavior in Pr$_{0.5}$Ca$_{0.5}$MnO$_3$ thin films: competition between Joule heating and nonlinear conduction mechanism

Thin films of Pr0.5Ca0.5MnO3 manganites exhibiting charge/orbital-ordered properties with colossal magnetoresistance have been synthesized by the pulsed laser deposition technique on both (100)-SrTiO3 and (100)-LaAlO3 substrates. The effects of current-induced metallic-behavior of the films are investigated as a function of the temperature and the magnetic field. Calculations based on a heat transfer model across the substrate, and our resistivity measurements reveal effects of Joule heating on charge transport over certain ranges of temperatures and magnetic fields. Our results also indicate that a nonlinear conduction, which cannot be explained by homogeneous Joule heating of the film, is observed when the material is less resistive (10-2 W.cm). The origin of this behavior is explained with a model based on local thermal instabilities associated with phase-separation mechanism and a change in the long range charge-ordered state.

cond-mat.str-el↗

arXiv2004

Interfacial strain measurements in $SrRuO_3/SrMnO_3$ magnetic multilayers

Magnetic multilayers of $(SrRuO_3)_m(SrMnO_3)_n$ were grown artificially using the pulsed laser deposition technique on (001)-oriented $SrTiO_3$ substrates. The state of strain at the interfaces and the structural coherency are studied in details utilizing asymmetrical $X$-ray diffraction and the $\sin ^2ψ$ method. First, the evolution of the lattice parameters, the crystallinity and the epitaxy of the films are evaluated as a function of the number of $SrMnO_3$ unit cells using $X$-rays diffraction and transmission electron microscopy. Second, our results on the stress indicate that the $SrRuO_3/SrMnO_3$ superlattices show a larger residual strain as compared to the single layer film of $SrRuO_3$. This suggests that the lattice stiffening from interfacial strain and inhibiting the dislocation by composition modulation. Finally, these results bring insights on the interfacial stress measurements of oxide multilayers that can be used to control the physical properties at the level of the atomic scale.

cond-mat.str-el↗

arXiv2004

Structural and magnetic properties of a series of low doped Zn$_{1-x}$Co$_x$O thin films deposited from Zn and Co metal targets on (0001) Al$_2$O$_3$ substrates

We report on the synthesis of low doping Zn$_{1-x}$Co$_x$O ($0<x<0.1$) thin films on (0001)-Al$_2$O$_3$ substrates. The films were prepared in an oxidizing atmosphere, using the pulsed laser deposition technique starting from Zn and Co metallic targets. We first studied the influence of the strains of ZnO and their stuctural properties. Second, we have investigated the structural and the magnetic properties of the Zn$_{1-x}$Co$_x$O films. We show that at low doping, the lattice parameters and the magnetization of the Zn$_{1-x}$Co$_x$O films depend strongly on the Co concentration.

cond-mat.mtrl-sci↗