arXiv subjects

P. Pedrazzini

Publications and source records attributed to P. Pedrazzini.

16 recordsLinked to original sources

arXiv2024

Enhanced weak superconductivity in trigonal $γ$-PtBi$_2$

Electrical resistivity experiments show superconductivity at $T_c = 1.1\,$K in a high-quality single crystal of trigonal $γ$-PtBi$_2$, with an enhanced critical magnetic field $μ_0H_{c2}(0) \gtrsim 1.5\,$Tesla and a low critical current-density $J_c(0)\approx 40\,\mathrm{A}/\mathrm{cm}^2$ at $H=0$. Both $T_c$ and $H_{c2}(0)$ are the highest reported values for stoichiometric bulk samples at ambient pressure. We found a weak $H_{c2}$ anisotropy with $Γ=H_{c2}^{ab}/H_{c2}^{c} < 1$, which is unusual among superconductors. Under a magnetic field, the superconducting transition becomes broader and asymmetric. Along with the low critical currents, this observation suggests an inhomogeneous superconducting state. In fact, no trace of superconductivity is observed through field-cooling--zero-field-cooling magnetization experiments.

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arXiv2022

Low-temperature thermal expansion of the topological material candidates $β$-PtBi$_2$ and $β$-Bi$_2$Pd

We report on the low-temperature ($T <$ 120 K) thermal expansion of the bismuth-based topological semimetal $β$-PtBi$_2$ and topological superconductor $β$-Bi$_2$Pd candidates. The linear thermal-expansion coefficient of tetragonal $β$-Bi$_2$Pd shows a pronounced anisotropy between the $a$- and $c$-axis while the volume thermal-expansion coefficient $α_V$($β$-Bi$_2$Pd) is considerable larger than $α_V$($β$-PtBi$_2$). The coefficient $α_V$($β$-PtBi$_2$) nearly matches the experimental specific heat, from which a Debye temperature $θ_D =$ 199 K is obtained. On the other hand, $α_V$($β$-Bi$_2$Pd) reasonably fits the Debye model with $θ_D =$ 138 K, extracted from the low-temperature specific heat. An almost constant Grüneisen parameter $Γ\approx$ 2 is obtained for both compounds. No magnetostriction is observed in any of both compounds up to $μ_0 H =$ 16 T. We compare our results with other Bi-based topological materials.

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arXiv2019

Entropy jump at the first-order vortex phase transition in Bi2Sr2CaCu2O8+δ with columnar defects

We study the entropy jump associated with the first-order vortex melting transition (FOT) in Bi2Sr2CaCu2O8+δ crystals by means of Hall probe magnetometry. The samples present a diluted distribution of columnar defects (CD) introduced by irradiation with Xe ions. The FOT is detected in ac transmittivity measurements as a paramagnetic peak, the height of which is proportional to the enthalpy difference entailed by the transition. By applying the Clausius-Clapeyron relation, we quantify the evolution of the entropy jump Δs as a function of the FOT temperature, TFOT, in both pristine crystals and crystals with CD. On increasing the density of CD, Δs decreases monotonically with respect to values found in pristine samples. The Δs versus TFOT dependence in the case of pristine samples follows reasonably well the theoretical prediction of dominant electromagnetic coupling for a model neglecting the effect of disorder. The data for samples with a diluted distribution of CD are not properly described by such a theoretical model.

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arXiv2019

Strong magnetoelastic effect in CeCo$_{1-x}$Fe$_{x}$Si as Néel order is suppressed

A very strong magnetoelastic effect in the CeCo$_{1-x}$Fe$_{x}$Si alloys is reported. The strength of the magnetostrictive effect can be tuned upon changing $x$. The moderate low-temperature linear magnetostriction observed at low Fe concentrations becomes very large ($\frac {ΔL}{L} \left(16 T,2 K\right) =$ 3$\times$10$^{-3}$) around the critical concentration ($x_c \approx$ 0.23) at which the long-range antiferromagnetic order vanishes. Upon increasing doping through the non-magnetic region ($x > x_c$), the magnetostriction strength gradually weakens again. Remarkably the low-temperature magnetostriction at the critical concentration shows a pronounced $S$-like shape (centered at $B_m \sim$ 6 T) resembling other well-known Ce-based metamagnetic systems like CeRu$_2$Si$_2$ and CeTiGe. Unlike what is observed in these compounds, however, the field dependence of the magnetization shows only a minor upturn around $B_m$ vaguely resembling a metamagnetic behavior. The subtle interplay between magnetic order and the Kondo screening seems to originate an enhanced valence susceptibility slightly changing the Ce ions valence, ultimately triggering the large magnetostriction observed around the critical concentration.

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arXiv2017

Unconventional superconductivity in the strong-coupling limit for the heavy fermion system CeCoIn$_5$

We present scanning tunneling spectroscopy measurements of the local quasiparticles' excitation spectra of CeCoIn$_5$ between 440mK and 3K in samples with a bulk $T_{\rm c}=2.25$K. The spectral shape of our low-temperature tunneling data, quite textbook nodal-gap conductance, allow us to confidently fit the spectra with a d-wave density of states considering also a shortening of quasiparticles' lifetime term $Γ$. The $Δ(0)$ value obtained from the fits yields a BCS ratio $2Δ/kT_{\rm c} =7.73$ suggesting that CeCoIn$_5$ is an unconventional superconductor in the strong coupling limit. The fits also suggest that the height of coherence peaks in CeCoIn$_5$ is reduced with respect to a pure BCS spectra and therefore the coupling of quasiparticles with spin excitations should play a relevant role. In addition, the tunneling conductance shows a depletion at energies smaller than $Δ$ for temperatures larger than the bulk $T_{\rm c}$, giving further support to the existence of a pseudogap phase that in our samples span up to $T^{*}\sim 1.2 T_{\rm c}$. The phenomenological scaling of the pseudogap temperature observed in various families of cuprates, $2Δ/kT^{*} \sim 4.3 $, is not fulfilled in our measurements. This suggests that in CeCoIn$_5$ the strong magnetic fluctuations might conspire to close the local superconducting gap at a smaller pesudogap temperature-scale than in cuprates.

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arXiv2014

Local character of the highest antiferromagnetic Ce-system CeTi{1-x}Sc{x} Ge

The highest antiferromagnetic (AFM) temperature in Ce based compounds has been reported for CeScGe with Tn=47K, but its local or itinerant nature was not deeply investigated yet. In order to shed more light into this unusually high ordering temperature we have investigated structural, magnetic, transport and thermal properties of CeTi{1-x}Sc{x}Ge alloys within the range of stability of the CeScSi-type structure: 0.25<x<1. Along this concentration range, this strongly anisotropic system presents a complex magnetic phase diagram with a continuous modification of its magnetic behavior, from ferromagnetism (FM)for 0.25<x<0.50 (with 7K<Tc<16K) to AFM for 0.60<x<1 (with 19K<Tn<47K). The onset of the AFM phase is associated to a metamagnetic transition with a critical field increasing from H{cr}=0 at x~0.55 to ~6Tesla at x=1, coincident with an increasing contribution of the first excited crystal electric field doublet. At a critical point x{cr}=0.65 a second transition appears at Tl<Tn. In contrast to observations in itinerant systems like CeRh{2}Si{2} or CeRh{3}B{2}, no evidences for significant hybridization of the 4f electrons at large Sc contents were found. Therefore, the exceptionally large Tn of CeScGe can be attributed to an increasing RKKY inter-layer interaction as Sc content grows.

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arXiv2014

Effect of quenched disorder in the entropy-jump at the first-order vortex phase transition of Bi$_{2}$Sr$_{2}$CaCu$_{2}$O$_{8 + δ}$

We study the effect of quenched disorder in the thermodynamic magnitudes entailed in the first-order vortex phase transition of the extremely layered Bi$_{2}$Sr$_{2}$CaCu$_{2}$O$_{8 + δ}$ compound. We track the temperature-evolution of the enthalpy and the entropy-jump at the vortex solidification transition by means of AC local magnetic measurements. Quenched disorder is introduced to the pristine samples by means of heavy-ion irradiation with Pb and Xe producing a random columnar-track pins distribution with different densities (matching field $B_Φ$). In contrast with previous magneto-optical reports, we find that the first-order phase transition persists for samples with $B_Φ$ up to 100\,Gauss. For very low densities of quenched disorder (pristine samples), the evolution of the thermodynamic properties can be satisfactorily explained considering a negligible effect of pinning and only electromagnetic coupling between pancake vortices lying in adjacent CuO planes. This description is not satisfactory on increasing magnitude of quenched disorder.

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arXiv2014

Low-temperature physical properties of GdCoIn$_5$

A comprehensive experimental and theoretical study of the low temperature properties of GdCoIn$_5$ was performed. Specific heat, thermal expansion, magnetization and electrical resistivity were measured in good quality single crystals down to $^4$He temperatures. All the experiments show a second-order-like phase transition at 30 K probably associated with the onset of antiferromagnetic order. Total energy GGA+U calculations indicate a ground state with magnetic moments localized at the Gd ions and allowed a determination of the Gd-Gd magnetic interactions. Band structure calculations of the electron and phonon contributions to the specific heat and Quantum Monte Carlo calculations of the magnetic contributions to the thermodynamic quantities reproduce quite well the experimental data.

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arXiv2014

Exploring high temperature magnetic order in CeTi_1-xSc_xGe

Most of magnetic transitions related to Ce ordering are found below T_ord~12K. Among the few cases exceeding that temperature, two types of behaviors can be distinguished. One of them is related to the rare cases of Ce binary compounds formed in BCC structures, with a quartet ground state, whose degeneracy is reduced by undergoing different types of transitions mostly structural. The other group shows evidences of itinerant character with the outstanding example of CeRh_3B_2 showing the highest T_ord=115K. The second highest ordering temperature has been reported for CeScGe with T_ord=47K, but the nature of this magnetic state has not been investigated very deeply. In order to shed more light into this unusual high temperature ordering we studied the structural, magnetic, transport and thermal properties of CeTi_1-xSc_xGe alloys in the stability range of the CeScSi-type structure 0.25 0.65, the magnetic phase boundary splits into two transitions, with an intermediate phase presenting incommensurate spin density waves features.

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arXiv2013

Effect of pressure cycling on Iron: Signatures of an electronic instability and unconventional superconductivity

High pressure electrical resistivity and x-ray diffraction experiments have been performed on Fe single crystals. The crystallographic investigation provides direct evidence that in the martensitic $bcc \rightarrow hcp$ transition at 14 GPa the $\lbrace 110\rbrace_{bcc}$ become the $\lbrace 002\rbrace_{hcp}$ directions. During a pressure cycle, resistivity shows a broad hysteresis of 6.5 GPa, whereas superconductivity, observed between 13 and 31 GPa, remains unaffected. Upon increasing pressure an electronic instability, probably a quantum critical point, is observed at around 19 GPa and, close to this pressure, the superconducting $T_{c}$ and the isothermal resistivity ($0<T<300\,$K) attain maximum values. In the superconducting pressure domain, the exponent $n = 5/3$ of the temperature power law of resistivity and its prefactor, which mimics $T_{c}$, indicate that ferromagnetic fluctuations may provide the glue for the Cooper pairs, yielding unconventional superconductivity.

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arXiv2011

Pressure cycle of superconducting Cs0.8Fe2Se2: a transport study

We report measurements of the temperature and pressure dependence of the electrical resistivity of single crystalline iron-based chalcogenide Cs0.8Fe2Se2. In this material superconductivity Tc~30K develops from a normal state with extremely large resistivity. At ambient pressure a large "hump" in the resistivity is observed around 200K. Under pressure, the resistivity decreases by two orders of magnitude, concomitant with a sudden Tc suppression around p~8GPa. Even at 9GPa a metallic resistivity state is not recovered, and the ρ(T) "hump" is still detected. A comparison of the data measured upon increasing and decreasing the external pressure leads us to suggest that superconductivity is not related to this hump.

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arXiv2006

Metallic State in Cubic FeGe beyond its Quantum Phase Transition

We report on results of electrical resistivity and structural investigations on the cubic modification of FeGe under high pressure. The long-wavelength helical order ($T_C=280$ K) is suppressed at a critical pressure $p_c\approx 19$ GPa. An anomaly in the resistivity data at $T_X(p)$ and strong deviations from a Fermi-liquid behavior in a wide pressure range above $p_c$ suggest that the suppression of $T_C$ disagrees with the standard notion of a quantum critical phase transition. The metallic ground state persisting at high pressure can be described by band-structure calculations if structural disorder due to zero-point motion is included. Discontinuous changes in the pressure dependence of the shortest Fe-Ge interatomic distance occurring close to the $T_C(p)$ phase line could be interpreted as a symmetry-conserving transition of first order.

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arXiv2005

Probing the extended non-Fermi liquid regimes of MnSi and Fe

Recent studies show that the non-Fermi liquid (NFL) behavior of MnSi and Fe spans over an unexpectedly broad pressure range, between the critical pressure p_c and around 2p_c. In order to determine the extension of their NFL regions, we analyze the evolution of the resistivity rho(T) A(p)T^n at higher pressures. We find that in MnSi the n=3/2 exponent holds below 4.8 GPa=3 p_c, but it increases above that pressure. At 7.2 GPa we observe the low temperature Fermi liquid exponent n=2 whereas for T>1.5 K, n=5/3. Our measurements in Fe show that the NFL behavior rho T^{5/3} extends at least up to 30.5 GPa, above the entire superconducting (SC) region. In the studied pressure range, the onset of the SC transition reduces by a factor 10 down to T_c^onset(30.5 GPa)=0.23 K, while the A-coefficient diminishes monotonically by around 50%.

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arXiv2004

Low temperature magnetic phase diagram of the cubic non-Fermi liquid system CeIn_(3-x)Sn_x

In this paper we report a comprehensive study of the magnetic susceptibility (χ), resistivity (ρ), and specific heat (C_P), down to 0.5 K of the cubic CeIn_(3-x)Sn_x alloy. The ground state of this system evolves from antiferromagnetic (AF) in CeIn_3(T_N=10.2 K) to intermediate-valent in CeSn_3, and represents the first example of a Ce-lattice cubic non-Fermi liquid (NFL) system where T_N(x) can be traced down to T=0 over more than a decade of temperature. Our results indicate that the disappearance of the AF state occurs near x_c ~ 0.7, although already at x ~ 0.4 significant modifications of the magnetic ground state are observed. Between these concentrations, clear NFL signatures are observed, such as ρ(T)\approx ρ_0 + A T^n (with n<1.5) and C_P(T)\propto -T ln(T) dependencies. Within the ordered phase a first order phase transition occurs for 0.25 < x < 0.5. With larger Sn doping, different weak ρ(T) dependencies are observed at low temperatures between x=1 and x=3 while C_P/T shows only a weak temperature dependence.

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arXiv2004

Complex magnetic phase diagram of CePd_{2-x}Ni_xAl_3 around its critical concentration

Thermal, magnetic and transport measurements are reported on CePd_{2-x}Ni_xAl_3 in the 0<= x <= 1 range, including the effect of pressure (p) and magnetic field on some selected samples. The low temperature results indicate that long range antiferromagnetic order is stable up to x=0.2, while between 0.25 and 0.5 magnetic disorder gives rise to non-Fermi-liquid (NFL) behavior. In this region, the low temperature specific heat can be described by the sum of two components, the major one showing a C_P/T=gamma_0 -gamma_1 T^(1/2) dependence, while the minor one includes a decreasing number of degrees of freedom related to a residue of short range order. The latter extrapolates to zero between 0.45<x_{cr}<0.5. Electrical resistivity (rho) studies performed under pressure for x=0.5 allow to investigate the evolution of the NFL state right above the critical point, where the exponent of rho ~ T^n is found to increase from n=1 (for p=0) up to n=2 (for p=12 kbar). The latter is observed for x=1.0 already at normal pressure, indicating the onset of the Fermi Liquid behavior. Doping and pressure effects are compared by fitting high temperature resistivity data employing a unique function which allows to describe the evolution of the characteristic energy of this series through a large range of concentration and pressure.

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arXiv2001

Study of the Ce(Rh$_{1-x}$Pd$_x$)$_2$Si$_2$ alloy: evidence for itinerant character of the magnetic order in CeRh$_2$Si$_2$

We present electrical resistivity and specific heat measurements of alloys on the Rh rich side of the phase diagram of the Ce(Rh$_{1-x}$Pd$_x$)$_2$Si$_2$ system and compare the results with those obtained at intermediate and low Rh concentrations. The analysis of the x-evolution of the entropy and the scaling behaviour of $C_{el}(T)$ and $ρ(T)$ clearly confirm a separation of the magnetic phase diagram into two regions. The region $x\le0.3$, showing a concentration independent characteristic temperature $T_o\approx45 {\rm K}$, while for $x>0.3$ $T_o$ decreases down to $T_o(x=1)\approx15 {\rm K}$. This characteristic temperature is obtained by scaling the $C_{el}(T,x>0.3)$ results as a function of the reduced temperature $T/T_o$. At low Pd-content, $T_N$ decreases very rapidly from $T_N = 36 {\rm K}$ in pure CeRh$_2$Si$_2$ to $T_N=18 {\rm K}$ at x=0.1. With higher Pd concentration it stabilized at $T_N\approx15 {\rm K}$ whereas the magnitude of the anomalies in $C_{el}(T)$ and in the susceptibility around $T_N$ are further reduced and disappear at $x\approx0.3$. This is in contrast to the behavior found on the Pd-rich side, where $T_N$ decreases continuously to zero with increasing Rh content. The pronounced differences observed between both phase boundaries and the drastic effect of doping on the Rh rich side suggest an itinerant character in CeRh$_2$ Si$_2$, in contrast to the localized character of CePd$_2$Si$_2$. A further evidence for the itinerant character in CeRh$_2$Si$_2$ is given by the $ρ(T)$ dependence observed for $x\le0.3$, which scales with $ρ(T)$ of the prototype itinerant compound YCo$_2$.

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