arXiv subjects

P. Quemerais

Publications and source records attributed to P. Quemerais.

14 recordsLinked to original sources

arXiv2017

Theory of charge density wave depinning by electromechanical effect

We discuss the first theory for the depinning of low dimensional, incommensurate, charge density waves (CDWs) in the strong electron-phonon (e-p) regime. Arguing that most real CDWs systems invariably develop a gigantic dielectric constant (GDC) at very low frequencies, we propose an electromechanical mechanism which is based on a local field effect. At zero electric field and large enough e-p coupling the structures are naturally pinned by the lattice due to its discreteness, and develop modulation functions which are characterized by discontinuities. When the electric field is turned on, we show that it exists a finite threshold value for the electric field above which the discontinuities of the modulation functions vanish due to CDW deformation. The CDW is then free to move. The signature of this pinning/depinning transition as a function of the increasing electric field can be directly observed in the phonon spectrum by using inelastic neutrons or X-rays experiments.

cond-mat.mtrl-sci↗

arXiv2007

Role of commensurate arrangements in the optical response of metallic gratings

Light localization on commensurate arrangements of metallic sub-wavelength grooves is studied. We theoretically show that as the degree of commensuration tends to an irrational number new light localization states are produced. These have properties close to that reported for hot spots on disordered surfaces and are not permitted for simple period gratings. Some theoretical predictions are experimentally provided in the infra-red region by reflectivity measurements performed on two commensurate samples with respectively two and three slits per period.

cond-mat.other↗

arXiv2007

Why metallic surfaces with grooves a few nanometers deep and wide may strongly absorb visible light

It is theoretically shown that nanometric silver lamellar gratings present very strong visible light absorption inside the grooves, leading to electric field intensities by several orders of magnitude larger than that of the impinging light. This effect, due to the excitation of long wave vector surface plasmon polaritons with particular small penetration depth in the metal, may explain the abnormal optical absorption observed a long time ago on almost flat Ag films. Surface enhanced Raman scattering in rough metallic films could also be due to the excitation of such plasmon polaritons in the grain boundaries or notches of the films.

cond-mat.other↗

arXiv2006

Controlling Strong Electromagnetic Fields at a Sub-Wavelength Scale

We investigate the optical response of two sub-wavelength grooves on a metallic screen, separated by a sub-wavelength distance. We show that the Fabry-Perot-like mode, already observed in one-dimensional periodic gratings and known for a single slit, splits into two resonances in our system : a symmetrical mode with a small Q-factor, and an antisymmetric one which leads to a much stronger light enhancement. This behavior results from the near-field coupling of the grooves. Moreover, the use of a second incident wave allows to control the localization of the photons in the groove of our choice, depending on the phase difference between the two incident waves. The system exactly acts as a sub-wavelength optical switch operated from far-field.

physics.optics↗

arXiv2006

Enhancement of Wigner crystallization in quasi low-dimensional solids

The crystallization of electrons in quasi low-dimensional solids is studied in a model which retains the full three-dimensional nature of the Coulomb interactions. We show that restricting the electron motion to layers (or chains) gives rise to a rich sequence of structural transitions upon varying the particle density. In addition, the concurrence of low-dimensional electron motion and isotropic Coulomb interactions leads to a sizeable stabilization of the Wigner crystal, which could be one of the mechanisms at the origin of the charge ordered phases frequently observed in such compounds.

cond-mat.str-el↗

arXiv2005

Polarization catastrophe at low densities of polarons: from Cuprates to Metal-Ammonia Solutions

We review some results on the role played by dielectric polarons at the metal-insulator transition in polarizable materials, taking into account the long-range nature of the Coulomb interactions. The occurrence of a polarization catastrophe is examined in a model describing a Wigner crystal of polarons. The possible relevance of this scenario in the cuprates and in metal-ammonia solutions is discussed.

cond-mat.supr-con↗

arXiv2004

On the stability of hole crystals in layered cuprates

Recent STM measurements have revealed the existence of periodic charge modulations at the surface of certain cuprate superconductors. Here we show that the observed patterns are compatible with the formation of a three-dimensional crystal of doped holes, with space correlations extending between different Cu-O layers. This puts severe constraints on the dynamical stability of the crystallised hole structure, resulting in a close relationship between the periodicity of the electronic modulation and the interlayer distance.

cond-mat.supr-con↗

arXiv2004

Efficient excitation of cavity resonances of subwavelength metallic gratings

One dimensional rectangular metallic gratings enable enhanced transmission of light for specific resonance frequencies. Two kinds of modes participating to enhanced transmission have already been demonstrated : (i) waveguide modes and (ii) surface plasmon polaritons (SPP). Since the original paper of Hessel and Oliner \cite{hessel} pointing out the existence of (i), no progress was made in their understanding. We present here a carefull analysis, and show that the coupling between the light and such resonances can be tremendously improved using an {\it evanescent} wave. This leads to enhanced localisation of light in cavities, yielding, in particular, to a very selective light transmission through these gratings.

physics.optics↗

arXiv2002

Polarization catastrophe in doped cuprates and metal-ammonia solutions: an analogy

On doping polar dielectrics, such as the cuprates or liquid ammonia, the long range polarization leads to the formation of bound states (polarons or solvated electrons). However, the exact role of such entities in the metal-insulator transition (MIT) still remains unclear. We suggest that the driving mechanism of the MIT is a polarization catastrophe that occurs due to their unscreened Coulomb interaction. This phenomenon is associated to a negative static dielectric constant, which could be the origin of both the superconducting transition in the cuprates -- where the doping ions are frozen in the lattice structure -- and the phase separation observed in liquid metal-ammonia solutions -- where the counter-ions are mobile.

cond-mat↗

arXiv2002

Polarization catastrophe in the polaronic Wigner crystal

We consider a three dimensional Wigner crystal of electrons lying in a host ionic dielectric. Owing to their interaction with the lattice polarization, each localized electron forms a polaron. We study the collective excitations of such a polaronic Wigner crystal at zero temperature, taking into account the quantum fluctuations of the polarization within the Feynman harmonic approximation. We show that, contrary to the ordinary electron crystal, the system undergoes a polarization catastrophe when the density is increased. An optical signature of this instability is derived, whose trend agrees with the experiments carried out in Nd-based cuprates.

cond-mat.str-el↗

arXiv2000

Is the Quantum Melting of a Polaron Wigner Crystal an Insulator-to-Superconductor transition ?

On examining the stability of a Wigner Crystal (WC) in an ionic dielectric, two competitive effects due to Polaron formation are found to be important: (i) the screening of the Coulomb forces which destabilizes the crystal, compensated by (ii) the increase of the carrier mass (polaron mass). The quantum melting of the Polaron Wigner Crystal (PWC) is examined. By calculating the quantum fluctuations of both the electrons and the polarization, we show that there is a competition between the dissociation of the Polarons at the insulator-to-metal transition (IMT), and a melting towards a polaron liquid. We find that at strong coupling ($α> α^*$), a liquid state of polarons cannot exist, and the IMT is driven by polaron dissociation. Next, we show that the dipolar interactions between localized polarons are responsible for a phonon instability of the PWC as the density increases. This provides a new mechanism for the IMT in doped dielectrics. Examining the sign of the dielectric constant of the PWC, we conjecture that such an instability could yield an Insulator-to-Superconductor transition.

cond-mat.supr-con↗

arXiv1999

Melting of a Wigner Crystal in an Ionic Dielectric

The melting of a Wigner Crystal of electrons placed into a host polar material is examined as a function of the density and the temperature. When the coupling to the longitudinal optical modes of the host medium is turned on, the WC is progressively transformed into a polaronic Wigner Crystal. We estimate the critical density for crystal melting at zero temperature using the Lindeman criterion. We show that above a certain critical value of the Frohlich electron-phonon coupling, the melting towards a quantum liquid of polarons is not possible, and the insulator-to-metal transition is driven by the ionization of the polarons (polaron dissociation). The phase diagram at finite temperature is obtained by making use of the same Lindeman criterion. Results are also provided in the case of an anisotropic electron band mass, showing that the scenario of polaron dissociation can be relevant in anisotropic compounds such as the superconducting cuprates at rather moderate e-ph couplings.

cond-mat.str-el↗

arXiv1998

Polaron Crystallization and Melting: Effects of the Long-Range Coulomb Forces

On examining the stability of a Wigner crystal in an ionic dielectric, two competitive effects due to the polaron formation are found to be important: (i) the screening of the Coulomb force, which destabilizes the crystal, compensated by (ii) the increase of the carrier mass (polaron mass). The competition between the two effects is carefully studied, and the quantum melting of the polaronic Wigner crystal is examined by varying the density at zero temperature. By calculating the quantum fluctuations of both the electron and the polarization, we show that there is a competition between the dissociation of the polarons at the insulator-to-metal transition (IMT), and a melting towards a polaron liquid. We find that at strong coupling, a liquid state of dielectric polarons cannot exist, and the IMT is driven by the polaron dissociation. Next, taking into account the dipolar interactions between localized carriers, we show that these are responsible for an instability of the transverse vibrational modes of the polaronic Wigner crystal as the density increases. This provides a new mechanism for the IMT in doped dielectrics, which yields interesting dielectric properties below and beyond the transition. An optical signature of such a mechanism for the IMT is provided.

cond-mat.supr-con↗

arXiv1997

Polaron Dissociation at the Insulator-to-Metal Transition

Considering the long range Coulomb interactions between large polarons in dielectrics, we propose a model for their crystallization when no bipolarons are formed. As the density increases, the melting is examined at $T=OK$. One possibility is the delocalization towards a liquid state of polarons. However, we show that this cannot happen if the electron-phonon coupling is larger than some critical value. The other competing mechanism is the dissociation of the polarons themselves, favored owing to their large mass at strong coupling. Finally, we propose a phase diagram for the insulator-to metal transition as a function of the density and electron-phonon coupling.

cond-mat↗