arXiv subjects

P. Reiter

Publications and source records attributed to P. Reiter.

At least 19 recordsLinked to original sources

arXiv2026

Direct transfer to $^{46,48}$K as a survey of the $\pi(s_{1/2})$$-\nu(sdpf)$ interaction

The collapse of the canonical $N=28$ magic number in nuclei with $Z<20$ has drawn significant interest as it relates to the emergence of an island of inversion centered on $^{42}$Si and $^{44}$S. In particular, interactions between the $\pi s_{1/2}$ orbital -- empty in $^{42}$Si and full in $^{44}$S -- and the neutron orbitals just above and below the $N=28$ gap are expected to be critical in this region, but remain relatively unexplored. In this paper, we expand upon the results of our previous study of the direct transfer reaction $^{47}$K(d,p$\gamma$)$^{48}$K [C.\,J.~Paxman \textit{et al.}, Phys. Rev. Lett. 134, 162504 (2025)] with the results of the complementary $^{47}$K(d,t$\gamma$)$^{46}$K reaction. Through this study, we present a comprehensive scan of the interaction between the critical $\pi s_{1/2}$ orbital and a broad range of neutron orbitals spanning nearly two full shells. We identify several discrepancies between the experimental results and state-of-the-art shell model calculations, which suggest a deficiency of the shell model to fully capture the complex proton configuration mixing in this region, highlighting a significant challenge for single-particle descriptions of the island of inversion.

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arXiv2025

Fusion of 12C+28Si at deep sub-barrier energies

The existence of fusion hindrance is not well established in light heavy-ion systems. Studying slightly heavier cases allows extrapolating the trend to light systems of astrophysical interest. Fusion of 12C + 28Si has been measured down to deep sub-barrier energies, using 28Si beams from the XTU Tandem accelerator of LNL on thin 12C targets. The fusion-evaporation residues were detected by a detector telescope following an electrostatic beam separator, and coincidences between the gamma-ray array AGATA and segmented silicon detectors DSSD were performed, where the evaporated light charged particles were identified by pulse shape analysis. Fusion cross sections have been obtained in the wide range 150 mb-42 nb. Coupled-channel (CC) calculations using a Woods-Saxon potential reproduce the data above 0.1 mb. Below that, hindrance shows up and the CC results overestimate the cross sections which get close to the one-dimensional potential tunnelling limit. This suggests that the coupling strengths gradually vanish, as predicted by the adiabatic model. The hindrance threshold follows a recently updated phenomenological systematics.

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arXiv2024

Shape evolution in even-mass $^{98-104}$Zr isotopes via lifetime measurements using the $\gamma\gamma$-coincidence technique

The Zirconium (Z = 40) isotopic chain has attracted interest for more than four decades. The abrupt lowering of the energy of the first $2^+$ state and the increase in the transition strength B(E2; $2_1^\rightarrow 0_1^+$ going from $^{98}$Zr to $^{100}$Zr has been the first example of "quantum phase transition" in nuclear shapes, which has few equivalents in the nuclear chart. Although a multitude of experiments have been performed to measure nuclear properties related to nuclear shapes and collectivity in the region, none of the measured lifetimes were obtained using the Recoil Distance Doppler Shift method in the $\gamma\gamma$-coincidence mode where a gate on the direct feeding transition of the state of interest allows a strict control of systematical errors. This work reports the results of lifetime measurements for the first yrast excited states in $^{98-104}$Zr carried out to extract reduced transition probabilities. The new lifetime values in $\gamma\gamma$-coincidence and $\gamma$-single mode are compared with the results of former experiments. Recent predictions of the Interacting Boson Model with Configuration Mixing, the Symmetry Conserving Configuration Mixing model based on the Hartree-Fock-Bogoliubov approach and the Monte Carlo Shell Model are presented and compared with the experimental data.

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arXiv2024

Probing exotic cross-shell interactions at N=28 with single-neutron transfer on 47K

We present the first measurement of the $^{47}$K($d,p\gamma$)$^{48}$K transfer reaction, performed in inverse kinematics using a reaccelerated beam of $^{47}$K. The level scheme of $^{48}$K has been greatly extended with nine new bound excited states identified and spectroscopic factors deduced. Detailed comparisons with SDPF-U and SDPF-MU shell-model calculations reveal a number of discrepancies with these results, and a preference for SDPF-MU is found. Intriguingly, an apparent systematic overestimation of spectroscopic factors and a poor reproduction of the energies for 1$^-$ states suggests that the mixing between the $\pi s^{\,\,\,1}_{1/2} d^{\,\,\,4}_{3/2}$ and $\pi s^{\,\,\,2}_{1/2} d^{\,\,\,3}_{3/2}$ proton configurations in $^{48}$K is not correctly described using current interactions, challenging our descriptions of light $N=28$ nuclei.

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arXiv2024

High-precision spectroscopy of $^{20}$O benchmarking ab-initio calculations in light nuclei

The excited states of unstable $^{20}$O were investigated via $\gamma$-ray spectroscopy following the $^{19}$O$(d,p)^{20}$O reaction at 8 $A$MeV. By exploiting the Doppler Shift Attenuation Method, the lifetime of the 2$^+_2$ and 3$^+_1$ states were firmly established. From the $\gamma$-ray branching and E2/M1 mixing ratios for transitions deexciting the 2$^+_2$ and 3$^+_1$ states, the B(E2) and B(M1) were determined. Various chiral effective field theory Hamiltonians, describing the nuclear properties beyond ground states, along with a standard USDB interaction, were compared with the experimentally obtained data. Such a comparison for a large set of $\gamma$-ray transition probabilities with the valence space in medium similarity renormalization group ab-initio calculations was performed for the first time in a nucleus far from stability. It was shown that the ab-initio approaches using chiral EFT forces are challenged by detailed high-precision spectroscopic properties of nuclei. The reduced transition probabilities were found to be a very constraining test of the performance of the ab-initio models.

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arXiv2023

Nuclear Level Density and $\gamma$-ray Strength Function of $^{67}\mathrm{Ni}$ and the impact on the i-process

Proton-$\gamma$ coincidences from $(\mathrm{d},\mathrm{p})$ reactions between a $^{66}\mathrm{Ni}$ beam and a deuterated polyethylene target have been analyzed with the inverse-Oslo method to find the nuclear level density (NLD) and $\gamma$-ray strength function ($\gamma$SF) of $^{67}\mathrm{Ni}$. The $^{66}\mathrm{Ni}(n,\gamma)$ capture cross section has been calculated using the Hauser-Feshbach model in TALYS using the measured NLD and $\gamma$SF as constraints. The results confirm that the $^{66}\mathrm{Ni}(n,\gamma)$ reaction acts as a bottleneck when relying on one-zone nucleosynthesis calculations. However, the impact of this reaction is strongly dampened in multi-zone models of low-metallicity AGB stars experiencing i-process nucleosynthesis.

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arXiv2022

Search for $^{22}$Na in novae supported by a novel method for measuring femtosecond nuclear lifetimes

Classical novae are thermonuclear explosions in stellar binary systems, and important sources of $^{26}$Al and $^{22}$Na. While gamma rays from the decay of the former radioisotope have been observed throughout the Galaxy, $^{22}$Na remains untraceable. The half-life of $^{22}$Na (2.6 yr) would allow the observation of its 1.275 MeV gamma-ray line from a cosmic source. However, the prediction of such an observation requires good knowledge of the nuclear reactions involved in the production and destruction of this nucleus. The $^{22}$Na($p,\gamma$)$^{23}$Mg reaction remains the only source of large uncertainty about the amount of $^{22}$Na ejected. Its rate is dominated by a single resonance on the short-lived state at 7785.0(7) keV in $^{23}$Mg. In the present work, a combined analysis of particle-particle correlations and velocity-difference profiles is proposed to measure femtosecond nuclear lifetimes. The application of this novel method to the study of the $^{23}$Mg states, combining magnetic and highly-segmented tracking gamma-ray spectrometers, places strong limits on the amount of $^{22}$Na produced in novae, explains its non-observation to date in gamma rays (flux < 2.5x$10^{-4}$ ph/(cm$^2$s)), and constrains its detectability with future space-borne observatories.

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arXiv2022

Muonic atom spectroscopy with microgram target material

Muonic atom spectroscopy -- the measurement of the x rays emitted during the formation process of a muonic atom -- has a long standing history in probing the shape and size of nuclei. In fact, almost all stable elements have been subject to muonic atom spectroscopy measurements and the absolute charge radii extracted from these measurements typically offer the highest accuracy available. However, so far only targets of at least a few hundred milligram could be used as it required to stop a muon beam directly in the target to form the muonic atom. We have developed a new method relying on repeated transfer reactions taking place inside a 100-bar hydrogen gas cell with an admixture of 0.25% deuterium that allows us to drastically reduce the amount of target material needed while still offering an adequate efficiency. Detailed simulations of the transfer reactions match the measured data, suggesting good understanding of the processes taking place inside the gas mixture. As a proof of principle we demonstrate the method with a measurement of the 2p-1s muonic x rays from a 5-{\mu}g gold target.

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arXiv2021

Narrow resonances in the continuum of the unbound nucleus $^{15}$F

The structure of the unbound $^{15}$F nucleus is investigated using the inverse kinematics resonant scattering of a radioactive $^{14}$O beam impinging on a CH$_2$ target. The analysis of $^{1}$H($^{14}$O,p)$^{14}$O and $^{1}$H($^{14}$O,2p)$^{13}$N reactions allowed the confirmation of the previously observed narrow $1/2^{-}$ resonance, near the two-proton decay threshold, and the identification of two new narrow 5/2$^{-}$ and 3/2$^{-}$ resonances. The newly observed levels decay by 1p emission to the ground of $^{14}$O, and by sequential 2p emission to the ground state (g.s.) of $^{13}$N via the $1^-$ resonance of $^{14}$O. Gamow shell model (GSM) analysis of the experimental data suggests that the wave functions of the 5/2$^{-}$ and 3/2$^{-}$ resonances may be collectivized by the continuum coupling to nearby 2p- and 1p- decay channels. The observed excitation function $^{1}$H($^{14}$O,p)$^{14}$O and resonance spectrum in $^{15}$F are well reproduced in the unified framework of the GSM.

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arXiv2021

Evidence for enhanced neutron-proton correlations from the level structure of the $N=Z+1$ nucleus $^{87}_{43}$Tc$^{\ }_{44}$

The low-lying excited states in the neutron-deficient $N=Z+1$ nucleus $^{87}_{43}$Tc$^{\ }_{44}$ have been studied via the fusion-evaporation reaction $^{54}$Fe($^{36}$Ar, $2n1p$)$^{87}$Tc at the Grand Acc\'el\'erateur National d'Ions Lourds (GANIL), France. The AGATA spectrometer was used in conjunction with the auxiliary NEDA, Neutron Wall, and DIAMANT detector arrays to measure coincident prompt $\gamma$-rays, neutrons, and charged particles emitted in the reaction. A level scheme of $^{87}$Tc from the (9/2$^{+}_{g.s.}$) state to the (33/2$^{+}_{1}$) state was established based on 6 mutually coincident $\gamma$-ray transitions. The constructed level structure exhibits a rotational behavior with a sharp backbending at $\hbar\omega\approx 0.50$ MeV. A decrease in alignment frequency and increase in alignment sharpness in the odd-mass isotonic chains around $N=44$ is proposed as an effect of the enhanced isoscalar neutron-proton interactions in odd-mass nuclei when approaching the $N=Z$ line.

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arXiv2020

The observation of vibrating pear shapes in radon nuclei: update

There is a large body of evidence that atomic nuclei can undergo octupole distortion and assume the shape of a pear. This phenomenon is important for measurements of electric-dipole moments of atoms, which would indicate CP violation and hence probe physics beyond the standard model of particle physics. Isotopes of both radon and radium have been identified as candidates for such measurements. Here, we have observed the low-lying quantum states in $^{224}$Rn and $^{226}$Rn by accelerating beams of these radioactive nuclei. We report here additional states not assigned in our 2019 publication. We show that radon isotopes undergo octupole vibrations but do not possess static pear-shapes in their ground states. We conclude that radon atoms provide less favourable conditions for the enhancement of a measurable atomic electric-dipole moment.

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arXiv2020

Testing ab initio nuclear structure in neutron-rich nuclei: lifetime measurements of second 2+ states in 16C and 20O

To test the predictive power of ab initio nuclear structure theory, the lifetime of the second 2+ state in neutron-rich 20O, tau(2+_2 ) = 150(+80-30) fs, and an estimate for the lifetime of the second 2+ state in 16C have been obtained, for the first time. The results were achieved via a novel Monte Carlo technique that allowed us to measure nuclear state lifetimes in the tens-to-hundreds femtoseconds range, by analyzing the Doppler-shifted gamma-transition line shapes of products of low-energy transfer and deep-inelastic processes in the reaction 18O (7.0 MeV/u) + 181Ta. The requested sensitivity could only be reached owing to the excellent performances of the AGATA gamma-tracking array, coupled to the PARIS scintillator array and to the VAMOS++ magnetic spectrometer. The experimental lifetimes agree with predictions of ab initio calculations using two- and three-nucleon interactions, obtained with the valence-space in-medium similarity renormalization group for 20O, and with the no-core shell model for 16C. The present measurement shows the power of electromagnetic observables, determined with high-precision gamma spectroscopy, to assess the quality of first-principles nuclear structure calculations, complementing common benchmarks based on nuclear energies. The proposed experimental approach will be essential for short lifetimes measurements in unexplored regions of the nuclear chart, including r-process nuclei, when intense ISOL-type beams become available.

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arXiv2020

Evolution of Octupole Deformation in Radium Nuclei from Coulomb Excitation of Radioactive $^{222}$Ra and $^{228}$Ra Beams

There is sparse direct experimental evidence that atomic nuclei can exhibit stable pear shapes arising from strong octupole correlations. In order to investigate the nature of octupole collectivity in radium isotopes, electric octupole ($E3$) matrix elements have been determined for transitions in $^{222,228}$Ra nuclei using the method of sub-barrier, multi-step Coulomb excitation. Beams of the radioactive radium isotopes were provided by the HIE-ISOLDE facility at CERN. The observed pattern of $E$3 matrix elements for different nuclear transitions is explained by describing $^{222}$Ra as pear-shaped with stable octupole deformation, while $^{228}$Ra behaves like an octupole vibrator.

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arXiv2019

Effects of one valence proton on seniority and angular momentum of neutrons in neutron-rich $^{122-131}$Sb$_{51}$ isotopes

The neutron-rich $^{122-131}$Sb isotopes were produced as fission fragments in the reaction $^{9}$Be($^{238}$U,~f) with 6.2 MeV/u beam energy. An unique setup, consisting of AGATA, VAMOS++ and EXOGAM detectors, was used which enabled the prompt-delayed gamma-ray ($\gamma$) spectroscopy of fission fragments in the time range of 100 ns - 200 $\mu$s. New isomers, prompt and delayed transitions were established in the even-A $^{122-130}$Sb isotopes. In the odd-A $^{123-131}$Sb isotopes, new prompt and delayed $\gamma$-ray transitions were identified, in addition to the confirmation of the previously known isomers. The half-lives of the isomeric states and the $B(E2)$ transition probabilities of the observed transitions depopulating these isomers were extracted. The experimental data was compared with the theoretical results obtained in the framework of Large-Scale Shell-Model (LSSM) calculations in a restricted model space. Modifications of several components of the shell model interaction were introduced to obtain a consistent agreement with the excitation energies and the $B(E2)$ transition probabilities in neutron-rich Sn and Sb isotopes. The isomeric configurations in Sn and Sb were found to be relatively pure. Further, the calculations revealed that the presence of a single valence proton, mainly in the $g_{7/2}$ orbital in Sb isotopes, leads to significant mixing (due to the $\nu\pi$ interaction) of: (i) the neutron seniorities ($\upsilon_{\nu}$) and (ii) the neutron angular momentum ($I_{\nu}$). The above features have a weak impact on the excitation energies, but have an important impact on the $B(E2)$ transition probabilities. In addition, a constancy of the relative excitation energies irrespective of neutron seniority and neutron number in Sn and Sb was observed.

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arXiv2019

Pairing-quadrupole interplay in the neutron-deficient tin nuclei: first lifetime measurements of low-lying states in $^{106,108}$Sn

The lifetimes of the low-lying excited states $2^+$ and $4^+$ have been directly measured in the neutron-deficient $^{106,108}$Sn isotopes. The nuclei were populated via a deep-inelastic reaction and the lifetime measurement was performed employing a differential plunger device. The emitted $\gamma$ rays were detected by the AGATA array, while the reaction products were uniquely identified by the VAMOS++ magnetic spectrometer. Large-Scale Shell-Model calculations with realistic forces indicate that, independently of the pairing content of the interaction, the quadrupole force is dominant in the $B(E2; 2_1^+ \to 0_{g.s.}^+)$ values and it describes well the experimental pattern for $^{104-114}$Sn; the $B(E2; 4_1^+ \to 2_1^+)$ values, measured here for the first time, depend critically on a delicate pairing-quadrupole balance, disclosed by the very precise results in $^{108}$Sn. This result provides insight in the hitherto unexplained $B(E2; 4_1^+ \to 2_1^+)/B(E2; 2_1^+ \to 0_{g.s.}^+) < 1$ anomaly.

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arXiv2016

Spectroscopy of 46Ar by the (t,p) two-neutron transfer reaction

States in the $N=28$ nucleus $^{46}$Ar have been studied by a two-neutron transfer reaction at REX-ISOLDE (CERN). A beam of radioactive $^{44}$ at an energy of 2.16~AMeV and a tritium loaded titanium target were used to populate $^{46}$ by the t($^{44}$,p) two-neutron transfer reaction. Protons emitted from the target were identified in the T-REX silicon detector array. The excitation energies of states in $^{46}$ have been reconstructed from the measured angles and energies of recoil protons. Angular distributions for three final states were measured and based on the shape of the differential cross section an excited state at 3695~keV has been identified as $J^\pi = 0^+$. The angular differential cross section for the population of different states are compared to calculations using a reaction model employing both sequential and direct transfer of two neutrons. Results are compared to shell model calculations using state-of-the-art effective interactions.

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arXiv2016

The structure of low-lying states in ${}^{140}$Sm studied by Coulomb excitation

The electromagnetic structure of $^{140}$Sm was studied in a low-energy Coulomb excitation experiment with a radioactive ion beam from the REX-ISOLDE facility at CERN. The $2^+$ and $4^+$ states of the ground-state band and a second $2^+$ state were populated by multi-step excitation. The analysis of the differential Coulomb excitation cross sections yielded reduced transition probabilities between all observed states and the spectroscopic quadrupole moment for the $2_1^+$ state. The experimental results are compared to large-scale shell model calculations and beyond-mean-field calculations based on the Gogny D1S interaction with a five-dimensional collective Hamiltonian formalism. Simpler geometric and algebraic models are also employed to interpret the experimental data. The results indicate that $^{140}$Sm shows considerable $\gamma$ softness, but in contrast to earlier speculation no signs of shape coexistence at low excitation energy. This work sheds more light on the onset of deformation and collectivity in this mass region.

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arXiv2015

Low-energy Coulomb excitation of $^{62}$Fe and $^{62}$Mn following in-beam decay of $^{62}$Mn

Sub-barrier Coulomb-excitation was performed on a mixed beam of $^{62}$Mn and $^{62}$Fe, following in-trap $\beta^{-}$ decay of $^{62}$Mn at REX-ISOLDE, CERN. The trapping and charge breeding times were varied in order to alter the composition of the beam, which was measured by means of an ionisation chamber at the zero-angle position of the Miniball array. A new transition was observed at 418~keV, which has been tentatively associated to a $(2^{+},3^{+})\rightarrow1^{+}_{g.s.}$ transition. This fixes the relative positions of the $\beta$-decaying $4^{+}$ and $1^{+}$ states in $^{62}$Mn for the first time. Population of the $2^{+}_{1}$ state was observed in $^{62}$Fe and the cross-section determined by normalisation to the $^{109}$Ag target excitation, confirming the $B(E2)$ value measured in recoil-distance lifetime experiments.

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