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P. Roulleau

Publications and source records attributed to P. Roulleau.

At least 19 recordsLinked to original sources

Interferometry reveals spin-singlet fractional quantum Hall edges in graphene

The edge modes of spin-singlet fractional quantum Hall (FQH) phases are manifestations of multicomponent topological order and SU(2) spin symmetry. An archetype is the spin-unpolarized state at $ν$=2/3, whose edge is expected to host spatially coexisting yet counter-propagating charge and neutral spin modes. Despite efforts, its edge properties, including spin coherence and spin-charge separation, have remained elusive owing to the difficulty of resolving spins in FQH edge transport. Here, we develop a spin-sensitive probe of graphene FQH edges by using a p-n junction to interface a target FQH state with a probe integer quantum Hall (QH) state of opposite polarity. An Aharonov-Bohm (AB) interferometer forms along the interface, when the target and probe edge channels carry the same spin. We identify the spin-unpolarized and polarized edges of the $ν$=2/3 states at lower and higher magnetic fields, respectively, through spin-dependent interference. A novel multiparticle AB interference between two electrons of opposite spin emerges from spin-charge separation and recombination on the unpolarized edge, featuring a spin swap. Our results establish edge transport as a probe of spin-singlet topological orders, with implications for parafermion platforms in graphene-superconductor hybrids.

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Flying qubits Surfing on Plasmons

The rapid emergence of flying qubits in graphene and other low-dimensional conductors is pushing quantum electronics into an ultrafast regime where conventional transport theories no longer apply. In these systems, single-electron wave packets propagate coherently over micrometer scales while interacting with collective charge excitations on comparable time scales. Yet existing theoretical frameworks describe either fermionic single-particle dynamics or bosonic plasmonic modes, without reconciling the two. Here we introduce a unified theory of dynamical quantum transport that bridges this long-standing divide. Starting from a gauge-invariant scattering approach, we show how a time-dependent single-electron excitation self-consistently generates a propagating internal potential that behaves as a collective plasmonic mode. Electrons propagate at the Fermi velocity while simultaneously 'surfing' on this self-induced plasmon wave, whose velocity is renormalized by Coulomb interactions and screening. This dynamical mean-field framework captures photon-assisted transport, charge relaxation, and edge magnetoplasmon dynamics within a single description and remains valid far beyond the low-frequency limit. By unifying single-electron and plasmonic pictures, our results provide a timely foundation for the interpretation and control of flying-qubit experiments in graphene at gigahertz/terahertz frequencies.

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Enhanced shot noise in graphene quantum point contacts with electrostatic reconstruction

Shot noise measurements in quantum point contacts are a powerful tool to investigate charge transport in the integer and fractional quantum Hall regime, in particular to unveil the charge, quantum statistics and tunneling dynamics of edge excitations. In this letter, we describe shot noise measurements in a graphene quantum point contact in the quantum Hall regime. At large magnetic field, the competition between confinement and electronic interactions gives rise to a quantum dot located at the saddle point of the quantum point contact. We show that the presence of this quantum dot leads to a $50-100~\%$ increase in the shot noise, which we attribute to correlated charge tunneling. Our results highlight the role played by the electrostatic environment in those graphene devices.

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Emission and Coherent Control of Levitons in Graphene

Flying qubits encode quantum information in propagating modes instead of stationary discrete states. Although photonic flying qubits are available, the weak interaction between photons limits the efficiency of conditional quantum gates. Conversely, electronic flying qubits can use Coulomb interactions, but the weaker quantum coherence in conventional semiconductors has hindered their realization. In this work, we engineered on-demand injection of a single electronic flying qubit state and its manipulation over the Bloch sphere. The flying qubit is a Leviton propagating in quantum Hall edge channels of a high-mobility graphene monolayer. Although single-shot qubit readout and two-qubit operations are still needed for a viable manipulation of flying qubits, the coherent manipulation of an itinerant electronic state at the single-electron level presents a highly promising alternative to conventional qubits.

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Absence of heat flow in ν = 0 quantum Hall ferromagnet in bilayer graphene

The charge neutrality point of bilayer graphene, denoted as ν = 0 state, manifests competing phases marked by spontaneously broken isospin (spin/valley/layer) symmetries under external magnetic and electric fields. However, due to their electrically insulating nature, identifying these phases through electrical conductance measurements remains challenging. A recent theoretical proposal introduces a novel approach, employing thermal transport measurements to detect these competing phases. Here, we experimentally explore the bulk thermal transport of the ν = 0 state in bilayer graphene to investigate its ground states and collective excitations associated with isospin. While the theory anticipates a finite thermal conductance in the ν = 0 state, our findings unveil an absence of detectable thermal conductance. Through variations in the external electric field and temperature-dependent measurements, our results suggest towards gapped collective excitations at ν = 0 state. Our findings underscore the necessity for further investigations into the nature of ν = 0.

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Two-particle time-domain interferometry in the Fractional Quantum Hall Effect regime

Quasi-particles are elementary excitations of condensed matter quantum phases. Demonstrating that they keep quantum coherence while propagating is a fundamental issue for their manipulation for quantum information tasks. Here, we consider anyons, the fractionally charged quasi-particles 20 of the Fractional Quantum Hall Effect occurring in two-dimensional electronic conductors in high magnetic fields. They obey anyonic statistics, intermediate between fermionic and bosonic. Surprisingly, anyons show large quantum coherence when transmitted through the localized states of electronic Fabry-Pérot interferometers, but almost no quantum interference when transmitted via the propagating states of Mach-Zehnder interferometers. Here, using a novel interferometric 25 approach, we demonstrate that anyons do keep quantum coherence while propagating. Performing two-particle time-domain interference measurements sensitive to the two-particle Hanbury Brown Twiss phase, we find 53% and 60% visibilities for anyons with charges e/5 and e/3. Our results give a positive message for the challenge of performing controlled quantum coherent braiding of anyons.

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How do edge states position themselves in a quantum Hall graphene pn junction?

Recent experiments have shown that electronic Mach-Zehnder interferometers of unprecedented fidelities could be built using a graphene pn junction in the quantum Hall regime. In these junctions, two different edge states corresponding to two different valley configurations are spatially separated and form the two arms of the interferometer. The observed separation, of several tens of nanometers, has been found to be abnormally high and thus associated to unrealistic values of the exchange interaction. In this work, we show that, although the separation is due to exchange interaction, its actual value is entirely governed by the sample geometry and independent of the value of the exchange splitting. Our analysis follows the lines of the classical work of Chklovski-Shklovskii- Glazman on electrostatically induced edge state reconstruction and includes quantitative numerical calculations in the experimental geometries.

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Quantum Hall valley splitters and tunable Mach-Zehnder interferometer in graphene

Graphene is a very promising test-bed for the field of electron quantum optics. However, a fully tunable and coherent electronic beam splitter is still missing. We report the demonstration of electronic beam splitters in graphene that couple quantum Hall edge channels having opposite valley polarizations. The electronic transmission of our beam splitters can be tuned from zero to near unity. By independently setting the beam splitters at the two corners of a graphene PN junction to intermediate transmissions, we realize a fully tunable electronic Mach-Zehnder interferometer. This tunability allows us to unambiguously identify the quantum interferences due to the Mach-Zehnder interferometer, and to study their dependence with the beam-splitter transmission and the interferometer bias voltage. The comparison with conventional semiconductor interferometers points towards universal processes driving the quantum decoherence in those two different 2D systems, with graphene being much more robust to their effect.

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Unveiling excitonic properties of magnons in a quantum Hall ferromagnet

Magnons enable transferring a magnetic moment or spin over macroscopic distance. In quantum Hall ferromagnet, it has been predicted in the early 90s that spin and charges are entangled, meaning that any change of the spin texture modifies the charge distribution. As a direct consequence of this entanglement, magnons carry an electric dipole moment. Here we report the first evidence of the existence of this electric dipole moment in a graphene quantum Hall ferromagnet using a Mach-Zehnder interferometer as a quantum sensor. By propagating towards the interferometer through an insulating bulk, the magnon electric dipole moment modifies the Aharonov-Bohm flux through the interferometer, changing both its phase and its visibility. In particular, we relate the phase shift to the sign of this electric dipole moment, and the exponential loss of visibility to the flux of emitted magnons. Finally, we probe the emission energy threshold of the magnons close to filling factor v=1. Approaching v=0, we observe that the emission energy threshold diminishes towards zero, which might be linked to the existence of gapless mode in the canted-antiferromagnetic (CAF) phase at v=0. The detection and manipulation of magnons based on their electric dipole open the field for a new type of coherent magnon quantum circuits that will be electrostatically controlled.

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Relaxation and revival of quasiparticles injected in an interacting quantum Hall liquid

The one-dimensional, chiral edge channels of the quantum Hall effect are a promising platform in which to implement electron quantum optics experiments; however, Coulomb interactions between edge channels are a major source of decoherence and energy relaxation. It is therefore of large interest to understand the range and limitations of the simple quantum electron optics picture. Here we confirm experimentally for the first time the predicted relaxation and revival of electrons injected at finite energy into an edge channel. The observed decay of the injected electrons is reproduced theoretically within a Tomonaga-Luttinger liquid framework, including an important dissipation towards external degrees of freedom. This gives us a quantitative empirical understanding of the strength of the interaction and the dissipation.

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A Josephson frequency for fractionally charged anyons

Anyons occur in two-dimensional electron systems as excitations with fractional charge in the topologically ordered states of the Fractional Quantum Hall Effect (FQHE). Their dynamics are of utmost importance for topological quantum phases and possible decoherence free quantum information approaches, but observing these dynamics experimentally is challenging. Here we report on a dynamical property of anyons: the long predicted Josephson relation fJ=e*V/h for charges e*=e/3 and e/5, where e is the charge of the electron and h is Planck's constant. The relation manifests itself as marked signatures in the dependence of Photo Assisted Shot Noise (PASN) on voltage V when irradiating contacts at microwaves frequency fJ. The validation of FQHE PASN models indicates a path towards realizing time-resolved anyon sources based on levitons.

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Quantum Hall effect in epitaxial graphene with permanent magnets

We have observed the well-kown quantum Hall effect (QHE) in epitaxial graphene grown on silicon carbide (SiC) by using, for the first time, only commercial NdFeB permanent magnets at low temperature. The relatively large and homogeneous magnetic field generated by the magnets, together with the high quality of the epitaxial graphene films, enables the formation of well-developed quantum Hall states at Landau level filling factors $ν=\pm 2$, commonly observed with superconducting electro-magnets. Furthermore, the chirality of the QHE edge channels can be changed by a top gate. These results demonstrate that basic QHE physics are experimentally accessible in graphene for a fraction of the price of conventional setups using superconducting magnets, which greatly increases the potential of the QHE in graphene for research and applications.

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Photon-assisted shot noise in graphene in the Terahertz range

When subjected to electromagnetic radiation, the fluctuation of the electronic current across a quantum conductor increases. This additional noise, called photon-assisted shot noise, arises from the generation and subsequent partition of electron-hole pairs in the conductor. The physics of photon-assisted shot noise has been thoroughly investigated at microwave frequencies up to 20 GHz, and its robustness suggests that it could be extended to the Terahertz (THz) range. Here, we present measurements of the quantum shot noise generated in a graphene nanoribbon subjected to a THz radiation. Our results show signatures of photon-assisted shot noise, further demonstrating that hallmark time-dependant quantum transport phenomena can be transposed to the THz range.

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Shot noise generated by graphene p-n junctions in the quantum Hall effect regime

Owing to a linear and gapless band structure and a tunability of the charge carrier type, graphene offers a unique system to investigate transport of Dirac Fermions at p-n junctions (PNJs). In a magnetic field, combination of quantum Hall physics and the characteristic transport across PNJs leads to a fractionally quantized conductance associated with the mixing of electron-like and hole-like modes and their subsequent partitioning. The mixing and partitioning suggest that a PNJ could be used as an electronic beam-splitter. Here we report the shot noise study of the mode mixing process and demonstrate the crucial role of the PNJ length. For short PNJs, the amplitude of the noise is consistent with an electronic beam-splitter behavior, whereas, for longer PNJs, it is reduced by the energy relaxation. Remarkably, the relaxation length is much larger than typical size of mesoscopic devices, encouraging using graphene for electron quantum optics and quantum information processing.

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Robust quantum coherence above the Fermi sea

In this paper we present an experiment where we measured the quantum coherence of a quasiparticle injected at a well-defined energy above the Fermi sea into the edge states of the integer quantum Hall regime. Electrons are introduced in an electronic Mach-Zehnder interferometer after passing through a quantum dot that plays the role of an energy filter. Measurements show that above a threshold injection energy, the visibility of the quantum interferences is almost independent of the energy. This is true even for high energies, up to 130~$μ$eV, well above the thermal energy of the measured sample. This result is in strong contradiction with our theoretical predictions, which instead predict a continuous decrease of the interference visibility with increasing energy. This experiment raises serious questions concerning the understanding of excitations in the integer quantum Hall regime.

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Intrinsic and extrinsic decay of edge magnetoplasmons in graphene

We investigate intrinsic and extrinsic decay of edge magnetoplasmons (EMPs) in graphene quantum Hall (QH) systems by high-frequency electronic measurements. From EMP resonances in disk shaped graphene, we show that the dispersion relation of EMPs is nonlinear due to interactions, giving rise to intrinsic decay of EMP wavepacket. We also identify extrinsic dissipation mechanisms due to interaction with localized states in bulk graphene from the decay time of EMP wavepackets. We indicate that, owing to the unique linear and gapless band structure, EMP dissipation in graphene can be lower than that in GaAs systems.

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Fractionalization of minimal excitations in integer quantum Hall edge channels

A theoretical study of the single electron coherence properties of Lorentzian and rectangular pulses is presented. By combining bosonization and the Floquet scattering approach, the effect of interactions on a periodic source of voltage pulses is computed exactly. When such excitations are injected into one of the channels of a system of two copropagating quantum Hall edge channels, they fractionalize into pulses whose charge and shape reflects the properties of interactions. We show that the dependence of fractionalization induced electron/hole pair production in the pulses amplitude contains clear signatures of the fractionalization of the individual excitations. We propose an experimental setup combining a source of Lorentzian pulses and an Hanbury Brown and Twiss interferometer to measure interaction induced electron/hole pair production and more generally to reconstruct single electron coherence of these excitations before and after their fractionalization.

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Coherent Electron-Phonon Coupling in Tailored Quantum Systems

The coupling between a two-level system and its environment leads to decoherence. Within the context of coherent manipulation of electronic or quasiparticle states in nanostructures, it is crucial to understand the sources of decoherence. Here, we study the effect of electron-phonon coupling in a graphene and an InAs nanowire double quantum dot. Our measurements reveal oscillations of the double quantum dot current periodic in energy detuning between the two levels. These periodic peaks are more pronounced in the nanowire than in graphene, and disappear when the temperature is increased. We attribute the oscillations to an interference effect between two alternative inelastic decay paths involving acoustic phonons present in these materials. This interpretation predicts the oscillations to wash out when temperature is increased, as observed experimentally.

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