arXiv subjects

P. Ryan

Publications and source records attributed to P. Ryan.

At least 19 recordsLinked to original sources

arXiv2026

Antiferromagnetic order and lattice response in DyCuAs$_2$

We report high-resolution synchrotron X-ray diffraction and X-ray resonant magnetic scattering (XRMS) studies of the low-temperature crystal and magnetic structures of DyCuAs$_2$, a member of the \RE{}CuAs$_2$ family exhibiting a resistivity minimum above the antiferromagnetic transition temperature. Synchrotron diffraction measurements reveal that DyCuAs$_2$ preserves tetragonal symmetry down to low temperature within the experimental resolution, although pronounced anomalies in both lattice parameters $a$ and $c$ are observed near the antiferromagnetic transition temperature, $T_{\mathrm N}\approx7$~K, indicating strong magnetoelastic coupling. XRMS measurements at the Dy $L_3$ edge establish commensurate antiferromagnetic ordering below $T_{\mathrm N}$ with AFM Bragg peaks at \qq{} = (0, 0, 0.5). Representation analysis and calculations of the AFM Bragg peak intensities identify the magnetic structure as the $\Gamma_{10}$ representation, consisting of in-plane Dy moments stacked along the \cc{} axis in a $++--$ sequence. The magnetic structure is therefore identical to that previously reported for SmCuAs$_2$. Comparison among DyCuAs$_2$, SmCuAs$_2$, and GdCuAs$_2$ suggests that in-plane AFM order and the associated magnetic frustration on the tetragonal lattice are closely connected to the emergence of the resistivity minimum in the \RE{}CuAs$_2$ family. At the same time, the enhanced lattice response and stronger magnetic-field sensitivity observed in DyCuAs$_2$ imply that magnetoelastic and spin-orbit interactions additionally play important roles in determining the robustness of this anomalous transport behavior.

cond-mat.str-el↗

arXiv2026

Evidence for parity violation in gravitational fields

Discrete symmetries in gravity have only been tested for low energy, non-relativistic matter, confirming the perfectly symmetric general relativity. A hint for high energy $\cal{CP}$ violation in gravitational fields has recently been found in the HERA Compton polarimeter's two spectra, measured with electron and positron beams. Here we report results of the analysis of the same polarimeter's 314896 spectra, acquired during 2004--2007 and tagged by laser polarization states allowing the separation of charge ($\cal C$) and space parity ($\cal P$) contributions. The measured Compton edge energy asymmetry, induced by the laser helicity flips, is as high as $(4.9\pm0.5)\cdot10^{-5}$ which corresponds to a helicity-dependent difference in the gravitational potentials of $(1.7\pm0.2)\cdot10^{-14}$. In the case of the observed anomalous coupling's energy independence, the spin asymmetric gravity will contribute to the galactic rotational curves. Further analysis and calculations can determine whether the observed magnitude of the gravitational parity violation is sufficient for detaching this famous phenomena from the dark matter theory.

hep-ex↗

arXiv2026

Initial observations in X-point target divertor discharges on MAST-U

The first high-power (> 3 MW) H-mode experiments using a double-null X-point-target (XPT) divertor configuration have been performed on MAST-U. The XPT geometry is obtained by combining a large strike point radius, similar to the Super-X divertor (SXD), with an additional X-point near the separatrix in the baffled outer divertor chambers and leads to additional exhaust benefits over the SXD. The broader electron density profile near the secondary X-point leads to additional plasma-neutral interactions, evidenced by a broader hydrogenic emission profile, and resulting in larger power and ion sinks. The increase in plasma-neutral interactions also leads to lower target electron temperatures and heat fluxes. These benefits appear to extend to transients, and preliminary evidence of improved ELM buffering in the XPT is presented. These results showcase how multiple alternative divertor configuration strategies can be combined to improve momentum, power, and particle losses, which may be required for the challenging exhaust conditions of future reactors.

physics.plasm-ph↗

arXiv2024

Ion Temperature Measurements in the MAST-U Divertor During Steady State Plasmas and ELM Burn Through Phenomena

This study presents ion temperature ($T_i$) measurements in the MAST-U divertor, using a Retarding Field Energy Analyzer (RFEA). Steady state measurements were made during an L-Mode plasma with the strike point on the RFEA. ELM measurements were made with the strike point swept over the RFEA. The scenarios are characterized by a plasma current ($I_p$) of 750 kA, line average electron density ($n_e$) between $1.6 \times 10^{19}$ and $4.5 \times 10^{19}\,\text{m}^{-3}$, and Neutral Beam Injection (NBI) power ranging from 1.1 MW to 1.6 MW. The ion temperatures, peaking at approximately 10 eV in steady state, were compared with electron temperatures ($T_e$) obtained from Langmuir probes (LP) at the same radial positions. Preliminary findings reveal a $T_i/T_e$ ratio in the divertor region less than 1 for shot 48008. High temporal resolution measurements captured the dynamics of Edge Localized Modes (ELMs) Burn Through, providing $T_i$ data as a radial distance from the probe peaking around 20 eV.

physics.plasm-ph↗

arXiv2024

A novel understanding of the role of plasma-molecular kinetics on divertor power exhaust

During detachment, a buffer of neutral atoms and molecules builds up between the target and the ionising plasma. Collisions between the plasma and the molecules play an important role in the detachment process. Studies of plasma-molecular kinetics indicate that the gas temperature is increased during detachment for a wide range of conditions on the MAST-U and TCV tokamaks. This is related to an increased $\mathrm{D}_2$ lifetime during detachment, leading to more plasma-molecule collisions that raise the molecular temperature. Such collisions subsequently result in significant power and momentum losses to the divertor plasma during detachment. Using a simplified inference, these losses are estimated using the rotational temperature, neutral pressure and ionisation front position. Significant power losses (about $10\%$ of $P_{SOL}$) and dominant momentum losses (majority of the upstream pressure) from plasma-molecule collisions are inferred experimentally in long-legged, strongly baffled, detached divertors (MAST-U Super-X divertor), consistent with SOLPS-ITER simulations. The vibrational distribution obtained is compared to a collisional-radiative model setup using the same rate data as SOLPS-ITER, indicating some qualitative agreements and disagreements, potentially highlighting model gaps with regard to the default rates used. These interpretations highlight the importance of plasma-molecular collisions, leading to power and momentum losses during detachment. Our analysis and reduced modelling of these processes provide further insights into detachment control observations, the workings of long-legged divertors and divertor power balance.

physics.plasm-ph↗

arXiv2024

2D electron density profile evolution during detachment in Super-X divertor L-mode discharges on MAST-U

2D electron density profiles obtained from coherence imaging spectroscopy in different MAST-U divertor conditions are compared. The data includes variations of strike point position, core electron density, and heating power. The improved performance of the long-legged divertors results in a lower electron density and particle flux at the target compared to configurations with smaller strike point major radius, while also being characterized by lower temperatures and deeper detachment. Comparisons against SOLPS simulations generally show good agreement in profile shape along and across the separatrix. The peaking of the electron density downstream of the detachment front is associated with significant neutral drag acting on the plasma flow.

physics.plasm-ph↗

arXiv2024

First Ion Temperature Measurements in the MAST-U Divertor via Retarding Field Energy Analyzer

This study presents the first ion temperature ($T_i$) measurements from the MAST-U divertor using a Retarding Field Energy Analyzer (RFEA). Embedded within the flat tile of the closed divertor chamber, the RFEA captures $T_i$ profiles across various plasma scenarios, including transitions to the Super-X configuration. Measurements were conducted under steady-state and transient plasma conditions characterized by a plasma current ($I_p$) of 750 kA, electron density ($n_e$) between $2.2 \times 10^{19}$ and $4.45 \times 10^{19}\,\text{m}^{-3}$, and Neutral Beam Injection (NBI) power ranging from 3.0 MW to 3.2 MW. The ion temperatures, peaking at approximately 17 eV in steady state, were compared with electron temperatures ($T_e$) obtained from Langmuir probes (LP) at identical radial positions. The study also examined ion saturation current density ($J_{\text{sat}}$) signals to using methodologies similar to previous MAST experiments. Preliminary findings reveal a $T_i/T_e$ ratio ranging from 1 to 2.2. Additionally, high temporal resolution measurements (100 $\mu s$) captured the dynamics of Edge Localized Modes (ELMs), showing $T_i$ peaks at 16.03 +- 1.84 eV during ELM events, nearly three times higher than inter-ELM temperatures.

physics.plasm-ph↗

arXiv2023

Investigations of atomic \& molecular processes of NBI-heated discharges in the MAST Upgrade Super-X divertor with implications for reactors

This experimental study presents an in-depth investigation of the performance of the MAST-U Super-X divertor during NBI-heated operation (up to 2.5 MW) focussing on volumetric ion sources and sinks as well as power losses during detachment. The particle balance and power loss analysis revealed the crucial role of Molecular Activated Recombination and Dissociation (MAR and MAD) ion sinks in divertor particle and power balance, which remain pronounced in the change from ohmic to higher power (NBI heated) L-mode conditions. The importance of MAR and MAD remains with double the absorbed NBI heating. MAD results in significant power dissipation (up to $\sim 20 \%$ of $P_{SOL}$), mostly in the cold ($T_e < 5$ eV) detached region. Theoretical and experimental evidence is found for the potential contribution of $D^-$ to MAR and MAD, which warrants further study. These results suggest that MAR and MAD can be relevant in higher power conditions than the ohmic conditions studied previously. Post-processing reactor-scale simulations shows that MAR and MAD can play a significant role in divertor physics and synthetic diagnostic signals of reactor-scale devices, which are currently underestimated in exhaust simulations. This raises implications for the accuracy of reactor-scale divertor simulations of particularly tightly baffled (alternative) divertor configurations.

physics.plasm-ph↗

arXiv2023

Divertor shaping with neutral baffling as a solution to the tokamak power exhaust challenge

Exhausting power from the hot fusion core to the plasma-facing components is one of the biggest challenges in fusion energy. The MAST Upgrade tokamak uniquely integrates strong containment of neutrals within the exhaust area (divertor) with extreme divertor shaping capability. By systematically altering the divertor shape, this study shows the strongest evidence to date that long-legged divertors with a high magnetic field gradient (total flux expansion) deliver key power exhaust benefits without adversely impacting the hot fusion core. These benefits are already achieved with relatively modest geometry adjustments that are more feasible to integrate in reactor designs. Benefits include reduced target heat loads and improved access to, and stability of, a neutral gas buffer that 'shields' the target and enhances power exhaust (detachment). Analysis and model comparisons shows these benefits are obtained by combining multiple shaping aspects: long-legged divertors have expanded plasma-neutral interaction volume that drive reductions in particle and power loads, while total flux expansion enhances detachment access and stability. Containing the neutrals in the exhaust area with physical structures further augments these shaping benefits. These results demonstrate strategic variation in the divertor geometry and magnetic topology is a potential solution to one of fusion's biggest challenges: power exhaust.

physics.plasm-ph↗

arXiv2023

Initial Fulcher band observations from high resolution spectroscopy in the MAST-U divertor

High resolution Fulcher band spectroscopy was used in the MAST-U divertors during Super-X and elongated conventional divertor density ramps with $\text{D}_{2}$ fuelling from the mid-plane high-field side. In the Super-X case (density ramp from Greenwald fraction 0.12 to 0.24), the upper divertor showed ground state rotational temperatures of the $\text{D}_{2}$ molecules increasing from $\sim$6000 K, starting at the detachment onset, to $\sim$9000 K during deepening detachment. This was correlated with the movement of the Fulcher emission region, which is correlated with the ionisation source. The increase in rotational temperature did not occur near the divertor entrance, where the plasma was still ionising. Qualitative agreement was obtained between the lower and upper divertor. Similar rotational temperatures were obtained in the elongated divertor before the detachment onset, although the increase in rotational temperature during detachment was less clearly observed as less deep detachment was obtained. %In the elongated conventional divertor there was some qualitative agreement of this effect impeded by low signal. The measured vibrational distribution of the upper Fulcher state (first four bands) does not agree with a ground state Boltzmann distribution but shows a different characteristic with an elevated population especially in the $\nu = 2$ and $\nu = 3$ bands. The populations of the $\nu = 2$ and $\nu = 3$ band relative to the $\nu = 0$ band are roughly proportional to the $\textit{rotational}$ temperature.

physics.plasm-ph↗

arXiv2015

Response to Comment (arXiv:1506.02787v1) on Selective Interface Control of Order Parameters in Complex Oxides

In response to Lu et al, (arXiv:1506.02787v1), here we present a detailed writeup concerning the questions raised in their comment on our eprint (arXiv:1505.07451). The key question raised by Lu et al was if the bulk-like charge ordered state becomes indetectable with resonant scattering due to ultrathin film thickness. In this reply, we first detail the relation of our work to past work on the same compound by Staub et al to demonstrate that the presented data are indeed sufficient to support our claims of no charge order on ultra thin films of NdNiO3 (NNO) on NdGaO3 (NGO). Further, we demonstrate that if a well defined charge ordered phase exists in ultra thin films, it is indeed resolvable such as that in EuNiO3 (ENO).

cond-mat.str-el↗

arXiv2015

Engineered Mott ground state in LaTiO$_{3+\delta}$/LaNiO$_3$ heterostructure

In pursuit of creating cuprate-like electronic and orbital structures, artificial heterostructures based on LaNiO$_3$ have inspired a wealth of exciting experimental and theoretical results. However, to date there is a very limited experimental understanding of the electronic and orbital states emerging after interfacial charge-transfer and their connections to the modified band structure at the interface. Towards this goal, we have synthesized a prototypical superlattice composed of correlated metal LaNiO$_3$ and doped Mott insulator LaTiO$_{3+\delta}$, and investigated its electronic structure by resonant X-ray absorption spectroscopy combined with X-ray photoemission spectroscopy, electrical transport and theory calculations. The heterostructure exhibits interfacial charge-transfer from Ti to Ni sites giving rise to an insulating ground state with orbital polarization and $e_\textrm{g}$ orbital band splitting. Our findings demonstrate how the control over charge at the interface can be effectively used to create exotic electronic, orbital and spin states.

cond-mat.str-el↗

arXiv2015

Epitaxial Growth of (1 1 1)-Oriented Spinel CoCr$_2$O$_4$/Al$_2$O$_3$ Heterostructures

High quality (1 1 1)-oriented CoCr$_2$O$_4$/Al$_2$O$_3$ heterostructures were synthesized on the sapphire (0 0 0 1) single crystal substrates in a layer-by-layer mode. The structural properties are demonstrated by $in$-$situ$ reflection high energy electron diffraction, atomic force microscopy, X-ray reflectivity and X-ray diffraction. X-ray photoemission spectroscopy confirms that the films possess the proper chemical stoichiometry. This work offers a pathway to fabricating spinel type artificial quasi-two-dimensional frustrated lattices by means of geometrical engineering.

cond-mat.str-el↗

arXiv2014

Epitaxial stabilization of ultra thin films of electron doped manganites

Ultra-thin films of the electron doped manganite La$_{0.8}$Ce$_{0.2}$MnO$_3$ were grown in a layer-by-layer growth mode on SrTiO$_3$ (001) substrates by pulsed laser interval deposition. High structural quality and surface morphology was confirmed by a combination of synchrotron based x-ray diffraction and atomic force microscopy. Resonant X-ray absorption spectroscopy measurements confirm the presence of Ce$^{+4}$ and Mn$^{+2}$ ions. In addition, the electron doping signature was corroborated by Hall effect measurements. All grown films show ferromagnetic ground state as revealed by both XMCD and magnetoresistance measurements and remain insulating contrary to earlier reports of metal-insulator transition. Our results hint at the possibility of electron-hole asymmetry in the colossal magnetoresistive (CMR) manganite phase diagram akin to high-$T_c$ cuprates.

cond-mat.str-el↗

arXiv2012

Metal-insulator transition and orbital reconstruction in Mott quantum wells of NdNiO$_{3}$

The metal-insulator transition (MIT) and the underlying electronic and orbital structure in $e_{g}^{1}$ quantum wells based on NdNiO$_{3}$ was investigated by d.c. transport and resonant soft x-ray absorption spectroscopy. By comparing quantum wells of the same dimension but with two different confinement structures, we explicitly demonstrate that the quantum well boundary condition of correlated electrons is critical to selecting the many-body ground state. In particular, the long-range orderings and the MIT are found to be strongly enhanced under quantum confinement by sandwiching NdNiO$_{3}$ with the wide-gap dielectric LaAlO$_{3}$, while they are suppressed when one of the interfaces is replaced by a surface (interface with vacuum). Resonant spectroscopy reveals that the reduced charge fluctuations in the sandwich structure are supported by the enhanced propensity to charge ordering due to the suppressed $e_g$ orbital splitting when interfaced with the confining LaAlO$_{3}$ layer.

cond-mat.str-el↗

arXiv2011

Quantum confinement of Mott electrons in ultrathin LaNiO3/LaAlO3 superlattice

We investigate the electronic reconstruction in (LaNiO$_{3}$)$_n$/(LaAlO$_{3}$)$_3$ (n=3, 5 and 10) superlattices due to the quantum confinement (QC) by d.c. transport and resonant soft x-ray absorption spectroscopy. In proximity to the QC limit, a Mott-type transition from an itinerant electron behavior to a localized state is observed. The system exhibits tendency towards charge-order during the transition. ab initio cluster calculations are in good agreement with the absorption spectra, indicating that the apical ligand hole density is highly suppressed resulting in a strong modification of the electronic structure. At the dimensional crossover cellular dynamical-mean-field calculations support the emergence of a Mott insulator ground state in the heterostructured ultra-thin slab of LaNiO$_{3}$.

cond-mat.str-el↗

arXiv2010

Orbital control in strained ultra-thin LaNiO$_3$/LaAlO$_3$ superlattices

In pursuit of rational control of orbital polarization, we present a combined experimental and theoretical study of single unit cell superlattices of the correlated metal LaNiO$_3$ and the band insulator LaAlO$_3$. Polarized x-ray absorption spectra show a distinct asymmetry in the orbital response under strain. A splitting of orbital energies consistent with octahedral distortions is found for the case of compressive strain. In sharp contrast, for tensile strain, no splitting is found although a strong orbital polarization is present. Density functional theory calculations including a Hubbard U term reveal that this asymmetry is a result of the interplay of strain and confinement induces octahedral rotations and distortions and altered covalency in the bonding across the interfacial Ni-O-Al apical oxygen, leading to a charge disporportionation at the Ni sites for tensile strain.

cond-mat.str-el↗

arXiv2010

Sub-monolayer nucleation and growth of complex oxide heterostructures at high supersaturation and rapid flux modulation

We report on the non-trivial nanoscale kinetics of the deposition of novel complex oxide heterostructures composed of a unit-cell thick correlated metal LaNiO3 and dielectric LaAlO3. The multilayers demonstrate exceptionally good crystallinity and surface morphology maintained over the large number of layers, as confirmed by AFM, RHEED, and synchrotron X-ray diffraction. To elucidate the physics behind the growth, the temperature of the substrate and the deposition rate were varied over a wide range and the results were treated in the framework of a two-layer model. These results are of fundamental importance for synthesis of new phases of complex oxide heterostructures.

cond-mat.str-el↗