arXiv subjects

P. S. Julienne

Publications and source records attributed to P. S. Julienne.

At least 19 recordsLinked to original sources

arXiv2018

Narrow-line photoassociation spectroscopy and mass-scaling of bosonic strontium

Using new experimental measurements of photoassociation resonances near the $^1\mathrm{S}_0 \rightarrow \phantom{ }^3\mathrm{P}_1$ intercombination transition in $^{84}$Sr and $^{86}$Sr, we present an updated study into the mass-scaling behavior of bosonic strontium dimers. A previous mass-scaling model [Borkowski et al., Phys. Rev. A 90, 032713 (2014)] was able to incorporate a large number of photoassociation resonances for $^{88}$Sr, but at the time only a handful of resonances close to the dissociation limit were known for $^{84}$Sr and $^{86}$Sr. In this work, we perform a more thorough measurement of $^{84}$Sr and $^{86}$Sr bound states, identifying multiple new resonances at deeper binding energies out to $E/h=-5$ GHz. We also identify several previously measured resonances that cannot be experimentally reproduced and provide alternative binding energies instead. With this improved spectrum, we develop a mass-scaled model that reproduces the observed binding energies of $^{86}$Sr and $^{88}$Sr to within 1 MHz. In order to accurately reproduce the deeper bound states, our model includes a second $1_u$ channel and more faithfully reproduces the depth of the potential. As determined by the previous mass-scaling study, $^{84}$Sr $0_u^+$ levels are strongly perturbed by the avoided crossing between the $^1\mathrm{S}_0 + \phantom{ }^3\mathrm{P}_1$ $0_u^+$ $(^3Π_u)$ and $^1\mathrm{S}_0 + \phantom{ }^1\mathrm{D}_2$ $0_u^+$ $(^1Σ_u^+)$ potential curves and therefore are not included in this mass-scaled model, but are accurately reproduced using an isotope-specific model with slightly different quantum defect parameters. In addition, the optical lengths of the $^{84}$Sr $0_u^+,\ ν=-2$ to $ν=-5$ states are measured and compared to numerical estimates to characterize their use as optical Feshbach resonances.

physics.atom-ph↗

arXiv2018

Emergence of multi-body interactions in few-atom sites of a fermionic lattice clock

Alkaline-earth (AE) atoms have metastable clock states with minute-long optical lifetimes, high-spin nuclei, and SU($N$)-symmetric interactions that uniquely position them for advancing atomic clocks, quantum information processing, and quantum simulation. The interplay of precision measurement and quantum many-body physics is beginning to foster an exciting scientific frontier with many opportunities. Few particle systems provide a window to view the emergence of complex many-body phenomena arising from pairwise interactions. Here, we create arrays of isolated few-body systems in a fermionic ${}^{87}$Sr three-dimensional (3D) optical lattice clock and use high resolution clock spectroscopy to directly observe the onset of both elastic and inelastic multi-body interactions. These interactions cannot be broken down into sums over the underlying pairwise interactions. We measure particle-number-dependent frequency shifts of the clock transition for atom numbers $n$ ranging from 1 to 5, and observe nonlinear interaction shifts, which are characteristic of SU($N$)-symmetric elastic multi-body effects. To study inelastic multi-body effects, we use these frequency shifts to isolate $n$-occupied sites and measure the corresponding lifetimes. This allows us to access the short-range few-body physics free from systematic effects encountered in a bulk gas. These measurements, combined with theory, elucidate an emergence of multi-body effects in few-body systems of sites populated with ground-state atoms and those with single electronic excitations. By connecting these few-body systems through tunneling, the favorable energy and timescales of the interactions will allow our system to be utilized for studies of high-spin quantum magnetism and the Kondo effect.

cond-mat.quant-gas↗

arXiv2018

Spectral Asymmetry of Atoms in the van der Waals Potential of an Optical Nanofiber

We measure the modification of the transmission spectra of cold $^{87}$Rb atoms in the proximity of an optical nanofiber (ONF). Van der Waals interactions between the atoms an the ONF surface decrease the resonance frequency of atoms closer to the surface. An asymmetric spectra of the atoms holds information of their spatial distribution around the ONF. We use a far-detuned laser beam coupled to the ONF to thermally excite atoms at the ONF surface. We study the change of transmission spectrum of these atoms as a function of heating laser power. A semi-classical phenomenological model for the thermal excitation of atoms in the atom-surface van der Waals bound states is in good agreement with the measurements. This result suggests that van der Waals potentials could be used to trap and probe atoms at few nanometers from a dielectric surfaces, a key tool for hybrid photonic-atomic quantum systems.

physics.atom-ph↗

arXiv2017

Incorporating the Stern-Gerlach delayed-choice quantum eraser into the undergraduate quantum mechanics curriculum

As "Stern-Gerlach first" becomes the new paradigm within the undergraduate quantum mechanics curriculum, we show how one can extend the treatment found in conventional textbooks to cover some of the exciting new developments within the quantum field. Namely, we illustrate how one can employ Dirac notation and conventional quantum rules to describe a delayed choice variant of the quantum eraser which is realized within the Stern-Gerlach framework. Covering this material, allows the instructor to reinforce notions of changes of basis functions, quantum superpositions, quantum measurement, and the complementarity principle as expressed in whether we know "which-way" information or not. It also allows the instructor to dispel common misconceptions of when a measurement occurs and when a system is in a superposition of states. We comment at the end how a similar methodology can be employed when the more conventional two-slit experiment is treated.

physics.ed-ph↗

arXiv2017

Enhancing quantum order with fermions by increasing species degeneracy

One of the challenges for fermionic cold atom experiments in optical lattices is to cool the systems to low enough temperature that they can form quantum degenerate ordered phases. In particular, there has been significant work in trying to find the antiferromagnetic phase transition of the Hubbard model in three dimensions, without success. Here, we attack this problem from a different angle by enhancing the ordering temperature via an increase in the degeneracy of the atomic species trapped in the optical lattice. In addition to developing the general theory, we also discuss some potential systems where one might be able to achieve these results experimentally.

cond-mat.quant-gas↗

arXiv2016

Isotopic shift of atom-dimer Efimov resonances in K-Rb mixtures: Critical effect of multichannel Feshbach physics

The multichannel Efimov physics is investigated in ultracold heteronuclear admixtures of K and Rb atoms. We observe a shift in the scattering length where the first atom-dimer resonance appears in the $^{41}$K-$^{87}$Rb system relative to the position of the previously observed atom-dimer resonance in the $^{40}$K-$^{87}$Rb system. This shift is well explained by our calculations with a three-body model including the van der Waals interactions, and, more importantly, the multichannel spinor physics. With only minor difference in the atomic masses of the admixtures, the shift in the atom-dimer resonance positions can be cleanly ascribed to the isolated and overlapping Feshbach resonances in the $^{40}$K-$^{87}$Rb and $^{41}$K-$^{87}$Rb systems, respectively. Our study demonstrates the role of the multichannel Feshbach physics in determining Efimov resonances in heteronuclear three-body systems.

physics.atom-ph↗

arXiv2015

Optical Feshbach resonances: Field-dressed theory and comparison with experiments

Optical Feshbach resonances (OFRs) have generated significant experimental interest in recent years. These resonances are promising for many-body physics experiments, yet the practical application of OFRs has been limited. The theory of OFRs has been based on an approximate model that fails in important detuning regimes, and the incomplete theoretical understanding of this effect has hindered OFR experiments. We present the most complete theoretical treatment of OFRs to date, demonstrating important characteristics that must be considered in OFR experiments and comparing OFRs to the well-studied case of magnetic Feshbach resonances. We also present a comprehensive treatment of the approximate OFR model, including a study of the range of validity for this model. Finally, we derive experimentally useful expressions that can be applied to real experimental data to extract important information about the resonance structure of colliding atoms.

physics.atom-ph↗

arXiv2014

Few-body physics of ultracold atoms and molecules with long-range interactions

The quantum mechanical few-body problem at ultracold energies poses severe challenges to theoretical techniques, particularly when long-range interactions are present that decay only as a power-law potential. In this paper we review the techniques and progress in studies of universal few-body physics for ultracold atoms, particularly those related to long-range interactions.

physics.atom-ph↗

arXiv2013

Precise characterization of ^6Li Feshbach resonances using trap-sideband resolved RF spectroscopy of weakly bound molecules

We have performed radio-frequency dissociation spectroscopy of weakly bound ^6Li_2 Feshbach molecules using low-density samples of about 30 molecules in an optical dipole trap. Combined with a high magnetic field stability this allows us to resolve the discrete trap levels in the RF dissociation spectra. This novel technique allows the binding energy of Feshbach molecules to be determined with unprecedented precision. We use these measurements as an input for a fit to the ^6Li scattering potential using coupled-channel calculations. From this new potential, we determine the pole positions of the broad ^6Li Feshbach resonances with an accuracy better than 7 \times 10^{-4} of the resonance widths. This eliminates the dominant uncertainty for current precision measurements of the equation of state of strongly interacting Fermi gases. For example, our results imply a corrected value for the Bertsch parameter ξmeasured by Ku et al. [Science 335, 563 (2012)], which is ξ= 0.370(5)(8).

cond-mat.quant-gas↗

arXiv2011

Universality of the Three-Body Parameter for Efimov States in Ultracold Cesium

We report on the observation of triatomic Efimov resonances in an ultracold gas of cesium atoms. Exploiting the wide tunability of interactions resulting from three broad Feshbach resonances in the same spin channel, we measure magnetic-field dependent three-body recombination loss. The positions of the loss resonances yield corresponding values for the three-body parameter, which in universal few-body physics is required to describe three-body phenomena and in particular to fix the spectrum of Efimov states. Our observations show a robust universal behavior with a three-body parameter that stays essentially constant.

cond-mat.quant-gas↗

arXiv2011

Systematic study of Optical Feshbach Resonances in an ideal gas

Using a narrow intercombination line in alkaline earth atoms to mitigate large inelastic losses, we explore the Optical Feshbach Resonance (OFR) effect in an ultracold gas of bosonic $^{88}$Sr. A systematic measurement of three resonances allows precise determinations of the OFR strength and scaling law, in agreement with coupled-channels theory. Resonant enhancement of the complex scattering length leads to thermalization mediated by elastic and inelastic collisions in an otherwise ideal gas. OFR could be used to control atomic interactions with high spatial and temporal resolution.

physics.atom-ph↗

arXiv2010

Feshbach resonances in the 6Li-40K Fermi-Fermi mixture: Elastic versus inelastic interactions

We present a detailed theoretical and experimental study of Feshbach resonances in the 6Li-40K mixture. Particular attention is given to the inelastic scattering properties, which have not been considered before. As an important example, we thoroughly investigate both elastic and inelastic scattering properties of a resonance that occurs near 155 G. Our theoretical predictions based on a coupled channels calculation are found in excellent agreement with the experimental results. We also present theoretical results on the molecular state that underlies the 155G resonance, in particular concerning its lifetime against spontaneous dissociation. We then present a survey of resonances in the system, fully characterizing the corresponding elastic and inelastic scattering properties. This provides the essential information to identify optimum resonances for applications relying on interaction control in this Fermi-Fermi mixture.

cond-mat.quant-gas↗

arXiv2009

Quantum-State Controlled Chemical Reactions of Ultracold KRb Molecules

How does a chemical reaction proceed at ultralow temperatures? Can simple quantum mechanical rules such as quantum statistics, single scattering partial waves, and quantum threshold laws provide a clear understanding for the molecular reactivity under a vanishing collision energy? Starting with an optically trapped near quantum degenerate gas of polar $^{40}$K$^{87}$Rb molecules prepared in their absolute ground state, we report experimental evidence for exothermic atom-exchange chemical reactions. When these fermionic molecules are prepared in a single quantum state at a temperature of a few hundreds of nanoKelvins, we observe p-wave-dominated quantum threshold collisions arising from tunneling through an angular momentum barrier followed by a near-unity probability short-range chemical reaction. When these molecules are prepared in two different internal states or when molecules and atoms are brought together, the reaction rates are enhanced by a factor of 10 to 100 due to s-wave scattering, which does not have a centrifugal barrier. The measured rates agree with predicted universal loss rates related to the two-body van der Waals length.

physics.atom-ph↗

arXiv2009

Radio-frequency dressing of multiple Feshbach resonances

We demonstrate and theoretically analyze the dressing of several proximate Feshbach resonances in Rb-87 using radio-frequency (rf) radiation. We present accurate measurements and characterizations of the resonances, and the dramatic changes in scattering properties that can arise through the rf dressing. Our scattering theory analysis yields quantitative agreement with the experimental data. We also present a simple interpretation of our results in terms of rf-coupled bound states interacting with the collision threshold.

cond-mat.quant-gas↗

arXiv2009

Two-orbital SU(N) magnetism with ultracold alkaline-earth atoms

Fermionic alkaline-earth atoms have unique properties that make them attractive candidates for the realization of novel atomic clocks and degenerate quantum gases. At the same time, they are attracting considerable theoretical attention in the context of quantum information processing. Here we demonstrate that when such atoms are loaded in optical lattices, they can be used as quantum simulators of unique many-body phenomena. In particular, we show that the decoupling of the nuclear spin from the electronic angular momentum can be used to implement many-body systems with an unprecedented degree of symmetry, characterized by the SU(N) group with N as large as 10. Moreover, the interplay of the nuclear spin with the electronic degree of freedom provided by a stable optically excited state allows for the study of spin-orbital physics. Such systems may provide valuable insights into strongly correlated physics of transition metal oxides, heavy fermion materials, and spin liquid phases.

cond-mat.quant-gas↗

arXiv2009

Improving the efficiency of ultracold dipolar molecule formation by first loading onto an optical lattice

Ultracold ground state dipolar 40K-87Rb molecules have recently been produced in a loose harmonic trap by employing a magnetic field sweep across a Feshbach resonance followed by stimulated Raman adiabatic passage [K.-K. Ni et al., Science 322, 231 (2008)]. The overall experimental efficiency for molecule formation was around 20%. We show that the efficiency can be increased to nearly 100% if one first loads the atomic gases into an optical lattice of the appropriate depth and tunes the interspecies attraction to have exactly one atom of each species at an occupied lattice site. Our proposed scheme provides a large enhancement to the dipolar molecule density even at relatively high temperatures, and avoids three-body recombination loss by preventing lattice sites from being triply occupied.

cond-mat.quant-gas↗

arXiv2009

Line shapes of optical Feshbach resonances near the intercombination transition of bosonic Ytterbium

The properties of bosonic Ytterbium photoassociation spectra near the intercombination transition $^{1}S_{0}$--$^{3}P_{1}$ are studied theoretically at ultra low temperatures. We demonstrate how the shapes and intensities of rotational components of optical Feshbach resonances are affected by mass tuning of the scattering properties of the two colliding ground state atoms. Particular attention is given to the relationship between the magnitude of the scattering length and the occurrence of shape resonances in higher partial waves of the van der Waals system. We develop a mass scaled model of the excited state potential that represents the experimental data for different isotopes. The shape of the rotational photoassociation spectrum for various bosonic Yb isotopes can be qualitatively different.

physics.atom-ph↗

arXiv2008

Ultracold polar molecules near quantum degeneracy

We report the creation and characterization of a near quantum-degenerate gas of polar $^{40}$K-$^{87}$Rb molecules in their absolute rovibrational ground state. Starting from weakly bound heteronuclear KRb Feshbach molecules, we implement precise control of the molecular electronic, vibrational, and rotational degrees of freedom with phase-coherent laser fields. In particular, we coherently transfer these weakly bound molecules across a 125 THz frequency gap in a single step into the absolute rovibrational ground state of the electronic ground potential. Phase coherence between lasers involved in the transfer process is ensured by referencing the lasers to two single components of a phase-stabilized optical frequency comb. Using these methods, we prepare a dense gas of $4\cdot10^4$ polar molecules at a temperature below 400 nK. This fermionic molecular ensemble is close to quantum degeneracy and can be characterized by a degeneracy parameter of $T/T_F=3$. We have measured the molecular polarizability in an optical dipole trap where the trap lifetime gives clues to interesting ultracold chemical processes. Given the large measured dipole moment of the KRb molecules of 0.5 Debye, the study of quantum degenerate molecular gases interacting via strong dipolar interactions is now within experimental reach.

physics.atom-ph↗