arXiv subjects

P. W. Brouwer

Publications and source records attributed to P. W. Brouwer.

At least 19 recordsLinked to original sources

arXiv2026

Observation of Ultrafast Coherent and Incoherent Spin Torques via Terahertz Spin-Hall Magnetoresistance

Spin Hall magnetoresistance (SMR) is a cornerstone effect in spintronics, enabling the electrical readout of magnetic states through spin-orbit coupling at interfaces. Despite its widespread use, experimental studies of SMR are limited to static (DC) or low-frequency (GHz) regimes, leaving the ultrafast dynamics of interfacial spin transport in the terahertz (THz) frequency window entirely unexplored. Here, we report the observation of SMR spanning from DC to 1.5 THz in the model SMR system YIG/Pt, bridging the divide between electronic transport and THz optics. We demonstrate that the SMR response exhibits a pronounced low-pass behavior, decreasing significantly with frequency and vanishing above 1.5 THz. Through a dynamic model, we reveal that this unexpected spectral decay arises from a fundamental competition between two distinct interfacial spin-magnetization coupling mechanisms: the frequency-independent coherent spin torque, and an incoherent torque mediated by thermal magnons. Our analysis shows that the reduced THz SMR signal reflects the nonzero response time of the magnon chemical potential, which facilitates the increased outflow of incoherent magnons through the interface at high frequencies. These results resolve the microscopic nature of spin-torque generation at ultrafast timescales. Crucially, this work establishes THz SMR as a powerful, non-contact methodology capable of probing spin-magnon coupling in magnetic thin films, providing the essential tool for advancing the next generation of spintronic devices, particularly those based on high-frequency antiferromagnets and emerging altermagnetic materials.

cond-mat.mes-hall↗

arXiv2026

Long-range spin-polarized Josephson effect in ballistic S/F/S junctions with precessing magnetization

We present a theory of ballistic N/F/S and S/F/S junctions with a uniformly precessing magnetization, which generates long-range equal-spin superconducting correlations [Takahashi et al., Phys. Rev. Lett. 99, 057003 (2007), Houzet, Phys. Rev. Lett. 101, 057009 (2008)]. The non-equilibrium distribution of Andreev bound states leads to a strongly non-sinusoidal current-phase relationship for large precession angles. We derive detailed results for ballistic junctions involving partially and fully polarized ferromagnets. In the fully polarized half-metal limit, the magnetization precession switches the junction from an "off" state with vanishing subgap current to an "on" state with finite Andreev conductance and finite Josephson current.

cond-mat.mes-hall↗

arXiv2023

Terahertz spin conductance probes of coherent and incoherent spin tunneling through MgO tunnel junctions

We study femtosecond spin currents through MgO tunneling barriers in CoFeB(2 nm)|MgO($d$)|Pt(2 nm) stacks by terahertz emission spectroscopy. To obtain transport information independent of extrinsic experimental factors, we determine the complex-valued spin conductance $\tilde{G}_d (ω)$ of the MgO layer (thickness d= 0-6 Å over a wide frequency range $(ω/2π=$ 0.5-8 THz). In the time $(t)$ domain,$ G_d (t)$ has an instantaneous and delayed component that point to (i) spin transport through Pt pinholes in MgO, (ii) coherent spin tunneling and (iii) incoherent resonant spin tunneling mediated by defect states in MgO. A remarkable signature of (iii) is its relaxation time that grows monotonically with $d$ to as much as 270 fs at $d= 6$ Å, in full agreement with an analytical model. Our results indicate that terahertz spin conductance spectroscopy will yield new and relevant insights into ultrafast spin transport for a wide range of materials.

physics.app-ph↗

arXiv2021

Ultrafast demagnetization of iron induced by optical vs terahertz pulses

We study ultrafast magnetization quenching of ferromagnetic iron following excitation by an optical vs a terahertz pump pulse. While the optical pump (photon energy of 3.1 eV) induces a strongly nonthermal electron distribution, terahertz excitation (~4 meV) results in a quasi-thermal perturbation of the electron population. The pump-induced spin and electron dynamics are interrogated by the magneto-optic Kerr effect (MOKE). A deconvolution procedure allows us to push the time resolution down to 130 fs, even though the driving terahertz pulse is more than 0.5 ps long. Remarkably, the MOKE signals exhibit an almost identical time evolution for both optical and terahertz pump pulses, despite the three orders of magnitude different number of excited electrons. We are able to quantitatively explain our results using a model based on quasi-elastic spin-flip scattering. It shows that in the small-perturbation limit, the rate of demagnetization of a metallic ferromagnet is proportional to the excess energy of the electrons, independent of the precise shape of their distribution. Our results reveal that the dynamics of ultrafast demagnetization and of the closely related terahertz spin transport do not depend on the pump photon energy.

physics.optics↗

arXiv2021

Laser-induced terahertz spin transport in magnetic nanostructures arises from the same force as ultrafast demagnetization

Laser-induced terahertz spin transport (TST) and ultrafast demagnetization (UDM) are central but so far disconnected phenomena in femtomagnetism and terahertz spintronics. Here, we use broadband terahertz emission spectroscopy to reliably measure both processes in one setup. We find that the rate of UDM of a single ferromagnetic metal film F has the same time evolution as the flux of TST from F into an adjacent normal-metal layer N. This remarkable agreement shows that UDM and TST are driven by the same force, which is fully determined by the state of the ferromagnet. An analytical model consistently and quantitatively explains our observations. It reveals that both UDM in F and TST in the F|N stack arise from a generalized spin voltage, which is defined for arbitrary, nonthermal electron distributions. We also conclude that contributions due to a possible temperature difference between F and N are minor and that the spin-current amplitude can, in principle, be increased by one order of magnitude. In general, our findings allow one to apply the vast knowledge of UDM to TST, thereby opening up new pathways toward large-amplitude terahertz spin currents and, thus, energy-efficient ultrafast spintronic devices.

cond-mat.mes-hall↗

arXiv2020

Continuous-Variable Tomography of Solitary Electrons

A method for characterising the wave-function of freely-propagating particles would provide a useful tool for developing quantum-information technologies with single electronic excitations. Previous continuous-variable quantum tomography techniques developed to analyse electronic excitations in the energy-time domain have been limited to energies close to the Fermi level. We show that a wideband tomography of single-particle distributions is possible using energy-time filtering and that the Wigner representation of the mixed-state density matrix can be reconstructed for solitary electrons emitted by an on-demand single-electron source. These are highly localised distributions, isolated from the Fermi sea. While we cannot resolve the pure state Wigner function of our excitations due to classical fluctuations, we can partially resolve the chirp and squeezing of the Wigner function imposed by emission conditions and quantify the quantumness of the source. This tomography scheme, when implemented with sufficient experimental resolution, will enable quantum-limited measurements, providing information on electron coherence and entanglement at the individual particle level.

cond-mat.mes-hall↗

arXiv2018

Femtosecond formation dynamics of the spin Seebeck effect revealed by terahertz spectroscopy

Understanding the transfer of spin angular momentum is essential in modern magnetism research. A model case is the generation of magnons in magnetic insulators by heating an adjacent metal film. Here, we reveal the initial steps of this spin Seebeck effect with <27fs time resolution using terahertz spectroscopy on bilayers of ferrimagnetic yttrium-iron garnet and platinum. Upon exciting the metal with an infrared laser pulse, a spin Seebeck current $j_\textrm{s}$ arises on the same ~100fs time scale on which the metal electrons thermalize. This observation highlights that efficient spin transfer critically relies on carrier multiplication and is driven by conduction electrons scattering off the metal-insulator interface. Analytical modeling shows that the electrons' dynamics are almost instantaneously imprinted onto $j_\textrm{s}$ because their spins have a correlation time of only ~4fs and deflect the ferrimagnetic moments without inertia. Applications in material characterization, interface probing, spin-noise spectroscopy and terahertz spin pumping emerge.

cond-mat.mes-hall↗

arXiv2015

Noiseless manipulation of helical edge state transport by a quantum magnet

The current through a helical edge state of a quantum-spin-Hall insulator may be fully transmitted through a magnetically gapped region due to a combination of spin-transfer torque and spin pumping [Meng {\em et al.}, Phys. Rev. B {\bf 90}, 205403 (2014)]. Using a scattering approach, we here argue that in such a system the current is effectively carried by electrons with energies below the magnet-induced gap and well below the Fermi energy. This has striking consequences, such as the absence of shot noise, an exponential suppression of thermal noise, and an obstruction of thermal transport. For two helical edges covered by the same quantum magnet, the device can act as robust noiseless current splitter.

cond-mat.mes-hall↗

arXiv2014

Time-delay matrix, midgap spectral peak, and thermopower of an Andreev billiard

We derive the statistics of the time-delay matrix (energy derivative of the scattering matrix) in an ensemble of superconducting quantum dots with chaotic scattering (Andreev billiards), coupled ballistically to $M$ conducting modes (electron-hole modes in a normal metal or Majorana edge modes in a superconductor). As a first application we calculate the density of states $ρ_0$ at the Fermi level. The ensemble average $\langleρ_0\rangle=δ_0^{-1}M[\max(0,M+2α/β)]^{-1}$ deviates from the bulk value $1/δ_0$ by an amount depending on the Altland-Zirnbauer symmetry indices $α,β$. The divergent average for $M=1,2$ in symmetry class D ($α=-1$, $β=1$) originates from the mid-gap spectral peak of a closed quantum dot, but now no longer depends on the presence or absence of a Majorana zero-mode. As a second application we calculate the probability distribution of the thermopower, contrasting the difference for paired and unpaired Majorana edge modes.

cond-mat.mes-hall↗

arXiv2013

Reentrant topological phase transitions in a disordered spinless superconducting wire

In a one-dimensional spinless p-wave superconductor with coherence length ξ, disorder induces a phase transition between a topologically nontrivial phase and a trivial insulating phase at the critical mean free path l=ξ/2. Here, we show that a multichannel spinless p-wave superconductor goes through an alternation of topologically trivial and nontrivial phases upon increasing the disorder strength, the number of phase transitions being equal to the channel number N. The last phase transition, from a nontrivial phase into the trivial phase, takes place at a mean free path l = ξ/(N+1), parametrically smaller than the critical mean free path in one dimension. Our result is valid in the limit that the wire width W is much smaller than the superconducting coherence length ξ.

cond-mat.mes-hall↗

arXiv2012

Spin and Charge Structure of the Surface States in Topological Insulators

We investigate the spin and charge densities of surface states of the three-dimensional topological insulator $Bi_2Se_3$, starting from the continuum description of the material [Zhang {\em et al.}, Nat. Phys. 5, 438 (2009)]. The spin structure on surfaces other than the 111 surface has additional complexity because of a misalignment of the contributions coming from the two sublattices of the crystal. For these surfaces we expect new features to be seen in the spin-resolved ARPES experiments, caused by a non-helical spin-polarization of electrons at the individual sublattices as well as by the interference of the electron waves emitted coherently from two sublattices. We also show that the position of the Dirac crossing in spectrum of surface states depends on the orientation of the interface. This leads to contact potentials and surface charge redistribution at edges between different facets of the crystal.

cond-mat.mes-hall↗

arXiv2012

Near-zero-energy end states in topologically trivial spin-orbit coupled superconducting nanowires with a smooth confinement

A one-dimensional spin-orbit coupled nanowire with proximity-induced pairing from a nearby s-wave superconductor may be in a topological nontrivial state, in which it has a zero energy Majorana bound state at each end. We find that the topological trivial phase may have fermionic end states with an exponentially small energy, if the confinement potential at the wire's ends is smooth. The possible existence of such near-zero energy levels implies that the mere observation of a zero-bias peak in the tunneling conductance is not an exclusive signature of a topological superconducting phase even in the ideal clean single channel limit.

cond-mat.mes-hall↗

arXiv2012

Endstates in multichannel spinless p-wave superconducting wires

Multimode spinless p-wave superconducting wires with a width W much smaller than the superconducting coherence length ξare known to have multiple low-energy subgap states localized near the wire's ends. Here we compare the typical energies of such endstates for various terminations of the wire: A superconducting wire coupled to a normal-metal stub, a weakly disordered superconductor wire and a wire with smooth confinement. Depending on the termination, we find that the energies of the subgap states can be higher or lower than for the case of a rectangular wire with hard-wall boundaries.

cond-mat.mes-hall↗

arXiv2011

Low-energy sub-gap states in multi-channel Majorana wires

One-dimensional p-wave superconductors are known to harbor Majorana bound states at their ends. Superconducting wires with a finite width W may have fermionic subgap states in addition to possible Majorana end states. While they do not necessarily inhibit the use of Majorana end states for topological computation, these subgap states can obscure the identification of a topological phase through a density-of-states measurement. We present two simple models to describe low-energy fermionic subgap states. If the wire's width W is much smaller than the superconductor coherence length ξ, the relevant subgap states are localized near the ends of the wire and cluster near zero energy, whereas the lowest-energy subgap states are delocalized if $W \gtrsim ξ$. Notably, the energy of the lowest-lying fermionic subgap state (if present at all) has a maximum for W ~ ξ.

cond-mat.mes-hall↗

arXiv2010

Aharonov-Bohm oscillations in disordered topological insulator nanowires

A direct signature of electron transport at the metallic surface of a topological insulator is the Aharonov-Bohm oscillation observed in a recent study of Bi_2Se_3 nanowires [Peng et al., Nature Mater. 9, 225 (2010)] where conductance was found to oscillate as a function of magnetic flux $ϕ$ through the wire, with a period of one flux quantum $ϕ_0=h/e$ and maximum conductance at zero flux. This seemingly agrees neither with diffusive theory, which would predict a period of half a flux quantum, nor with ballistic theory, which in the simplest form predicts a period of $ϕ_0$ but a minimum at zero flux due to a nontrivial Berry phase in topological insulators. We show how h/e and h/2e flux oscillations of the conductance depend on doping and disorder strength, provide a possible explanation for the experiments, and discuss further experiments that could verify the theory.

cond-mat.mes-hall↗

arXiv2009

Signatures of Klein tunneling in disordered graphene p-n-p junctions

We present a method for obtaining quantum transport properties in graphene that uniquely combines three crucial features: microscopic treatment of charge disorder, fully quantum mechanical analysis of transport, and the ability to model experimentally relevant system sizes. As a pertinent application we study the disorder dependence of Klein tunneling dominated transport in p-n-p junctions. Both the resistance and the Fano factor show broad resonance peaks due to the presence of quasi bound states. This feature is washed out by the disorder when the mean free path becomes of the order of the distance between the two p-n interfaces.

cond-mat.mes-hall↗

arXiv2009

Electrostatic confinement of electrons in an integrable graphene quantum dot

We compare the conductance of an undoped graphene sheet with a small region subject to an electrostatic gate potential for the cases that the dynamics in the gated region is regular (disc-shaped region) and classically chaotic (stadium). For the disc, we find sharp resonances that narrow upon reducing the area fraction of the gated region. We relate this observation to the existence of confined electronic states. For the stadium, the conductance looses its dependence on the gate voltage upon reducing the area fraction of the gated region, which signals the lack of confinement of Dirac quasiparticles in a gated region with chaotic classical electron dynamics.

cond-mat.mes-hall↗

arXiv2008

Quantum limit of the triplet proximity effect in half-metal - superconductor junctions

We apply the scattering matrix approach to the triplet proximity effect in superconductor-half metal structures. We find that for junctions that do not mix different orbital modes, the zero bias Andreev conductance vanishes, while the zero bias Josephson current is nonzero. We illustrate this finding on a ballistic half-metal--superconductor (HS) and superconductor -- half-metal -- superconductor (SHS) junction with translation invariance along the interfaces, and on HS and SHS systems where transport through the half-metallic region takes place through a single conducting channel. Our calculations for these physically single mode setups -- single mode point contacts and chaotic quantum dots with single mode contacts -- illustrate the main strength of the scattering matrix approach: it allows for studying systems in the quantum mechanical limit, which is inaccessible for quasiclassical Green's function methods, the main theoretical tool in previous works on the triplet proximity effect.

cond-mat.supr-con↗