arXiv subjects

P. W. Zhao

Publications and source records attributed to P. W. Zhao.

At least 37 records · Page 2Linked to original sources

arXiv2024

Principal components of nuclear mass models

The principal component analysis approach is employed to extract the principal components contained in nuclear mass models for the first time. The effects coming from different nuclear mass models are reintegrated and reorganized in the extracted principal components. These extracted principal components are recombined to build new mass models, which achieve better accuracy than the original theoretical mass models. This indicates that the effects contained in different mass models can work together to improve the nuclear mass predictions with the help of the principal component analysis approach.

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arXiv2024

Neutrinoless double-$β$ decay and double Gamow-Teller transitions

The neutrinoless double-$β$ ($0νββ$) decay and the double Gamow-Teller (DGT) transition are investigated with the state-of-the-art Relativistic Configuration-interaction Density functional theory. A strong linear correlation between the nuclear matrix elements (NMEs) of the $0νββ$ decay and the DGT transition is demonstrated. This linear correlation is found to originate from the similarity of the leading-order term of the $0νββ$-decay operator and the DGT-transition one, as revealed by expanding the $0νββ$-decay operator in terms of the spherical harmonics. The present results provide a strong support to constrain the $0νββ$-decay NMEs through the double charge-exchange reactions.

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arXiv2024

Ternary quasifission in collisions of actinide nuclei

The microscopic framework of time-dependent covariant density functional theory is applied to a systematic study of ternary quasifission in collisions of pairs of $^{238}$U nuclei. It is shown that the inclusion of octupole degree of freedom in the case of head-to-head collisions, extends the energy window in which ternary quasifission occurs, and greatly enhances the number of nucleons contained in a middle fragment. Dynamical pairing correlations, included here in the time-dependent BCS approximation, prevent the occurrence of ternary quasifission in head-to-head collisions, and have an effect on the location of the energy window in which a middle fragment is formed in tail-to-tail collisions. In the latter case, as well as for tail-to-side collisions, the formation of very heavy neutron-rich systems in certain energy intervals is predicted.

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arXiv2024

Multinucleon transfer with time-dependent covariant density functional theory

The microscopic framework of time-dependent covariant density functional theory is applied to study multinucleon transfer reactions, with transfer probabilities calculated using the particle number projection method. It is found that similar total cross sections are obtained with two different relativistic density functionals, PC-PK1 and DD-ME2, as well as with the Skyrme functional SLy5 in a previous study, for multinucleon transfer in the reactions: $^{40}{\rm Ca}+{}^{124}{\rm Sn}$ at $E_{\rm lab} = 170$ MeV, $^{40}{\rm Ca}+{}^{208}{\rm Pb}$ at $E_{\rm lab} = 249$ MeV, and $^{58}{\rm Ni}+{}^{208}{\rm Pb}$ at $E_{\rm lab} = 328.4$ MeV. We report the first microscopic calculation of total cross sections for the reactions: $^{40}{\rm Ar}+{}^{208}{\rm Pb}$ at $E_{\rm lab} = 256$ MeV and $^{206}{\rm Pb}+{}^{118}{\rm Sn}$ at $E_{\rm lab} = 1200$ MeV. Compared to the results obtained with the GRAZING model, the cross sections predicted by the time-dependent covariant density functional theory are in much better agreement with data, and demonstrate the potential of microscopic models based on relativistic density functionals for the description of reaction dynamics.

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arXiv2024

Generalized time-dependent generator coordinate method for induced fission dynamics

The generalized time-dependent generator coordinate method (TD-GCM) is extended to include pairing correlations. The correlated GCM nuclear wave function is expressed in terms of time-dependent generator states and weight functions. The particle-hole channel of the effective interaction is determined by a Hamiltonian derived from an energy density functional, while pairing is treated dynamically in the standard BCS approximation with time-dependent pairing tensor and single-particle occupation probabilities. With the inclusion of pairing correlations, various time-dependent phenomena in open-shell nuclei can be described more realistically. The model is applied to the description of saddle-to-scission dynamics of induced fission. The generalized TDGCM charge yields and total kinetic energy distribution for the fission of 240Pu, are compared to those obtained using the standard time-dependent density functional theory (TD-DFT) approach, and with available data.

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arXiv2023

Effects of rotation and valence nucleons in molecular-like $α$-chain nuclei

Effects of rotation and valence nucleons in molecular-like linear $α$-chain nuclei are analyzed using a three-dimensional lattice cranking model based on covariant density functional theory. The structure of $^{16}$C and $^{16}$Ne is investigated as a function of rotational frequency. The valence nucleons, with respect to the 3$α$ linear chain core of $^{12}$C, at low frequency occupy the $π$ molecular orbital. With increasing rotational frequency these nucleons transition from the $π$ orbital to the $σ$ molecular orbital, thus stabilizing the 3$α$ linear chain structure. It is predicted that the valence protons in $^{16}$Ne change occupation from the $π$ to the $σ$ molecular orbital at $\hbarω\approx 1.3$ MeV, a lower rotational frequency compared to $\hbarω\approx 1.7$ MeV for the valence neutrons in $^{16}$C. The same effects of valence protons are found in $^{20}$Mg, compared to the four valence neutrons in $^{20}$O. The model is also used to examine the effect of alignment of valence nucleons on the relative positions and size of the three $α$-clusters in $^{16}$C and $^{16}$Ne.

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arXiv2023

Generalized time-dependent generator coordinate method for small and large amplitude collective motion

An implementation of the generalized time-dependent generator coordinated method (TD-GCM) is developed, that can be applied to the dynamics of small- and large-amplitude collective motion of atomic nuclei. Both the generator states and weight functions of the GCM correlated wave function depend on time. The initial generator states are obtained as solutions of deformation-constrained self-consistent mean-field equations, and are evolved in time by the standard mean-field equations of nuclear density functional theory (TD-DFT). The TD-DFT trajectories are used as a generally non-orthogonal and overcomplete basis in which the TD-GCM wave function is expanded. The weights, expressed in terms of a collective wave function, obey a TD-GCM (integral) equation. In this explorative paper, the generalized TD-GCM is applied to the excitation energies and spreading width of giant resonances, and to the dynamics of induced fission. The necessity of including pairing correlations in the basis of TD-DFT trajectories is demonstrated in the latter example.

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arXiv2023

Shape and multiple shape coexistence of nuclei within covariant density functional theory

Shape and multiple shape coexistence of nuclei are investigated throughout the nuclear chart by calculating the low-lying spectra and the quadrupole shape invariants for even-even nuclei with $10\leq Z\leq 104$ from the proton drip line to the neutron one within a five-dimensional collective Hamiltonian based on the covariant density functional PC-PK1. The quadrupole shape invariants are implemented to characterize the quadrupole deformations of low-lying $0^+$ states and predict nuclear mass regions of shape and multiple shape coexistence. The predicted low-lying spectra and the shape or multi-shape coexisting nuclei are overall in good agreement with the available experimental results. In addition, the present work predicts a wealth of nuclei with shape or multiple shape coexistence in the neutron-rich regions. The connection between the strong $E0$ transition strength and the occurrence of shape coexistence is analyzed systemically. It is found that nuclei with pronounced shape coexistence generally have strong $E0$ transition strengths, while the reverse may not be true. The present results can serve as useful guidelines for experimental searches and theoretical studies of shape and multiple shape coexistence, especially in neutron-rich regions.

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arXiv2022

Fission dynamics, dissipation and clustering at finite temperature

The saddle-to-scission dynamics of the induced fission process is explored using a microscopic finite-temperature model based on time-dependent nuclear density functional theory (TDDFT), that allows to follow the evolution of local temperature along fission trajectories. Starting from a temperature that corresponds to the experimental excitation energy of the compound system, the model propagates the nucleons along isentropic paths toward scission. For the four illustrative cases of induced fission of $^{240}$Pu, $^{234}$U, $^{244}$Cm, and $^{250}$Cf, characteristic fission trajectories are considered, and the partition of the total energy into various kinetic and potential energy contributions at scission is analyzed, with special emphasis on the energy dissipated along the fission path and the prescission kinetic energy. The model is also applied to the dynamics of neck formation and rupture, characterized by the formation of few-nucleon clusters in the low-density region between the nascent fragments.

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arXiv2022

Multi-task learning on nuclear masses and separation energies with the kernel ridge regression

A multi-task learning (MTL) framework, called gradient kernel ridge regression, for nuclear masses and separation energies is developed by introducing gradient kernel functions to the kernel ridge regression (KRR) approach. By taking the WS4 mass model as an example, the gradient KRR network is trained with the mass model residuals, i.e., deviations between experimental and theoretical values of masses and one-nucleon separation energies, to improve the accuracy of theoretical predictions. Significant improvements are achieved by the gradient KRR approach in both the interpolation and the extrapolation predictions of nuclear masses and separation energies. This demonstrates the advantage of the present MTL framework that integrates the information of nuclear masses and separation energies and improves the predictions for both of them.

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arXiv2022

Relativistic effects and three-body interactions in atomic nuclei

Based on the leading-order covariant pionless effective field theory, a relativistic nuclear Hamiltonian is derived and solved using the variational Monte Carlo approach for $A\le 4$ nuclei by representing the nuclear many-body wave functions with a symmetry-based artificial neural network. It is found that the relativistic effects rescue the renormalizability of the theory, and overcome the energy collapse problem for $^3$H and $^4$He without promoting a repulsive three-nucleon interaction to leading order as in nonrelativistic calculations. Nevertheless, to exactly reproduce the experimental ground-state energies, a three-nucleon interaction is needed and its interplay with the relativistic effects plays a crucial role. The strongly repulsive relativistic effects suppress the energy contribution given by the three-nucleon interactions, so a strong strength for the three-nucleon interaction could be required to reproduce the experimental energies. These results shed light on a consistent understanding of relativistic effects and three-body interactions in atomic nuclei.

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arXiv2022

Dynamical synthesis of 4He in the scission phase of nuclear fission

In the exothermic process of fission decay, an atomic nucleus splits into two or more independent fragments. Several aspects of nuclear fission are not properly understood, in particular the formation of the neck between the nascent fragments, and the subsequent mechanism of scission into two or more independent fragments. Using an implementation of time-dependent density functional theory, based on a relativistic energy density functional and including pairing correlations, we analyze the final phase of the process of induced fission of $^{240}$Pu, and show that the time-scale of neck formation coincides with the assembly of two $α$-like clusters (less than 1 zs = 10$^{-21}$ s). Because of its much larger binding energy, the dynamical synthesis of 4He in the neck predominates over other light clusters, e.g., $^3$H and $^6$He. At the instant of scission the neck ruptures exactly between the two $α$-like clusters, which separate because of the Coulomb repulsion and are eventually absorbed by the two emerging fragments. The newly proposed mechanism of light charged clusters formation at scission provides a natural explanation of ternary fission.

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arXiv2022

Microscopic analysis of induced nuclear fission dynamics

The dynamics of low-energy induced fission is explored using a consistent microscopic framework that combines the time-dependent generator coordinate method (TDGCM) and time-dependent nuclear density functional theory (TDDFT). While the former presents a fully quantum mechanical approach that describes the entire fission process as an adiabatic evolution of collective degrees of freedom, the latter models the dissipative dynamics of the final stage of fission by propagating the nucleons independently toward scission and beyond. By combining the two methods, based on the same nuclear energy density functional and pairing interaction, we perform an illustrative calculation of the charge distribution of yields and total kinetic energy for induced fission of $^{240}$Pu. For the saddle-to-scission phase a set of initial points for the TDDFT evolution is selected along an iso-energy curve beyond the outer fission barrier on the deformation energy surface, and the TDGCM is used to calculate the probability that the collective wave function reaches these points at different times. Fission observables are computed with both methods and compared with available data. The relative merits of including quantum fluctuations (TDGCM) and the one-body dissipation mechanism (TDDFT) are discussed.

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arXiv2022

Configuration interaction projected density functional theory: effects of four-quasiparticle configurations and time-odd interactions

The effects of four-quasiparticle configurations and time-odd interactions are investigated in the framework of configuration interaction projected density functional theory by taking the yrast states of 60Fe as examples. Based on the universal PC-PK1 density functional, the energies of the yrast states with spin up to 20\hbar and the available B(E2) transition probabilities are well reproduced. The yrast states are predicted to be of four-quasiparticle structure above spin I = 16\hbar. The inclusion of the time-odd interactions increases the kinetic moments of inertia and delays the appearance of the first band crossing, and, thus, improves the description of the data.

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arXiv2022

Nuclear energy density functionals from machine learning

Machine learning is employed to build an energy density functional for self-bound nuclear systems for the first time. By learning the kinetic energy as a functional of the nucleon density alone, a robust and accurate orbital-free density functional for nuclei is established. Self-consistent calculations that bypass the Kohn-Sham equations provide the ground-state densities, total energies, and root-mean-square radii with a high accuracy in comparison with the Kohn-Sham solutions. No existing orbital-free density functional theory comes close to this performance for nuclei. Therefore, it provides a new promising way for future developments of nuclear energy density functionals for the whole nuclear chart.

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arXiv2022

Nuclear landscape in a mapped collective Hamiltonian from covariant density functional theory

The nuclear landscape has been investigated within the triaxial relativistic Hartree-Bogoliubov theory with the PC-PK1 density functional, and the beyond-mean-field dynamical correlation energies are taken into account by a microscopically mapped five-dimensional collective Hamiltonian without additional free parameters. The effects of triaxial deformation and dynamical correlations on the nuclear landscape are analyzed. The present results provide the best description of the experimental binding energies, in particular for medium and heavy mass regions, in comparison with the results obtained previously with other state-of-the-art covariant density functionals. The inclusion of the dynamical correlation energies plays an important role in the PC-PK1 results. It is emphasized that the nuclear landscape is considerably extended by the PC-PK1 functional in comparison with the previous results with other density functionals, which may be due to the different isovector properties in the density functionals.

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arXiv2022

Dynamics of rotation in chiral nuclei

The dynamics of chiral nuclei is investigated for the first time with the time-dependent and tilted axis cranking covariant density functional theories on a three-dimensional space lattice in a microscopic and self-consistent way. The experimental energies of the two pairs of the chiral doublet bands in $^{135}$Nd are well reproduced without any adjustable parameters beyond the well-defined density functional. A novel mechanism, i.e., chiral precession, is revealed from the microscopic dynamics of the total angular momentum in the body-fixed frame, whose harmonicity is associated with a transition from the planar into aplanar rotations with the increasing spin. This provides a fully microscopic and dynamical view to understand the chiral excitations in nuclei.

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arXiv2021

High-precision nuclear chronometer for the cosmos

Nuclear chronometer, which predicts the ages of the oldest stars by comparing the present and initial abundances of long-lived radioactive nuclides, provides an independent dating technique for the cosmos. A new nuclear chronometer called Th-U-X chronometer is proposed, which imposes stringent constraints on the astrophysical conditions in the $r$-process simulation by synchronizing the previous Th/X, U/X and Th/U chronometers. The astrophysical uncertainties of nuclear chronometer are significantly reduced from more than $\pm2$ billion years to within 0:3 billion years by the Th-U-X chronometer. The proposed chronometer is then applied to estimate the ages of the six metal-poor stars with observed uranium abundances, and the predicted ages are compatible with the cosmic age 13.8 billion years predicted from the cosmic microwave background radiation, but in contradictory with the new cosmic age 11.4 billion years from the gravitational lenses measurement.

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