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P. Walters

Publications and source records attributed to P. Walters.

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Hydrofluoric acid-free titanium etching for rare-event searches

Rare-event search experiments require construction materials with high radiopurity to minimise background contributions. Thanks to its high mechanical strength, low density, machinability, and commercial availability in relatively radiopure forms, titanium is a suitable material for structural elements in rare-event searches. In such applications, a chemical etching stage is typically performed to remove surface contamination or to prepare the surface for further treatment. However, due to its chemical resistance, the etching of titanium conventionally requires hydrofluoric acid, posing serious health and safety concerns that are further exacerbated in deep underground laboratory settings. An alternative approach is proposed, which uses sulphuric acid. Grade 1 titanium samples were etched in 20\% and 40\% sulphuric acid solutions at 20$^\circ$C and 40$^\circ$C for up to 24\,h. The effects of etching were quantified through mass change measurements, surface roughness analysis, and scanning electron microscopy. Sulphuric acid effectively etches titanium, with up to $3.5\,\pm\,0.3$ mg/cm$^2$ of titanium removed for an unagitated solution of 40\% sulphuric acid at $40^\circ$C for 24\,h. Furthermore, sulphuric acid is shown to be effective at etching at lower concentration and temperature. The formation of a passivation layer during the etching may enable control of the total mass removed.

physics.ins-det

Titanium for rare-event searches: Hydrofluoric acid-free etching

Rare-event search experiments require construction materials with high radiopurity to minimise background contributions. Thanks to its high mechanical strength, low density, machinability, and commercial availability in relatively radio-pure forms, titanium is a suitable material for structural elements in rare event searches. To remove surface deposits on materials used, a chemical etching stage is usually performed. However, the chemical resistance of titanium means that, conventionally, such etching is done with hydrofluoric acid. Hydrofluoric acid presents serious health risks to users, and such hazards are compounded in the case of construction in deep underground laboratories. An alternative chemical etching using sulphuric acid is presented. This is demonstrated to etch titanium, removing 3.7 $\mu$m of material from the surface over the course of 20 hours. Scanning electron microscopy with back-scattered electron spectroscopy was used to study the surface and contamination of the titanium, demonstrating the removal of surface contaminants after etching. The proposed method is a potential alternative to those currently employed.

physics.ins-det

Participant and spectator scaling of spectator fragments in Au+Au and Cu+Cu collisions at sqrt(sNN) = 19.6 and 22.4 GeV

Spectator fragments resulting from relativistic heavy ion collisions, consisting of single protons and neutrons along with groups of stable nuclear fragments up to Nitrogen (Z=7), are measured in PHOBOS. These fragments are observed in Au+Au (sqrt(sNN)=19.6 GeV) and Cu+Cu (22.4 GeV) collisions at high pseudorapidity ($\eta$). The dominant multiply-charged fragment is the tightly bound Helium ($\alpha$), with Lithium, Beryllium, and Boron all clearly seen as a function of collision centrality and pseudorapidity. We observe that in Cu+Cu collisions, it becomes much more favorable for the $\alpha$ fragments to be released than Lithium. The yields of fragments approximately scale with the number of spectator nucleons, independent of the colliding ion. The shapes of the pseudorapidity distributions of fragments indicate that the average deflection of the fragments away from the beam direction increases for more central collisions. A detailed comparison of the shapes for $\alpha$ and Lithium fragments indicates that the centrality dependence of the deflections favors a scaling with the number of participants in the collision.

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Phobos results on charged particle multiplicity and pseudorapidity distributions in Au+Au, Cu+Cu, d+Au, and p+p collisions at ultra-relativistic energies

Pseudorapidity distributions of charged particles emitted in $Au+Au$, $Cu+Cu$, $d+Au$, and $p+p$ collisions over a wide energy range have been measured using the PHOBOS detector at RHIC. The centrality dependence of both the charged particle distributions and the multiplicity at midrapidity were measured. Pseudorapidity distributions of charged particles emitted with $|η|<5.4$, which account for between 95% and 99% of the total charged-particle emission associated with collision participants, are presented for different collision centralities. Both the midrapidity density, $dN_{ch}/dη$, and the total charged-particle multiplicity, $N_{ch}$, are found to factorize into a product of independent functions of collision energy, $\sqrt{s_{_{NN}}}$, and centrality given in terms of the number of nucleons participating in the collision, $N_{part}$. The total charged particle multiplicity, observed in these experiments and those at lower energies, assumes a linear dependence of $(\ln s_{_{NN}})^2$ over the full range of collision energy of $\sqrt{s_{_{NN}}}$=2.7-200 GeV.

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Scaling properties in bulk and p$_{\rm T}$-dependent particle production near midrapidity in relativistic heavy ion collisions

The centrality dependence of the midrapidity charged-particle multiplicity density ($|η|$$<$1) is presented for Au+Au and Cu+Cu collisions at RHIC over a broad range of collision energies. The multiplicity measured in the Cu+Cu system is found to be similar to that measured in the Au+Au system, for an equivalent N$_{\rm part}$, with the observed factorization in energy and centrality still persistent in the smaller Cu+Cu system. The extent of the similarities observed for bulk particle production is tested by a comparative analysis of the inclusive transverse momentum distributions for Au+Au and Cu+Cu collisions near midrapidity. It is found that, within the uncertainties of the data, the ratio of yields between the various energies for both Au+Au and Cu+Cu systems are similar and constant with centrality, both in the bulk yields as well as a function of p$_{\rm T}$, up to at least 4 GeV/$c$. The effects of multiple nucleon collisions that strongly increase with centrality and energy appear to only play a minor role in bulk and intermediate transverse momentum particle production.

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System size, energy, centrality and pseudorapidity dependence of charged-particle density in Au+Au and Cu+Cu collisions at RHIC

Charged particle pseudorapidity distributions are presented from the PHOBOS experiment at RHIC, measured in Au+Au and Cu+Cu collisions at sqrt{s_NN}=19.6, 22.4, 62.4, 130 and 200 GeV, as a function of collision centrality. The presentation includes the recently analyzed Cu+Cu data at 22.4 GeV. The measurements were made by the same detector setup over a broad range in pseudorapidity, |eta|<5.4, allowing for a reliable systematic study of particle production as a function of energy, centrality and system size. Comparing Cu+Cu and Au+Au results, we find that the total number of produced charged particles and the overall shape (height and width) of the pseudorapidity distributions are determined by the number of nucleon participants, N_part. Detailed comparisons reveal that the matching of the shape of the Cu+Cu and Au+Au pseudorapidity distributions over the full range of eta is better for the same N_part/2A value than for the same N_part value, where A denotes the mass number. In other words, it is the geometry of the nuclear overlap zone, rather than just the number of nucleon participants that drives the detailed shape of the pseudorapidity distribution and its centrality dependence.

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Non-flow correlations and elliptic flow fluctuations in Au+Au collisions at sqrt(s_NN)=200GeV

We present first results on event-by-event elliptic flow fluctuations in nucleus-nucleus collisions corrected for effects of non-flow correlations where the magnitude of non-flow correlations has been independently measured in data. Over the measured range in centrality, we see large relative fluctuations of 25-50%. The results are consistent with predictions from both color glass condensate and Glauber type initial condition calculations of the event-by-event participant eccentricity fluctuations.

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The Importance of Correlations and Fluctuations on the Initial Source Eccentricity in High-Energy Nucleus-Nucleus Collisions

In this paper, we investigate various ways of defining the initial source eccentricity using the Monte Carlo Glauber (MCG) approach. In particular, we examine the participant eccentricity, which quantifies the eccentricity of the initial source shape by the major axes of the ellipse formed by the interaction points of the participating nucleons. We show that reasonable variation of the density parameters in the Glauber calculation, as well as variations in how matter production is modeled, do not significantly modify the already established behavior of the participant eccentricity as a function of collision centrality. Focusing on event-by-event fluctuations and correlations of the distributions of participating nucleons we demonstrate that, depending on the achieved event-plane resolution, fluctuations in the elliptic flow magnitude $v_2$ lead to most measurements being sensitive to the root-mean-square, rather than the mean of the $v_2$ distribution. Neglecting correlations among participants, we derive analytical expressions for the participant eccentricity cumulants as a function of the number of participating nucleons, $\Npart$,keeping non-negligible contributions up to $\ordof{1/\Npart^3}$. We find that the derived expressions yield the same results as obtained from mixed-event MCG calculations which remove the correlations stemming from the nuclear collision process. Most importantly, we conclude from the comparison with MCG calculations that the fourth order participant eccentricity cumulant does not approach the spatial anisotropy obtained assuming a smooth nuclear matter distribution. In particular, for the Cu+Cu system, these quantities deviate from each other by almost a factor of two over a wide range in centrality.

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System Size, Energy and Centrality Dependence of Pseudorapidity Distributions of Charged Particles in Relativistic Heavy Ion Collisions

We present the first measurements of the pseudorapidity distribution of primary charged particles in Cu+Cu collisions as a function of collision centrality and energy, \sqrtsnn = 22.4, 62.4 and 200 GeV, over a wide range of pseudorapidity, using the PHOBOS detector. Making a global comparison of Cu+Cu and Au+Au results, we find that the total number of produced charged particles and the rough shape (height and width) of the pseudorapidity distributions are determined by the number of nucleon participants. More detailed studies reveal that a more precise matching of the shape of the Cu+Cu and Au+Au pseudorapidity distributions over the full range of pseudorapidity occurs for the same Npart/2A value rather than the same Npart value. In other words, it is the collision geometry rather than just the number of nucleon participants that drives the detailed shape of the pseudorapidity distribution and its centrality dependence at RHIC energies.

nucl-ex