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P. Wilhelm

Publications and source records attributed to P. Wilhelm.

13 recordsLinked to original sources
arXiv2018

Photoionization of metastable heliumlike C4+(1s 2s 3S1) ions: Precision study of intermediate doubly excited states

In a joint experimental and theoretical endeavour, photoionization of metastable C4+(1s 2s 3S1) ions via intermediate levels with hollow, double-K-vacancy configurations 2s2p, 2s3p, 2p3s, 2p3d, 2s4p, 2p4s and 2p4d has been investigated. High-resolution photon-ion merged-beams measurements were carried out with the resolving power reaching up to 25,000 which is sufficient to separate the leading fine-structure components of the 2s2p 3P term. Many-body perturbation theory was employed to determine level-to-level cross sections for K-shell excitation with subsequent autoionization. The resonance energies were calculated with inclusion of electron correlation and radiative contributions. Their uncertainties are estimated to be below $\pm$1 meV. Detailed balance confirms the present photoionization cross-section results by comparison with previous dielectronic-recombination measurements. The high accuracy of the theoretical transition energies together with the present experimental results qualify photoabsorption resonances in heliumlike ions as new, greatly improved energy-reference standards at synchrotron radiation facilities.

physics.atom-ph↗
arXiv2016

Molecular polygons probe the role of intramolecular strain in the photophysics of pi-conjugated chromophores

Pi-conjugated segments - chromophores - constitute the electronically active units of polymer materials used in organic electronics. To elucidate the effect of bending of these linear moieties on elementary electronic properties such as luminescence colour and radiative rate we introduce a series of molecular polygons. The pi-system in these molecules becomes so distorted in bichromophores (digons) that these absorb and emit light of arbitrary polarisation: any part of the chain absorbs and emits radiation with equal probability. Bending leads to a cancellation of transition dipole moment (TDM), increasing excited-state lifetime. Simultaneously, fluorescence shifts to the red as radiative transitions require mixing of the excited state with vibrational modes. However, strain can become so large that excited-state localisation on shorter units of the chain occurs, compensating TDM cancellation. Since these effects counteract, underlying correlations between shape and photophysics can only be resolved in single molecules.

physics.chem-ph↗
arXiv1997

Meson retardation in deuteron photodisintegration above pi-threshold

Photodisintegration of the deuteron above pi-threshold is studied in a coupled channel approach including N Delta- and pi d-channels with pion retardation in potentials and exchange currents. A much improved description of total and differential cross sections in the energy region between pi-threshold and 400-450 MeV is achieved.

nucl-th↗
arXiv1997

On the extraction of electromagnetic properties of the Delta(1232) excitation from pion photoproduction

Several methods for the treatment of pion photoproduction in the region of the Delta(1232) resonance are discussed, in particular the effective Lagrangian approach and the speed plot analysis are compared to a dynamical treatment. As a main topic, we discuss the extraction of the genuine resonance parts of the magnetic dipole and electric quadrupole multipoles of the electromagnetic excitation of the resonance. To this end, we try to relate the various values for the ratio R_{EM} of the E2 to M1 multipole excitation strengths for the Delta(1232) resonance as extracted by the different methods to corresponding ratios of a dynamical model. Moreover, it is confirmed that all methods for extracting resonance properties suffer from an unitary ambiguity which is due to some phenomenological contributions entering the models.

nucl-th↗
arXiv1997

Unitarity constraint for threshold coherent pion photoproduction on the deuteron and chiral perturbation theory

The contribution of the two-step process gamma + d -> p + n -> pi0 + d to the imaginary part of the amplitude for coherent pion production on the deuteron is calculated exploiting unitarity constraints. The result shows that this absorptive process is not negligible and has to be considered in an extraction of the elementary neutron production amplitude from the gamma + d -> pi0 + d cross section at threshold. In addition, it is argued that a consistent calculation of gamma + d -> pi0 + d in baryon chiral perturbation theory beyond next-to-leading order requires the inclusion of this absorptive process.

nucl-th↗
arXiv1997

Treatment of the $\Delta$ current in electromagnetic two-nucleon knockout reactions

The contribution of the $\Delta$(1232) isobar to the electromagnetic current of the two-nucleon system and its role in ($\gamma$,NN) processes is investigated. The difference between the genuine $\Delta$-excitation current and that part of the current connected to the deexcitation of a preformed $\Delta$ in the target nucleus is stressed. The latter cannot lead to a resonant behaviour of matrix elements for energies in the $\Delta$ region. The reaction $^{16}O(\gamma,pp)^{14}C$, where the $\Delta$ contribution is dominant at intermediate energies, is considered. The large variations found in the cross sections for different treatments stress the need for a proper treatment of the $\Delta$ current for a clear understanding of the reaction mechanism of two-nucleon emission processes.

nucl-th↗
arXiv1997

On the Gerasimov-Drell-Hearn sum rule for the deuteron

The Gerasimov-Drell-Hearn sum rule is evaluated for the deuteron by explicit integration up to a photon energy of 550 MeV including contributions from the photodisintegration channel and from coherent and incoherent single pion production as well. The photodisintegration channel converges fast enough in this energy range and gives a large negative contribution, essentially from the $^1S_0$ resonant state near threshold. Its absolute value is about the same size than the sum of proton and neutron GDH values. It is only partially cancelled by the single pion production contribution. But the incoherent channel has not reached convergence at 550 MeV.

nucl-th↗
arXiv1996

Quasifree pion photoproduction on the deuteron in the $\Delta$ region

Photo production of pions on the deuteron is studied in the spectator nucleon model. The Born terms of the elementary production amplitude are determined in pseudovector $\pi$N coupling and supplied with a form factor. The $\Delta$ resonance is considered both in the $s$ and the $u$ channel. The parameters of the $\Delta$ resonance and the cutoff of the form factors are fixed on the leading photoproduction multipoles. Results for total and differential cross sections are compared with experimental data. Particular attention is paid to the role of Pauli correlations of the final state nucleons in the quasifree case. The results are compared with those for pion photoproduction on the nucleon.

nucl-th↗
arXiv1996

Unitary ambiguity in the extraction of the E2/M1 ratio for the $γN\leftrightarrowΔ$ transition

The resonant electric quadrupole amplitude in the transition $γN\leftrightarrowΔ(1232)$ is of great interest for the understanding of baryon structure. Various dynamical models have been developed to extract it from the corresponding photoproduction multipole of pions on nucleons. It is shown that once such a model is specified, a whole class of unitarily equivalent models can be constructed, all of them providing exactly the same fit to the experimental data. However, they may predict quite different resonant amplitudes. Therefore, the extraction of the E2/M1($γN\leftrightarrowΔ$) ratio (bare or dressed) which is based on a dynamical model using a largely phenomenological $πN$ interaction is not unique.

nucl-th↗
arXiv1996

Rescattering effects in coherent pion photoproduction on the deuteron in the $Δ$ resonance region

Within a dynamical model, rescattering effects are studied in coherent pion photoproduction on the deuteron in the $Δ$(1232) resonance region. The model consists of a system of coupled equations for the N$Δ$, NN$π$ and NN channels. Pion rescattering leads in general to a significant reduction of total and differential cross sections resulting in a better description of experimental data. Only a few polarization observables are sensitive to rescattering effects. In particular $T_{20}$ allows an analysis of the reaction mechanism for specific kinematics. The question how rescattering affects the sensitivity to the E2 excitation of the $Δ$ resonance is also studied.

nucl-th↗
arXiv1994

Quasifree photoabsorption on neutron-proton pairs in 3He

Three-body photodisintegration of 3He is calculated in the photon energy range 200 - 400 MeV assuming quasifree absorption on np pairs both in initial quasideuteron and singlet configurations. The model includes the normal nucleonic current, explicit meson exchange currents and the Delta(1232)-isobar excitation. The total cross section is increased by a factor of about 1.5 compared with free deuteron photodisintegration. Well below and above the Delta region also some spin observables differ significantly from the ones of free deuteron disintegration due to the more compressed wave function of the correlated np pairs in 3He compared to the deuteron. The initial singlet state causes a significant change in the analyzing power Ay. These differences could presumably be seen at the conjugate angles where two-body effects are maximized and where photoreactions could complement similar pion absorption experiments. Figures by fax or post from janiskanen@phcu.helsinki.fi

nucl-th↗
arXiv1994

Photon absorption on a neutron-proton pair in $^3$He

The cross section of the reaction $^3$He$(γ,pn)p_{spec}$ in the energy range 150 - 450 MeV has been calculated in a quasifree two-body model and compared with a recent kinematically complete experiment. In comparison with free deuteron disintegration the cross section is increased by a factor of about 1.5 in reasonable agreement with the data for photon energies above 200 MeV. At lower energies the data deviate from the two-body behaviour and thus suggest a more important role of the spectator requiring a more exact treatment.

nucl-th↗