arXiv subjects

P. Wu

Publications and source records attributed to P. Wu.

17 recordsLinked to original sources

arXiv2025

Versatile multi-q antiferromagnetic charge order in correlated vdW metals

Following the discovery of graphene, interest in van der Waals (vdW) materials has surged; however, advancing physics beyond graphene requires quantum vdW materials platforms that host versatile, strongly interacting many-body states. Here, using scanning tunneling microscopy and spectroscopy at 300 mK, we uncover multiple competing electronic states in the van der Waals metal CeTe3: charge-ordered antiferromagnetic phases forming stripe and checkerboard orders. Remarkably, their competition is tuned by a modest in-plane magnetic field (~1.5 T), revealing strongly intertwined multiple frustrations involving antiferromagnetism, charge order, and Fermi-surface instabilities. Quasiparticle-interference imaging directly identifies the momentum-space origin of these competitions on the representative semimetals Fermi surface. While the observations can be understood at a basic level in terms of Kondo coupling between localized Ce 4f moments and itinerant Te 5p electrons, our results reveal a much richer phenomenology: an unusually broad electronic reconstruction extending to an energy scale of roughly 30 meV from EF, which realizes and deforms antiferromagnetic charge-ordered states and signals strongly correlated interactions beyond a weak-coupling description. Beyond establishing CeTe3 as a model platform, our results demonstrate that competing instabilities in antiferromagnetic two-dimensional metals/semimetals generate versatile electronic phases, opening a route to tunable nanoscale quantum states governed by the intertwined effects of correlation, symmetry, and topology.

cond-mat.str-el↗

arXiv2024

Uncovering hidden Fermi surface instabilities through visualizing unconventional quasiparticle interference in CeTe3

The charge density wave (CDW) state is a widespread phenomenon in low-dimensional metals/semimetals. The spectral weight of the associated folded bands (shadow bands) can be an intriguing trigger leading to additional Fermi surface instability and unexplored phase transitions. The rare earth tri-telluride CeTe3 exhibits a single CDW stabilized below ~400 K and antiferromagnetism below ~3 K. The distinct periodicities between the Te-square net, the CeTe block layer, and the CDW give rise to rich shadow band formations. In this work, we reveal the predominant scattering between the original and shadow bands at 4 K, with the scattering within the original bands being relatively suppressed at Fermi energy. This unconventional quasi-particle scattering collectively underscores the vital role of the shadow bands' spectral weight and the hidden matrix element effect, which are crucial for controlling electronic properties in this system. Furthermore, our finding points to the existence of rich and unexplored Fermi surface instabilities, which potentially play a role in controlling the nature of long-range antiferromagnetism at lower temperatures in the presence of finite charge-spin interaction.

cond-mat.str-el↗

arXiv2019

Observation of Multiphoton Frequency Conversion in Superconducting Circuits

Multiphoton up/down conversion in a transmon circuit, driven by a pair of microwaves tuned near and far off the qubit resonance, has been observed. The experimental realization of these high order non-linear processes is accomplished in the three-photon regime, when the transmon is coupled to weak bichromatic microwave fields with the same Rabi frequencies. A many-mode Floquet formalism, with longitudinal coupling, is used to simulate the quantum interferences in the absorption spectrum that manifest the multiphoton pumping processes in the transmon qubit. An intuitive graph theoretic approach is used to introduce effective Hamiltonians that elucidate main features of the Floquet results. The analytical solutions also illustrate how controllability is achievable for desired single- or multiphoton pumping processes in a wide frequency range.

quant-ph↗

arXiv2016

Results of the ASY-EOS experiment at GSI: The symmetry energy at suprasaturation density

Directed and elliptic flows of neutrons and light charged particles were measured for the reaction 197Au+197Au at 400 MeV/nucleon incident energy within the ASY-EOS experimental campaign at the GSI laboratory. The detection system consisted of the Large Area Neutron Detector LAND, combined with parts of the CHIMERA multidetector, of the ALADIN Time-of-flight Wall, and of the Washington-University Microball detector. The latter three arrays were used for the event characterization and reaction-plane reconstruction. In addition, an array of triple telescopes, KRATTA, was used for complementary measurements of the isotopic composition and flows of light charged particles. From the comparison of the elliptic flow ratio of neutrons with respect to charged particles with UrQMD predictions, a value γ= 0.72 \pm 0.19 is obtained for the power-law coefficient describing the density dependence of the potential part in the parametrization of the symmetry energy. It represents a new and more stringent constraint for the regime of supra-saturation density and confirms, with a considerably smaller uncertainty, the moderately soft to linear density dependence deduced from the earlier FOPI-LAND data. The densities probed are shown to reach beyond twice saturation.

nucl-ex↗

arXiv2015

Robust diamond-like Fe-Si network in the zero-strain NaxFeSiO4 Cathode

Sodium orthosilicates Na2MSiO4 (M denotes transition metals) have attracted much attention due to the possibility of exchanging two electrons per formula unit. In this work, we report a group of sodium iron orthosilicates Na2FeSiO4, the crystal structures of which are characterized by a diamond-like Fe-Si network. The Fe-Si network is quite robust against the charge/discharge process, which explains the high structural stability observed in experiment. Using the density functional theory within the GGA+U framework and X-ray diffraction studies, the crystal structures and structural stabilities during the sodium insertion/deinsertion process are systematically investigated. The calculated average deintercalation voltages are in good agreement with the experimental result.

cond-mat.mtrl-sci↗

arXiv2014

Electron Heating During Magnetic Reconnection: A Simulation Scaling Study

Electron bulk heating during magnetic reconnection with symmetric inflow conditions is examined using kinetic particle-in-cell (PIC) simulations. The degree of electron heating is well correlated with the inflowing Alfvén speed $c_{Ar}$ based on the reconnecting magnetic field through the relation $ΔT_e = 0.033 \,m_i\,c_{Ar}^2$, where $ΔT_{e}$ is the increase in electron temperature. For the range of simulations performed, the heating shows almost no correlation with inflow total temperature $T_{tot} = T_i + T_e$ or plasma $β$. An out-of-plane (guide) magnetic field of similar magnitude to the reconnecting field does not affect the total heating, but it does quench perpendicular heating, with almost all heating being in the parallel direction. These results are qualitatively consistent with a recent statistical survey of electron heating in the dayside magnetopause, which also found that $ΔT_e$ was proportional to the inflowing Alfvén speed. The net electron heating varies very little with distance downstream of the x-line. The simulations show at most a very weak dependence of electron heating on the ion to electron mass ratio. In the antiparallel reconnection case, the largely parallel heating is eventually isotropized downstream due a scattering mechanism such as stochastic particle motion or instabilities. The study highlights key properties that must be satisfied by an electron heating mechanism: (1) Preferential heating in the parallel direction; (2) Heating proportional to $m_i\,c_{Ar}^2$; (3) At most a weak dependence on electron mass; and (4) An exhaust electron temperature that varies little with distance from the x-line.

physics.plasm-ph↗

arXiv2013

Accelerating charging dynamics in sub-nanometer pores

Having smaller energy density than batteries, supercapacitors have exceptional power density and cyclability. Their energy density can be increased using ionic liquids and electrodes with sub-nanometer pores, but this tends to reduce their power density and compromise the key advantage of supercapacitors. To help address this issue through material optimization, here we unravel the mechanisms of charging sub-nanometer pores with ionic liquids using molecular simulations, navigated by a phenomenological model. We show that charging of ionophilic pores is a diffusive process, often accompanied by overfilling followed by de-filling. In sharp contrast to conventional expectations, charging is fast because ion diffusion during charging can be an order of magnitude faster than in bulk, and charging itself is accelerated by the onset of collective modes. Further acceleration can be achieved using ionophobic pores by eliminating overfilling/de-filling and thus leading to charging behavior qualitatively different from that in conventional, ionophilic pores.

cond-mat.mtrl-sci↗

arXiv2013

von Kármán energy decay and heating of protons and electrons in a kinetic turbulent plasma

Decay in time of undriven weakly collisional kinetic plasma turbulence in systems large compared to the ion kinetic scales is investigated using fully electromagnetic particle-in-cell simulations initiated with transverse flow and magnetic disturbances, constant density, and a strong guide field. The observed energy decay is consistent with the von Kármán hypothesis of similarity decay, in a formulation adapted to magnetohydrodyamics (MHD). Kinetic dissipation occurs at small scales, but the overall rate is apparently controlled by large scale dynamics. At small turbulence amplitude the electrons are preferentially heated. At larger amplitudes proton heating is the dominant effect. In the solar wind and corona the protons are typically hotter, suggesting that these natural systems are in large amplitude turbulence regime.

physics.plasm-ph↗

arXiv2012

The ASY-EOS experiment at GSI: investigating the symmetry energy at supra-saturation densities

The elliptic-flow ratio of neutrons with respect to protons in reactions of neutron rich heavy-ions systems at intermediate energies has been proposed as an observable sensitive to the strength of the symmetry term in the nuclear Equation Of State (EOS) at supra-saturation densities. The recent results obtained from the existing FOPI/LAND data for $^{197}$Au+$^{197}$Au collisions at 400 MeV/nucleon in comparison with the UrQMD model allowed a first estimate of the symmetry term of the EOS but suffer from a considerable statistical uncertainty. In order to obtain an improved data set for Au+Au collisions and to extend the study to other systems, a new experiment was carried out at the GSI laboratory by the ASY-EOS collaboration in May 2011.

nucl-ex↗

arXiv2011

Cosmic acceleration and phantom crossing in $f(T)$-gravity

In this paper, we propose two new models in $f(T)$ gravity to realize universe acceleration and phantom crossing due to dark torsion in the formalism. The model parameters are constrained and the observational test are discussed. The best fit results favors an accelerating universe with possible phantom crossing in the near past or future followed respectively by matter and radiation dominated era.

physics.gen-ph↗

arXiv2010

Local Probing of Mesoscopic Physics of Ferroelectric Domain Walls

Domain wall dynamics in ferroic materials underpins functionality of data storage and information technology devices. Using localized electric field of a scanning probe microscopy tip, we experimentally demonstrate a surprisingly rich range of polarization reversal behaviors in the vicinity of the initially flat 180°ferroelectric domain wall. The nucleation bias is found to increase by an order of magnitude from a 2D nucleus at the wall to 3D nucleus in the bulk. The wall is thus significantly ferroelectrically softer than the bulk. The wall profoundly affects switching on length scales of the order of micrometers. The mechanism of correlated switching is analyzed using analytical theory and phase-field modeling. The long-range effect is ascribed to wall bending under the influence of a tip bias well below the bulk nucleation field and placed many micrometers away from the wall. These studies provide an experimental link between the macroscopic and mesoscopic physics of domain walls and atomistic models of nucleation.

cond-mat.mtrl-sci↗

arXiv2010

Evidence of Dirac insulator properties in poly 1,5-dihydro-1,5-diazocine diazene

Existence of heteroaromatic graphene analog is predicted based upon periodic first principles density functional theory calculations. The new material, poly 1,5-dihydro 1,5-diazocine diazene, is a monolayered aromatic (planar) cross-linked polymer with cohesion energy - 6.03 eV/atom. Calculations reveal its Dirac insulator properties with narrow (~ 0.057 eV) and nearly direct band gap in close vicinity of Γ-point of Brillouin Zone. The predicted Fermi velocity of charge carriers ranges from ~3.41x105 m/s to ~1.63x106 m/s; thus effective mass of those could be up to ~2260 times lower than free electron one. These make proposed material a good alternative to graphene.

cond-mat.mtrl-sci↗

arXiv2009

Differential Neutron-Proton Squeeze-out

The elliptic flow (squeeze-out) of neutrons, protons and light complex particles in reactions of neutron-rich systems at relativistic energies is proposed as an observable sensitive to the strength of the symmetry term in the equation of state at supra-normal densities. Preliminary results from a study of the existing FOPI/LAND data for 197Au + 197Au collisions at 400 A MeV with the UrQMD model favor a moderately soft symmetry term with a density dependence of the potential term proportional to (rho/rho_0)^gamma with gamma = 0.6+-0.3.

nucl-ex↗

arXiv2007

Spin dependent resonant tunneling through 6 micron diameter double barrier resonant tunneling diode

A vertical resonant tunneling diode (RTD) based on the paramagnetic Zn1-x-yMnyCdxSe system has been fabricated with a pillar diameter down to ~ 6 micron. The diode exhibits high quality resonant tunneling characteristics through the electron sub-band of the quantum well at a temperature of 4.2K, where a clear phonon replica was observable in addition to the primary peak. Both peaks show a giant Zeeman splitting in an applied magnetic field. Employing a self-consistent real-time Green's function method, the current-voltage characteristic was simulated, showing good agreement with the measured result.

cond-mat.mes-hall↗

arXiv2000

CMB Analysis of Boomerang & Maxima & the Cosmic Parameters {Omega_tot,Omega_b h^2,Omega_cdm h^2,Omega_Lambda,n_s}

We show how estimates of parameters characterizing inflation-based theories of structure formation localized over the past year when large scale structure (LSS) information from galaxy and cluster surveys was combined with the rapidly developing cosmic microwave background (CMB) data, especially from the recent Boomerang and Maxima balloon experiments. All current CMB data plus a relatively weak prior probability on the Hubble constant, age and LSS points to little mean curvature (Omega_{tot} = 1.08\pm 0.06) and nearly scale invariant initial fluctuations (n_s =1.03\pm 0.08), both predictions of (non-baroque) inflation theory. We emphasize the role that degeneracy among parameters in the L_{pk} = 212\pm 7 position of the (first acoustic) peak plays in defining the $Ω_{tot}$ range upon marginalization over other variables. Though the CDM density is in the expected range (Ω_{cdm}h^2=0.17\pm 0.02), the baryon density Omega_bh^2=0.030\pm 0.005 is somewhat above the independent 0.019\pm 0.002 nucleosynthesis estimate. CMB+LSS gives independent evidence for dark energy (Omega_Λ=0.66\pm 0.06) at the same level as from supernova (SN1) observations, with a phenomenological quintessence equation of state limited by SN1+CMB+LSS to w_Q<-0.7 cf. the w_Q=-1 cosmological constant case.

astro-ph↗

arXiv2000

The Cosmic Background Radiation circa nu2K

We describe the implications of cosmic microwave background (CMB) observations and galaxy and cluster surveys of large scale structure (LSS) for theories of cosmic structure formation, especially emphasizing the recent Boomerang and Maxima CMB balloon experiments. The inflation-based cosmic structure formation paradigm we have been operating with for two decades has never been in better shape. Here we primarily focus on a simplified inflation parameter set, {omega_b,omega_{cdm},Omega_{tot}, Omega_Λ,n_s,τ_C, σ_8}. Combining all of the current CMB+LSS data points to the remarkable conclusion that the local Hubble patch we can access has little mean curvature (Omega_{tot}=1.08\pm 0.06) and the initial fluctuations were nearly scale invariant (n_s=1.03\pm 0.08), both predictions of (non-baroque) inflation theory. The baryon density is found to be slightly larger than that preferred by independent Big Bang Nucleosynthesis estimates (omega_b=0.030\pm 0.005 cf. 0.019\pm 0.002). The CDM density is in the expected range (omega_{cdm}=0.17 \pm 0.02). Even stranger is the CMB+LSS evidence that the density of the universe is dominated by unclustered energy akin to the cosmological constant (Omega_Λ=0.66\pm 0.06), at the same level as that inferred from high redshift supernova observations. We also sketch the CMB+LSS implications for massive neutrinos.

astro-ph↗

arXiv2000

The Quintessential CMB, Past & Future

The past, present and future of cosmic microwave background (CMB) anisotropy research is discussed, with emphasis on the Boomerang and Maxima balloon experiments. These data are combined with large scale structure (LSS) information and high redshift supernova (SN1) observations to explore the inflation-based cosmic structure formation paradigm. Here we primarily focus on a simplified inflation parameter set, {omega_b,omega_{cdm},Omega_{tot}, Omega_Q,w_Q, n_s,tau_C, sigma_8}. After marginalizing over the other cosmic and experimental variables, we find the current CMB+LSS+SN1 data gives Omega_{tot}=1.04\pm 0.05, consistent with (non-baroque) inflation theory. Restricting to Omega_{tot}=1, we find a nearly scale invariant spectrum, n_s =1.03 \pm 0.07. The CDM density, omega_{cdm}=0.17\pm 0.02, is in the expected range, but the baryon density, omega_b=0.030\pm 0.004, is slightly larger than the current nucleosynthesis estimate. Substantial dark energy is inferred, Omega_Q\approx 0.68\pm 0.05, and CMB+LSS Omega_Q values are compatible with the independent SN1 estimates. The dark energy equation of state, parameterized by a quintessence-field pressure-to-density ratio w_Q, is not well determined by CMB+LSS (w_Q<-0.3 at 95%CL), but when combined with SN1 the resulting w_Q<-0.7 limit is quite consistent with the w_Q=-1 cosmological constant case. Though forecasts of statistical errors on parameters for current and future experiments are rosy, rooting out systematic errors will define the true progress.

astro-ph↗