arXiv subjects

P. Wustelt

Publications and source records attributed to P. Wustelt.

5 recordsLinked to original sources

arXiv2021

High-order phase-dependent asymmetry in the above-threshold ionization plateau

Above-threshold ionization spectra from cesium are measured as a function of the carrier-envelope phase (CEP) using laser pulses centered at 3.1 $μ$m wavelength. The directional asymmetry in the energy spectra of backscattered electrons oscillates three times, rather than once, as the CEP is changed from $0$ to $2π$. Using the improved strong-field approximation, we show that the unusual behavior arises from the interference of few quantum orbits. We discuss the conditions for observing the high-order CEP dependence, and draw an analogy with time-domain holography with electron wave packets.

physics.atom-ph↗

arXiv2018

Goldilocks Zone for Enhanced Ionization in Strong Laser Fields

Utilizing a benchmark measurement of laser-induced ionization of an H$_2^+$ molecular ion beam target at infrared wavelength around 2 $μ$m, we show that the characteristic two-peak structure predicted for laser-induced enhanced ionization of H$_2^+$ and diatomic molecules in general, is a phenomenon which is confined to a small laser parameter space --- a Goldilocks Zone. Further, we control the effect experimentally and measure its imprint on the electron momentum. We replicate the behavior with simulations, which reproduce the measured kinetic-energy release as well as the correlated-electron spectra. Based on this, a model, which both maps out the Goldilocks Zone and illustrates why enhanced ionization has proven so elusive in H$_2^+$, is derived.

physics.atom-ph↗

arXiv2018

Heteronuclear Limit of Strong-Field Ionization: Fragmentation of HeH$^+$ by Intense Ultrashort Laser Pulses

The laser-induced fragmentation dynamics of this most fundamental polar molecule HeH$^+$ are measured using an ion beam of helium hydride and an isotopologue at various wavelengths and intensities. In contrast to the prevailing interpretation of strong-field fragmentation, in which stretching of the molecule results primarily from laser-induced electronic excitation, experiment and theory for nonionizing dissociation, single ionization and double ionization both show that the direct vibrational excitation plays the decisive role here. We are able to reconstruct fragmentation pathways and determine the times at which each ionization step occurs as well as the bond length evolution before the electron removal. The dynamics of this extremely asymmetric molecule contrast the well-known symmetric systems leading to a more general picture of strong-field molecular dynamics and facilitating interpolation to systems between the two extreme cases.

physics.chem-ph↗

arXiv2015

Momentum-resolved study of the saturation intensity in multiple ionization

We present a momentum-resolved study of strong field multiple ionization of ionic targets. Using a deconvolution method we are able to reconstruct the electron momenta from the ion momentum distributions after multiple ionization up to four sequential ionization steps. This technique allows an accurate determination of the saturation intensity as well as of the electron release times during the laser pulse. The measured results are discussed in comparison to typically used models of over-the-barrier ionization and tunnel ionization.

physics.atom-ph↗

arXiv2013

Coherent control at its most fundamental: CEP-dependent electron localization in photodissoziation of a H2+ molecular ion beam target

Measurements and calculations of the absolute carrier-envelope phase (CEP) effects in the photodissociation of the simplest molecule, H2+, with a 4.5-fs Ti:Sapphire laser pulse at intensities up to (4 +- 2)x10^14 Watt/cm^2 are presented. Localization of the electron with respect to the two nuclei (during the dissociation process) is controlled via the CEP of the ultra-short laser pulses. In contrast to previous CEP-dependent experiments with neutral molecules, the dissociation of the molecular ions is not preceded by a photoionization process, which strongly influences the CEP dependence. Kinematically complete data is obtained by time- and position-resolved coincidence detection. The phase dependence is determined by a single-shot phase measurement correlated to the detection of the dissoziation fragments. The experimental results show quantitative agreement with ab inito 3D-TDSE calculations that include nuclear vibration and rotation.

physics.chem-ph↗