arXiv subjects

P. de Marcillac

Publications and source records attributed to P. de Marcillac.

At least 55 records · Page 3Linked to original sources

arXiv2021

Calibration of nuclear recoils at the 100 eV scale using neutron capture

The development of low-threshold detectors for the study of coherent elastic neutrino-nucleus scattering and for the search for light dark matter necessitates methods of low-energy calibration. We suggest this can be provided by the nuclear recoils resulting from the $γ$ emission following thermal neutron capture. In particular, several MeV-scale single-$γ$ transitions induce well-defined nuclear recoil peaks in the 100 eV range. Using the FIFRELIN code, complete schemes of $γ$-cascades for various isotopes can be predicted with high accuracy to determine the continuous background of nuclear recoils below the calibration peaks. We present a comprehensive experimental concept for the calibration of CaWO$_4$ and Ge cryogenic detectors at a research reactor. For CaWO$_4$ the simulations show that two nuclear recoil peaks at 112.5 eV and 160.3 eV should be visible above background simply in the spectrum of the cryogenic detector. Then we discuss how the additional tagging for the associated $γ$ increases the sensitivity of the method and extends its application to a wider energy range and to Ge cryogenic detectors.

physics.ins-det↗

arXiv2021

Phonon-mediated crystal detectors with metallic film coating capable of rejecting $α$ and $β$ events induced by surface radioactivity

Phonon-mediated particle detectors based on single crystals and operated at millikelvin temperatures are used in rare-event experiments for neutrino physics and dark-matter searches. In general, these devices are not sensitive to the particle impact point, especially if the detection is mediated by thermal phonons. In this Letter, we demonstrate that excellent discrimination between interior and surface $β$ and $α$ events can be achieved by coating a crystal face with a thin metallic film, either continuous or in the form of a grid. The coating affects the phonon energy down-conversion cascade that follows the particle interaction, leading to a modified signal shape for close-to-film events. An efficient identification of surface events was demonstrated with detectors based on a rectangular $20 \times 20 \times 10$ mm$^3$ Li$_2$MoO$_4$ crystal coated with a Pd normal-metal film (10~nm thick) and with Al-Pd superconductive bi-layers (100~nm-10~nm thick) on a $20 \times 20$ mm$^2$ face. Discrimination capabilities were tested with $^{238}$U sources emitting both $α$ and $β$ particles. Surface events are identified for energy depositions down to millimeter-scale depths from the coated surface. With this technology, a substantial improvement of the background figure can be achieved in experiments searching for neutrinoless double-beta decay.

physics.ins-det↗

arXiv2021

New Limit for Neutrinoless Double-Beta Decay of $^{100}$Mo from the CUPID-Mo Experiment

The CUPID-Mo experiment at the Laboratoire Souterrain de Modane (France) is a demonstrator for CUPID, the next-generation ton-scale cryogenic $0νββ$ experiment. It consists of a 4.2 kg array of 20 enriched Li$_{2}$$^{100}$MoO$_4$ scintillating bolometers to search for the lepton number violating process of $0νββ$ decay in $^{100}$Mo. With more than one year of operation (2.16 kg$\times$yr of physics data), no event in the region of interest and hence no evidence for $0νββ$ is observed. We report a new limit on the half-life of $0νββ$ decay in $^{100}$Mo of $T_{1/2} > 1.5 \times 10^{24}\,$yr at 90 % C.I. The limit corresponds to an effective Majorana neutrino mass $\langle m_{ββ} \rangle$ $<$ (0.31--0.54)$\,$eV, dependent on the nuclear matrix element in the light Majorana neutrino exchange interpretation.

nucl-ex↗

arXiv2021

Pulse Shape Discrimination in CUPID-Mo using Principal Component Analysis

CUPID-Mo is a cryogenic detector array designed to search for neutrinoless double-beta decay ($0νββ$) of $^{100}$Mo. It uses 20 scintillating $^{100}$Mo-enriched Li$_2$MoO$_4$ bolometers instrumented with Ge light detectors to perform active suppression of $α$ backgrounds, drastically reducing the expected background in the $0νββ$ signal region. As a result, pileup events and small detector instabilities that mimic normal signals become non-negligible potential backgrounds. These types of events can in principle be eliminated based on their signal shapes, which are different from those of regular bolometric pulses. We show that a purely data-driven principal component analysis based approach is able to filter out these anomalous events, without the aid of detector response simulations.

physics.data-an↗

arXiv2020

Characterization of cubic Li$_{2}$$^{100}$MoO$_4$ crystals for the CUPID experiment

The CUPID Collaboration is designing a tonne-scale, background-free detector to search for double beta decay with sufficient sensitivity to fully explore the parameter space corresponding to the inverted neutrino mass hierarchy scenario. One of the CUPID demonstrators, CUPID-Mo, has proved the potential of enriched Li$_{2}$$^{100}$MoO$_4$ crystals as suitable detectors for neutrinoless double beta decay search. In this work, we characterised cubic crystals that, compared to the cylindrical crystals used by CUPID-Mo, are more appealing for the construction of tightly packed arrays. We measured an average energy resolution of (6.7$\pm$0.6) keV FWHM in the region of interest, approaching the CUPID target of 5 keV FWHM. We assessed the identification of $α$ particles with and without a reflecting foil that enhances the scintillation light collection efficiency, proving that the baseline design of CUPID already ensures a complete suppression of this $α$-induced background contribution. We also used the collected data to validate a Monte Carlo simulation modelling the light collection efficiency, which will enable further optimisations of the detector.

physics.ins-det↗

arXiv2020

A CUPID Li$_{2}$$^{100}$MoO$_4$ scintillating bolometer tested in the CROSS underground facility

A scintillating bolometer based on a large cubic Li$_{2}$$^{100}$MoO$_4$ crystal (45 mm side) and a Ge wafer (scintillation detector) has been operated in the CROSS cryogenic facility at the Canfranc underground laboratory in Spain. The dual-readout detector is a prototype of the technology that will be used in the next-generation $0\nu2β$ experiment CUPID. The measurements were performed at 18 and 12 mK temperature in a pulse tube dilution refrigerator. This setup utilizes the same technology as the CUORE cryostat that will host CUPID and so represents an accurate estimation of the expected performance. The Li$_{2}$$^{100}$MoO$_4$ bolometer shows a high energy resolution of 6 keV FWHM at the 2615 keV $γ$ line. The detection of scintillation light for each event triggered by the Li$_{2}$$^{100}$MoO$_4$ bolometer allowed for a full separation ($\sim$8$σ$) between $γ$($β$) and $α$ events above 2 MeV. The Li$_{2}$$^{100}$MoO$_4$ crystal also shows a high internal radiopurity with $^{228}$Th and $^{226}$Ra activities of less than 3 and 8 $μ$Bq/kg, respectively. Taking also into account the advantage of a more compact and massive detector array, which can be made of cubic-shaped crystals (compared to the cylindrical ones), this test demonstrates the great potential of cubic Li$_{2}$$^{100}$MoO$_4$ scintillating bolometers for high-sensitivity searches for the $^{100}$Mo $0\nu2β$ decay in CROSS and CUPID projects.

physics.ins-det↗

arXiv2020

The CROSS Experiment: Rejecting Surface Events by PSD Induced by Superconducting Films

Neutrinoless double beta ($0νββ$) decay is a hypothetical rare nuclear transition ($T_{1/2}>10^{26}$ y). Its observation would provide an important insight about the nature of neutrinos (Dirac or Majorana particle) demonstrating that the lepton number is not conserved. This decay can be investigated with bolometers embedding the double beta decay isotope ($^{76}$Ge, $^{82}$Se, $^{100}$Mo, $^{116}$Cd, $^{130}$Te...), which perform as low temperature calorimeters (10 mK) detecting particle interactions via a small temperature rise read out by a dedicated thermometer. CROSS (Cryogenic Rare-event Observatory with Surface Sensitivity) aims at the development of bolometric detectors (Li$_{2}$MoO$_{4}$ and TeO$_{2}$) capable of discriminating surface $α$ and $β$ interactions by exploiting superconducting properties of Al film deposited on the crystal surface. We report in this paper the results of tests on prototypes performed at CSNSM (Orsay, France) that showed the capability of a-few-$μ$m-thick superconducting Al film deposited on crystal surface to discriminate surface $α$ from bulk events, thus providing the detector with the required surface sensitivity capability. The CROSS technology would further improve the background suppression and simplify the detector construction with a view to future competitive double beta decay searches.

physics.ins-det↗

arXiv2019

Precise measurement of $2νββ$ decay of $^{100}$Mo with the CUPID-Mo detection technology

We report the measurement of the two-neutrino double-beta ($2νββ$) decay of $^{100}$Mo to the ground state of $^{100}$Ru using lithium molybdate (\crystal) scintillating bolometers. The detectors were developed for the CUPID-Mo program and operated at the EDELWEISS-III low background facility in the Modane underground laboratory. From a total exposure of $42.235$ kg$\times$d, the half-life of $^{100}$Mo is determined to be $T_{1/2}^{2ν}=[7.12^{+0.18}_{-0.14}\,\mathrm{(stat.)}\pm0.10\,\mathrm{(syst.)}]\times10^{18}$ years. This is the most accurate determination of the $2νββ$ half-life of $^{100}$Mo to date. We also confirm, with the statistical significance of $>3σ$, that the single-state dominance model of the $2νββ$ decay of $^{100}$Mo is favored over the high-state dominance model.

nucl-ex↗

arXiv2019

First data from the CUPID-Mo neutrinoless double beta decay experiment

The CUPID-Mo experiment is searching for neutrinoless double beta decay in $^{100}$Mo, evaluating the technology of cryogenic scintillating Li$_{2}^{100}$MoO$_4$ detectors for CUPID (CUORE Upgrade with Particle ID). CUPID-Mo detectors feature background suppression using a dual-readout scheme with Li$_{2}$MoO$_4$ crystals complemented by Ge bolometers for light detection. The detection of both heat and scintillation light signals allows the efficient discrimination of $α$ from $γ$&$β$ events. In this proceedings, we discuss results from the first 2 months of data taking in spring 2019. In addition to an excellent bolometric performance of 6.7$\,$keV (FWHM) at 2615$\,$keV and an $α$ separation of better than 99.9\% for all detectors, we report on bulk radiopurity for Th and U. Finally, we interpret the accumulated physics data in terms of a limit of $T_{1/2}^{0ν}\,> 3\times10^{23}\,$yr for $^{100}$Mo and discuss the sensitivity of CUPID-Mo until the expected end of physics data taking in early 2020.

hep-ex↗

arXiv2019

The $0\nu2β$-decay CROSS experiment: preliminary results and prospects

Neutrinoless double-beta decay is a key process in particle physics. Its experimental investigation is the only viable method that can establish the Majorana nature of neutrinos, providing at the same time a sensitive inclusive test of lepton number violation. CROSS (Cryogenic Rare-event Observatory with Surface Sensitivity) aims at developing and testing a new bolometric technology to be applied to future large-scale experiments searching for neutrinoless double-beta decay of the promising nuclei $^{100}$Mo and $^{130}$Te. The limiting factor in large-scale bolometric searches for this rare process is the background induced by surface radioactive contamination, as shown by the results of the CUORE experiment. The basic concept of CROSS consists of rejecting this challenging background component by pulse-shape discrimination, assisted by a proper coating of the faces of the crystal containing the isotope of interest and serving as energy absorber of the bolometric detector. In this paper, we demonstrate that ultra-pure superconductive Al films deposited on the crystal surfaces act successfully as pulse-shape modifiers, both with fast and slow phonon sensors. Rejection factors higher than 99.9% of $α$ surface radioactivity have been demonstrated in a series of prototypes based on crystals of Li$_2$MoO$_4$ and TeO$_2$. We have also shown that point-like energy depositions can be identified up to a distance of $\sim 1$ mm from the coated surface. The present program envisions an intermediate experiment to be installed underground in the Canfranc laboratory (Spain) in a CROSS-dedicated facility. This experiment, comprising $\sim 3\times 10^{25}$ nuclei of $^{100}$Mo, will be a general test of the CROSS technology as well as a worldwide competitive search for neutrinoless double-beta decay, with sensitivity to the effective Majorana mass down to 70 meV in the most favorable conditions.

nucl-ex↗

arXiv2019

The CUPID-Mo experiment for neutrinoless double-beta decay: performance and prospects

CUPID-Mo is a bolometric experiment to search for neutrinoless double-beta decay ($0νββ$) of $^{100}$Mo. In this article, we detail the CUPID-Mo detector concept, assembly, installation in the underground laboratory in Modane in 2018, and provide results from the first datasets. The demonstrator consists of an array of 20 scintillating bolometers comprised of $^{100}$Mo-enriched 0.2 kg Li$_2$MoO$_4$ crystals. The detectors are complemented by 20 thin cryogenic Ge bolometers acting as light detectors to distinguish $α$ from $γ$/$β$ events by the detection of both heat and scintillation light signals. We observe good detector uniformity, facilitating the operation of a large detector array as well as excellent energy resolution of 5.3 keV (6.5 keV) FWHM at 2615 keV, in calibration (physics) data. Based on the observed energy resolutions and light yields a separation of $α$ particles at much better than 99.9\% with equally high acceptance for $γ$/$β$ events is expected for events in the region of interest for $^{100}$Mo $0νββ$. We present limits on the crystals' radiopurity ($\leq$3 $μ$Bq/kg of $^{226}$Ra and $\leq$2 $μ$Bq/kg of $^{232}$Th). Based on these initial results we also discuss a sensitivity study for the science reach of the CUPID-Mo experiment, in particular, the ability to set the most stringent half-life limit on the $^{100}$Mo $0νββ$ decay after half a year of livetime. The achieved results show that CUPID-Mo is a successful demonstrator of the technology - developed in the framework of the LUMINEU project - selected for the CUPID experiment, a proposed follow-up of CUORE, the currently running first tonne-scale cryogenic $0νββ$ experiment.

physics.ins-det↗

arXiv2019

First test of a $\mathrm{CdMoO_4}$ scintillating bolometer for neutrinoless double beta decay experiments with $\mathrm{{}^{116}Cd}$ and $\mathrm{{}^{100}Mo}$ nuclides

A large cylindrical cadmium molybdate crystal with natural isotopic abundance has been used to fabricate a scintillating bolometer. The measurement was performed above ground at milli-Kelvin temperature, with simultaneous readout of the heat and the scintillation light. The energy resolution as FWHM has achieved from 5 keV (at 238 keV) to 13 keV (at 2615 keV). We present the results of the $α$ versus $β$/$γ$ events discrimination. The low internal trace contamination of the $\mathrm{CdMoO_4}$ crystal was evaluated as well. The detector performance with preliminary positive indications proves that cadmium molybdate crystal is a promising absorber for neutrinoless double beta decay scintillating bolometric experiments with $\mathrm{{}^{116}Cd}$ and $\mathrm{{}^{100}Mo}$ nuclides in the next-generation technique.

physics.ins-det↗

arXiv2019

Charge-to-heat transducers exploiting the Neganov-Trofimov-Luke effect for light detection in rare-event searches

In this work we present how to fabricate large-area (15 cm2), ultra-low threshold germanium bolometric photo-detectors and how to operate them to detect few (optical) photons. These detectors work at temperatures as low as few tens of mK and exploit the Neganov-Trofimov-Luke (NTL) effect. They are operated as charge-to-heat transducers: the heat signal is linearly increased by simply changing a voltage bias applied to special metal electrodes, fabricated onto the germanium absorber, and read by a (NTD-Ge) thermal sensor. We fabricated a batch of five prototypes and ran them in different facilities with dilution refrigerators. We carefully studied how impinging spurious infrared radiation impacts the detector performances, by shining infrared photons via optical-fiber-guided LED signals, in a controlled manner, into the bolometers. We hence demonstrated how the radiation-tightness of the test environment tremendously enhances the detector performances, allowing to set electrode voltage bias up to 90 volts without any leakage current and signal-to-noise gain as large as a factor 12 (for visible photons). As consequence, for the first time we could operate large-area NTD-Ge-sensor-equipped NTL bolometric photo-detectors capable to reach sub 10-eV baseline noise (RMS). Such detectors open new frontiers for rare-event search experiments based on low light yield Ge-NTD equipped scintillating bolometers, such the CUPID neutrinoless double-beta decay experiment.

physics.ins-det↗

arXiv2018

Complete event-by-event $α$/$γ(β)$ separation in a full-size TeO$_2$ CUORE bolometer by Neganov-Luke-magnified light detection

In the present work, we describe the results obtained with a large ($\approx 133$ cm$^3$) TeO$_2$ bolometer, with a view to a search for neutrinoless double-beta decay ($0νββ$) of $^{130}$Te. We demonstrate an efficient $α$ particle discrimination (99.9\%) with a high acceptance of the $0νββ$ signal (about 96\%), expected at $\approx 2.5$ MeV. This unprecedented result was possible thanks to the superior performance (10 eV rms baseline noise) of a Neganov-Luke-assisted germanium bolometer used to detect a tiny (70 eV) light signal from the TeO$_2$ detector, dominated by $γ$($β$)-induced Cherenkov radiation but exhibiting also a clear scintillation component. The obtained results represent a major breakthrough towards the TeO$_2$-based version of CUORE Upgrade with Particle IDentification (CUPID), a ton-scale cryogenic $0νββ$ experiment proposed as a follow-up to the CUORE project with particle identification. The CUORE experiment began recently a search for neutrinoless double-beta decay of $^{130}$Te with an array of 988 125-cm$^3$ TeO$_2$ bolometers. The lack of $α$ discrimination in CUORE makes $α$ decays at the detector surface the dominant background component, at the level of $\approx 0.01$ counts/(keV kg y) in the region of interest. We show here, for the first time with a CUORE-size bolometer and using the same technology as CUORE for the readout of both heat and light signals, that surface $α$ background can be fully rejected.

physics.ins-det↗

arXiv2018

First scintillating bolometer tests of a CLYMENE R&D on Li$_2$MoO$_4$ scintillators towards a large-scale double-beta decay experiment

A new R&D on lithium molybdate scintillators has begun within a project CLYMENE (Czochralski growth of Li$_2$MoO$_4$ crYstals for the scintillating boloMeters used in the rare EveNts sEarches). One of the main goals of the CLYMENE is a realization of a Li$_2$MoO$_4$ crystal growth line to be complementary to the one recently developed by LUMINEU in view of a mass production capacity for CUPID, a next-generation tonne-scale bolometric experiment to search for neutrinoless double-beta decay. In the present paper we report the investigation of performance and radiopurity of 158-g and 13.5-g scintillating bolometers based on a first large-mass (230 g) Li$_2$MoO$_4$ crystal scintillator developed within the CLYMENE project. In particular, a good energy resolution (2--7 keV FWHM in the energy range of 0.2--5 MeV), one of the highest light yield (0.97 keV/MeV) amongst Li$_2$MoO$_4$ scintillating bolometers, an efficient alpha particles discrimination (10$σ$) and potentially low internal radioactive contamination (below 0.2--0.3 mBq/kg of U/Th, but 1.4 mBq/kg of $^{210}$Po) demonstrate prospects of the CLYMENE in the development of high quality and radiopure Li$_2$MoO$_4$ scintillators for CUPID.

physics.ins-det↗

arXiv2018

Growth and characterization of a Li2Mg2(MoO4)3 scintillating bolometer

Lithium magnesium molybdate (Li$_2$Mg$_2$(MoO$_4$)$_3$) crystals were grown by the low-thermal-gradient Czochralski method. Luminescence properties of the material (emission spectra, thermally stimulated luminescence, dependence of intensity on temperature, phosphorescence) have been studied under X-Ray excitation in the temperature interval from 8 K to 400 K, while at the same being operated as a scintillating bolometer at 20 mK for the first time. We demonstrated that Li$_2$Mg$_2$(MoO$_4)_3$ crystals are a potentially promising detector material to search for neutrinoless double beta decay of $^{100}$Mo.

physics.ins-det↗

arXiv2017

Development of $^{100}$Mo-containing scintillating bolometers for a high-sensitivity neutrinoless double-beta decay search

This paper reports on the development of a technology involving $^{100}$Mo-enriched scintillating bolometers, compatible with the goals of CUPID, a proposed next-generation bolometric experiment to search for neutrinoless double-beta decay. Large mass ($\sim$1~kg), high optical quality, radiopure $^{100}$Mo-containing zinc and lithium molybdate crystals have been produced and used to develop high performance single detector modules based on 0.2--0.4~kg scintillating bolometers. In particular, the energy resolution of the lithium molybdate detectors near the $Q$-value of the double-beta transition of $^{100}$Mo (3034~keV) is 4--6~keV FWHM. The rejection of the $α$-induced dominant background above 2.6~MeV is better than 8$σ$. Less than 10~$μ$Bq/kg activity of $^{232}$Th ($^{228}$Th) and $^{226}$Ra in the crystals is ensured by boule recrystallization. The potential of $^{100}$Mo-enriched scintillating bolometers to perform high sensitivity double-beta decay searches has been demonstrated with only 10~kg$\times$d exposure: the two neutrino double-beta decay half-life of $^{100}$Mo has been measured with the up-to-date highest accuracy as $T_{1/2}$ = [6.90 $\pm$ 0.15(stat.) $\pm$ 0.37(syst.)] $\times$ 10$^{18}$~yr. Both crystallization and detector technologies favor lithium molybdate, which has been selected for the ongoing construction of the CUPID-0/Mo demonstrator, containing several kg of $^{100}$Mo.

physics.ins-det↗

arXiv2016

Rejection of randomly coinciding events in Li$_2$$^{100}$MoO$_4$ scintillating bolometers using light detectors based on the Neganov-Luke effect

Random coincidences of nuclear events can be one of the main background sources in low-temperature calorimetric experiments looking for neutrinoless double-beta decay, especially in those searches based on scintillating bolometers embedding the promising double-beta candidate $^{100}$Mo, because of the relatively short half-life of the two-neutrino double-beta decay of this nucleus. We show in this work that randomly coinciding events of the two-neutrino double decay of $^{100}$Mo in enriched Li$_2$$^{100}$MoO$_4$ detectors can be effectively discriminated by pulse-shape analysis in the light channel if the scintillating bolometer is provided with a Neganov-Luke light detector, which can improve the signal-to-noise ratio by a large factor, assumed here at the level of $\sim 750$ on the basis of preliminary experimental results obtained with these devices. The achieved pile-up rejection efficiency results in a very low contribution, of the order of $\sim 6\times10^{-5}$ counts/(keV$\cdot$kg$\cdot$y), to the background counting rate in the region of interest for a large volume ($\sim 90$ cm$^3$) Li$_2$$^{100}$MoO$_4$ detector. This background level is very encouraging in view of a possible use of the Li$_2$$^{100}$MoO$_4$ solution for a bolometric tonne-scale next-generation experiment as that proposed in the CUPID project.

physics.ins-det↗